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Exact Geometric Relationships, Symmetry Breaking and Structural Stability for Single-Walled Carbon Nanotubes

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Nano-Micro Letters 2011年第4期3卷 228-235页

作者： Tong Zhang ze shuai yuan Li Hao Tan Research Center for Solid Mechanics Beihang University

We pioneered a study about how the geometric relationship of single-walled carbon nanotubes(SWCNT) is influenced by curvature factor and non-planar geometry factor in cylindrical coordinate system based on the assumption of complete symmetry. The bond length and angle of every carbon-carbon bonds are determined by using the principle of the minimum energy. The results of the paper include(1) From the calculation result, the symmetry breaking appears for chiral carbon nanotubes, while the part symmetry appears for achiral carbon nanotubes with increasing curvature.(2) The synergistic effect of bond lengths and bond angles is first found.(3) We conclude that the influence of non-planar geometry factor can be completely ignored on bond lengths and bond angles when the curvature parameter has been included in the model.(4)The two fractal dimensions are given from the nanoscale to the macroscale for zigzag topology and armchair topology respectively. Fractal dimensions of SWCNT show special characteristics, varying with the length of SWCNT until the lengths approach infinity. The close and inevitable correlations among curvature, symmetry breaking and stability of SWCNTs can be summed up as: the increase of curvature causes symmetry breaking,and such symmetry breaking will further reduce the structural stability.

关键词： Geometry Structural Stability Symmetry Breaking Fractal Dimension

Phosphorus-doping activates carbon nanotubes for efficient electroreduction of nitrogen to ammonia

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Nano Research 2020年第5期13卷 1376-1382页

作者： Lu-Pan yuan ze-yuan Wu Wen-Jie Jiang Tang Tang shuai Niu Jin-Song Hu Beijing National Laboratory for Molecular Sciences(BNLMS) CAS Key Laboratory of Molecular Nanostructure and NanotechnologyInstitute of ChemistryChinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China

The electrochemical nitrogen reduction reaction(NRR)as an energy-efficient approach for ammonia synthesis is hampered by the low ammonia yield and ambiguous reaction ***,phosphorus-doped carbon nanotube(P-CNTs)is developed as an efficient metal-free electrocatalyst for NRR with a remarkable NH3 yield of 24.4μg·h^−1·mg^−*** partial current density of 0.61 mA·cm^−*** superior activity is found to be from P doping and highly conjugated CNTs *** and theoretical investigations discover that the electron-deficient phosphorus sites with Lewis acidity should be genuine active sites and NRR on P-CNTs follows the distal *** findings provide insightful understanding on NRR processes on P-CNTs,opening up opportunities for the rational design of highly-active cost-effective metal-free catalysts for electrochemical ammonia synthesis.

关键词： P-doped carbon nanotubes nitrogen reduction reaction active sites reaction pathway electrocatalysis

Inhibition of the cGAS–STING pathway:contributing to the treatment of cerebral ischemia-reperfusion injury

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Neural Regeneration Research 2025年第7期20卷 1900-1918页

作者： Hang Yang Yulei Xia Yue Ma Mingtong Gao shuai Hou Shanshan Xu Yanqiang Wang School of Clinical Medicine Shandong Second Medical UniversityWeifangShandong ProvinceChina Department of Emergency The Affiliated Hospital of Weifang Medical UniversityWeifangShandong ProvinceChina Department of Neurology Ⅱ The Affiliated Hospital of Weifang Medical UniversityWeifangShandong ProvinceChina

The cGAS–STING pathway plays an important role in ischemia-reperfusion injury in the heart,liver,brain,and kidney,but its role and mechanisms in cerebral ischemia-reperfusion injury have not been systematically ***,we outline the components of the cGAS–STING pathway and then analyze its role in autophagy,ferroptosis,cellular pyroptosis,disequilibrium of calcium homeostasis,inflammatory responses,disruption of the blood–brain barrier,microglia transformation,and complement system activation following cerebral ischemia-reperfusion *** further analyze the value of cGAS–STING pathway inhibitors in the treatment of cerebral ischemia-reperfusion injury and conclude that the pathway can regulate cerebral ischemia-reperfusion injury through multiple *** of the cGAS–STING pathway may be helpful in the treatment of cerebral ischemia-reperfusion injury.

关键词： calcium homeostasis cellular autophagy cerebral ischemia-reperfusion injury cGAS–STING pathway ferroptosis gut–brain–microbiota axis inflammatory light chain 3 microglial cells Syntaxin-17 protein

Preparation and properties of T-ZnO_(w) enhanced BCP scaffolds with double-layer structure by digital light processing

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Journal of Advanced Ceramics 2022年第4期11卷 570-581页

作者： Ming-Zhu PAN shuai-Bin HUA Jia-Min WU Xi yuan ze-Lin DENG Jun XIAO Yu-Sheng SHI State Key Laboratory of Materials Processing and Die&Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074China Engineering Research Center of Ceramic Materials for Additive Manufacturing Ministry of EducationWuhan 430074China Department of Orthopedic Surgery Tongji HospitalTongji Medical CollegeHuazhong University of Science and TechnologyWuhan 430030China

Bone scaffolds require both good bioactivity and mechanical properties to keep shape and promote bone *** this work,T-ZnO_(w) enhanced biphasic calcium phosphate(BCP)scaffolds with triply periodic minimal surface(TPMS)-based double-layer porous structure were fabricated by digital light processing(DLP)with high *** of suspension was first discussed to obtain better printing *** sintering,T-ZnO_(w) reacts with b-tricalcium phosphate(β-TCP)to form Ca_(19)Zn_(2)(PO_(4))14,and inhibits the phase transition toα-*** the content of T-ZnO_(w) increasing from 0 to 2 wt%,the flexural strength increases from 40.9 to 68.5 MPa because the four-needle whiskers can disperse stress,and have the effect of pulling out as well as fracture ***,excessive whiskers will reduce the cure depth,and cause more printing defects,thus reducing the mechanical ***,T-ZnO_(w) accelerates the deposition of apatite,and the sample with 2 wt%T-ZnO_(w) shows the fastest mineralization *** good biocompatibility has been proved by cell proliferation *** confirmed that doping T-ZnO_(w) can improve the mechanical strength of BCP scaffolds,and keep good biological property,which provides a new strategy for better bone repair.

关键词： biphasic calcium phosphate(BCP) T-ZnO_(w) digital light processing(DLP) double-layer structure cure property mechanical strength

A multi-fidelity prediction model for vertical bending moment and total longitudinal stress of a ship based on composite neural network

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Journal of Hydrodynamics 2023年第1期35卷 27-35页

作者： Cai-xia Jiang Yu-bo Liu Zi-yuan Wang shuai Chen Sheng-ze Cai Qi Gao Xue-ming Shao Science and Technology on Advanced Composites in Special Environments Key Laboratory Harbin Institute of TechnologyHarbin150001China China Ship Scientific Research Center Wuxi214082China School of Aeronautics and Astronautics Zhejiang UniversityHangzhou310027China College of Control Science and Engineering Zhejiang UniversityHangzhou310027China

In ship engineering,the prediction of vertical bending moment(VBM)and total longitudinal stress(TLS)during ship navigation is of utmost *** this work,we propose a new prediction paradigm,the multi-fidelity regression model based on multi-fidelity data and artificial neural network(MF-ANN).Specifically,an ANN is used to learn the fundamental physical laws from low-fidelity data and construct an initial input-output *** predicted values of this initial model are of low accuracy,and then the high-fidelity data are utilized to establish a correction model that can correct the low-fidelity prediction ***,the overall accuracy of prediction can be improved *** feasibility of the multi-fidelity regression model is demonstrated by predicting the VBM,and the robustness of the model is evaluated at the same *** prediction of TLS on the deck indicates that just a small amount of high-fidelity data can make the prediction accuracy reach a high level,which further illustrates the validity of the proposed MF-ANN.

关键词： Artificial neural network multi-fidelity vertical bending moment total longitudinal stress

Random forest-based prediction of decay modes and half-lives of superheavy nuclei

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Nuclear Science and Techniques 2023年第12期34卷 271-280页

作者： Bo‑shuai Cai Cen‑Xi yuan Sino‑French Institute of Nuclear Engineering and Technology Sun Yat-sen UniversityZhuhai 519082China

Information on the decay process of nuclides in the superheavy region is critical in investigating new elements beyond oganesson and the island of *** paper presents the application of a random forest algorithm to examine the competition among different decay modes in the superheavy region,includingα decay,β^(-)decay,β^(+)decay,electron capture and spontaneous *** observed half-lives and dominant decay mode are well *** dominant decay mode of 96.9%of the nuclei beyond ^(212) Po is correctly ***,α decay is predicted to be the dominant decay mode for isotopes in new elements Z=119-122,except for spontaneous fission in certain even–even elements owing to the increased Coulomb repulsion and odd–even *** predicted half-lives demonstrate the existence of a long-lived spontaneous fission island southwest of ^(298) Fl caused by the competition between the fission barrier and Coulomb repulsion.A better understanding of spontaneous fission,particularly beyond ^(286)Fl,is crucial in the search for new elements and the island of stability.

关键词： Decay mode Superheavy nuclide Random forest

Joint method for reconstructing three-dimensional temperature of flame using Lucy-Richardson and nearest neighbor filtering using light-field imaging

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Science China(Technological Sciences) 2019年第7期62卷 1232-1243页

作者： LI TianJiao yuan yuan shuai Yong TAN HePing Key Laboratory of Aerospace Thermophysics Ministry of Industry and Information Technology Harbin Institute of Technology

The real-time measurement and reconstruction of three-dimensional temperature are essential when studying the combustion process inside a flame. In the proposed sectioned flame light field imaging model, flame sections are reconstructed based on the characteristics identified using the Lucy-Richardson or nearest neighbor filtering methods, or a joint method involving a combination of both, to improve on the accuracy of two-dimensional temperature reconstruction. Compared to the results of a previous work, the proposed method increases the resolution in the depth of field direction and the extraction of the flame temperature of all sections from the same height ensures the accuracy of the reconstructed temperature distribution across the cross-section of the flame. The relative error when compared to the actual flame is less than 10%. Thus, this approach allows the accurate estimation of the three-dimensional temperature distribution inside a flame, and enables the rapid and effective reconstruction of the three-dimensional temperature field.

关键词： radiative transfer flame light field imaging temperature estimation

Synergistic regulation of temperature resistance and thermal insulation performance of zirconia-based ceramic fibers

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Rare Metals 2023年第12期42卷 4189-4200页

作者： Yong-shuai Xie Ying Peng Zhe-Zhe Deng ze Zhu yuan Cheng De-Hua Ma Lu-Yi Zhu Xing-Hong Zhang State Key Laboratory of Crystal Materials School of Crystal MaterialsShandong UniversityJinan 250100China National Key Laboratory of Science and Technology on Advanced Composites in Special Environments Harbin Institute of TechnologyHarbin 150001China

ZrO_(2) fiber is a promising high-temperature resistant and heat-insulating fiber ***,the decrease in mechanical properties caused by grain growth at high temperatures seriously affects its *** to achieve the synergy of its temperature resistance and the thermal insulation performance is still the focus of the current *** this work,we started with doping inequivalent elements and studied the phase composition,temperature resistance,and thermal insulation properties of Y_(2)O_(3)-ZrO_(2) ceramic fibers by adjusting the Y/Zr molar *** results showed that Y_(2)O_(3) could enter the crystal lattice of ZrO_(2) and form a solid *** the increase in Y_(2)O_(3) content,the structure of fibers changed from a tetragonal phase to a cubic phase,and the configurational entropy of the system *** larger configuration entropy in the sample could produce a robust steric hindrance effect,inhibiting grain *** heat treatment at 1300℃,the grain size of Y_(2)Zr_(2)O_(7)(Y5Z5)fibers was only 61.8%that of Y_(0.1)Zr_(0.9)O_(1.95)(Y1Z9)*** smaller grain size made the Y5Z5 fibers still have excellent flexibility and deformation recovery performance after heat treatment at 1300℃and could still return to the original state after 85%compression or folded in *** addition,due to the larger configurational entropy,the mean free path of phonon scattering was shortened,thereby improving the thermal insulation performance of the *** short,this work achieves the synergistic effect of temperature resistance and thermal insulation properties of zirconia-based fiber materials only through simple inequivalent element doping.

关键词： Ceramics fiber ZrO_(2) Y_(2)O_(3) Thermal insulation Temperature resistance

新疆小麦过氧化物酶活性基因TaPod-A1、TaPod-A3和TaPod-D1等位变异及分布规律

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作物学报 2025年第1期51卷 68-78页

作者：刘鑫源程宇坤王丽丽战帅帅马孟瑶郭玲耿洪伟新疆农业大学农学院/新疆优质专用麦类作物工程技术研究中心新疆乌鲁木齐830052 新疆作物遗传改良与种质创新重点实验室新疆乌鲁木齐830052

小麦面粉的颜色是其品质分级的重要指标,为了使小麦面粉的品质得到进一步提升,本研究利用位于TaPod-A1、TaPod-A3和TaPod-D1位点基因的功能标记对110份新疆小麦品种(系)进行等位变异基因检测。基因型与表型方差分析结果显示, TaPod-A1、... 详细信息

小麦面粉的颜色是其品质分级的重要指标,为了使小麦面粉的品质得到进一步提升,本研究利用位于TaPod-A1、TaPod-A3和TaPod-D1位点基因的功能标记对110份新疆小麦品种(系)进行等位变异基因检测。基因型与表型方差分析结果显示, TaPod-A1、TaPod-A3和TaPod-D1位点的等位变异类型TaPod-A1b (35.5%)、TaPod-A3c (53.6%)和TaPod-D1b(60%)较其他等位变异类型TaPod-A1a (64.5%)、TaPod-A3a (46.4%)和TaPod-D1a(40%)均具有较高的POD活性。在新疆小麦材料中, TaPod-A1、TaPod-A3和TaPod-D1的3个不同基因位点上高POD活性的优异等位变异类型的分布频率均表现为引进品种(系)≈自育品种(系)>地方品种。TaPod-A3b在110份新疆小麦材料中并未检测出,说明该等位变异为稀有等位变异。具有TaPod-A1、TaPod-A3和TaPod-D1基因等位变异组合品种(系)的平均POD活性高低依次为TaPod-A1b/TaPod-A3c/TaPod-D1b (2836.25 U g^(–1) min^(–1))> TaPod-A1b/TaPod-A3c/TaPod-D1a (2796.00 U g^(–1)min^(–1))> TaPod-A1b/TaPod-A3a/TaPod-D1b(2520.31Ug^(–1)min^(–1))> TaPod-A1a/TaPod-A3c/TaPod-D1b(2473.91Ug^(–1)min^(–1))> TaPod-A1a/TaPod-A3a/TaPod-D1b(2407.65Ug^(–1)min^(–1))> TaPod-A1b/TaPod-A3a/TaPod-D1a(2339.06Ug^(–1)min^(–1))> TaPod-A1a/TaPod-A3c/TaPod-D1a(2320.38Ug^(–1)min^(–1))> TaPod-A1a/TaPod-A3a/TaPod-D1a(2210.69Ug^(–1)min^(–1))。其中,具有TaPod-A1b/TaPod-A3c/TaPod-D1b等位变异基因的活性(2836.25Ug^(–1)min^(–1))极显著高于具有TaPod-A1a/TaPod-A3a/TaPod-D1a(2210.69Ug^(–1)min^(–1))(P<0.01)的品种,说明具有较多优异等位变异类型的品种具有较高的POD活性。

关键词：小麦过氧化物酶等位变异分子标记检测