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A healable, mechanically robust and ultrastretchable ionic conductive elastomer for durably wearable sensor

Nano Research 2024年第4期17卷 3369-3378页

作者： Guoxian zhang Chunmei Li JiaoJun Tan Mingqi Wang yafeng Ren Feijie Ge Qiuyu zhang Key Laboratory of Special Functional and Smart Polymer Materials of Ministry of Industry and Information Technology School of Chemistry and Chemical EngineeringNorthwestern Polytechnical UniversityXi'an 710072China College of Bioresources Chemical and Materials Engineering National Demonstration Center for Experimental Light Chemistry Engineering EducationShaanxi University of Science&TechnologyXi’an 710021China

The ionic conductive elastomers show great promise in multifunctional wearable electronics,but they currently suffer from liquid leakage/evaporation or mechanical compliance.Developing ionic conductive elastomers integrating non-volatility,mechanical robustness,superior ionic conductivity,and ultra-stretchability remains urgent and challenging.Here,we developed a healable,robust,and conductive elastomer via impregnating free ionic liquids(ILs)into the ILs-multigrafted poly(urethane-urea)(PUU)elastomer networks.A crucial strategy in the molecular design is that imidazolium cations are largely introduced by double-modification of PUU and centipede-like structures are obtained,which can lock the impregnated ILs through strong ionic interactions.In this system,the PUU matrix contributes outstanding mechanical properties,while the hydrogen bonds and ionic interactions endow the elastomer with self-healing ability,conductivity,as well as non-volatility and transparency.The fabricated ionic conductive elastomers show good conductivity(3.8×10^(-6) S·cm^(-1)),high mechanical properties,including tensile stress(4.64 MPa),elongation(1470%),and excellent healing ability(repairing efficiency of 90%after healing at room temperature for 12 h).Significantly,the conductive elastomers have excellent antifatigue properties,and demonstrate a highly reproducible response after 1000 uninterrupted extension-release cycles.This work provides a promising strategy to prepare ionic conductive elastomers with excellent mechanical properties and stable sensing capacity,and further promote the development of mechanically adaptable intelligent sensors.

关键词： ionic conductive elastomers poly(urethane-urea)(PUU) ionic interactions centipede-like self-healing

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Tribological Behaviors of Electroless Nickel-Boron Coating on Titanium Alloy Surface

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Chinese Journal of Mechanical Engineering 2024年第1期37卷 309-320页

作者： Yao Jia Jianping Lai Jiaxin Yu Huimin Qi yafeng zhang Hongtu He Key Laboratory of Testing Technology for Manufacturing Process in Ministry of Education State Key Laboratory of Environment-Friendly Energy MaterialsSouthwest University of Science and TechnologyMianyang 621010China

Titanium alloys are excellent structural materials in engineering fields,but their poor tribological properties limit their further applications.Electroless plating is an effective method to enhance the tribological performance of alloys,but it is difficult to efficiently apply to titanium alloys,due to titanium alloy’s strong chemical activity.In this work,the electroless Nickel-Boron(Ni-B)coating was successfully deposited on the surface of titanium alloy(Ti-6AL-4V)via a new pre-treatment process.Then,linearly reciprocating sliding wear tests were performed to evaluate the tribological behaviors of titanium alloy and its electroless Ni-B coatings.It was found that the Ni-B coatings can decrease the wear rate of the titanium alloy from 19.89×10^(−3)mm^(3)to 0.41×10^(−3)mm^(3),which attributes to the much higher hardness of Ni-B coatings.After heat treatment,the hardness of Ni-B coating further increases corresponding to coating crystallization and hard phase formation.However,heat treatment does not improve the tribological performance of Ni-B coating,due to the fact that higher brittleness and more severe oxidative wear exacerbate the damage of heat-treated coatings.Furthermore,the Ni-B coatings heat-treated both in air and nitrogen almost present the same tribological performance.The finding of this work on electroless coating would further extend the practical applications of titanium alloys in the engineering fields.

关键词： Electroless coating Titanium alloy Tribology Wear Heat treatment Nanoindentation

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End-group modulation of phenazine based non-fullerene acceptors for efficient organic solar cells with high open-circuit voltage

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Journal of Energy Chemistry 2024年第1期88卷 461-468,I0011页

作者： Yahui zhang yafeng Li Ruixiang Peng Yi Qiu Jingyu Shi Zhenyu Chen Jinfeng Ge Cuifen zhang Zheng Tang Ziyi Ge School of Materials Science and Engineering Shanghai UniversityShanghai 200444China Zhejiang Business Technology Institute Ningbo 315012ZhejiangChina Zhejiang Provincial Engineering Research Center of Energy Optoelectronic Materials and Devices Ningbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingbo 315201ZhejiangChina Center for Advanced Low-dimension Materials College of Materials Science and EngineeringDonghua UniversityShanghai 201620China

Phenazine-based non-fullerene acceptors(NFAs)have demonstrated great potential in improving the power conversion efficiency(PCE)of organic solar cells(OSCs).Halogenation is known to be an effective strategy for increasing optical absorption,refining energy levels,and improving molecular packing in organic semiconductors.Herein,a series of NFAs(Pz IC-4H,Pz IC-4F,Pz IC-4Cl,Pz IC-2Br)with phenazine as the central core and with/without halogen-substituted(dicyanomethylidene)-indan-1-one(IC)as the electron-accepting end group were synthesized,and the effect of end group matched phenazine central unit on the photovoltaic performance was systematically studied.Synergetic photophysical and morphological analyses revealed that the PM6:Pz IC-4F blend involves efficient exciton dissociation,higher charge collection and transfer rates,better crystallinity,and optimal phase separation.Therefore,OSCs based on PM6:Pz IC-4F as the active layer exhibited a PCE of 16.48%with an open circuit voltage(Voc)and energy loss of 0.880 V and 0.53 e V,respectively.Accordingly,this work demonstrated a promising approach by designing phenazine-based NFAs for achieving high-performance OSCs.

关键词： Organic solar cells Non-fullerene acceptor Phenazine Central core End group

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Nutrient enrichment driven by canopy rainfall redistribution:Mechanism,quantification,and pattern

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Science China Earth Sciences 2024年第5期67卷 1529-1544页

作者： Chuan YUAN Xiaoping YUE yafeng zhang Yu zhang Yanting HU Qiang TANG Li GUO Shuai WANG Xingwu DUAN Wenhua XIANG Xiaohua WEI Xiaoyan LI College of Forestry and Biotechnology Zhejiang A&F UniversityHangzhou 311300China Chongqing Jinfo Mountain Karst Ecosystem National Observation and Research Station School of Geographical SciencesSouthwest UniversityChongqing 400715China Shapotou Desert Research and Experiment Station Northwest Institute of Eco-Environment and ResourcesChinese Academy of SciencesLanzhou 730000China School of Geographical Sciences Hebei Normal UniversityShijiazhuang 050024China Faculty of Life Science and Technology Central South University of Forestry and TechnologyChangsha 410004China State Key Laboratory of Hydraulics and Mountain River Engineering College of Water Resource and HydropowerSichuan UniversityChengdu 610065China State Key Laboratory of Earth Surface Processes and Resource Ecology Faculty of Geographical ScienceBeijing Normal UniversityBeijing 100875China Yunnan Key Laboratory of Soil Erosion Prevention and Green Development Institute of International Rivers and Eco-securityYunnan UniversityKunming 650091China Department of Earth Environmental and Geographic SciencesUniversity of British Columbia(Okanagan)KelownaBritish Columbia V1V 1V7Canada

Vegetation canopies intercept and redistribute rainfall into throughfall and stemflow,which transfer substantial amounts of elements into the soil,influencing soil microbial community,plant survival,and plant community succession.Despite advancements in ecohydrological research,the implication of nutrient enrichment resulting from this redistribution of rainfall by canopies remains largely unexplored.To address this gap,we conducted a systematic review of 1020 papers published between 2000 and 2022,gathering data on nutrient concentration and enrichment for critical ions(including K^(+),Na^(+),Ca^(2+),Mg^(2+),NH_(4)^(+),Cl^(-),NO_(3)^(-)and SO_(4)^(2-))from the Web of Science and Chinese Knowledge Infrastructure databases.We aimed to synthesize the mechanisms,quantify the enrichments,and identify global patterns of nutrient enrichment in stemflow and throughfall across climate zones,and vegetation types and ecosystems.The results of this study indicate that stemflow exhibits,on average,2.1times greater ion concentration(6.13 mg L^(-1))compared to throughfall.In particular,among the investigated ions,SO_(4)^(2-)(12.45and 6.32 mg L^(-1))for stemflow and throughfall,respectively,and Cl^(-)(9.21 and 4.81 mg L^(-1))exhibit the highest concentrations in both rainfall redistribution components,while K^(+)(13.7 and 5.8)and Mg^(2+)(5.6 and 2.8)have the highest enrichment factors.Across climate zones,throughfall and stemflow show the lowest ion concentrations but the highest enrichment factors in extremely humid regions.Along the temperature gradient,ion concentrations are the highest in cold climates with no clear patterns observed for enrichment factors with increasing temperature.In addition,shrubs,conifers,mixed forests,and artificial ecosystems demonstrate enrichment factors 1.1 to 3.0 times greater than those of trees,broad-leaved plants,pure forests,and natural ecosystems.These findings emphasize the need for increased attentions to artificial ecosystems,such as urban and agricultural ecosystems,which often received

关键词： Ecohydrology Rainfall redistribution Nutrients transport Enrichment characteristics Climate zones

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Gas-phase synthesis of Ti_(2)CCl_(2) enables an efficient catalyst for lithiumsulfur batteries

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The Innovation 2024年第1期5卷 33-40页

作者： Maoqiao Xiang Zihan Shen Jie Zheng Miao Song Qiya He yafeng Yang Jiuyi Zhu Yuqi Geng Fen Yue Qinghua Dong Yu Ge Rui Wang Jiake Wei Weiliang Wang Haiming Huang Huigang zhang Qingshan Zhu Chuanfang John zhang State Key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China School of Chemical Engineering University of the Chinese Academy of SciencesBeijing 100049China Innovation Academy for Green Manufacture Chinese Academy of SciencesBeijing 100190China China Nuclear Power Engineering Co. Ltd.117 West Third Ring RoadNorth SectionBeijing 100840China College of Materials Science&Engineering Sichuan UniversityChengdu 610065China State Key Laboratory of Catalysis Dalian Institute of Chemical PhysicsChinese Academy of SciencesDalian 116023China School of Physics Guangdong Province Key Laboratory of Display Material and TechnologyCenter for Neutron Science and TechnologySun Yat-sen UniversityGuangzhou 510275China Solid State Physics&Material Research Laboratory School of Physics and Materials ScienceGuangzhou UniversityGuangzhou 510006China

MXenes have aroused intensive enthusiasm because of their exotic properties and promising applications.However,to date,they are usually synthesized by etching technologies.Developing synthetic technologies provides more opportunities for innovation and may extend unexplored applications.Here,we report a bottom-up gas-phase synthesis of Cl-terminated MXene(Ti_(2)CCl_(2)).The gas-phase synthesis endows Ti_(2)CCl_(2) with unique surface chemistry,high phase purity,and excellent metallic conductivity,which can be used to accelerate polysulfide conversion kinetics and dramatically prolong the cyclability of Li-S batteries.In-depth mechanistic analysis deciphers the origin of the formation of Ti_(2)CCl_(2) and offers a paradigm for tuning MXene chemical vapor deposition.In brief,the gas-phase synthesis transforms the synthesis of MXenes and unlocks the hardly achieved potentials of MXenes.

关键词： synthesis phase lithium

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A型代数的多重张量代数表示有限的充分必要条件

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中国科学：数学 2024年第1期54卷 25-38页

作者：刘雨喆张亚峰贵州大学数学与统计学院贵阳550025 兰州财经大学信息工程与人工智能学院兰州730020

本文考虑A型代数的多重张量代数的表示型,给出多重张量代数表示有限的判定条件.此外,本文还为一些表示有限张量代数提供了用于计算不可分解模同构类数的计数公式.

关键词：箭图表示 Auslander-Reiten箭图表示型模范畴

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数字平台“二选一”垄断行为与监管策略

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运筹与管理 2024年第1期33卷 219-225页

作者：孙勇杨瑞佳张亚峰广州大学公共管理学院广东广州510006 河海大学商学院江苏南京211100 中国科学院大学公共政策与管理学院北京100049

数字平台发展模式的成功离不开各利益相关方的共同努力,其反垄断问题越来越受到各国重视。本文构建了政府、数字平台和商家三方的反垄断演化博弈模型,研究数字平台“二选一”垄断行为与监管策略。结果表明:当满足一定条件时,可以实现政... 详细信息

数字平台发展模式的成功离不开各利益相关方的共同努力,其反垄断问题越来越受到各国重视。本文构建了政府、数字平台和商家三方的反垄断演化博弈模型,研究数字平台“二选一”垄断行为与监管策略。结果表明:当满足一定条件时,可以实现政府反垄断监管,数字平台不垄断且商家合作的理想稳态均衡;政府反垄断强度对数字平台垄断策略选择具有负向影响,但超过一定强度阈值,会导致数字平台和政府的策略选择概率进入震荡的不均衡状态;数字平台垄断地位越高其选择垄断行为的意愿就越高,政府选择反垄断监管策略的意愿越强,同时商家选择不合作策略的意愿也越强;反垄断惩罚与垄断损害赔偿力度均能降低数字平台的垄断意愿,但反垄断惩罚对数字平台具有更强的约束作用。

关键词：数字平台数字经济反垄断演化博弈二选一

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Therapeutic efficacy of traditional Chinese exercises and massage treatment on lumbar instability:a randomized controlled trial

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Journal of Traditional Chinese Medicine 2020年第6期40卷 1026-1032页

作者： Chen Wenjin Wang Jianwei Zhou Zhiyi Ren Yide Hua Zhen Yan Zheng zhang yafeng Department of Orthopedics Wuxi Affiliated Hospital of Nanjing University of Chinese MedicineJiangsu 214071China Wuxi Huishan Traditional Chinese Medicine hospital Jiangsu 214071China College of Information Science and Engineering Huaqiao University Fujian 361021China

OBJECTIVE:To determine the effect of traditional Chinese exercises combined with traditional Chinese massage on lumbar instability.METHODS:Seventy patients with lumbar instability were randomly divided into experimental group and control group.The experimental group was treated with traditional Chinese exercises combined with traditional Chinese massage,while the control group was only treated with traditional Chinese exercises.The Japanese Orthopaedic Association(JOA)scores,Oswestry Disability Index(ODI)and dynamic imaging indexes were used to assess treatment outcomes.RESULTS:After 8 weeks of treatment,the JOA scores of both groups were significantly higher than those before treatment(P<0.05),while ODI was significantly lower(P<0.05).In addition,compared with the control group,the JOA score of the experimental group was significantly increased(P<0.05),and the ODI was significantly decreased(P<0.05).Besides,the dynamic imaging indexes of patients with lumbar instability significantly changed after treatment.The lumbar vertebral laxity was significantly decreased(P<0.05)than those before treatment.CONCLUSION:The traditional Chinese exercises and massage may improve the symptoms of lumbar instability,and traditional Chinese exercises combined with massage treatment may be better than exercises alone.

关键词： Joint instability Exercise therapy Massage Medicine Chinese traditional Randomized controlled trial

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结合Cokriging模型和单目标函数的随机模型修正

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机械科学与技术 2024年第1期43卷 1-8页

作者：彭珍瑞张雪萍张亚峰兰州交通大学机电工程学院兰州730070

将Cokriging代理模型技术和单目标函数进行结合,提出了一种随机模型修正方法。该方法将不确定性模型修正问题转化为较简单的待修正参数统计特征的修正问题,能够在保证模型修正精度的同时,有效缓解模型修正中由于分步修正和多目标修正造... 详细信息

将Cokriging代理模型技术和单目标函数进行结合,提出了一种随机模型修正方法。该方法将不确定性模型修正问题转化为较简单的待修正参数统计特征的修正问题,能够在保证模型修正精度的同时,有效缓解模型修正中由于分步修正和多目标修正造成的计算成本高的问题。首先,假设待修正参数和响应均服从高斯分布,采用拉丁超立方抽样获取训练集样本,构造满足精度要求的Cokriging模型替代复杂的有限元模型参与迭代计算。然后,建立有限元模型计算响应统计特征与试验响应统计特征的加权残差目标函数,引入土狼优化算法最小化该单目标函数来得到待修正参数的统计特征。最后,通过二维和三维桁架结构验证了所提方法的可行性。

关键词：不确定性模型修正单目标函数全局优化 Cokriging模型

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Fabrication,microstructures,and properties of copper matrix composites reinforced by molybdenum-coated carbon nanotubes

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Rare Metals 2011年第4期30卷 401-407页

作者： NIE Junhui JIA Chengchang JIA Xian zhang yafeng SHI Na LI Yi School of Matertals Sctence and Engmeermg Umverszty of Sctence and Technology Beijing Beijing 100083 China China Iron ＆ Steel Research Institute Group Beijing 100081 China

Multiwalled carbon nanotubes （CNTs） were coated by a molybdenum layer using carbonyl thermal decomposition process with a precursor of molybdenum hexacarbonyl. The Mo-coated CNTs （Mo-CNTs） were added into copper powders to fabricate Mo-CNT/Cu composites by means of mechanical milling followed by spark plasma sintering. The Mo-CNTs were uniform dispersion in the Cu matrix when their contents were 2.5 vo1.%-7.5 vol.%, while some Mo-CNT clusters were clearly observed at additions of 10.0 vo1.%-15.0 vol.% Mo-CNTs in the mixture. The mechanical, electrical, and thermal properties of the Mo-CNT/Cu composites were characterized, and the results showed that the tensile strength and hardness were 2.0 and 2.2 times higher than those of CNT-free specimens, respectively. Moreover, the Mo-CNT/Cu composites exhibited an enhanced thermal conductivity but inferior electrical conductivity compared with sintered pure Cu. The uncoated CNT/Cu composites were fabricated by the similar processes, and the measured tensile strength, hardness, thermal conductivity, and electrical conductivity of the CNT/Cu composites were lower than those of the Mo-CNT/Cu composites.

关键词： metallic matrix composites mechanical properties ball milling molybdenum carbon nanotubes

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