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Science China(Life Sciences) 2024年第8期67卷 1769-1771页

作者： tao liu Jutao He Chang Xiao jie liu jie Sun Minling Li Yuanhua Hong Weiwei zhang Fuwen Wei Jiangxi Provincial Key Laboratory of Conservation Biology Jiangxi Agricultural UniversityNanchang 330045China Forestry Bureau of Wuyuan Shangrao 333299China

Dear Editor,Population size is a crucial indicator in evaluating the conservation status of a *** the patterns of population fluctuation and the distribution range of endangered species is important for biodiversity c... 详细信息

关键词： Population crown dynamics

Construction of RuO2-Ru/MoO2@carbon cloth bifunctional electrocatalyst for efficient overall water splitting

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Rare Metals 2024年第10期43卷 5095-5104页

作者： Jia-Lin cai Jing-Yi Fan Xu-Dong zhang Xin Xie Wan-Yu Tian Xin-Gang zhang jie Ding Yu-Shan liu College of Material Henan Key Laboratory of Aeronautical Materials and Application TechnologyZhengzhou University of Aeronautics The Green Catalysis Center and College of ChemistryZhengzhou University

Efficient bifunction electrocatalyst is extremely interesting for electrochemical overall water splitting （OWS）.Herein,a new RuO2-Ru/MoO2@CC（RRM/CC） bifunctional electrocatalyst was prepared via a solid phase reaction *** obtain a suitable precursor for SPR,MoS2nanosheets and RuO2nanoparticles （NPs）were sequentially loaded onto carbon cloth conductive ***,the prepared RuO2/MoS2/CC precursor was sealed in a furnace and annealed in Ar to trigger the redox *** SPR,active RuO2-Ru/MoO2units containing metal–metal oxide interfaces were formed on CC substrate *** optimized RRM/CC sample annealed at 400℃ exhibited a overpotential of 13 m V for hydrogen evolution reaction （HER） and 231 mV for oxygen evolution reaction （OER） at 10 mA·cm-2under alkaline condition,respectively,which can be deduced to the modulated electronic structure and unique hierarchica *** addition,a low cell voltage of 1.48 V for OWS was required at 10 mA·cm-2under alkaline condition Meanwhile,RRM/CC exhibited excellent pH-independent durability.

关键词： Bifunctional Electrocatalyst Overall water splitting Ru RuO2

The lactylation index predicts the immune microenvironment and prognosis of pan-cancer patients

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BIOCELL 2024年第8期48卷 1223-1239页

作者： XUEJIA ZHAI jie liu JINWEI XIAO tao zhang JUN WANG JIANJUN LI SHICANG YU Department of Oncology Southwest HospitalThird Military Medical University(Army Medical University)Chongqing400038China Department of Stem Cell and Regenerative Medicine Institute of Pathology and Southwest Cancer CenterSouthwest HospitalThird Military Medical University(Army Medical University)Chongqing400038China Key Laboratory of Cancer Immunopathology Ministry of EducationChongqing400038China International Joint Research Center for Precision Biotherapy Ministry of Science and TechnologyChongqing400038China Jin-feng Laboratory Chongqing401329China

Background:Protein lactylation is a new way for the“metabolic waste”lactic acid to perform novel ***,our understanding of the contribution of protein lactylation to both tumor progression and therapeutic interventions remains *** construction of a scoring system for lactylation to predict the prognosis of pancancer patients and to evaluate the tumor immune microenvironment(TIME)would improve our understanding of the clinical significance of ***:Consensus clustering analysis of lactylation-related genes was used to cluster 177 pancreatic adenocarcinoma(PAAD)***,a scoring system was developed using the least absolute shrinkage and selection operator(LASSO)*** validation and external validation were both conducted to assess and confirm the predictive accuracy of the scoring ***,leucine rich repeat containing 1(LRRC1),a newly discovered lactylation-related gene,was analyzed in PAAD in ***:Utilizing the profiles of 332 lactylation-related genes,a total of 177 patients with PAAD were segregated into two distinct ***^(high) patients had a poorer prognosis than LacCluster^(low) *** the differential analysis between the LacCluster^(high) and LacCluster^(low) groups,we identified additional genes associated with *** genes were then integrated to construct the LacCluster-enhanced system,which enabled more accurate prognosis prediction for patients with ***,a lactylation index containing three genes(LacI-3)was constructed using LASSO *** was done to enhance the usability of the LacCluster-enhanced system in the *** to those in the LacI-3^(high) subgroup,patients in the LacI-3^(low) subgroup exhibited increased expression of immune checkpoint-related genes,more immune cell infiltration,lower tumor mutation burdens,and better prognoses,indicating a“hot tumor”***,knocking down the expression of LRRC1,

关键词： Pancreatic adenocarcinoma Pan-cancer Lactylation Prognosis Tumor immune microenvironment LRRC1

White matter disease derived from vascular and demyelinating origins

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Stroke & Vascular Neurology 2024年第4期9卷 344-350页

作者： Lin-jie zhang De-cai Tian Li Yang Kaibin Shi Yaou liu Yilong Wang Fu-Dong Shi Department of Neurology Tianjin Medical University General HospitalTianjinTianjinChina National Clinical Research Center for Neurological Diseases of China Beijing Tiantan HospitalCapital Medical UniversityBeijingBeijingChina

Damage or microstructural alterations of the white matter can cause dysfunction of the intrinsic neural networks in a condition termed as white matter disease(WMD).Frequently detected on brain computed tomography and magnetic resonance imaging scans,WMD is commonly presented in inflammatory demyelinating diseases like multiple sclerosis(MS)and vascular diseases such as cerebral small vessel disease(CSVD).Prevention of MS and CSVD progression requires early treatments with drastically different medications and approaches,as such,early and accurate diagnosis of WMD,derived from vascular or demyelinating etiologies,is of paramount ***,the clinical and imaging similarities between MS,especially during the early stage,and CSVD,pose a significant dilemma in differentiating these two *** this review,we attempt to summarize and contrast the distinguishing features of MS and CSVD for aiding accurate diagnosis to ensure timely corresponding management in the early stages of MS and CSVD.

关键词： diagnosis myelin alterations

Nd^(3)+:YAG-Al_(2)O_(3) nanocrystalline transparent ceramics with high inflexion concentration quenching of Nd^(3+) prepared by amorphous crystallization

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Journal of Advanced Ceramics 2024年第8期13卷 1242-1253页

作者： Xiujuan Wan Guangfan Tan Liang cai jie Fu Jianqiang Li Yingchun zhang School of Materials Science and Engineering University of Science and Technology BeijingBeijing 100083China State Key Laboratory of New Ceramics and Fine Processing School of Materials Science and EngineeringTsinghua UniversityBeijing 100080China State Key Lab for Mesoscience and Engineering Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China

Rare earth ion-doped Y_(3)Al_(5)O_(12)(YAG)-based transparent ceramics have been used as important laser gain media for a long time,yet the doping concentration of active ions is limited due to concentration quenching,wherein the inflexion concentration quenching of Nd^(3+)is recognized as 1.0 at%.In this work,YAG-Al_(2)O_(3) nanocrystalline transparent ceramics with a concentration of Nd^(3+)(O-5.0 at%)were fabricated via amorphous crystallization,and the crystal structure evolution,morphology,and optical properties were systematically investigated by differential scanning calorimetry(DSC),X-ray powder diffraction(XRD),transmission electron microscopy(TEM),magnetic resonation(MAS),nuclear magnetic resonation(NMR),and fluorescence *** doping of Nd^(3+)can promote the transition of Al[5]and Al[6]to Al[14],indicating improvements in the ability of the amorphous material to form Nd^(3+):Y_(2)O_(3)-Al_(2)O_(3) vitrified beads,and 1.5 at%Nd^(3+):YAG-Al_(2)O_(3) nanocrystalline transparent ceramics can be obtained by crystallization at 1050℃ with a matrix composed of YAG and concomitant δ-Al_(2)O_(3) and θ-Al_(2)O_(3).The nanocrystalline transparent ceramics show an internal transmitance of 89.56%at 1064 nm,and the strongest emission peak corresponds to the energy transfer from 4F_(3/2) to 4l_(11/2) of Nd^(3+)with a fluorescence lifetime of 231μs when pumped by an 808 nm ***,spectral broadening begins to occur,indicating the onset of concentration quenching,when the concentration of Nd^(3+)exceeds 1.5 at%,substantially higher than the 1.0 at% observed in YAG ***-Al_(2)O_(3) nanocrystalline transparent ceramics obtained by amorphous crystalization can be utilized as the matrix to increase the inflexion point of doping concentration quenching of Nd^(3+),and this material may have great potential as a laser gain medium.

关键词： Y_(3)Al_(5)O_(12)(YAG)-Al_(2)O_(3) nanocrystalline transparent ceramics laser gain medium Nd^(3+)

Cardiac-Adaptive Conductive Hydrogel Patch Enabling Construction of Mechanical–Electrical Anisotropic Microenvironment for Heart Repair

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Research 2024年第1期2023卷 489-507页

作者： Xiaoping Song Jifeng zhang Si Shen Dan liu jie zhang Wenming Yin Genlan Ye Leyu Wang liu cai Honghao Hou Xiaozhong Qiu Central Laboratory The Fifth Affiliated HospitalSouthern Medical UniversityGuangzhouGuangdong 510910China Department of Anatomy Neuroscience Laboratory for Cognitive and Developmental DisordersMedical College of Jinan UniversityGuangzhou 510630China Guangdong Provincial Key Laboratory of Construction and Detection in Tissue Engineering School of Basic Medical ScienceBiomaterials Research CenterSchool of Biomedical EngineeringSouthern Medical UniversityGuangzhouGuangdong 510515China

The biomimetic construction of a microstructural–mechanical–electrical anisotropic microenvironment adaptive to the native cardiac tissue is essential to repair myocardial infarction(MI).Inspired by the 3D anisotropic characteristic of the natural fish swim bladder(FSB),a novel flexible,anisotropic,and conductive hydrogel was developed for tissue-specific adaptation to the anisotropic structural,conductive,and mechanical features of the native cardiac extracellular *** results revealed that the originally stiff,homogeneous FSB film was tailored to a highly flexible anisotropic hydrogel,enabling its potential as a functional engineered cardiac patch(ECP).In vitro and in vivo experiments demonstrated the enhanced electrophysiological activity,maturation,elongation,and orientation of cardiomyocytes(CMs),and marked MI repair performance with reduced CM apoptosis and myocardial fibrosis,thereby promoting cell retention,myogenesis,and vascularization,as well as improving electrical *** findings offer a potential strategy for functional ECP and provides a novel strategy to bionically simulate the complex cardiac repair environment.

关键词： bladder thereby patch

Interface optimization of graphene paper-Cu composite prepared by electrodeposition

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Journal of Iron and Steel Research International 2024年第1期31卷 64-73页

作者： Jing Guo Hai-jing Wang Shuang-juan liu Peng zhang Jing-yu Tang Wei-yang zhang Han-jie Guo Peng-cheng Wang cai Meng School of Metallurgical and Ecological Engineering University of Science and Technology BeijingBeijing100083China Institute of High Energy Physics Chinese Academy of SciencesBeijing100049China Advanced Technology and Materials Co. Ltd.Beijing100083China School of Nuclear Science and Technology University of Science and Technology of ChinaHefei230027AnhuiChina

A room-temperature electrodeposition method with an organic electrolyte was developed to fabricate a HNO3-pretreated graphene paper Cu(GP'-Cu)*** improve the interfacial bonding of GP'-Cu composite,magnetron sputtering technology was used to create a"sandwich"structural gradient GP'-Cu *** selection of the intermediate transition layer metal was based on two-dimensional *** electron microscopy,X-ray photoelectron spectroscopy,and other analytical methods confirmed that the addition of an intermediate transition metal(Cr,Ni)layer reduced the gap distance and enhanced the interfacial bonding of the GP'and Cu deposited *** GP'-Ni-Cu composite exhibited the largest increase in tensile strength and *** addition,it had the highest thermal diffusivity and elongation at break among the GP'-Cu,GP'-Cr-Cu and GP'-Ni-Cu composites.

关键词： Graphene paper Two-dimensional disregistry Magnetron sputtering Metal composite

From Digital Human Modeling to Human Digital Twin: Framework and Perspectives in Human Factors

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Chinese Journal of Mechanical Engineering 2024年第1期37卷 1-14页

作者： Qiqi He Li Li Dai Li tao Peng Xiangying zhang Yincheng cai Xujun zhang Renzhong Tang State Key Laboratory of Fluid Power Components and Mechatronic Systems Zhejiang UniversityHangzhou 310027China ZJU-Sunon Joint Research Center for Smart Furniture Zhejiang UniversityHangzhou 310027China PICO-Lab Bytedance Inc.Shanghai 200233China Sunon Technology Co. Ltd.Hangzhou 311215China

The human digital twin(HDT)emerges as a promising human-centric technology in Industry 5.0,but challenges remain in human modeling and *** human modeling(DHM)provides solutions for modeling and simulating human physical and cognitive aspects to support ergonomic ***,it has limitations in real-time data usage,personalized services,and timely *** emerging HDT concept offers new possibilities by integrating multi-source data and artificial intelligence for continuous monitoring and ***,this paper reviews the evolution from DHM to HDT and proposes a unified HDT framework from a human factors *** framework comprises the physical twin,the virtual twin,and the linkage between these *** virtual twin integrates human modeling and AI engines to enable model-data-hybrid-enabled *** can potentially upgrade traditional ergonomic methods to intelligent services through real-time analysis,timely feedback,and bidirectional ***,the future perspectives of HDT for industrial applications as well as technical and social challenges are *** general,this study outlines a human factors perspective on HDT for the first time,which is useful for cross-disciplinary research and human factors innovation to enhance the development of HDT in industry.

关键词： Human digital twin Digital human modeling Human factors Human-centric technology

Enhancing layered perovskite ferrites with ultra-high-density nanoparticles via cobalt doping for ceramic fuel cell anode

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Journal of Energy Chemistry 2024年第9期96卷 39-48页

作者： Shuo Zhai Rubao Zhao Hailong Liao Ling Fu Senran Hao Junyu cai Yifan Wu Jian Wang Yunhong Jiang jie Xiao tao liu Heping Xie State Key Laboratory of Intelligent Construction and Healthy Operation and Maintenance of Deep Underground Engineering Shenzhen University&Sichuan UniversityShenzhen 518060GuangdongChina National and Local Joint Engineering Research Center for Lithium-ion Batteries and Materials Preparation Technology Key Laboratory of Advanced Battery Materials of Yunnan ProvinceFaculty of Metallurgical and Energy EngineeringKunming University of Science and TechnologyKunming 650093YunnanChina School of Energy and Environment City University of Hong KongKowloon 999077Hong KongChina

Nanoparticles anchored on the perovskite surface have gained considerable attention for their wide-ranging applications in heterogeneous catalysis and energy conversion due to their robust and integrated structural ***,we employ controlled Co doping to effectively enhance the nanoparticle exsolution process in layered perovskite ferrites *** alloy nanoparticles with ultra-high-density are exsolved on the(PrBa)_(0.95)(Fe_(0.8)Co_(0.1)Nb_(0.1))2O_(5+δ)(PBFCN_(0.1))surface under reducing atmosphere,providing significant amounts of reaction sites and good durability for hydrocarbon *** a reducing atmosphere,cobalt facilitates the reduction of iron cations within PBFCN_(0.1),leading to the formation of CoFe alloy *** formation is accompanied by a cation exchange process,wherein,with the increase in temperature,partial cobalt ions are substituted by ***,Co doping significantly enhance the electrical conductivity due to the stronger covalency of the Cosingle bondO bond compared with Fesingle bondO bond.A single cell with the configuration of PBFCN_(0.1)-Sm_(0.2)Ce_(0.8)O_(1.9)(SDC)|SDC|Ba_(0.5)Sr_(0.5)Co_(0.8)Fe_(0.2)O_(3−δ)(BSCF)-SDC achieves an extremely low polarization resistance of 0.0163Ωcm^(2)and a high peak power density of 740 mW cm^(−2)at 800℃.The cell also shows stable operation for 120 h in H_(2)with a constant current density of 285 mA cm^(−2).Furthermore,employing wet C_(2)H_(6)as fuel,the cell demonstrates remarkable performance,achieving peak power densities of 455 mW cm^(−2)at 800℃and 320 mW cm^(−2)at 750℃,marking improvements of 36%and 70%over the cell with(PrBa)_(0.95)(Fe_(0.9)Nb_(0.1))_(2)O_(5+δ)(PBFN)-SDC at these respective *** discovery emphasizes how temperature influences alloy nanoparticles exsolution within doped layered perovskite ferrites materials,paving the way for the development of high-performance ceramic fuel cell anodes.

关键词： Solid oxide fuel cell Anode Ethane fuel Nanoparticle Exsolution Layered perovskite Ferrites

Evaluating two stages of silicone-containing arylene resin oxidation via experiment and molecular simulation

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Chinese Journal of Chemical Engineering 2024年第2期66卷 189-202页

作者： Jiangtao cai Qingfu Huang Huan Chen tao zhang Bo Niu Yayun zhang Donghui Long Key Laboratory of Chemical Engineering East China University of Science and TechnologyShanghai 200237China Key Laboratory of Special Functional Polymeric Materials and Related Technology(Ministry of Education) School of Chemical EngineeringEast China University of Science and TechnologyShanghai 200237China

Silicon-containing aryl acetylene resin(PSA)is a new type of high-temperature resistant resin with excellent oxidation resistance,whereas antioxidant reaction mechanism of PSA resin under ultra-high temperatures still remains ***,the oxidation behavior and mechanisms of PSA resin are systematically investigated combining kinetic analysis and Reax FF molecular dynamics(MD)*** analysis indicates that the oxidation process of PSA resin undergoes two main steps:oxidative mass gain and oxidative *** distributed activation energy model(DAEM)is employed for describing oxidation processes and the best-fit one is obtained using genetic algorithms and differential *** model demonstrates that the oxidative weight gain stage is dominated by two virtual reactants and the oxidative degradation stage consists of three virtual ***,the observation of MD reaction pathways indicates that oxygen oxidation of unsaturated structures occurs in the initial stage,which results in the formation of PSA resin ***,cracked pieces react with O_(2)to generate CO and other chemicals in the second *** resin matrix's great antioxidation resilience is illustrated by the formation of SiO_(2).The analysis based on MD simulations exhibits an efficient computational proof with the experiments and DAEM *** on the results,a two-stage reaction mechanism is proposed,which provides important theoretical support for the subsequent study of the oxidation behavior of silica-based resins.

关键词： PSA resin Oxidative degradation Thermogravimetric analysis DAEM reaction kinetics ReaxFF simulation