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Effects of Interaction between Axial and Radial Secondary Air and Reductive Intensity in Reduction Region on Combustion Characteristics and NO_(x) Emission of Coal Preheated by a Self-Preheating Burner

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Journal of Thermal Science 2024年第1期33卷 249-267页

作者： SU Kun DINg Hongliang OUYANg Ziqu zhang Jinyang zhu Shujun Institute of Engineering Thermophysics Chinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China School of Energy and Power Engineering Jiangsu UniversityZhenjiang 212013China

The study focused on the effects of the interaction between axial and radial secondary air and the reductive intensity in reduction region on combustion characteristics and NO_(x) emission in a 30 kW preheating combustion *** results revealed that the interaction and reductive intensity influenced the combustion in the down-fired combustor(DFC) and NO_(x) emission *** the temperature distribution,the interaction caused the position of the main combustion region to shift down as R_(2-12)(ratio of axial secondary air flow to radial secondary air flow) decreased or λ_(2)(total secondary air ratio) increased,and there was the interplay between both of their *** R_(3-12)(ratio of first-staged tertiary air flow to second-staged tertiary air flow)increased,the decrease in the reductive intensity also caused the above phenomenon,and the peak temperature increased in this *** the NO_(x) emission,the interaction affected the NO_(x) reduction adversely when λ_(2) or R_(2-12) was higher,and the range of this effect was larger,so that the NO_x emission increased obviously as they *** decrease in the reductive intensity caused the NO_(x) emission increased under the homogeneous reduction mechanism,while was unchanged at a high level under the heterogeneous reduction *** the combustion efficiency,the interaction improved the combustion efficiency as λ_(2) increased when R_(2-12) was lower,while reduced it as λ_(2) increased excessively when R_(2-12) was *** proper decrease in the reductive intensity caused the combustion efficiency increased obviously,while was hardly improved further when the intensity decreased *** this study,the lowest NO_(x) emission was only 41.75 mg/m^(3) without sacrificing the combustion efficiency by optimizing the interaction and reductive intensity.

关键词： self-preheating interaction of axial and radial secondary air reductive intensity combustion characteristic NO_(x)emission

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Dissolution behavior of Al_(2)O_(3)inclusions into CaO-MgO-SiO_(2)-Al_(2)O_(3)-TiO_(2)system ladle slags

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International Journal of Minerals,Metallurgy and Materials 2024年第5期31卷 977-987页

作者： Zhiyin Deng Xiaomeng zhang guangyu Hao Chunxin Wei Miaoyong zhu Key Laboratory for Ecological Metallurgy of Multimetallic Mineral(Ministry of Education) Northeastern UniversityShenyang 110819China School of Metallurgy Northeastern UniversityShenyang 110819China TBEA Shenyang Transformer group Co. Ltd.Shenyang 110141China Angang Steel Co. Ltd.Anshan 114021China

To investigate the dissolution behaviors of Al_(2)O_(3)inclusions in CaO-5wt%MgO-SiO_(2)-30wt%Al_(2)O_(3)-TiO_(2)system ladle slags,confocal scanning laser microscopy was conducted on the slags with different TiO_(2)contents(0-10wt%),and scanning electron microscopy was performed to study the interfacial reaction between Al_(2)O_(3)and this slag *** results disclose that the dissolution of Al_(2)O_(3)inclusions does not result in the formation of new phases at the boundary between the slag and the *** TiO_(2)-bearing and TiO_(2)-free ladle slags,there is no difference in the dissolution mechanism of Al_(2)O_(3)inclusions at steelmaking *** layer diffusion is found as the controlling step of the dissolution of Al_(2)O_(3),and the diffusion coefficient is in the range of 4.18×10^(-10)to 2.18×10^(-9)m^(2)/s at 1450-1500℃.Compared with the solubility of Al_(2)O_(3)in the slags,slag viscosity and temperature play a more profound role in the dissolution of Al_(2)O_(3)inclusions.A lower viscosity and a lower melting point of the slags are beneficial for the *** addition of TiO_(2)(e.g.,5wt%)in ladle slags can enhance the dissolution of Al_(2)O_(3)inclusions because of the low viscosity and melting point of the slags,while excessive addition of TiO_(2)(e.g.,10wt%)shows the opposite trend.

关键词： inclusions dissolution ladle refining slag titanium dioxide confocal scanning laser microscopy

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Durable poly(binaphthyl-co-p-terphenyl piperidinium)-based anion exchange membranes with dual side chains

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Journal of Energy Chemistry 2024年第2期89卷 324-335,I0008页

作者： Weiting gao Xuelang gao Qiugen zhang Aimei zhu Qinglin Liu Department of Chemical&Biochemical Engineering Fujian Provincial Key Laboratory of Theoretical and Computational ChemistryThe College of Chemistry and Chemical EngineeringXiamen UniversityXiamen 361005FujianChina Department of Chemistry Pohang University of Science and Technology(POSTECH)Pohang 790-784South Korea

Building well-developed ion-conductive highways is highly desirable for anion exchange membranes(AEMs).grafting side chain is a highly effective approach for constructing a well-defined phaseseparated morphological structure and forming unblocked ion pathways in AEMs for fast ion *** of side chains can further enhance phase separation due to the superhydrophobic nature of fluorine ***,their electronic effect on the alkaline stability of side chains and membranes is rarely ***,fluorine-containing and fluorine-free side chains are introduced into the polyaromatic backbone in proper configuration to investigate the impact of the fluorine terminal group on the stability of the side chains and membrane *** poly(binaphthyl-co-p-terphenyl piperidinium)AEM(QBNp TP)has the highest molecular weight and most dimensional stability due to its favorable backbone arrangement among ortho-and meta-terphenyl based ***,by introducing both a fluorinated piperidinium side chain and a hexane chain into the p-terphenyl-based backbone,the prepared AEM(QBNp TP-QFC)presents an enhanced conductivity(150.6 m S cm^(-1))and a constrained swelling at 80℃.The electronic effect of fluorinated side chains is contemplated by experiments and *** results demonstrate that the presence of strong electro-withdrawing fluorine groups weakens the electronic cloud of adjacent C atoms,increasing OH^(-)attack on the C atom and improving the stability of piperidinium *** QBNp TP-QFC possesses a robust alkaline stability at 80℃(95.3%conductivity retention after testing in 2 M Na OH for 2160 h).An excellent peak power density of 1.44 W cm^(-2)and a remarkable durability at 80℃(4.5%voltage loss after 100 h)can be observed.

关键词： Anion exchange membranes Backbone structure Fluorinated side chain Alkaline stability

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The Role of grain Boundaries in Organic-Inorganic Hybrid Perovskite Solar Cells and its Current Enhancement Strategies:A Review

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Energy & Environmental Materials 2024年第4期7卷 175-204页

作者： Jindan zhang Shicheng Tang Mengqi zhu Zhenghong Li Zhibin Cheng Shengchang Xiang zhangjing zhang College of Chemistry and Materials Science Fujian Key Laboratory of Polymer Materials Fujian Normal University

grain boundaries (gBs) in perovskite polycrystalline films are the most sensitive place for the formation of the defect states and the accumulation of ***,abundant works have been carried out to explore their properti... 详细信息

关键词： additives charge carrier dynamics grain boundaries perovskite solar cells

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Theory of small-scale self-focusing of spatially partially coherent beams and its implications for high-power laser systems

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High Power Laser Science and Engineering 2024年第3期12卷 84-89页

作者： Ruifeng Wang Xiaoqi zhang Yanli zhang Fanglun Yang Jianhao Tang Ziang Chen Jianqiang zhu Key Laboratory of High Power Laser and Physics Shanghai Institute of Optics and Fine MechanicsChinese Academy of SciencesShanghaiChina Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijingChina

Based on the paraxial wave equation,this study extends the theory of small-scale self-focusing(SSSF)from coherent beams to spatially partially coherent beams(PCBs)and derives a general theoretical equation that reveals the underlying physics of the reduction in the B-integral of spatially *** the analysis of the simulations,the formula for the modulational instability(MI)gain coefficient of the SSSF of spatially PCBs is obtained by introducing a decrease factor into the formula of the MI gain coefficient of the SSSF of coherent *** decrease can be equated to a drop in the injected light intensity or an increase in the critical *** to this formula,the reference value of the spatial coherence of spatially PCBs is given,offering guidance to overcome the output power limitation of the high-power laser driver due to SSSF.

关键词： B-integral complex screen method nonlinearity small-scale self-focusing spatially partially coherent beams

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Improving mechanical properties and high-temperature oxidation of press hardened steel by adding Cr and Si

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International Journal of Minerals,Metallurgy and Materials 2024年第8期31卷 1865-1875页

作者： Rong zhu Yonggang Yang Baozhong zhang Borui zhang Lei Li Yanxin Wu Zhenli Mi National Engineering Research Center for Advanced Rolling and Intelligent Manufacturing University of Science and Technology BeijingBeijing 102206China Manufacturing Management Department Ningbo Iron&Steel Co.Ltd.Ningbo 315800China Hunan Valin Lianyuan Iron and Steel Co. Ltd.Loudi 417009China

This work investigated the effect of Cr and Si on the mechanical properties and oxidation resistance of press hardened *** indicated that the microstructure of the Cr-Si micro-alloyed press hardened steel consisted of lath martensite,M_(23)C_(6)carbides,and retained *** retained austenite and carbides are responsible for the increase in elongation of the micro-alloyed *** addition,after oxidation at 930℃for 5 min,the thickness of the oxide scales on the Cr-Si micro-alloyed press hardened steel is less than 5μm,much thinner than 45.50μm-thick oxide scales on *** oxide scales of the Cr-Si micro-alloyed steel are composed of Fe_(2)O_(3),Fe_(3)O_(4),mixed spinel oxide(FeCr_(2)O_(4)and Fe_(2)SiO_(4)),and amorphous SiO_(2).Adding Cr and Si significantly reduces the thickness of the oxide scales and prevents the generation of the FeO *** to the increase of spinel FeCr_(2)O_(4)and Fe_(2)SiO_(4)phase in the inner oxide scale and the amorphous SiO_(2)close to the substrate,the oxidation resistance of the Cr-Si micro-alloyed press hardened steel is improved.

关键词： Cr-Si micro-alloyed press hardened steel mechanical properties oxidation resistance amorphous SiO_(2)

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In^(3+)-doped Sr_(2)Fe_(1.5)Mo_(0.5)O_(6−δ)cathode with improved performance for an intermediate-temperature solid oxide fuel cell

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Nano Research 2024年第1期17卷 407-415页

作者： Yumei Ma Lijie zhang Kang zhu Binze zhang Ranran Peng Changrong Xia Ling Huang State Key Laboratory of Chemistry and Utilization of Carbon Based Energy Resources College of ChemistryXinjiang UniversityUrumqi 830046China Department of Materials Science and Engineering University of Science and Technology of ChinaHefei 230026China

Promoting the oxygen reduction reaction(ORR)is critical for commercialization of intermediate-temperature solid oxide fuel cells(IT-SOFCs),where Sr_(2)Fe_(1.5)Mo_(0.5)O_(6)−δ(SFM)is a promising cathode by working as a mixed ionic and electronic *** this work,dopi.g of In^(3+)greatly increases the oxygen vacancy concentration and the content of adsorbed oxygen species in Sr_(2)Fe_(1.5)Mo_(0.5−x)InxO_(6−δ)(SFMInx),and thus effectively promotes the ORR *** a typical example,SFMIn_(0.1)reduces the polarization resistance(R_(p))from 0.089 to 0.046Ω∙cm^(2)at 800°C,which is superior to those doped with other metal *** addition,SFMIn0.1 increases the peak power density from 0.92 to 1.47 W∙cm^(−2)at 800°C with humidified H_(2)as the fuel,indicating that In3+dopi.g at the Mo site can effectively improve the performance of SOFC cathode material.

关键词： solid oxide fuel cell cathode In3+dopi.g oxygen reduction reaction(ORR) Sr_(2)Fe_(1.5)Mo_(0.5)O_(6-δ)

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An efficient CuZr-based metallic glasses electrode material for electrocatalytic degradation of azo dyes

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Journal of Environmental Sciences 2024年第2期136卷 537-546页

作者： Zhiwang Deng Bowen Zhao Songtao Li Zhengkun Li Shiming zhang Kewei zhang Zhengwang zhu Taiyuan University of Science and Technology School of materials science and engineeringTaiyuan 030024China Shi-changxu Innovation Center for Advanced Materials Institute of Metal ResearchChinese Academy of SciencesShenyang 110016China Chinese Academy of Sciences Key Laboratory of Nuclear Materials and Safety Assessment Institute of Metal ResearchChinese Academy of SciencesShenyang 110016China Qingdao Yunlu Advanced Materials Technology Co. Ltd.Qingdao 266232China

Metallic glasses have received a lot of attention on wastewater treatment due to their unique atomic structure,and the use of metallic glasses as electrodes has produced unexpected electrocatalytic degradation effects for many pollutants through combining with electrochemical ***,it still is a formidable challenge to find a metallic glass electrode material with both efficient and clean for the catalytic degradation of *** this work,the Cu_(55)Zr_(45)metallic glassy ribbons are used as an electrode to degrade azo dyes and show the excellent degradation effect,which can reach 95.6%within 40 *** the degradation process,almost no additives are produced and Cu_(55)Zr_(45)metallic glassy ribbons have excellent effects under different pH ***,it exhibits good stability for degradation efficiency during the 8 cycle degradation tests of the amorphous alloy *** the copper nanoparticles are exposed on the surface of the ribbons,the oxidized copper obtained synergistically produce activated radicals is the primary degradation mechanism,where the auxiliary degradation mechanisms include electron transfer and the promotion of active *** research develops a new type of electrode material for wastewater treatment,and the economy and high efficiency of Cu55Zr45metallic glass endow it the expandable functional applications.

关键词： Metallic glasses Azo dyes Electrocatalytic Degradation Oxidized copper

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Transient synthesis of carbon-supported high-entropy alloy sulfide nanoparticles via flash Joule heating for efficient electrocatalytic hydrogen evolution

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Nano Research 2024年第4期17卷 3379-3389页

作者： Yuntian Liao Rongtao zhu Wenjun zhang Haiyang zhu Yang Sun Jiale Chen Zhenhua Dong Ronghuan Lv School of Chemical Engineering and Technology China University of Mining and TechnologyXuzhou 221116China

High entropy alloys(HEA)are frequently employed as catalysts in electrocatalytic hydrogen ***,the traditional high entropy alloy synthesis methods are time-consuming,energy-intensive,and environmentally polluting,which limits their application in the hydrogen evolution reaction(HER).This study leveraged the capabilities of flash Joule heating(FJH)to synthesize carbon-supported high-entropy alloy sulfide nanoparticles(CC-S-HEA)on carbon cloth(CC)with good self-standing properties within 300 *** carbon thermal shock generated by the Joule heating could pyrolyze the sulfur source into gas,resulting in numerous pore structures and defects on CC,forming an S-doped carbon substrate(CC-S).Then the S atoms were used to stably anchor the metal atoms on CC-S to form high-density uniformly dispersed HEA *** electrochemical test results demonstrated that CC-S-HEA prepared at 60 V flash voltage had HER performance comparable to Pt/*** density functional theory(DFT)calculation indicated that the S atoms on CC-S accelerated the electron transfer between the carbon substrate and HEA ***,the unique electronic structure of CC-S-HEA was beneficial to H*adsorption and promoted catalytic *** simplicity and versatility of FJH synthesis are of great significance for optimizing the synthesis of HEA and improving the quality of HEA products,which provides a broad application prospect for the synthesis of nanocatalysts with efficient HER performance.

关键词： high entropy alloy flash Joule heating carbon thermal shock hydrogen evolution reaction density functional theory

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Achievable hole concentration at room temperature as a function of Mg concentration for MOCVD-grown p-gaN after sufficient annealing

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Journal of Semiconductors 2024年第8期45卷 67-73页

作者： Siyi Huang Masao Ikeda Feng zhang Minglong zhang Jianjun zhu Shuming zhang Jianpi.g Liu School of Nano-Tech and Nano-Bionics University of Science and Technology of ChinaHefei 230026China Suzhou Institute of Nano-Tech and Nano-Bionics Chinese Academy of SciencesSuzhou 215123China Key Laboratory of Nanodevices and Applications Chinese Academy of SciencesSuzhou 215123China

Relationship between the hole concentration at room temperature and the Mg dopi.g concentration in p-gaN grown by MOCVD after sufficient annealing was studied in this *** annealing conditions were applied to obtain sufficient activation for p-gaN samples with different Mg dopi.g *** concentration,resistivity and mobility were characterized by room-temperature Hall *** Mg dopi.g concentration and the residual impurities such as H,C,O and Si were measured by secondary ion mass spectroscopy,confirming negligible compensations by the *** hole concentration,resistivity and mobility data are presented as a function of Mg concentration,and are compared with literature *** appropriate curve relating the Mg dopi.g concentration to the hole concentration is derived using a charge neutrality equation and the ionized-acceptor-density[N-(A)^(-)](cm^(−3))dependent ionization energy of Mg acceptor was determined asE_(A)^(Mg)=184−2.66×10^(−5)×[N_(A)^(-)]1/3 meV.

关键词： p-gaN hole concentration electrical properties annealing ionization energy

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