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dual-donor-Induced Crystallinity m.d.lation Enables 19.23% Efficiency Organic Solar Cells

NANO-mICRO LETTERS 2025年第1期17卷 1-13页

作者： Liang, Anhai Sun, Yuqing Chung, Sein Shin, Jiyeong Sun, Kangbo Zhu, Chaofeng zhao, Jingjing zhao, Zhenmin Zhong, Yufei Zhang, Guangye Cho, Kilwon Kan, Zhipeng Guangxi Univ Inst Sci & Technol Carbon Peak & Neutral Ctr Nanoenergy Res Sch Phys Sci & Technol Nanning 530004 Peoples R China Pohang Univ Sci & Technol Dept Chem Engn Pohang 37673 South Korea Shenzhen Technol Univ Coll New Mat & New Energies Shenzhen 518118 Peoples R China NingboTech Univ Zhejiang Engn Res Ctr Fabricat & Applicat Adv Phot Sch Mat Sci & Engn Ningbo 315100 Peoples R China State Key Lab Featured met mat & Life Cycle Safety Nanning 530004 Peoples R China

By m.d.lating the crystalline properties of the active layer with dual donors, the efficiency of organic solar cells reaches 19.23%.The introduction of PTzBI-dF suppresses the accumulation of traps and charge recombination, allowing ternary devices to maintain 82% of their initial power conversion efficiency (PCE) after illumination for 800 *** dual-donor strategy for m.d.lating the crystallinity of the active layer is applicable to a variety of Y6 derivatives, and the increase in PCE exceeds 1%. Trap-assisted charge recombination is one of the primary limitations of restricting the performance of organic solar cells. However, effectively reducing the presence of traps in the photoactive layer remains challenging. Herein, wide bandgap polymer donor PTzBI-dF is demonstrated as an effective m.d.lator for enhancing the crystallinity of the bulk heterojunction active layers composed of d18 derivatives blended with Y6, leading to dense and ordered molecular packings, and thus, improves photoluminescence quenching properties. As a result, the photovoltaic devices exhibit reduced trap-assisted charge recombination losses, achieving an optimized power conversion efficiency of over 19%. Besides the efficiency enhancement, the devices comprised of PTzBI-dF as a third component simultaneously attain decreased current leakage, improved charge carrier mobilities, and suppressed bimolecular charge recombination, leading to reduced energy losses. The advanced crystalline structures induced by PTzBI-dF and its characteristics, such as well-aligned energy level, and complementary absorption spectra, are ascribed to the promising performance improvements. Our findings suggest that donor phase engineering is a feasible approach to tuning the molecular packings in the active layer, providing guidelines for designing effective morphology m.d.lators for high-performance organic solar cells.

关键词： Trap-assisted charge recombination Photoluminescence miscibility Current leakage Power conversion efficiency

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Subretinal fibrosis secondary to neovascular age-related macular degeneration:mechanisms and potential therapeutic targets

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Neural Regeneration Research 2025年第2期20卷 378-393页

作者： Jingxiang Zhang Xia Sheng Quanju ding Yujun Wang Jiwei zhao Jingfa Zhang department of Ophthalmology People’s Hospital of Huangdao DistrictQingdaoShandong ProvinceChina department of Urology People’s Hospital of Huangdao DistrictQingdaoShandong ProvinceChina department of Ophthalmology Shanghai General Hospital(Shanghai First People’s Hospital)Shanghai Jiao Tong University School of MedicineShanghaiChina National Clinical Research Center for Eye diseases Shanghai Key Laboratory of Ocular Fundus DiseasesShanghai Engineering Center for Visual Science and PhotomedicineShanghai Engineering Center for Precise Diagnosis and Treatment of Eye DiseasesShanghaiChina

Subretinal fibrosis is the end-stage sequelae of neovascular age-related macular *** causes local damage to photoreceptors,retinal pigment epithelium,and choroidal vessels,which leads to permanent central vision loss of patients with neovascular age-related macular *** pathogenesis of subretinal fibrosis is complex,and the underlying mechanisms are largely ***,there are no effective treatment options.A thorough understanding of the pathogenesis of subretinal fibrosis and its related mechanisms is important to elucidate its complications and explore potential *** current article reviews several aspects of subretinal fibrosis,including the current understanding on the relationship between neovascular age-related macular degeneration and subretinal fibrosis;multim.d.l imaging techniques for subretinal fibrosis;animal m.d.ls for studying subretinal fibrosis;cellular and non-cellular constituents of subretinal fibrosis;pathophysiological mechanisms involved in subretinal fibrosis,such as aging,infiltration of macrophages,different sources of mesenchymal transition to myofibroblast,and activation of complement system and immune cells;and several key molecules and signaling pathways participating in the pathogenesis of subretinal fibrosis,such as vascular endothelial growth factor,connective tissue growth factor,fibroblast growth factor 2,platelet-derived growth factor and platelet-derived growth factor receptor-β,transforming growth factor-βsignaling pathway,Wnt signaling pathway,and the axis of heat shock protein 70-Toll-like receptors 2/*** review will improve the understanding of the pathogenesis of subretinal fibrosis,allow the discovery of molecular targets,and explore potential treatments for the management of subretinal fibrosis.

关键词： choroidal neovascularization epithelial-mesenchymal transition mesenchymal transition myofibroblast neovascular age-related macular degeneration submacular fibrosis subretinal fibrosis therapeutic targets transforming growth factor-β vascular endothelial growth factor

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Hydrogen Storage Capacity of C120 Nanocapsules： density Functional Theory Based Treatments

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Communications in Theoretical Physics 2011年第3期55卷 519-526页

作者： m.d. Ganji Gh. Valizadeh m. Jahan-tigh department of Chemistry Islamic Azad University Ghaemshahr Branch Mazandaran Iran

The adsorption of hydrogen molecule on the external surface of pure 0120 nanocapsule and endohedrallyH2 @C120 complex has been examined using the density functional theory calculations. Several different bonding configu- rations are considered for the hydrogen molecule approaching the outer surface of the considered nanocages. It has been found that the adsorbed H2 molecule bound weakly to the outer surface of the pure C1~0 nanocapsules in agreement with the recent experimental and theoretical results while, it prefers to be adsorbed rather strongly on the side wall of the endohedrally /-/2@C120 complex. The adsorption of a single layer and bi-layer of two tt2 molecules on the most stable states of the considered H2@C120 complex appears to be feasible, although the molecules of the second layer are weakly bound. Furthermore, it is found that the formation of 100% coverage is favorable therm.d.namically, which corresponds to about 20% by weight storage of 1-12 molecules. Thus, surprisingly, we arrive at the prediction that the C120 nanocapsules can be implemented as a novel material for energy storage.

关键词： adsorption encapsulation hydrogen storages carbon nanocapsule ab initio calculations

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Notes on the Landmark development of CBR in China

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中国康复医学杂志 2009年第1期24卷 3-4页

作者： dahong Zhuo, m.d. Faculty of Rehabilitation m.d.cine Sun Yat-Sen University WHO Collaborating Centre for Rehabilitation

Community-based rehabilitation has a history of 22 years in *** spite of the preliminary achievement and experiences obtained by the pioneering and trial projects,it was not until the beginning of the new century that CBR in China experienced a landmark *** is characterized by a number of favorable policy by the government for CBR;the mechanism facilitating primary health care with CBR,a new work-force system of CBR reorganized with better motivation and efficiency,99 demonstration projects of CBR bringing about benchmark promotion effect and the active involvement in CBR by social resources agents.

关键词： CBR 中国医疗卫生行业发展历史

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Leader-follower: Human-centered intention-guided controller for novel SuperLimb with application to load-carrying scenarios

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Science China Technological Sciences 2025年第1期 325-338页

作者： Qinghua ZHANG Xianglong LI Hongwei JING Kerui SUN Yuancheng LI Sikai zhao Lele LI Haotian JU Ziqi WANG Rui WU Tianjiao ZHENG Jie zhao Yanhe ZHU The State Key Laboratory of Robotics and System Harbin Institute of Technology The Learning Algorithms and Systems Laboratory School of Engineeringécole Polytechnique Fédérale de Lausanne

Supernumerary robotic arms(SuperLimb) are a new type of wearable robot that works closely with humans as a third hand to augment human operation capability. Accurate conveyance of wearers' intentions, allocation of roles, and humancentered interaction considerations are the key points in the process of human–SuperLimb collaboration. This paper proposes a human-centered intention-guided leader–follower controller that relies on the dynamic m.d.ling of SuperLimb with application to load-carrying scenarios. The proposed leader–follower controller takes the human as the leader and the SuperLimb as the follower, achieving effective information communication, autonomous coordination, and good force compliance between SuperLimb, humans, and the environment under human safety assurance. First, the human–SuperLimb dynamic system is m.d.led to achieve force interaction with the environment and wearer. Second, to achieve the precise intention extraction of humans, pose data from five visual odometry sensors are fused to capture the human state, the generalized position, the velocity of hands, and the surface electromyography signals from two myoelectric bracelets sensors are processed to recognize the natural hand gestures during load-carrying scenarios by a designed Swin transformer network. Then, based on the real-time distance detection between human and mechanical limbs, the security assurance and force-compliant interaction of the human–SuperLimb system are realized. Finally, the human hand muscle intention recognition, human–robot safety strategy verification,and comparative load-carrying experiments with and without the proposed method are conducted on the SuperLimb *** showed that the task parameters are well estimated to produce more reasonable planning trajectories, and SuperLimb could well understand the wearer's intentions to switch different SuperLimb actions. The proposed sensor-based human–robot communication framework motivates future studies of o

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PROPERTIES, WELdABILITY ANd APPLICATIONS OF AdVANCEd WROUGHT SUPERALLOYS FOR GAS TURBINE ENGINES

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Acta metallurgica Sinica(English Letters) 2005年第1期18卷 1-14页

作者： d.L. Klarstrom V.R. Ishwar m.d. Rowe Haynes International Inc. Kokomo Indiana IN 46904-9013 USAHaynes International Inc. Kokomo Indiana IN 46904-9013 USAHaynes International Inc. Kokomo Indiana IN 46904-9013 USA

Alloy selection and alloy design both require consideration of an array of material attributes, including in-service properties, weldability and fabricability. Critical properties of advanced wrought superalloys for gas turbine applications include high temperature strength, thermal stability, oxidation resistance and fatigue resistance. In this paper, the properties of twelve wrought solid-solution-strengthened and six age-hardenable superalloys are compared. Weldability is an important attribute and can be a major limiting factor in the use of certain alloys. Weldability test methods are discussed and the resistance of alloys to solidification cracking and strain-age cracking is compared. The use of weldability testing in the development of m.d.rn wrought su-peralloys is discussed with several examples cited. Finally, alloy selection for gas turbine components is outlined, taking into account both alloy properties and fabricability.

关键词： wrought superalloys mechanical properties strain-age cracking of weldments selection and application of wrought superalloys

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Establishing a new testing protocol of the electrochemical stability window for electric double-layer capacitors

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Science China Chemistry 2025年第01期 217-225页

作者： Ruilin Hou Xiaoxi zhao Tingting Liang Qingyun dou Shan Xu Xingbin Yan School of materials Science and Engineering Sun Yat-sen University Laboratory of Clean Energy Chemistry and materials Lanzhou Institute of Chemical Physics Chinese Academy of Sciences College of Engineering and Applied Sciences Nanjing University Center of Industrial Analysis and Testing Guangdong Academy of Science

The electrochemical stability window(ESW) is crucial for determining the energy density of electric double-layer capacitors(EdLCs). However, current ESW testing protocols of EdLCs are strongly affected by artificial factors, thereby leading to unreliable result. To solve this problem, we first identify the key shortcomings of the traditional protocols by analyzing their test principles. Subsequently, taking an aqueous carbon-based EdLC as an example, we design a side reaction descriptor to represent the response difference in the charging capacitance to side reactions between the cyclic voltammetry and galvanostatic chargedischarge methods. With the aid of this descriptor, we propose a new ESW testing protocol, which is not only able to completely avoid the adverse influence of subjective factors but also fully consider the operating condition limitations. The protocol can be extended from the single electrode to the full device. This work proposes a more rigorous definition of ESW and provides a reliable protocol for evaluating the ESW of EdLCs.

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Lipid droplets in the nervous system:involvement in cell metabolic homeostasis

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Neural Regeneration Research 2025年第3期20卷 740-750页

作者： Yuchen Zhang Yiqing Chen Cheng Zhuang Jingxuan Qi Robert Chunhua zhao Jiao Wang School of Life Sciences Shanghai UniversityShanghaiChina School of m.d.cine Shanghai UniversityShanghaiChina Institute of Basic m.d.cal Sciences Chinese Academy of m.d.cal Sciences School of Basic MedicinePeking Union Medical CollegeBeijingChina Center of Excellence in Tissue Engineering Chinese Academy of Medical SciencesBeijingChina Beijing Key Laboratory of New drug development and Clinical Trial of Stem Cell Therapy BeijingChina

Lipid droplets serve as primary storage organelles for neutral lipids in neurons,glial cells,and other cells in the nervous *** droplet formation begins with the synthesis of neutral lipids in the endoplasmic ***,lipid droplets were recognized for their role in maintaining lipid metabolism and energy homeostasis;however,recent research has shown that lipid droplets are highly adaptive organelles with diverse functions in the nervous *** addition to their role in regulating cell metabolism,lipid droplets play a protective role in various cellular stress ***,lipid droplets exhibit specific functions in neurons and glial *** of lipid droplet formation leads to cellular dysfunction,metabolic abnormalities,and nervous system *** review aims to provide an overview of the role of lipid droplets in the nervous system,covering topics such as biogenesis,cellular specificity,and ***,it will explore the association between lipid droplets and neurodegenerative *** the involvement of lipid droplets in cell metabolic homeostasis related to the nervous system is crucial to determine the underlying causes and in exploring potential therapeutic approaches for these diseases.

关键词： Alzheimer's disease lipid droplet biogenesis lipid droplets lipid metabolism nervous system neurodegenerative disorders oxidative stress Parkinson's disease

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Precise gradient separation of nanoparticles using reduced graphene oxide-polyoxomolybdate membranes

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Science China Chemistry 2025年第01期 209-216页

作者： Yixin Yang Wanlei zhao Ruoxuan Zheng Hongqiang Li Wei Chen Yu-Fei Song State Key Laboratory of Chemical Resource Engineering Beijing University of Chemical Technology Quzhou Institute for Innovation in Resource Chemical Engineering

The purification and size sieving of nanoparticles （NPs） represents a significant scientific ***,the r GO-polyoxometalates (POms=Pmo12,mo132and mo368) membranes were fabricated successfully via a simple and scalable POmsassisted in-situ photoreduction *** the mass ratio of r GO to Pmo12was 1:30,the resultant r GO-Pmo12membranes with highly ordered and uniform nanochannels of 1.0 nm can be obtained,which showed an accurate carbon quantum.d.ts（CQds） separation with a cut-off size approximately 1.0 *** increase of the size of the interlayered POms from Pmo12（1.0 nm）,{mo132}（2.9 nm） to{mo368}（3.8 nm）,the resultant r GO-Pmo12,r GO-mo132and r GO-mo368exhibited precise gradient separation of CQds and Au nanoparticles by size exclusion *** results pave a promising way to construct new twodimensional （2d） membranes for highly efficient size-selective separation.

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Percolation analysis of large-scale wireless balloon networks

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digital Communications and Networks 2019年第2期5卷 84-93页

作者： m.d. Nashid Anjum Honggang Wang Hua Fang University of massachusetts dartmouth 285 Old Westport RdDartmouthMA 02747USA

Recent advancements in wireless technology have tested Wireless Balloon Networks (WBNs) as an ideal solution for the provision of internet facilities in deprived and challenging areas. A few high profile companies, such as Google, Space data Inc., etc., have already m.d. news by initiating projects based on high-altitude WBNs in order to provide internet facilities in remote areas. Unfortunately, the technical details have mainly been kept confidential so far. In this paper, we attempt to analyze the percolation properties of large-scale WBNs, considering both homogenous and heterogenous wireless nodes. In order to do so, we m.d.led a WBN as a large-scale random network where the path-loss m.d.ls of homogenous and heterogenous WBNs were reduced to Gdm (Gilbert's disk m.d.l) and RGdm (Random Gilbert's disk m.d.l), respectively. The bounds of the critical density regime were derived for both percolation m.d.ls. Additionally, this paper implemented an experimental test bed for the WBN percolation m.d.l. Consequently, the findings of this research may prove crucial in estimating critical network properties.

关键词： Percolation Connectivity WBN PPP Gdm

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