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Predictive value of red blood cell distribution width and hematocrit for short-term outcomes and prognosis in colorectal cancer patients undergoing radical surgery

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World Journal of Gastroenterology 2024年第12期30卷 1714-1726页

作者： Dong peng Zi-Wei Li fei Liu Xu-Rui Liu Chun-Yi Wang Department of Gastrointestinal Surgery The First Affiliated Hospital of Chongqing Medical UniversityChongqing 400016China

BACKGROUND Previous studies have reported that low hematocrit levels indicate poor survival in patients with ovarian cancer and cervical cancer,the prognostic value of hematocrit for colorectal cancer(CRC)patients has not been *** prognostic value of red blood cell distribution width(RDW)for CRC patients was *** To investigate the impact of RDW and hematocrit on the short-term outcomes and long-term prognosis of CRC patients who underwent radical *** Patients who were diagnosed with CRC and underwent radical CRC resection between January 2011 and January 2020 at a single clinical center were *** short-term outcomes,overall survival(OS)and disease-free survival(DFS)were compared among the different *** analysis was also conducted to identify independent risk factors for OS and *** There were 4258 CRC patients who underwent radical surgery included in our study.A total of 1573 patients were in the lower RDW group and 2685 patients were in the higher RDW *** were 2166 and 2092 patients in the higher hematocrit group and lower hematocrit group,*** in the higher RDW group had more intraoperative blood loss(P<0.01)and more overall complications(P<0.01)than did those in the lower RDW ***,patients in the lower hematocrit group had more intraoperative blood loss(P=0.012),longer hospital stay(P=0.016)and overall complications(P<0.01)than did those in the higher hematocrit *** higher RDW group had a worse OS and DFS than did the lower RDW group for tumor node metastasis(TNM)stage I(OS,P<0.05;DFS,P=0.001)and stage II(OS,P=0.004;DFS,P=0.01)than the lower RDW group;the lower hematocrit group had worse OS and DFS for TNM stage II(OS,P<0.05;DFS,P=0.001)and stage III(OS,P=0.001;DFS,P=0.001)than did the higher hematocrit *** hematocrit was an independent risk factor for OS[P=0.017,hazard ratio(HR)=1.256,95%confidence interval(CI):1.041-1.515]and DFS(P=0.035,HR=1.194

关键词： Colorectal cancer Red blood cell distribution width Survival Short-term outcomes

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Synthesis,Characterization of Polyethylene Ionomers and Their Antibacterial Properties

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Chinese Journal of Polymer Science 2024年第8期42卷 1077-1084页

作者： Jia-Jia Wu fei Wang peng-Qi Wan Li Pan Chun-Sheng Xiao Zhe Ma Yue-Sheng Li Tianjin Key Lab Composite&Functional Materials School of Materials Science and EngineeringTianjin UniversityTianjin 300350China Key Lab Polymer Ecomaterials Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun 130022China

Owing to its high production volume and wide range of application s,polyethylene has gained a great deal of attention,but its low surface energy and non-polar nature have limited its application in some important *** this study,ethylene/11-iodo-1-undecene copolymers were prepared and used as the intermediates to afford a series of imidazolium-based ionomers bearing methanesulfonate(CH_(3)SO_(3)^(-)),trifluoromethanesulfonate(CF_(3)SO_(3)^(-)),or bis(trifluoromethane)sulfonimide(Tf_(2)N^(-))*** tensile test results showed that the stress-at-break(7.8-25.6 MPa)and the elongation-at-break(445%-847%)of the ionomers could be adjusted by changing the counterion species and the ionic group *** importantly,the ionomers exhibited marvelous antibacterial activities against Staphylococcus aureus(***)and Escherichia coli(***).The ionomers bearing Tf_(2)N^(-)exhibited antibacterial activities>99%against both *** and *** when ionic content reached 9.1%.The imidazolium-based ionomers prepared in this work demonstrated excellent comprehensive properties,especially highefficient and broad-spectrum antibacterial ability,exhibiting the potential fo r the application as the antibacterial materials in packaging,medical,and other fields.

关键词： Polyethylene Ionomer Polymerization catalysis Imidazolium Antibacterial material

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Boosting Li-ion storage kinetics via constructing layered TiO2 anode

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PARTICUOLOGY 2024年第10期93卷 22-29页

作者： Hou, Jiyue Wang, fei Zhang, Enfeng Wang, Ying Dong, peng Wang, Yunxiao Zhang, Yiyong Li, Xue Zhang, Yingjie Kunming Univ Sci & Technol Fac Met & Energy Engn Natl & Local Joint Engn Res Ctr Lithium ion Batter Kunming 650093 Peoples R China Panzhihua Univ Coll Elect Informat Engn Panzhihua 617000 Peoples R China Univ Wollongong Australian Inst Innovat Mat Inst Superconducting & Elect Mat Innovat Campus Squires Way Wollongong NSW 2500 Australia

Due to the typical intercalation-deintercalation mechanism, TiO 2 holds great promise as a sustainable anode for next-generation lithium -ion batteries (LIBs). However, commercial TiO 2 (C-TiO 2 ) is granular and shows slow ionic conductivity, which greatly hinders its development due to sluggish kinetics, leading to low reversible capacity and inferior rate capability. In this study, a two-dimensional layered TiO 2 (L-TiO 2 ) anode is prepared via a one-step calcination process, which can effectively shorten the lithium ions diffusion path and improve its lithium ions conductivity. We elucidated the enhanced electrochemical performance of L-TiO 2 as an anode in LIBs through pseudocapacitive acceleration of lithium ions intercalation and deintercalation using various characterization techniques, including different scan rate cyclic voltammetry tests, in situ electrochemical impedance spectroscopy, in situ Raman spectroscopy, and in situ X-ray diffraction. In comparison to C-TiO 2 material, L-TiO 2 material showcases remarkable electrochemical performance, achieving a capacity of 166 mAh/g after 100 cycles at 0.1 C. Additionally, the lithium -ion diffusion coef ficient calculated for the L-TiO 2 is two orders of magnitude greater, underscoring its potential as a negative electrode material for LIBs. (c) 2024 Chinese Society of Particuology and Institute of Process Engineering, Chinese Academy of Sciences. Published by Elsevier B.V. All rights are reserved, including those for text and data mining, AI training, and similar technologies.

关键词： Lithium-ion batteries Anode MXene LayeredTiO2 ELECTROCHEMICAL PROPERTIES ANATASE TIO2 LITHIUM NANOPARTICLE PERFORMANCE

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Molecular surface functionalization of In_(2)O_(3) to tune interfacial microenvironment for enhanced catalytic performance of CO_(2) electroreduction

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Nano Research 2024年第3期17卷 1242-1250页

作者： Suwen WangQiang GaoCui Xu Shuai Jiang Mengyang Zhang Xianjun Yin Hui-Qing peng Bin Liu Yu-fei Song State Key Laboratory of Chemical Resource Engineering Beijing Advanced Innovation Center for Soft Matter Science and EngineeringCollege of ChemistryBeijing University of Chemical TechnologyBeijing 100029China

Indium-based materials(e.g.,In_(2)O_(3))are a class of promising non-noble metal-based catalysts for electroreduction of carbon dioxide(CO_(2)).However,competitive hydrogen reduction reaction(HER)on indium-based catalysts hampers CO_(2) reduction reaction(CO_(2)RR)*** herein tune the interfacial microenvironment of In_(2)O_(3) through chemical graft of alkyl phosphoric acid molecules using a facile solution-processed strategy for the first time,which is distinguished from other researches that tailor intrinsic activity of In_(2)O_(3) *** surface functionalization of alkyl phosphoric acids over In_(2)O_(3) is demonstrated to remarkably boost CO_(2) *** example,octadecylphosphonic acid modified In_(2)O_(3) exhibits Faraday efficiency for H_(2) H_(2) H_(2)(FE)of as low as 6.6%and FEHCOOH of 86.5%at-0.67 V ***,which are far superior to parent In_(2)O_(3) counterparts(FE of 24.0%and FEHCOOH of 63.1%).Moreover,the enhancing effect of alkyl phosphoric acid functionalization is found to be closely related to the length of alkyl *** virtue of comprehensive experimental characterizations and molecular dynamics simulations,it is revealed that the modification of alkyl phosphoric acids significantly alters the interface microenvironment of the electrocatalyst,which changes the electrocatalyst surface from hydrophilic and aerophobic to hydrophobic and *** this case,the water molecules are pushed away and more CO_(2) molecules are trapped,increasing local CO_(2) concentration at In_(2)O_(3) active sites,thus leading to the significantly enhanced CO_(2)RR and suppressed *** work highlights the importance of regulating the interfacial microenvironment of inorganic catalysts by molecular surface functionalization as a means for promoting the electrochemical performance in electrosynthesis and beyond.

关键词： carbon dioxide(CO_(2))electroreduction interfacial microenvironment molecular surface functionalization In_(2)O_(3)catalyst water and CO_(2)diffusion

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Assessment of soil total phosphorus storage in a complex topography along China's southeast coast based on multiple mapping scales

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Pedosphere 2024年第1期34卷 236-251页

作者： Zhongxing CHEN Jing LI Kai HUANG Miaomiao WEN Qianlai zhuang Licheng LIU peng ZHU Zhenong JIN Shihe XING Liming ZHANG Fujian Provincial Key Laboratory of Soil Environmental Health and Regulation College of Resources and EnvironmentFujian Agriculture and Forestry UniversityFuzhou 350002China State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China Guangxi zhuang Autonomous Region Plant Protection Station Nanjing 530022China Department of Earth Atmosphericand Planetary SciencesPurdue UniversityWest Lafayette IN47907US Department of Bioproducts and Biosystems Engineering University of Minnesota-Twin CitiesSaint Paul MN 55108USA Department of Geography The University of Hong KongHong Kong 999077China

Soil phosphorus (P) plays a vital role in both ecological and agricultural ecosystems, where total P (TP) in soil serves as a crucial indicator of soil fertility and quality. Most of the studies covered in the literature employ a single or narrow range of soil databases, which largely overlooks the impact of utilizing multiple mapping scales in estimating soil TP, especially in hilly topographies. In this study, Fujian Province, a subtropical hilly region along China’s southeast coast covered by a complex topographic environment, was taken as a case study. The influence of the mapping scale on soil TP storage (TPS)estimation was analyzed using six digital soil databases that were derived from 3 082 unique soil profiles at different mapping scales, i.e., 1:50 000 (S5),1:200 000 (S20), 1:500 000 (S50), 1:1 000 000 (S100), 1:4 000 000 (S400), and 1:10 000 000 (S1000). The regional TPS in the surface soil (0–20 cm) based on the S5, S20, S50, S100, S400, and S1000 soil maps was 20.72, 22.17, 23.06, 23.05, 22.04, and 23.48 Tg, respectively, and the corresponding TPS at0–100 cm soil depth was 80.98, 80.71, 85.00, 84.03, 82.96, and 86.72 Tg, respectively. By comparing soil TPS in the S20 to S1000 maps to that in the S5map, the relative deviations were 6.37%–13.32%for 0–20 cm and 0.33%–7.09%for 0–100 cm. Moreover, since the S20 map had the lowest relative deviation among different mapping scales as compared to S5, it could provide additional soil information and a richer soil environment than other smaller mapping scales. Our results also revealed that many uncertainties in soil TPS estimation originated from the lack of detailed soil information, i.e., representation and spatial variations among different soil types. From the time and labor perspectives, our work provides useful guidelines to identify the appropriate mapping scale for estimating regional soil TPS in areas like Fujian Province in subtropical China or other places with similar complex topographies. Moreover,

关键词： agricultural management appropriate mapping scale digitized conventional soil map estimation uncertainty subtropical hilly region

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Simulation of optimal work extraction for quantum systems with work storage

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Chinese Physics B 2024年第2期33卷 195-203页

作者：宋鹏飞张旦波 Key Laboratory of Atomic and Subatomic Structure and Quantum Control(Ministry of Education) and School of PhysicsSouth China Normal UniversityGuangzhou 510006China Guangdong Provincial Key Laboratory of Quantum Engineering and Quantum Materials Guangdong–Hong Kong Joint Laboratory of Quantum Matterand Frontier Research Institute for PhysicsSouth China Normal UniversityGuangzhou 510006China

The capacity to extract work from a quantum heat machine is not only of practical value but also lies at the heart of understanding quantum *** this paper,we investigate optimal work extraction for quantum systems with work storage,where extracting work is completed by a unitary evolution on the composite *** consider the physical requirement of energy conservation both strictly and on *** both,we construct their corresponding unitaries and propose variational quantum algorithms for optimal work *** show that maximal work extraction in general can be feasible when energy conservation is satisfied on *** demonstrate with numeral simulations using a continuous-variable work *** work show an implementation of a variational quantum computing approach for simulating work extraction in quantum systems.

关键词： quantum algorithm quantum thermodyanmics

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Effect of Nb-content on the corrosion resistance of Co-free high entropy alloys in chloride environment

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Tungsten 2024年第4期6卷 778-793页

作者： peng-fei Dai Yang Zhang Sergey Rogozhkin Ji-Hong Han Shu-Wen Li Zhong-Wu Zhang Key Laboratory of Superlight Materials and Surface Technology Ministry of Education College of Materials Science and Chemical Engineering Harbin Engineering University National Research Nuclear University “MEPh I” National Research Center “Kurchatov Institute”

This study investigated the effect of Nb-content on the corrosion behavior of the Al7Cr20Fe35-xNi35Mo3Nbx（x=0,1 and 2）high-entropy alloys in a *** results indicated that only the face centered cubic phase existed in the NbO and Nbl alloys,while the emergence of Laves phase was observed when Nb-content reached 2 at.%.The NbO and Nb1alloys exhibited pitting corrosion,while the NiAl-rich phase experienced localized preferential corrosion in the Nb2 *** electrochemical results revealed that the corrosion current density of the Nbx（x=0,1 and 2） alloys fell within the range of 10-8-10-7A·cm-2,with a pitting corrosion potential exceeding 700 ***,the Nb1 alloy exhibited the most impressive corrosion resistance,as its corrosion current density(7 × 10-8A·cm-2) was merely half that of 316LN stainless *** is attributed to its rapid passivation process,resulting in the development of a protective film characterized by an increased Cr2O3/Al2O3+Cr（OH）*** study highlighted that the addition of Nb contributed to gram refinement,decreased corrosion current density,and elevated pitting potential,favoring passivation and improving corrosion ***,excessive Nb-content resulted in the emergence of the Laves phase,inducing galvanic corrosion and diminishing resistance to corrosion.

关键词： Corrosion High entropy alloys Microstructure Niobium Passive film

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Colonoscopy-assisted removal of an impaction foreign body at the rectosigmoid junction: A case report

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World Journal of Clinical Cases 2024年第11期12卷 1990-1995页

作者： peng-fei Zhou Jin-Gen Lu Jia-Dong Zhang Jia-Wen Wang Department of Anorectal Surgery Longhua Hospital Shanghai University of Traditional Chinese MedicineShanghai 200000China

BACKGROUND When an anorectal foreign body is found,its composition and shape should be evaluated,and a timely and effective treatment plan should be developed based on the patient's symptoms to avoid serious complications such as intestinal perforation caused by displacement of the foreign *** SUMMARY A 54-year-old male was admitted to our outpatient clinic on June 3,2023,due to a rectal foreign body that had been embedded for more than 24 *** patient reported using a glass electrode tube to assist in the recovery of prolapsed hemorrhoids,however,the electrode tube was inadvertently inserted into the anus and could not be removed by the *** hospitalization,the patient underwent surgery,and the foreign body was dragged into the rectum with the aid of *** anus was dilated with a comb-type pulling hook and an anal fistula pulling hook to widen the anus and remove the foreign body,and the local anal symptoms were then relieved with topical *** patient was allowed to eat and drink,and an entire abdominal Computed tomography(CT)and colonoscopy were reviewed 3 d after *** revealed no foreign body residue and colonoscopy showed no metal or other residues in the colon and rectum,and no apparent intestinal tract *** The timeliness and rationality of the surgical and therapeutic options for this patient were based on a literature review of the clinical signs and conceivable conditions in such *** type,material and the potential risks of rectal foreign bodies should be considered.

关键词： Foreign body impaction Surgical therapy Rectum-sigmoid colon Colonoscopy Case report

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Revealing the key role of non-solvating diluents for fast-charging and low temperature Li-ion batteries

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Journal of Energy Chemistry 2024年第7期94卷 171-180页

作者： Yuping Zhang Siyin Li Junkai Shi Jiawei Lai Ziyue zhuang Jingwen Liu Wenming Yang Liang Ma Yue-peng Cai Jijian Xu Qifeng Zheng School of Chemistry Guangzhou Key Laboratory of Materials for Energy Conversion and StorageSouth China Normal UniversityGuangzhou 510006GuangdongChina Guangzhou Foreign Language School Guangzhou 511455GuangdongChina Department of Chemistry City University of Hong KongHong Kong 999077China

Fast-charging and low temperature operation are of vital importance for the further development of lithium-ion batteries(LIBs),which is hindered by the utilization of conventional carbonate-based electrolytes due to their slow kinetics,narrow operating temperature and voltage ***,an acetonitrile(AN)-based localized high-concentration electrolyte(LHCE)is proposed to retain liquid state and high ionic conductivity at ultra-low temperatures while possessing high oxidation *** originally reveal the excellent thermal shielding effect of non-solvating diluent to prevent the aggregation of Li^(+) solvates as temperature drops,maintaining the merits of fast Li transport and facile desolvation as at room temperature,which bestows the graphite electrode with remarkable low temperature performance(264 mA h g^(-1) at-20 C).Remarkably,an extremely high capacity retention of 97%is achieved for high-voltage high-energy graphite||NCM batteries after 250 cycles at-20 C,and a high capacity of 110 mA h g^(-1)(71%of its room-temperature capacity)is retained at-30°*** study unveils the key role of the non-solvating diluents and provides instructive guidance in designing electrolytes towards fast-charging and low temperature LIBs.

关键词： Li-ion battery Fast-charging Low temperature Non-solvating diluent Shielding effect

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Astrometric Observations of NEA 1998 HH49 Using the Daocheng 50 cm Telescope

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Research in Astronomy and Astrophysics 2024年第7期24卷 71-78页

作者： Huan Xu Xiang-Ming Cheng Yi-Gong Zhang Teng-fei Song Zhen-Jun Zhang Qing-Yu peng Yunnan Observatories Chinese Academy of SciencesKunming 650216China University of Chinese Academy of Sciences Beijing 100049China Key Laboratory of the Structure and Evolution of Celestial Objects Chinese Academy of SciencesKunming 650216China Engineering Laboratory on Applied Astronomical Technology of Yunnan Kunming 650216China School of Information Engineering Kunming UniversityKunming 650214China School of Computer Science and Information Engineering Anyang Institute of TechnologyAnyang 455000China Department of Computer Science Jinan UniversityGuangzhou 510632China Sino-French Joint Laboratory for Astrometry Dynamics and Space ScienceJinan UniversityGuangzhou 510632China

This study details an astrometric observation campaign of the Near-Earth Asteroid 1998 HH49,conducted with the aim of refining our understanding of its physical *** the 50 cm telescope located at the Wumingshan Mountain in Daocheng,Sichuan,images were obtained over four nights,from 2023 October 19 to October *** observations were processed using Astrometrica software,facilitating the precise determination of the asteroid's *** observational results were compared with the ephemerides from three distinct sources to verify accuracy:the Jet Propulsion Laboratory(JPL)Horizons System,the Institut de Mécanique Céleste et de Calcul deséphémérides(IMCCE)Miriade,and the Near-Earth Objects Dynamic Site(NEODyS-2).When compared with the JPL ephemeris,a mean observed-minus-calculated(O-C)result of 0.″07 in the *** and-0.″35 in the *** was ***,the comparison with the IMCCE ephemeris yielded mean O-C results of 0.″08 in the *** and-0.″06 in the *** comparison with the NEODyS-2 ephemeris yielded the mean O-C results of 0.″06 in ***-0.″49 in *** study's findings demonstrate a general consistency between the observed data and the ephemeris predictions,with minor discrepancies observed across the data ***,both the JPL and NEODyS-2 ephemerides show that the residuals in the *** exceed those in the *** disparities may result from atmospheric differential color refraction,ephemeris discrepancies,observational errors,and other ***,it is worth noting that further investigation is required due to the potential influence of additional ***,the Daocheng 50 cm Telescope exhibits the ability to conduct high-precision positional measurements.

关键词： astrometry ephemerides time

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