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Lamellar water induced quantized interlayer spacing of nanochannels walls

Green Energy & Environment 2024年第2期9卷 356-365页

作者： Yue zhang Chenlu Wang chunlei Wang Yingyan zhang Junhua Zhao Ning Wei Jiangsu Key Laboratory of Advanced Food Manufacturing Equipment and Technology Jiangnan UniversityWuxi214122China Key Laboratory of Agricultural Soil and Water Engineering in Arid and Semiarid Areas Ministry of EducationNorthwest A&F UniversityYangling712100China zhangjiang Lab Interdisplinary Research CenterShanghai Advanced Research InstituteChinese Academy of SciencesShanghai201210China Key Laboratory of Interfacial Physics and Technology Shanghai Institute of Applied PhysicsChinese Academy of SciencesShanghai201800China Mechanical&Automotive Engineering School of EngineeringRMIT UniversityBundooraMelbourneVICVIC 3083Australia

The nanoscale confinement is of great important for the industrial applications of molecular sieve,desalination,and also essential in bio-logical transport systems.Massive efforts have been devoted to the influence of restricted spaces on the properties of confined fluids.However,the situation of channel-wall is crucial but attracts less attention and remains unknown.To fundamentally understand the mechanism of channel-walls in nanoconfinement,we investigated the interaction between the counter-force of the liquid and interlamellar spacing of nanochannel walls by considering the effect of both spatial confinement and surface wettability.The results reveal that the nanochannel stables at only a few discrete spacing states when its confinement is within 1.4 nm.The quantized interlayer spacing is attributed to water molecules becoming laminated structures,and the stable states are corresponding to the monolayer,bilayer and trilayer water configurations,respectively.The results can potentially help to understand the characterized interlayers spacing of graphene oxide membrane in water.Our findings are hold great promise in design of ion filtration membrane and artificial water/ion channels.

关键词： Nanoconfinement Quantized spacing Lamellar water layer MD simulations Entropy force

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Fabrication,Microstructure and Mechanical Properties of in situ GNPs Reinforced Magnesium Matrix Composites

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Acta Metallurgica Sinica(English Letters) 2024年第3期37卷 561-569页

作者： Peitang Zhao Xuejian Li Hailong Shi Xiaoshi Hu chunlei zhang Chao Xu Xiaojun Wang The 38th Research Institute of China Electronics Technology Group Corporation Hefei 230088China National Key Laboratory of Precision Hot Processing of Metal Harbin Institute of TechnologyHarbin 150001China

Graphene reinforced magnesium matrix composites have wide applications in automotive,electronics,aerospace and military fields due to the fascinating mechanical properties.However,it is difficult to realize the high strength and ductility simultaneously.In this work,the in situ liquid-state method was utilized to prepare GNPs/Mg6Zn composites via CO_(2)/Mg chemical reaction.Tensile strength of the GNPs/Mg6Zn composites was improved with increasing content of the GNPs.Meantime,the composites also exhibit a notable plastic deformation stage,and especially the ductility of 0.12 GNPs/Mg6Zn composites reaches 27.6%.Therefore,this novel preparation method has great potential application for fabricating Mg matrix composites with high strength and high ductility.

关键词： Magnesium matrix composite In situ composite Microstructure Mechanical properties

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Design of Ca-type todorokite catalysts with highly active for the selective reduction of NO_(x) by NH_(3) at low temperatures

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Journal of Environmental Sciences 2024年第4期138卷 697-708页

作者： Chuang Chang Zidi Yan chunlei zhang Yanshuang zhang Miao Jiang Luna Ruan Min Xiao Yunbo Yu Hong He School of Rare Earths University of Science and Technology of ChinaHefei 230026China Ganjiang Innovation Academy Chinese Academy of SciencesGanzhou 341000China State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China

Ca-type todorokite catalysts were designed and prepared by a simple redox method and applied to the selective reduction of NO_(x) by NH_(3)(NH_(3)-SCR)for the first time.Compared with the Na-type manjiroite prepared by the same method,the todorokite catalysts with different Mn/Ca ratios showed greatly improved catalytic activity for NO_(x) reduction.Among them,Mn8Ca4 catalyst exhibited the best NH_(3)-SCR performance,achieving 90%NO_(x) conversion within temperature range of 70-275℃ and having a high sulphur resistance.Compared to the Na-type manjiroite sample,Ca-type todorokite catalysts possessed an increased size of tunnel,resulting in a larger specific surface area.As increased the amounts of Ca doping,the Na content in Ca-type todorokite catalysts significantly decreased,providing larger amounts of Bronsted acid sites for NH_(3) adsorption to produce NH_(4)^(+).The NH_(4)^(+)species were highly active for reaction with NO+O_(2),playing a determining role in NH_(3)-SCR process at low temperatures.Meanwhile,larger amounts of surface adsorbed oxygen contained over the Ca-doping samples than that over Na-type manjiroite,promoting the oxidation of NO and fast SCR processes.Over the Ca-type todorokite catalysts,furthermore,nitrates produced during the flow of NO+O_(2),were more active for reaction with NH_(3) than that over Na-type manjiroite,benefiting the occurrence of NH_(3)-SCR process.This study provides novel insights into the design of NH_(3)-SCR catalysts with high performance.

关键词： NO_(x) NH_(3)-SCR Mn-based oxides Ca-type todorokite Bronsted acid sites

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Diagnostic Study of an Extreme Explosive Cyclone over the Kuroshio/Kuroshio Extension Region

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Journal of Ocean University of China 2024年第3期23卷 605-617页

作者： zhang Shuqin LIAO Qinghua LIU chunlei GAO Xiaoyu LONG Jingchao LI Pengyuan XU Jianjun College of Ocean and Meteorology Guangdong Ocean UniversityZhanjiang 524088China South China Sea Institute of Marine Meteorology Guangdong Ocean UniversityZhanjiang 524088China CMA-GDOU Joint Laboratory for Marine Meteorology Guangdong Ocean UniversityZhanjiang 524088China Key Laboratory of Climate Resources and Environment in Continental Shelf Sea and Deep Sea of Department of Education of Guangdong ProvinceGuangdong Ocean UniversityZhanjiang 524088China State Key Laboratory of Severe Weather Chinese Academy of Meteorological SciencesBeijing 100081China Department of Marine Meteorology Ocean-Atmosphere Interaction and Climate LaboratoryKey Laboratory of Physical OceanographyOcean University of ChinaQingdao 266100China

Explosive cyclones(ECs)occur frequently over the Kuroshio/Kuroshio Extension region.The most rapidly intensified EC over the Kuroshio/Kuroshio Extension region during the 42 years(1979-2020)of cold seasons(October-April)was studied to reveal the variations of the key factors at different explosive-developing stages.This EC had weak low-level baroclinicity,mid-level cyclonic-vorticity advection,and strong low-level water vapor convergence at the initial explosive-developing stage.The low-level baroclinicity and mid-level cyclonic-vorticity advection increased substantially during the maximum-deepening-rate stage.The diagnostic analyses using the Zwack-Okossi equation showed that diabatic heating was the main contributor to the initial rapid intensification of this EC.The cyclonic-vorticity advection and warm-air advection enhanced rapidly in the middle and upper troposphere and contributed to the maximum rapid intensification,whereas the diabatic heating weakened slightly in the mid-low troposphere.The relative contribution of the diabatic heating decreased from the initial explosive-developing stage to the maximum-deepening-rate stage due to the enhancement of other factors(the cyclonic-vorticity advection and warm-air advection).Furthermore,the physical factors contributing to this EC varied with the explosive-developing stage.The non-key factors at the initial explosive-developing stage need attention to forecast the rapid intensification.

关键词： explosive cyclone diabatic heating cyclonic-vorticity advection rapid intensification the Kuroshio/Kuroshio Extension region

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Hyperspectral Image Classification Based on Capsule Network

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Chinese Journal of Electronics 2022年第1期31卷 146-154页

作者： MA Qiaoyu zhang Xin zhang chunlei ZHOU Heng School of Science China University of Geosciences (Beijing) School of Statistics Beijing Normal University Beijing Zhongdi Runde Petroleum Technology Co. Ltd.

The conventional convolutional neural network performs not well enough in the ground objects classification because of its insufficient ability in maintaining sensitive spectral information and characterizing the covariance of spatial structure, resulting from the narrow sensitive frequency band and complex spatial structure with diversity of hyperspectral remote sensing data which caused more serious phenomena of "same material, different spectra" and "different material, same spectra".Therefore, an improved capsule network is proposed and introduced into hyperspectral image target recognition. A convolution structure combining shallow features and multi-scale depth features is put forward to reduce the phenomena of "different material, same spectra" firstly,and then the diversity of the spatial structure is expressed by the capsule vector and sub-capsule division in channel wise, so that the averaging effect of the convolution process is weakened in the spectral domain and the spatial domain to reduce the phenomena of "same material, different spectra". By comparing the experimental results on the hyperspectral data sets such as Indian Pines,Salinas, Tea Tree and Xiongan, the capsule network shows strong spatial structure expression ability, flexible deep and shallow feature fusion ability in multi-scale, and its accuracy in target recognition is better than that of conventional convolutional neural networks, so it is suitable for the recognition of complex targets in hyperspectral images.

关键词： Capsule network Space-spectrum fusion Hyperspectral Classification Deep learning

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Avoiding Sabatier's limitation through pulsed electrocatalysis for enhanced nitrogen oxidation performance

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Journal of Energy Chemistry 2024年第8期95卷 484-489页

作者： Xiping Guan Zhongfen Nie Linlin zhang Mingxia Guo Chuanwei Shi chunlei Gu Xia Liu Xin Ding College of Chemistry and Chemical Engineering Qingdao University State Key Laboratory of Fine Chemicals Dalian University of Technology(DUT)

1. Introduction The activation and conversion of the Earth’s abundant inert nitrogen resources into high-value-added products epitomize one of nature’s most critical processes[1–3]. Nitric acid （HNO3）, as a pivotal industrial raw material, showcases an extensive range of applications and possesses substantial economic value in the production of indispensable chemical compounds[4–6]. Currently,

关键词： AMMONIA

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A Distributed Computing Algorithm for Electricity Carbon Emission Flow and Carbon Emission Intensity

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Protection and Control of Modern Power Systems 2024年第2期9卷 138-146页

作者： Xingping Wu Wei Yang Ning zhang chunlei Zhou Jinwei Song Chongqing Kang Big Data Center of China Network Chinese Society of Electrical Engineering State Network Big Data Center Department of Electrical Engineering Tsinghua UniversityBeijingChina 不详 Big Data Center State Grid Corporation of ChinaBeijing 100052China Department of Electrical Engi-neering Tsinghua UniversityBeijingChina

The calculation of the indirect carbon emis-sion is essential for power system policy making,carbon market development,and power grid planning.The em-bedded carbon emissions of the electricity system are commonly calculated by carbon emission flow theory.However,the calculation procedure is time-consuming,especially for a country with 500-1000 thousand nodes,making it challenging to obtain nationwide carbon emis-sions intensity precisely.Additionally,the calculation procedure requires to gather all the grid data with high classified levels from different power grid companies,which can prevent data sharing and cooperation among different companies.This paper proposes a distributed computing algorithm for indirect carbon emission that can reduce the time consumption and provide privacy protection.The core idea is to utilize the sparsity of the nodes’flow matrix of the nationwide grid to partition the computing procedure into parallel sub-procedures exe-cuted in multiple terminals.The flow and structure data of the regional grid are transformed irreversibly for pri-vacy protection,when transmitted between terminals.A 1-master-and-N-slave layout is adopted to verify the method.This algorithm is suitable for large grid compa-nies with headquarter and branches in provinces,such as the State Grid Corporation of China.

关键词： Carbon emission flow cooperative computing carbon emission intensity matrix block par-tition power flow tracing parallel computing privacy protection

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Nucleotide excision repair gene polymorphisms and hepatoblastoma susceptibility in Eastern Chinese children:A five-center case-control study

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Chinese Journal of Cancer Research 2024年第3期36卷 298-306页

作者： Huimin Yin Xianqiang Wang Shouhua zhang Shaohua He Wenli zhang Hongting Lu Yizhen Wang Jing He chunlei Zhou Department of Pediatric Surgery Guangzhou Institute of Pediatrics Guangdong Provincial Key Laboratory of Research in Structural Birth Defect Disease Guangzhou Women and Children's Medical Center Guangzhou Medical University Department of Pediatric Surgery Senior Department of Pediatrics the Seventh Center of Chinese People's Liberation Army(PLA)General Hospital Department of General Surgery Jiangxi Provincial Children's Hospital Department of Pediatric Surgery Shengli Clinical Medical College of Fujian Medical University Department of Pediatric Surgery Qingdao Women and Children's Hospital Department of Pathology Anhui Provincial Children's Hospital Department of Pathology Children's Hospital of Nanjing Medical University

Objective: Nucleotide excision repair(NER) plays a vital role in maintaining genome stability, and the effect of NER gene polymorphisms on hepatoblastoma susceptibility is still under investigation. This study aimed to evaluate the relationship between NER gene polymorphisms and the risk of hepatoblastoma in Eastern Chinese Han children.Methods: In this five-center case-control study, we enrolled 966 subjects from East China(193 hepatoblastoma patients and 773 healthy controls). The TaqMan method was used to genotype 19 single nucleotide polymorphisms(SNPs) in NER pathway genes, including ERCC1, XPA, XPC, XPD, XPF, and XPG. Then, multivariate logistic regression analysis was performed, and odds ratios(ORs) and 95% confidence intervals(95% CIs) were utilized to assess the strength of associations.Results: Three SNPs were related to hepatoblastoma risk. XPC rs2229090 and XPD rs3810366 significantly contributed to hepatoblastoma risk according to the dominant model(adjusted OR=1.49, 95% CI=1.07-2.08,P=0.019; adjusted OR=1.66, 95% CI=1.12-2.45, P=0.012, respectively). However, XPD rs238406 conferred a significantly decreased risk of hepatoblastoma under the dominant model(adjusted OR=0.68, 95% CI=0.49-0.95;P=0.024). Stratified analysis demonstrated that these significant associations were more prominent in certain subgroups. Moreover, there was evidence of functional implications of these significant SNPs suggested by online expression quantitative trait loci(eQTLs) and splicing quantitative trait loci(sQTLs) analysis.Conclusions: In summary, NER pathway gene polymorphisms(XPC rs2229090, XPD rs3810366, and XPD rs238406) are significantly associated with hepatoblastoma risk, and further research is required to verify these findings.

关键词： Nucleotide excision repair polymorphisms hepatoblastoma susceptibility

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ALKBH5 gene polymorphisms and risk of neuroblastoma in Chinese children from Jiangsu Province

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Cancer Innovation 2024年第2期3卷 72-79页

作者： Qian Guan Xinxin zhang Jiabin Liu chunlei Zhou Jinhong Zhu Haiyan Wu Zhenjian Zhuo Jing He Department of Pediatric Surgery Guangzhou Institute of PediatricsGuangdong Provincial Key Laboratory of Research in Structural Birth Defect DiseaseGuangdong Provincial Clinical Research Center for Child HealthGuangzhou Women and Children's Medical CenterGuangzhou Medical UniversityGuangzhouGuangdongChina Department of Pathology Children's Hospital of Nanjing Medical UniversityNanjingJiangsuChina Department of Clinical Laboratory BiobankHarbin Medical University Cancer HospitalHarbinHeilongjiangChina Laboratory Animal Center School of Chemical Biology and BiotechnologyPeking University Shenzhen Graduate SchoolShenzhenGuangdongChina

Background:Neuroblastoma is one of the most common extracranial malignant solid tumors in children.AlkB homolog 5(ALKBH5)is an RNA N6-methyladenosine(m6A)demethylase that plays a critical role in tumorigenesis and development.We assessed the association between single nucleotide polymorphisms(SNPs)in ALKBH5 and the risk of neuroblastoma in a case-control study including 402 patients and 473 non-cancer controls.Methods:Genotyping was determined by the TaqMan method.The association between ALKBH5 polymorphisms(rs1378602 and rs8400)and the risk of neuroblastoma was evaluated using the odds ratio(OR)and 95%confidence interval(CI).Results:We found no strong association of ALKBH5 rs1378602 and rs8400 with neuroblastoma risk.Further stratification analysis by age,sex,primary site,and clinical stage showed that the rs1378602 AG/AA genotype was associated with a lower risk of neuroblastoma in males(adjusted OR=0.58,95%CI=0.35–0.97,p=0.036)and children with retroperitoneal neuroblastoma(adjusted OR=0.58,95%CI=0.34–0.98,p=0.040).Conclusions:ALKBH5 SNPs do not seem to be associated with neuroblastoma risk.More studies are required to confirm this negative result and reveal the relationship between gene polymorphisms of the m6A modifier ALKBH5 and neuroblastoma.

关键词： ALKBH5 neuroblastoma polymorphism susceptibility

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Wetting front migration model of ion-adsorption rare earth during the multi-hole unsaturated liquid injection

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第2期16卷 483-496页

作者： Yu Wang Xiaojun Wang Yuchen Qiu Hao Wang Gang Li Kaijian Hu Wen Zhong Zhongqun Guo Bing Li chunlei zhang Guangxiang Ye Jiangxi Key Laboratory of Mining Engineering Jiangxi University of Science and TechnologyGanzhou341000China School of Resources and Environment Engineering Jiangxi University of Science and TechnologyGanzhou341000China School of Civil Engineering and Surveying&Mapping Engineering Jiangxi University of Science and TechnologyGanzhou341000China Ganzhou Nonferrous Metallurgy Research Institute Ganzhou341000China

In the process of ion-adsorption rare earth ore leaching,the migration characteristics of the wetting front in multi-hole injection holes and the influence of wetting front intersection effect on the migration distance of wetting fronts are still unclear.Besides,wetting front migration distance and leaching time are usually required to optimize the leaching process.In this study,wetting front migration tests of ionadsorption rare earth ores during the multi-hole fluid injection(the spacing between injection holes was 10 cm,12 cm and 14 cm)and single-hole fluid injection were completed under the constant water head height.At the pre-intersection stage,the wetting front migration laws of ion-adsorption rare earth ores during the multi-hole fluid injection and single-hole fluid injection were identical.At the postintersection stage,the intersection accelerated the wetting front migration.By using the Darcy’s law,the intersection effect of wetting fronts during the multi-hole liquid injection was transformed into the water head height directly above the intersection.Finally,based on the Green-Ampt model,a wetting front migration model of ion-adsorption rare earth ores during the multi-hole unsaturated liquid injection was established.Error analysis results showed that the proposed model can accurately simulate the infiltration process under experimental conditions.The research results enrich the infiltration law and theory of ion-adsorption rare earth ores during the multi-hole liquid injection,and this study provides a scientific basis for optimizing the liquid injection well pattern parameters of ion-adsorption rare earth in situ leaching in the future.

关键词： Ion-adsorption rare earth ore Multi-hole unsaturated liquid injection In situ leaching Intersection effect Calculation model

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