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Structural and functional imaging of brains

Science china Chemistry 2023年第2期66卷 324-366页

作者： Zhichao Liu Ying zhu Liming zhang Weiping Jiang Yawei Liu Qiaowei Tang Xiaoqing Cai Jiang Li Lihua Wang Changlu Tao Xianzhen Yin Xiaowei Li Shangguo Hou Dawei Jiang Kai Liu Xin Zhou Hongjie zhang Maili Liu Chunhai Fan Yang Tian Shanghai Key Laboratory of Green Chemistry and Chemical Processes School of Chemistry and Molecular EngineeringEast China Normal UniversityShanghai200241China Interdisciplinary Research center Shanghai Synchrotron Radiation FacilityZhangjiang LaboratoryShanghai Advanced Research InstituteChinese Academy of SciencesUniversity of Chinese Academy of SciencesShanghai201210China State Key Laboratory of Magnetic Resonance and Atomic and Molecular physics Chinese Academy of SciencesWuhan National Laboratory for OptoelectronicsWuhan430071China State Key Laboratory of Rare Earth Resource Utilization Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun130022China department of Chemistry Tsinghua UniversityBeijing100084China School of Chemistry and Chemical Engineering Frontiers Science Center for Transformative MoleculesInstitute of Translational MedicineShanghai Jiao Tong UniversityShanghai200240China Interdisciplinary center for Brain Information Brain Cognition and Brain Disease InstituteShenzhen-Hong Kong Institute of Brain Science-Shenzhen Fundamental Research InstitutionsFaculty of Life and Health SciencesShenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen518055China lingang Laboratory Shanghai201602China School of Biomedical Engineering Shanghai Jiao Tong UniversityShanghai200240China Institute of Systems and Physical Biology Shenzhen Bay LaboratoryShenzhen518055China department of Nuclear Medicine Union HospitalTongji Medical CollegeHuazhong University of Science and TechnologyWuhan430022China

Analyzing the complex structures and functions of brain is the key issue to understanding the physiological and pathological *** neuronal morphology and local distribution of neurons/blood vessels in the brain have been known,the subcellular structures of cells remain challenging,especially in the live *** addition,the complicated brain functions involve numerous functional molecules,but the concentrations,distributions and interactions of these molecules in the brain are still poorly *** this review,frontier techniques available for multiscale structure imaging from organelles to the whole brain are first overviewed,including magnetic resonance imaging(MRI),computed tomography(CT),positron emission tomography(PET),serial-section electron microscopy(ss EM),light microscopy(LM)and synchrotron-based X-ray microscopy(XRM).Specially,XRM for three-dimensional(3D)imaging of large-scale brain tissue with high resolution and fast imaging speed is ***,the development of elegant methods for acquisition of brain functions from electrical/chemical signals in the brain is *** particular,the new electrophysiology technologies for neural recordings at the single-neuron level and in the brain are also *** also focus on the construction of electrochemical probes based on dual-recognition strategy and surface/interface chemistry for determination of chemical species in the brain with high selectivity and long-term stability,as well as electrochemophysiological microarray for simultaneously recording of electrochemical and electrophysiological signals in the ***,the recent development of brain MRI probes with high contrast-to-noise ratio(CNR)and sensitivity based on hyperpolarized techniques and multi-nuclear chemistry is ***,multiple optical probes and instruments,especially the optophysiological Raman probes and fiber Raman photometry,for imaging and biosensing in live brain are emphas

关键词： brain structure brain function brain chemistry chemical signal biosensing and bioimaging

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太赫兹辅助测量铷原子超快量子相干过程的理论研究

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物理学报 2020年第17期69卷 70-76页

作者：凌中火王帅张金仓张逸竹阎天民江玉海上海大学物理系材料基因组工程研究院上海200444 中国科学院上海高等研究院上海201210 天津大学精密仪器与光电子工程学院太赫兹研究中心天津300072 中国科学院大学北京100049 上海科技大学上海201210

太赫兹辅助光电离瞬态测量方法可以分辨超快量子拍频,同时对复杂量子系统的超快密度矩阵演化进行成像.本文依据这种方法提出了一种具体的实验方案,利用紫外脉冲(脉宽为30 fs)和高强度太赫兹脉冲(峰值场强:约1 MV/cm)组成复合探测电场,... 详细信息

太赫兹辅助光电离瞬态测量方法可以分辨超快量子拍频,同时对复杂量子系统的超快密度矩阵演化进行成像.本文依据这种方法提出了一种具体的实验方案,利用紫外脉冲(脉宽为30 fs)和高强度太赫兹脉冲(峰值场强:约1 MV/cm)组成复合探测电场,探测铷原子5S1/2.5P3/2.加态振荡周期约为2.6 fs的量子拍频过程,量子体系密度矩阵演化的布居项和相干项投影在光电子动量谱的不同位置,可以对密度矩阵演化实现完全信息测量.本文设计的实验方案不需要阿秒高次谐波或自由电子激光等复杂的先进光源,可以成为探索复杂量子体系超快相干动力学过程的新方案.

关键词：超快量子相干动力学密度矩阵量子拍频太赫兹激光

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Experimental evidence of the thickness- and electric-field-dependent topological phase transitions intopological crystalline insulator SnTe（111） thin films

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Nano Research 2018年第11期11卷 6045-6050页

作者： Yan Gong Kejing zhu Zhe Li Yunyi Zang Xiao Feng Ding zhang Canli Song Lili Wang Wei Li Xi Chen Xu-Cun Ma Qi-Kun Xue Yong Xu Ke He State Key Laboratory of Low-Dimensional Quantum physics Department of Physics Tsinghua University Beijing 100084 China Collaborative Innovation center of Quantum Matter 8eijing 100084 China

Using in situ angle-resolved photoemission spectroscopy, we systematically studied molecular-beam-epitaxy-grown topological crystalline insulator SnTe(111) thin films with varied thicknesses and substrate conditions. An oscillation in the band gap size with an increase in thickness was observed to depend on the electric field perpendicular to the films. The observations are consistent with the theoretically predicted thickness- and electric-field-dependent topological phase transitions between the normal insulator and the quantum spin Hall insulator phases in SnTe(111) films and demonstrate them to be an excellent and electrically tunable quantum spin Hall system.

关键词： topological crystalline insulator SnTe quantum spin Hall effect field effect

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Kinetic study of transverse electron-scale interface instability in relativistic shear flows

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Matter and Radiation at Extremes 2020年第5期5卷 12-19页

作者： Peilin Yao Hongbo Cai Xinxin Yan Wenshuai zhang Bao Du Jianmin Tian Enhao zhang Xuewu Wang Shaoping {2. department of Engineering physics Tsinghua UniversityBeijing 100084China Institute of Applied physics and Computational Mathematics Beijing 100094China center for Applied physics and Technology HEDPSand College of EngineeringPeking UniversityBeijing 100871China center for Applied physics and Technology HEDPSSchool of Physicsand College of EngineeringPeking UniversityBeijing 100871China Graduate School China Academy of Engineering PhysicsBeijing 100088China

Interfacial magnetic field structures induced by transverse electron-scale shear instability(mushroom instability)are found to be strongly associated with electron and ion dynamics,which in turn will influence the development of the instability *** find that high-frequency electron oscillations are excited normal to the shear ***,on a larger time scale,the bulk of the ions are gradually separated under the influence of local magnetic fields,eventually reaching an equilibrium related to the initial shear *** a theoretical model of this *** separation on the scale of the electron skin depth will prevent different ions from mixing and will thereafter restrain the growth of higher-order *** also analyze the role of electron thermal motion in the generation of the magnetic field,and we find an increase in the instability growth rate with increasing plasma *** results have potential for providing a more realistic description of relativistic plasma flows.

关键词： temperature. relativistic transverse

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The THU-NAOC transient survey: the performance and results from the first year

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Research in Astronomy and astrophysics 2015年第2期15卷 215-224页

作者： Tian-Meng zhang Xiao-Feng Wang Jun-Cheng Chen Ju-Jia zhang Li Zhou Wen-Xiong Li Qing Liu Jun Mo Kai-Cheng zhang Xin-Yu Yao Xu-Lin Zhao Xu Zhou Jun-Dan Nie Fang Huang Zhao-Ji Jiang Jun Ma ling-Zhi Wang Chao Wu Zhi-Min Zhou Hu Zou Li-Fan Wang Key Laboratory of Optical Astronomy National Astronomical Observatories Chinese Academy of Sciences physics department and {2. center for astrophysics Tsinghua University Yunnan Observatories Chinese Academy of Sciences Key Laboratory for the Structure and Evolution of Celestial Objects Chinese Academy of Sciences university of Chinese Academy of Sciences Purple Mountain Observatory Chinese Academy of Sciences Astronomy department Beijing Normal University National Astronomical Observatories Chinese Academy of Sciences

The tsinghua university-National Astronomical Observatories, Chinese Academy of Sciences （NAOC） Transient Survey is an automatic survey that conducts a systematic exploration of optical transients. This project utilizes a 60/90 cm Schmidt telescope at the Xinglong Station of NAOC. This survey repeatedly covers - 1000 square degrees of the northern sky with a cadence of 34 d. With an exposure of 60 s, the survey reaches a limiting unfiltered magnitude of about 19.5 mag, which enables us to discover supernovae in their relatively young stages. We describe the overall performance of our survey during the first year and present some preliminary results.

关键词： supernovae quasars and active galactic nuclei stars

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Determination of the number ofψ(3686)events taken at BESⅢ

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Chinese physics C 2024年第9期48卷 8-20页

作者： M.Ablikim M.N.Achasov P.Adlarson O.Afedulidis X.C.Ai R.Aliberti A.Amoroso Q.An Y.Bai O.Bakina I.Balossino Y.Ban H.-R.Bao V.Batozskaya K.Begzsuren N.Berger M.Berlowski M.Bertani D.Bettoni F.Bianchi E.Bianco A.Bortone I.Boyko R.A.Briere A.Brueggemann H.Cai X.Cai A.Calcaterra G.F.Cao N.Cao S.A.Cetin J.F.Chang G.R.Che G.Chelkov C.Chen C.H.Chen Chao Chen G.Chen H.S.Chen H.Y.Chen M.L.Chen S.J.Chen S.L.Chen S.M.Chen T.Chen X.R.Chen X.T.Chen Y.B.Chen Y.Q.Chen Z.J.Chen Z.Y.Chen S.K.Choi G.Cibinetto F.Cossio J.J.Cui H.L.Dai J.P.Dai A.Dbeyssi R.E.de Boer D.Dedovich C.Q.Deng Z.Y.Deng A.Denig I.Denysenko M.Destefanis F.De Mori B.Ding X.X.Ding Y.Ding Y.Ding J.Dong L.Y.Dong M.Y.Dong X.Dong M.C.Du S.X.Du Y.Y.Duan Z.H.Duan P.Egorov Y.H.Fan J.Fang J.Fang S.S.Fang W.X.Fang Y.Fang Y.Q.Fang R.Farinelli L.Fava F.Feldbauer G.Felici C.Q.Feng J.H.Feng Y.T.Feng M.Fritsch C.D.Fu J.L.Fu Y.W.Fu H.Gao X.B.Gao Y.N.Gao Yang Gao S.Garbolino I.Garzia L.Ge P.T.Ge Z.W.Ge C.Geng E.M.Gersabeck A.Gilman K.Goetzen L.Gong W.X.Gong W.Gradl S.Gramigna M.Greco M.H.Gu Y.T.Gu C.Y.Guan Z.L.Guan A.Q.Guo L.B.Guo M.J.Guo R.P.Guo Y.P.Guo A.Guskov J.Gutierrez K.L.Han T.T.Han F.Hanisch X.Q.Hao F.A.Harris K.K.He K.L.He F.H.Heinsius C.H.Heinz Y.K.Heng C.Herold T.Holtmann P.C.Hong G.Y.Hou X.T.Hou Y.R.Hou Z.L.Hou B.Y.Hu H.M.Hu J.F.Hu S.L.Hu T.Hu Y.Hu G.S.Huang K.X.Huang L.Q.Huang X.T.Huang Y.P.Huang T.Hussain F.Hölzken N.Hüsken N.in der Wiesche J.Jackson S.Janchiv J.H.Jeong Q.Ji Q.P.Ji W.Ji X.B.Ji X.L.Ji Y.Y.Ji X.Q.Jia Z.K.Jia D.Jiang H.B.Jiang P.C.Jiang S.S.Jiang T.J.Jiang X.S.Jiang Y.Jiang J.B.Jiao J.K.Jiao Z.Jiao S.Jin Y.Jin M.Q.Jing X.M.Jing T.Johansson S.Kabana N.Kalantar-Nayestanaki X.L.Kang X.S.Kang M.Kavatsyuk B.C.Ke V.Khachatryan A.Khoukaz R.Kiuchi O.B.Kolcu B.Kopf M.Kuessner X.Kui N.Kumar A.Kupsc W.Kühn J.J.Lane P.Larin L.Lavezzi T.T.Lei Z.H.Lei M.Lellmann T.Lenz C.Li C.Li C.H.Li Cheng Li D.M.Li F.Li G.Li H.B.Li H.J.Li H.N.Li Hui Li J.R.Li J.S.Li Ke Li L.J.Li L.K.Li Lei Li M.H.Li P.R.Li Q.M.Li Q.X.Li R.Li S.X.Li T.Li W.D.Li W.G.Li X.Li X.H.Li X.L.Li X.Z.Li Xi Institute of High Energy physics Beijing 100049China Beihang university Beijing 100191China Bochum Ruhr-university D-44780BochumGermany Budker Institute of Nuclear physics SB RAS(BINP) Novosibirsk 630090Russia Carnegie Mellon university PittsburghPennsylvania 15213USA Central china Normal university Wuhan 430079China Central South university Changsha 410083China china center of Advanced Science and Technology Beijing 100190China china university of Geosciences Wuhan 430074China Chung-Ang university Seoul06974Republic of Korea COMSATS university Islamabad Lahore CampusDefence RoadOff Raiwind Road54000LahorePakistan Fudan university Shanghai 200433China GSI Helmholtzcentre for Heavy Ion Research GmbH D-64291DarmstadtGermany Guangxi Normal university Guilin 541004China Guangxi university Nanning 530004China Hangzhou Normal university Hangzhou 310036China Hebei university Baoding 071002China Helmholtz Institute Mainz Staudinger Weg 18D-55099MainzGermany Henan Normal university Xinxiang 453007China Henan university Kaifeng 475004China Henan university of Science and Technology Luoyang 471003China Henan university of Technology Zhengzhou 450001China Huangshan College Huangshan 245000China Hunan Normal university Changsha 410081China Hunan university Changsha 410082China Indian Institute of Technology Madras Chennai 600036India Indiana university BloomingtonIndiana 47405USA INFN Laboratori Nazionali di Frascati (A)INFN Laboratori Nazionali di FrascatiI-00044FrascatiItaly(B)INFN Sezione di PerugiaI-06100PerugiaItaly(C)University of PerugiaI-06100PerugiaItaly INFN Sezione di Ferrara (A)INFN Sezione di FerraraI-44122FerraraItaly(B)University of FerraraI-44122FerraraItaly Inner Mongolia university Hohhot 010021China Institute of Modern physics Lanzhou 730000China Institute of physics and Technology Peace Avenue 54BUlaanbaatar 13330Mongolia Instituto de Alta Investigación Universidad de TarapacáCasilla 7DArica 1000000Chile Jilin university Changchun 130012China Joha

The number ofψ(3686)events collected by the BESⅢdetector during the 2.2. run period is determined to be(2.59.3±11.1)×10~6 by counting inclusiveψ(3686)hadronic *** uncertainty is systematic and the statistical uncertainty is ***,the numbers ofψ(3686)events collected during the 2.09 and 2.12.un periods are updated to be(107.7±0.6)×10~6 and(345.4±2.6)×10~6,*** numbers are consistent with the previous measurements within one standard *** total number ofψ(3686)events in the three data samples is(2.12.4±14.3)×10~6.

关键词： ψ(3686) inclusive process Hadronic events BESⅢdetector

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Bioresource Upgrade for Sustainable Energy,Environment,and Biomedicine

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Nano-Micro Letters 2023年第3期15卷 48-97页

作者： Fanghua Li Yiwei Li KSNovoselov Feng Liang Jiashen Meng Shih‑Hsin Ho Tong Zhao Hui Zhou Awais Ahmad Yinlong zhu Liangxing Hu Dongxiao Ji Litao Jia Rui Liu Seeram Ramakrishna Xingcai zhang center for Nanofibers and Nanotechnology National University of SingaporeSingapore 119260Singapore State Key Laboratory of Urban Water Resource and Environment Harbin Institute of TechnologyHarbin 150090People’s Republic of China School of Engineering Massachusetts Institute of TechnologyCambridgeMA 02139USA John A Paulson School of Engineering and Applied Sciences Harvard UniversityCambridgeMA 02138USA The Key Laboratory for Biomedical Photonics of MOE at Wuhan National Laboratory for Optoelectronics–department of Biomedical Engineering College of Life Science and TechnologyHuazhong University of Science and TechnologyWuhanHubei 430074People’s Republic of China Centre for Advanced 2. Materials National University of SingaporeSingapore 117546Singapore School of physics and Astronomy The University of ManchesterManchester M139PLUK department of Anesthesia Critical Care and Pain MedicineMassachusetts General Hospital and Harvard Medical SchoolBostonMA 02114USA department of Energy and Power Engineering Tsinghua UniversityBeijing 100084People’s Republic of China Departamento de Quimica Organica Universidad de CordobaEdificio Marie Curie(C‑3)Ctra Nnal IV‑AKm 39614014 CordobaSpain department of Chemical Engineering Monash UniversityClaytonVIC 3800Australia School of Mechanical and Aerospace Engineering Nanyang Technological UniversitySingapore 639798Singapore

We conceptualize bioresource upgrade for sustainable energy,environment,and biomedicine with a focus on circular economy,sustainability,and carbon neutrality using high availability and low utilization biomass(HALUB).We acme energy-efficient technologies for sustainable energy and material recovery and *** technologies of thermochemical conversion(TC),biochemical conversion(BC),electrochemical conversion(EC),and photochemical conversion(PTC)are summarized for *** biomass could contribute to a biofuel HHV of 35.72.MJ Kg^(-1)and total benefit of 749$/ton biomass via *** surface area of biochar reached 3000 m^(2.g^(-1)via pyrolytic carbonization of waste bean *** biomass can be effectively converted into bio-stimulants and biofertilizers via BC with a high conversion efficiency of more than 90%.Besides,lignocellulosic biomass can contribute to a current density of 672.mA m^(-2.via *** can be 100%selectively synthesized via electrocatalysis through EC and *** learning,techno-economic analysis,and life cycle analysis are essential to various upgrading approaches of *** biomaterials,sustainable living materials and technologies for biomedical and multifunctional applications like nano-catalysis,microfluidic and micro/nanomotors beyond are also *** techniques and systems for the complete conversion and utilization of HALUB for new energy and materials are further discussed.

关键词： High availability low utilization biomass(HALUB) Circular economy Machine learning Energy-efficient conversion Nano-catalysis

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Overview to the Hard X-ray Modulation Telescope (Insight-HXMT) Satellite

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Science china(physics,Mechanics & Astronomy) 2020年第4期63卷 2-19页

作者： Shuang-Nan zhang TiPei Li FangJun Lu LiMing Song YuPeng X u CongZhan Liu Yong Chen XueLei Cao QingCui Bu Zhi Chang Gang Chen Li Chen TianXiang Chen YiBao Chen YuPeng Chen Wei Cui WeiWei Cui JingKang Deng YongWei Dong Yuan Yuan Du MinXue Fu GuanHua Gao He Gao Min Gao MingYu Ge YuDong Gu Ju Guan Can Gungor ChengCheng Guo DaWei Han Wei Hu Yue Huang Jia Huo ShuMei Jia LuHua Jiang WeiChun Jiang Jing Jin YongJie Jin Bing Li ChengKui Li Gang Li MaoShun Li Wei Li Xian Li XiaoBo Li XuFang Li YanGuo Li ZiJian Li ZhengWei Li XiaoHua Liang JinYuan Liao GuoQing Liu HongWei Liu ShaoZhen Liu XiaoJing Liu Yuan Liu YiNong Liu Bo Lu XueFeng Lu Tao Luo Xiang Ma Bin Meng Yi Nang JianYin Nie Ge Ou JinLu Qu Na Sai RenCheng Shang GuoHong Shen Liang Sun Ying Tan Lian Tao YouLi Tuo Chen Wang ChunQin Wang GuoFeng Wang HuanYu Wang Juan Wang WenShuai Wang YuSa Wang XiangYang Wen BaiYang Wu BoBing Wu Mei Wu GuangCheng Xiao ShaoLin Xiong LinLi Yan JiaWei Yang Sheng Yang YanJi Yang QiBin Yi Bin Yuan AiMei zhang ChunLei zhang ChengMo zhang Fan zhang HongMei zhang Juan zhang Qiang zhang ShenYi zhangs Shu zhang Tong zhang WanChang zhang Wei zhang WenZhao zhang Yi zhang YiFei zhang YongJie zhang Yue zhang Zhao zhang Zhi zhang ZiLiang zhang HaiSheng Zhao XiaoFan Zhao ShiJie Zheng JianFeng Zhou YuXuan zhu Yue zhu RenLin zhuang Key Laboratory of Particle astrophysics Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China university of Chinese Academy of Sciences Beijing 100049China department of Astronomy Tsinghua UniversityBeijing 100084China department of physics Tsinghua UniversityBeijing 100084China department of Astronomy Beijing Normal UniversityBeijing 100088China department of Engineering physics Tsinghua UniversityBeijing 100084China National Astronomical Observatories Chinese Academy of SciencesBeijing 100101China National Space Science center Chinese Academy of SciencesBeijing 100190China

As china’s first X-ray astronomical satellite, the Hard X-ray Modulation Telescope (HXMT), which was dubbed as Insight-HXMT after the launch on June 15, 2.17, is a wide-band(1-2.0 ke V) slat-collimator-based X-ray astronomy satellite with the capability of all-sky monitoring in 0.2.3 Me V. It was designed to perform pointing, scanning and gamma-ray burst(GRB)observations and, based on the Direct Demodulation Method (DDM), the image of the scanned sky region can be *** we give an overview of the mission and its progresses, including payload, core sciences, ground calibration/facility, ground segment, data archive, software, in-orbit performance, calibration, background model, observations and some preliminary results.

关键词： X-and γ-ray telescopes and instrumentation neutron stars black holes X-ray binaries γ-ray bursts

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Review on recent progress in on-line monitoring technology for atmospheric pollution source emissions in china

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Journal of Environmental Sciences 2023年第1期123卷 367-386页

作者： Huanqin Wang Jitong Zhou Xue Li Qiang ling Hongyuan Wei Lei Gao Ying He Ming zhu Xiao Xiao Youjiang Liu Shan Li Chilai Chen Guotao Duan Zhimin Peng Peili Zhou Yufeng Duan Jianbing Wang Tongzhu Yu Yixin Yang Jiguang Wang Zhen Zhou Huaqiao Gui Yanjun Ding State Key Laboratory of Transducer Technology Institute of Intelligent MachinesHefei Institutes of Physical ScienceChinese Academy of SciencesHefei 230031China Institute of Mass Spectrometry and Atmospheric Environment Jinan UniversityGuangzhou 510632China department of Automation University of Science and Technology of ChinaHefei 230027China china Automotive Technology and Research center Tianjin 300300China Institute of Solid State physics Chinese Academy of SciencesHefei 230031China Key Laboratory of Environmental Optics and Technology Anhui Institute of Optics and Fine MechanicsChinese Academy of SciencesHefei 230031China School of Electronic Information and Communications Huazhong University of Science and TechnologyWuhan 430074China School of Optical and Electronic Information Huazhong University of Science and TechnologyWuhan 430074China State Key Laboratory of Power Systems Department of Energy and Power EngineeringTsinghua UniversityBeijing 100084China Key Laboratory of Energy Thermal Conversion and Control of Ministry of Education School of Energy and EnvironmentSoutheast UniversityNanjing 210096China School of Chemical and Environmental Engineering China University of Mining and Technology(Beijing)Beijing 100083China CAS center for Excellence in Regional Atmospheric Environment Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China

Emissions from mobile sources and stationary sources contribute to atmospheric pollution in china,and its components,which include ultrafine particles(UFPs),volatile organic compounds(VOCs),and other reactive gases,such as NH3and NOx,are the most harmful to human *** has released various regulations and standards to address pollution from mobile and stationary ***,it is urgent to develop online monitoring technology for atmospheric pollution source *** study provides an overview of the main progress in mobile and stationary source monitoring technology in china and describes the comprehensive application of some typical instruments in vital areas in recent *** instruments have been applied to monitor emissions from motor vehicles,ships,airports,the chemical industry,and electric power *** only has the level of atmospheric environment monitoring technology and equipment been improving,but relevant regulations and standards have also been constantly ***,the developed instruments can provide scientific assistance for the successful implementation of *** to the potential problem areas in atmospheric pollution in china,some research hotspots and future trends of atmospheric online monitoring technology are ***,more advanced atmospheric online monitoring technology will contribute to a comprehensive understanding of atmospheric pollution and improve environmental monitoring capacity.

关键词： Atmospheric pollution Mobile sources Stationary sources On-line monitoring technology

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Atomically dispersed Ni anchored on polymer-derived mesh-like Ndoped carbon nanofibers as an efficient CO_(2. electrocatalytic reduction catalyst

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Nano Research 2022年第5期15卷 3959-3963页

作者： Tai Cao Rui Lin Shoujie Liu Weng-Chon(Max)Cheong Zhi Li Konglin Wu Youqi zhu Xiaolu Wang Jian zhang Qiheng Li Xiao Liang Ninghua Fu Chen Chen Dingsheng Wang Qing Peng Yadong Li department of Chemistry Tsinghua UniversityBeijing 100084China College of Chemistry and Materials Science Anhui Normal UniversityWuhu 241000China department of physics and Chemistry Faculty of Science and TechnologyUniversity of MacaoMacao SARChina Research center of Materials Science Beijing Key Laboratory of Construction Tailorable Advanced Functional Materials and Green ApplicationsBeijing Institute of TechnologyBeijing 100081China

Efficient electroreduction of CO_(2. into CO and other chemicals turns greenhouse gases into fuels and value-added chemicals,holding great promise for a closed carbon cycle and the alleviation of climate ***,there are still challenges in the large-scale application of CO_(2. electroreduction due to the sluggish *** we develop a self-assembly strategy to synthesize a highly efficient CO_(2. reduction electrocatalyst with atomically dispersed Ni-N_(4) active centers anchored on polymerderived mesh-like N-doped carbon nanofibers(Ni-N_(4)/NC).The Ni-N_(4)/NC exhibits high selectivity for CO_(2. reduction reaction with CO Faradaic efficiency(CO FE)above 90% over a wide potential range from−0.6 to−1.0 V *** catalyst reaches a maximum CO FE up to 98.4% at−0.8 V with a TOF of 1.2.×10^(5) h^(–1) and Tafel slope of 113 mV·dec^(–1).The catalyst also exhibits remarkable stability,with little change in current density and CO FE over a 10-hour durability test at–0.8 V *** method provides a new route for the synthesis of highly efficient CO_(2. reduction electrocatalyst.

关键词： CO_(2.reduction reaction Ni-N_(4)site Ni single atoms self-assembly

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