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Selectively nucleotide-derived RuP on N,P-codoped carbon with engineered mesopores for energy-efficient hydrogen production assisted by hydrazine oxidation

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SusMat 2024年第1期4卷 166-177页

作者： Xiya Guan Yu Sun Simeng zhao Haibo Li Suyuan zeng Qingxia Yao Rui Li Hongyan Chen Konggang Qu School of Chemistry and Chemical Engineering Shandong Provincial Key Laboratory/Collaborative Innovation Center of Chemical Energy Storage&Novel Cell TechnologyLiaocheng UniversityLiaochengChina

Integrating hydrogen evolution reaction(HER)with hydrazine oxidation reaction(HzOR)has an encouraging prospect for the energy-saving hydrogen production,demanding the high-performance bifunctional HER/HzOR *** phosphide/doped carbon composites have exhibited superior activity towardmultiple electrocatalytic *** explore the decent water-soluble precursors containing bothNand P elements is highly attractive to facilely prepare metal phosphide/doped carbon ***,as one kind ecofriendly biomolecules,adenine nucleotide was first employed to selectively fabricate the highly pure RuP nanoparticles embedded into porous N,P-codoped carbons(RuP/PNPC)with a straightforward“mix-and-pyrolyze”*** newly prepared RuP/PNPC only requires 4.0 and−83.0 mV at 10 mA/cm^(2) separately in alkaline HER and HzOR,outperforming most of reported electrocatalysts,together with the outstanding neutral bifunctional ***,the two-electrode alkaline and neutral overall hydrazine splitting both exhibit significant power-efficiency superiority to the corresponding overall water splitting with the voltage difference of larger than 2 V,which can be also easily driven by the fuel cells and solar cells with considerableH2 *** report innovates the N-and P-bearing adenine nucleotide to effortlessly synthesize the high-quality RuP/doped carbon composite catalysts,highly potential as a universal platform for metal phosphide-related functional materials.

关键词： bifunctional electrocatalyst hydrazine oxidation hydrogen energy hydrogen evolution RuP

Bioinspired design of integral molded Janus silk fibroin-MXene evaporator for efficient solar vapor generation

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Nano Research 2024年第4期17卷 2824-2835页

作者： Ling-Qing Kong Zhi-Cheng zeng Guang-Zong Min zhao-Hui Meng Guo-Qing Meng Xiao-Xiao Guo Nai-Bo Lin Xiang-Yang Liu The Higher Educational Key Laboratory for Biomedical Engineering of Fujian Province Research Center of Biomedical Engineering of XiamenDepartment of BiomaterialsCollege of MaterialsXiamen UniversityXiamen 361005China The State Key Laboratory of Marine Environmental Science(MEL) College of Ocean and Earth SciencesXiamen UniversityXiamen 361005China

Solar vapor generation is a promising sustainable technology that uses solar distillation to produce fresh water from seawater and wastewater,helping relieve global water resource ***,inspired by naturally grown integrally molded mulberry leaves with a Janus hydrophilic and hydrophobic structure,a novel,simple,and efficient integrated molding method is proposed to break through the limitations of the traditional split manufacturing strategy and realizes the integrated formation of Janus *** on the spontaneous sedimentation characteristics of MXene in silk fibroin solution and its regulation of mesoscopic structure and hydrophilicity of silk fibroin,layered structures with different compositions and hydrophilicities were obtained in one ***,ethanol and glutaraldehyde were added to construct a physical crystallization-chemical crosslinking dual stabilization structure in silk *** evaporator has the evaporation rate of 3.07 kg·m^(-2)·h^(-1) and the efficiency of 86.8%under 1 sun and maintains high evaporation performance under various extreme test conditions including vigorous washing,repeated compression,and high-intensity ultraviolet(UV)***,the evaporator performs well in practical application scenarios,its evaporation rate in the simulated Dead Sea seawater exceeds 2.13 kg·m^(-2)·h^(-1),and more than 99.9%of the salt,heavy metal ions,oil pollution,and dyes are purified.

关键词： silk fibroin MXene bioinspired integrated molding Janus structure solar vapor generation

Enhanced SERS aptasensor for sensitive detection of saxitoxin based on HAuCl/HOreaction system and Pt/Au nanozyme

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Food Science and Human Wellness 2024年

作者： Yueqing Li Xuemei Tang wei zeng Ting Wu Long Wu School of Food Science and Engineering， Key Laboratory of Tropical Fruits and Vegetables Quality and Safety for State Market Regulation， Hainan University

Saxitoxin （STX） is a marine biotoxin produced by cyanobacteria and methanobacteria， which is harmful to humans and aquatic organisms. Therefore， it is urgent to establish an efficient， sensitive and selective method for the screening of STX. In this paper， based on the HAuCl4/H2O2reaction system， gold nanoparticles （Au NPs） decorated Fe3O4magnetic beads (Fe3O4@Au NPs) and Pt/Au nanozymes （Pt/Au NZs）， an enhanced SERS aptasensor was proposed for sensitive and selective detection of STX. Firstly， SERS tag （4-MBA） and aptamer modified Fe3O4@Au NPs were hybridized with complementary DNA modified Pt/Au NZs （Pt/Au-cDNA） to form the specific complexes. Wherein， aptamer acted as capture agent to specifically recognize STX， Pt/Au NZs catalyzed HAuCl4/H2O2reaction to enhance SERS signal， and Fe3O4facilitated the magnetic separation and simple detection operations. The SERS aptasensor achieved sensitive detection of STX with a wide linear range from 0.02 μmol/L to 0.8 μmol/L and a low detection limit of 13 nmol/L （LOD， S/N=3）. To evaluate the performance of this method， STX were detected in the spiked seafood samples with recoveries from 78.75% to 150% with relative errors below 6.52%. Besides， the SERS aptasensor behaved good stability and repeatability， revealing its promising potential in STX detection and food safety detection.

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Prescribed Performance Evolution Control for Quadrotor Autonomous Shipboard Landing

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IEEE/CAA Journal of Automatica Sinica 2024年第5期11卷 1151-1162页

作者： Yang Yuan Haibin Duan Zhigang zeng State Key Laboratory of Virtual Reality Technology and Systems the School of Automation Science and Electrical EngineeringBeihang UniversityBeijing 100083China State Key Laboratory of Virtual Reality Technology and Systems the School of Automation Science and Electrical EngineeringBeihang UniversityBeijing 100083 Virtual Reality Fundamental Research Laboratory Department of Mathematics and TheoriesPeng Cheng LaboratoryShenzhen 518000China School of Artificial Intelligence and Automation Huazhong University of Science and TechnologyWuhan 430074China

The shipboard landing problem for a quadrotor is addressed in this paper,where the ship trajectory tracking control issue is transformed into a stabilization control issue by building a relative position *** guarantee both transient performance and steady-state landing error,a prescribed performance evolution control(PPEC)method is developed for the relative position *** addition,a novel compensation system is proposed to expand the performance boundaries when the input saturation occurs and the error exceeds the predefined *** the wind and wave on the relative position model,an adaptive sliding mode observer(ASMO)is designed for the disturbance with unknown upper *** on the dynamic surface control framework,a shipboard landing controller integrating PPEC and ASMO is established for the quadrotor,and the relative position control error is guaranteed to be uniformly ultimately *** results have verified the feasibility and effectiveness of the proposed shipboard landing control scheme.

关键词： error integrating stabilization

Inhibition of the NF-κB Signaling Pathway Improves Cigarette Mainstream Smoke-Induced Lung Injury and Gut Microbiota Disturbance

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Biomedical and Environmental Sciences 2024年第6期37卷 676-681页

作者： Hong Huang Shengjie Li Lifang zeng Yan Zhang Ying Chen Yanbing Ma Jing wei Changwei Zou Tingtao Chen School of Resources and Environment Nanchang UniversityNanchang 330031JiangxiChina National Engineering Research Center for Bioengineering Drugs and the Technologies Institute of Translational MedicineJiangxi Medical CollegeNanchang UniversityNanchang 330031JiangxiChina School of Pharmacy Jiangxi Medical CollegeNanchang UniversityNanchang 330006JiangxiChina

Currently,cigarette smoke(CS)remains a major contributor to disease morbidity and *** can be divided into cigarette mainstream smoke(CMS)and side-stream smoke,depending on where it is produced by burning tobacco^([1]).CMS is inhaled by smokers from the filter end during cigarette combustion and is strongly associated with the development of several diseases^([2-4]).

关键词： smoke CMS cigarette

Role of adhesion molecules in cancer and targeted therapy

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Science China(Life Sciences) 2024年第5期67卷 940-957页

作者： Chunmei Fan Fang Xiong Shanshan Zhang zhaojian Gong Qianjin Liao Guiyuan Li Can Guo wei Xiong He Huang zhaoyang zeng NHC Key Laboratory of Carcinogenesis and Hunan Key Laboratory of Cancer Metabolism Hunan Cancer Hospital and the Affiliated Cancer Hospital of Xiangya School of MedicineCentral South UniversityChangsha 410000China Department of Histology and Embryology Xiangya School of MedicineCentral South UniversityChangsha410013China Department of Stomatology Xiangya HospitalCentral South UniversityChangsha 410078China Department of Oral and Maxillofacial Surgery The Second Xiangya HospitalCentral South UniversityChangsha 410011China Key Laboratory of Carcinogenesis and Cancer Invasion of the Chinese Ministry of Education Cancer Research InstituteCentral South UniversityChangsha 410078China

Adhesion molecules mediate cell-to-cell and cell-to-extracellular matrix interactions and transmit mechanical and chemical signals among *** mechanisms deregulate adhesion molecules in cancer,enabling tumor cells to proliferate without restraint,invade through tissue boundaries,escape from immune surveillance,and survive in the tumor *** studies have revealed that adhesion molecules also drive angiogenesis,reshape metabolism,and are involved in stem cell *** this review,we summarize the functions and mechanisms of adhesion molecules in cancer and the tumor microenvironment,as well as the therapeutic strategies targeting adhesion *** studies have implications for furthering our understanding of adhesion molecules in cancer and providing a paradigm for exploring novel therapeutic approaches.

关键词： adhesion molecules tumor microenvironment invasion and metastasis reshaping metabolism angiogenesis immune evasion tumor stemness therapeutic strategy

A social computing method for energy safety

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Journal of Safety Science and Resilience 2024年第1期5卷 64-82页

作者： Pengfei zhao Shuangqi Li Zhidong Cao Paul Jen-Hwa Hu Daniel Dajun zeng Da Xie Yichen Shen Jiangfeng Li Tianyi Luo Institute of Automation Chinese Academy of SciencesUniversity of Chinese Academy of SciencesBeijing 100090China Systems Engineering Cornell UniversityIthacaNY 14853USA David Eccles School of Business the University of UtahUtahUSA Department of Electrical Engineering Shanghai Jiao Tong UniversityShanghai 200240China China University of Mining and Technology China

Information and communication technologies enable the transformation of traditional energy systems into cyber-physical energy systems(CPESs),but such systems have also become popular targets of ***,available methods for evaluating the impacts of cyberattacks suffer from limited resilience,efficacy,and practical *** mitigate their potentially disastrous consequences,this study suggests a two-stage,discrepancy-based optimization approach that considers both preparatory actions and response measures,integrating concepts from social *** proposed Kullback-Leibler divergence-based,distributionally robust optimization(KDR)method has a hierarchical,two-stage objective function that incorporates the operating costs of both system infrastructures(e.g.,energy resources,reserve capacity)and real-time response measures(e.g.,load shedding,demand-side management,electric vehicle charging station management).By incorporating social computing principles,the optimization framework can also capture the social behavior and interactions of energy consumers in response to *** preparatory stage entails day-ahead operational decisions,leveraging insights from social computing to model and predict the behaviors of individuals and communities affected by potential *** mitigation stage generates responses designed to contain the consequences of the attack by directing and optimizing energy use from the demand side,taking into account the social context and preferences of energy consumers,to ensure resilient,economically efficient CPES *** method can determine optimal schemes in both stages,accounting for the social dimensions of the *** original disaster mitigation model uses an abstract formulation to develop a risk-neutral model that characterizes cyberattacks through KDR,incorporating social computing techniques to enhance the understanding and response to cyber *** approach can mitigate the impacts more

关键词： Cyberattacks Cyber-physical energy systems Distributionally robust optimization False data injections Two-stage modeling Social computing

Electrochemical conversion of organic compounds and inorganic small molecules

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Science China Chemistry 2024年第10期67卷 3223-3246页

作者： weimei zeng Youai Qiu Department of Chemistry Nankai University

Electrochemical synthesis presents a facile and sustainable strategy to produce valuable molecules. This review summarizes the most recent advances in electrosynthesizing value-added compounds with inorganic small molecules. While “small molecules”refers to a broad spectrum of chemicals, we mainly focus on the electrochemical conversion of CO2, H2O/D2O, NH3and SO2until March 2024. This review intends to compare the results and display general trends throughout the field, with an emphasis on the substrate scope and mechanical aspect. Furthermore, we propose several techniques and protocols that can enable a more fundamental understanding of the electrochemical reaction involving inorganic small molecules and help drive this methodology toward commercialization.

关键词： electrochemical synthesis inorganic small molecule organic synthesis carbon dioxide water

Self-synchronized multi-color Q-switched fiber laser using a parallel-integrated fiber Bragg grating

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Chinese Optics Letters 2024年第6期22卷 148-153页

作者： Chao zeng Guangwei Yang Dong Li Pengtao Luo Ruohui Wang Yueqing Du Dong Mao Jianlin zhao Key Laboratory of Light Field Manipulation and Information Acquisition Ministry of Industry and Information TechnologySchool of Physical Science and TechnologyNorthwestern Polytechnical UniversityXi’an 710072China Research&Development Institute of Northwestern Polytechnical University in Shenzhen Shenzhen 518063China School of Physics Northwest UniversityXi’an 720127China

We demonstrate an intracavity self-synchronized multi-color Q-switched fiber laser using a parallel-integrated fiber Bragg grating(PI-FBG), fabricated by a femtosecond laser with a point-by-point parallel inscription method. The multi-color Q-switched pulses can be always self-synchronized when the group delay differences between neighboring spectra range from-3.4 to 3.4 *** starting and evolution dynamics indicate that the saturable absorption effect of the carbon nanotube plays a dual role: synchronously triggering the startup of the pulse at successive colors by active Q-switching and spontaneously compensating to some extent the temporal walk-off of the multi-color pulses through the cross saturable absorption modulation. This work unveils the intracavity self-synchronization mechanism of the multi-color Q-switched pulses and also demonstrates the potential of PI-FBGs for the customizable generation of the synchronized multi-color pulse in a single cavity.

关键词： synchronized pulse sources Q-switched fiber lasers saturable absorption effect fiber Bragg grating