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秸秆与有机无机肥配施对潮土关键微生物及小麦产量的影响

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土壤学报 2024年第4期61卷 1134-1146页

作者：郭伟周云鹏陈美淇李丹丹王青霞周谈坛赵炳梓土壤与农业可持续发展国家重点实验室(中国科学院南京土壤研究所) 南京210008 中国科学院大学北京100049 中国科学院大学南京学院南京211135

秸秆与化肥和鸡粪配施改变了土壤微生物群落结构及微生物间的相互作用关系,但这种变化与小麦产量间的关系尚不清楚。依托7年长期定位试验,选取5个施肥处理:不施化肥+秸秆离田(N0S0)、不施化肥+秸秆还田(N0S)、常规施化肥+秸秆离田(NS0)... 详细信息

秸秆与化肥和鸡粪配施改变了土壤微生物群落结构及微生物间的相互作用关系,但这种变化与小麦产量间的关系尚不清楚。依托7年长期定位试验,选取5个施肥处理:不施化肥+秸秆离田(N0S0)、不施化肥+秸秆还田(N0S)、常规施化肥+秸秆离田(NS0)、常规施化肥+秸秆还田(NS)和施化肥+秸秆还田+鸡粪替代20%氮肥(NSM),研究不同施肥方式对细菌-真菌共现网络中微生物组成的影响,以及关键微生物与小麦产量间的相关关系。结果表明,与N0S0处理相比,NS0、NS和NSM处理的小麦籽粒产量分别提升539.20%、611.56%和676.56%,而N0S处理无显著变化。细菌和真菌群落组成均可分成显著不同的3组,分别为N0S0+N0S、NS0以及NS+NSM,即微生物群落组成在是否施用化肥之间显著不同;相同施用化肥情况下,在是否有施用有机物料之间显著不同。将重要性由高到低排序,导致不同处理细菌群落结构变化的主要土壤理化性质是有效磷(AP)、电导率(EC)、微生物生物量氮(MBN)、土壤有机碳(SOC)、易氧化有机碳(ROC)和颗粒有机碳(POC),导致不同处理真菌群落结构变化的主要土壤理化性质是EC、MBN、ROC、POC、AP和SOC。细菌-真菌共现网络中,两个关键模块(模块1和模块4)与小麦产量变化显著相关。NS+NSM处理提升了模块4中与小麦产量正相关的类诺卡氏菌属(Nocardioides)、纤维单胞菌属(Cellulomonas)、Pir4_lineage、金孢子菌属(Chrysosporium)、无茎真菌属(Acaulium)和裂壳菌属(Schizothecium)等有益菌的相对丰度,它们可降解纤维素和木质素、促进养分转化和循环或抑制病原菌生长;并显著降低了模块1中与小麦产量负相关的葡萄穗霉属(Stachybotrys)、无色穗孢属(Achroiostachys)和Fusicolla的相对丰度,它们为不利于土壤健康和作物生长的植物病原真菌。因此,化肥配施秸秆及化肥配施秸秆和鸡粪利于关键有益微生物增加及病原真菌减少,关键微生物的功能和相对丰度对小麦产量具有影响。

关键词：秸秆还田有机肥细菌-真菌共现网络关键微生物小麦产量

秸秆与有机无机肥配施对不同质地潮土土壤质量和小麦产量的影响

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土壤学报 2024年第5期61卷 1360-1373页

作者：郭伟李丹丹徐基胜周云鹏王青霞周谈坛赵炳梓土壤与农业可持续发展国家重点实验室(中国科学院南京土壤研究所) 南京211135 中国科学院大学北京100049 中国科学院大学南京学院南京211135

秸秆与化肥和粪肥配施是改善土壤质量的有效措施,但其在不同质地潮土中对小麦产量的影响及影响机制尚不清楚。本研究基于中国科学院封丘农业生态实验站设置的7年长期定位试验,选取砂质、壤质和黏质3种质地潮土(下文分别简称砂土、壤土... 详细信息

秸秆与化肥和粪肥配施是改善土壤质量的有效措施,但其在不同质地潮土中对小麦产量的影响及影响机制尚不清楚。本研究基于中国科学院封丘农业生态实验站设置的7年长期定位试验,选取砂质、壤质和黏质3种质地潮土(下文分别简称砂土、壤土和黏土),每种质地潮土均包含5个处理:不施化肥+秸秆离田(N0S0)、不施化肥+秸秆还田(N0S)、常规施化肥+秸秆离田(NS0)、常规施化肥+秸秆还田(NS)和施化肥+秸秆还田+鸡粪替代20%氮肥(NSM),研究了不同施肥模式在不同质地潮土中对土壤质量和小麦产量的影响。结果表明,在砂土、壤土和黏土中,与N0S0处理相比,NS处理的籽粒产量分别增加611.56%、440.00%和403.55%,NSM处理的籽粒产量分别增加676.56%、546.67%和492.86%。在砂土、壤土和黏土中,与N0S0处理相比,N0S和NS0处理的土壤质量指数(SQI)显著提升,NS处理则进一步提升。NSM处理在砂土中SQI优于NS处理,但在壤土和黏土中与NS处理无显著差异。随机森林分析表明,砂土中,pH、碱解氮(AHN)、可溶性有机氮(DON)、有效磷(AP)、有机碳(SOC)和速效钾(AK)是影响籽粒产量的关键土壤性质;壤土中,AP、pH、AK、AHN、微生物生物量碳(MBC)和SOC是影响籽粒产量的关键土壤性质;黏土中,AP、DON、AHN和pH是影响籽粒产量的关键土壤性质。偏最小二乘路径模型表明,在砂土、壤土和黏土中,影响小麦产量的关键土壤性质均受施肥模式显著调控,且均对SQI具有显著影响,而SQI均对小麦籽粒产量具有直接显著影响,影响小麦产量的关键土壤性质可以作为监测土壤质量和小麦产量变化的指标以指导优化施肥。此外,在壤土中,SQI还通过影响小麦产量构成因素而间接影响籽粒产量。因此,秸秆与化肥和鸡粪配施改善了土壤质量,并在不同质地潮土中通过不同作用方式直接或间接影响了小麦产量。

关键词：秸秆还田有机肥化肥土壤质量养分含量小麦产量

长期不同氮肥施用量对潮土团聚体分布和真菌群落组成的影响

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土壤学报 2024年第3期61卷 824-835页

作者：郭伟周云鹏陈美淇李丹丹王青霞马东豪赵炳梓土壤与农业可持续发展国家重点实验室(中国科学院南京土壤研究所) 南京210008 中国科学院大学北京100049 中国科学院大学南京学院南京211135

不同氮肥施用量显著改变团聚体分布、真菌群落组成及生物胶结物质的产生,但它们之间是否存在相关性尚不清楚。以中国科学院封丘农业生态实验站长期定位试验(2005—2020年)为研究平台,其包含5个施氮水平:0(F0)、150 kg·hm^(–2)(F1)、19... 详细信息

不同氮肥施用量显著改变团聚体分布、真菌群落组成及生物胶结物质的产生,但它们之间是否存在相关性尚不清楚。以中国科学院封丘农业生态实验站长期定位试验(2005—2020年)为研究平台,其包含5个施氮水平:0(F0)、150 kg·hm^(–2)(F1)、190 kg·hm^(–2)(F2)、230 kg·hm^(–2)(F3)和270 kg·hm^(–2)(F4),研究了不同施氮量对土壤团聚体组成(>2000μm、2000~250μm、250~53μm和<53μm)的影响,以及团聚体组成与生物胶结物质(球囊霉素相关土壤蛋白(GRSP)及微生物生物量碳(MBC))和土壤真菌之间的相关关系。结果表明,土壤团聚体分布和真菌群落组成分为显著不同的3组,分别为F0、F1和F2以及F3和F4,其中,(1)F1和F2处理团聚体平均重量直径(MWD)最高,同时大于2000μm团聚体的质量比例显著增加,并与拟棘壳孢属(Pyrenochaetopsis)富集有关;(2)F1和F2、F3和F4处理均表现为2000~250μm团聚体的质量比例增加,而小于53μm粉黏粒质量比例显著降低,2000~250μm团聚体的质量比例增加主要与易提取球囊霉素和总球囊霉素相关土壤蛋白比值(EE-GRSP/T-GRSP)以及易提取球囊霉素相关土壤蛋白(EE-GRSP)显著正相关,而与亚隔孢壳属(Didymella)和被孢霉属(Mortierella)相对丰度显著负相关;小于53μm粉黏粒质量比例显著降低主要与被孢霉属(Mortierella)、白腐菌属(Phlebia)、黑孢壳属(Melanospora)、Fusicolla、柄孢壳属(Podospora)和亚隔孢壳属(Didymella)相对丰度显著正相关,而与EE-GRSP和/或支顶孢属(Acremonium)、柱霉属(Scytalidium)、外瓶霉属(Exophiala)、EE-GRSP/T-GRSP、MBC显著负相关。因此,土壤团聚体稳定性的变异程度受氮肥施用水平影响。本研究条件下,150 kg·hm^(–2)和190 kg·hm^(–2)施氮水平下的团聚体稳定性超过230 kg·hm^(–2)和270 kg·hm^(–2)施氮水平,与不同施氮量下真菌群落组成及其胶结物质变化显著相关。

关键词：长期试验施氮水平团聚体稳定性生物胶结物质真菌群落

Dual-functional pyrene implemented mesoporous silicon material used for the detection and adsorption of metal ions

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中国化学工程学报:英文版 2023年第8期60卷 108-117页

作者： Jing Huang Honghui Cai Qian Zhao yunpeng zhou Haibo Liu Jing Wang School of Chemistry and Chemical Engineering Guangxi UniversityNanning 530004China

A fluorescent active organic–inorganic hybrid material Py N-SBA-15 was synthesized by implementing pyrene derivatives into mesoporous SBA-15 *** N-SBA-15 had detection and removal functionalities toward Al^(3+),Cu^(2+),and Hg^(2+).On the one hand,Py N-SBA-15 was used as a fluorescence sensor and displayed high sensitivity toward Al^(3+),Cu^(2+),and Hg^(2+)cations (limit of detection:8.0×10^(-7),1.1×10^(-7),and 2.9×10^(-6)mol·L^(–1),respectively) among various analytes with“turn-off”*** the other hand,the adsorption studies for these toxic analytes (Cu^(2+),Hg^(2+),and Al^(3+)) showed that the ion removal capacity could reach up to 45,581,and 85 mg·g^(-1),***,the Langmuir isotherm models were better fitted with the adsorption data,indicating that the adsorption was mono-layer *** analysis revealed that the adsorption process was well described by the pseudo-second-order kinetic model for Cu^(2+)and Hg^(2+)and pseudo-first-order kinetic model for Al^(3+).The prepared silica material could be reused in four recycles without significantly decreasing its adsorption ***,the Py N-SBA-15 material can serve as a promising candidate for the simultaneous rapid detection and efficient adsorption of metal ions.

关键词： Dual function Nanomaterials Mesoporous silica Metal ions Detection and adsorption

Rare Earth Ion Yb^3+ Doping of Bi2WO6 with Excellent Visible-light Photocatalytic Activity

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Journal of Wuhan University of Technology(Materials Science) 2020年第2期35卷 348-355页

作者： HE Jinyun YU Qi zhou yunpeng WANG Yanwu LONG Fei School of Materials Science and Engineering Guilin University of TechnologyGuilin 514004China Key Laboratory of Nonferrous Materials and New Processing Technology Ministry of EducationGuilin University of TechnologyGuilin 541004China College of En-vironmental Science and Engineering Guilin University of TechnologyGuilin 541004China

The rare earth ion Yb^3+ doped Bi2WO6 photocatalysts were synthesized by hydrothermal ***,XRD,XPS,FESEM,TEM,Ramam,N2 adsorption-desorption isotherm measurements and UV-vis diffusion reflectance spectra were used to characterize the Yb^3+ doped Bi2WO6 *** morphology,specific surface area,and pore volume distribution were greatly affected after Yb3+ ions *** performance of Bi2WO6 was effectively enhanced after Yb3+ ions doping,6% Yb^3+ doped Bi2WO6 had the best photocatalytic performance,and 96.2% Rhodamine B was degradated after irradiated 30 min,which was 1.29 times that of the pristine *** enhanced photocatalytic performance was due to the increased specific surface area,decreased energy band gap and inhibition of photoelectron-hole recombination after Yb3+ ions doping.

关键词： Bi2WO6 rare earth ion doping visible-light photocatalytic activity hydrothermal method

Dual-mode Switching Fault Ride-through Control Strategy for Self-synchronous Wind Turbines

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Journal of Modern Power Systems and Clean Energy 2023年第2期11卷 579-588页

作者： Xinshou Tian Yongning Chi Peng Cheng Wei He yunpeng zhou Jianzhu Hu China Institute of Energy and Transportation Integrated Development North China Electric Power UniversityBeijing 102206China State Key Laboratory of Operation and Control of Renewable Energy&Storage Systems China Electric Power Research InstituteBeijing 100192China State Grid Zhejiang Electric Power Co. Economic and Technological Research InstituteHangzhouChina

The installed capacity of renewable energy generation has continued to grow rapidly in recent years along with the global energy transition towards a 100%renewable-based power *** the same time,the grid-connected large-scale renewable energy brings significant challenges to the safe and stable operation of the power system due to the loss of synchronous ***,self-synchronous wind turbines have attracted wide attention from both academia and ***,the understanding of the physical operation mechanisms of self-synchronous wind turbines is not *** particular,the transient characteristics and dynamic processes of wind turbines are fuzzy in the presence of grid ***,it is difficult to design an adaptive fault ride-through(FRT)control ***,a dual-mode switching FRT control strategy for self-synchronous wind turbines is *** FRT control strategies are *** one strategy,the amplitude and phase of the internal potential are directly calculated according to the voltage drop when a minor grid fault *** other dual-mode switching control strategy in the presence of a deep grid fault includes three parts:vector control during the grid fault,fault recovery vector control,and self-synchronous *** proposed control strategy can significantly mitigate transient overvoltage,overcurrent,and multifrequency oscillation,thereby resulting in enhanced transient ***,simulation results are provided to validate the proposed control strategy.

关键词： Dual-mode switching self-synchronous wind turbine transient stability fault ride-through(FRT)control

Numerical simulation of the effect of coaxial and cross-axis injection modes on pulverized coal combustion in the raceway of blast furnace tuyere

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Particuology 2024年第10期93卷 154-169页

作者： yunpeng Wang Lei Gao Xiaolei zhou Faculty of Metallurgy and Energy Engineering Kunming University of Science and TechnologyKunming650093China

The aim of this study is to investigate the influence of the angle of the pulverized coal (PC) injection lance on the combustion characteristics of fuel in the raceway of blast furnace tuyeres. Using FLUENT software, a Euler-Lagrange three-dimensional numerical model was constructed to analyze the influence of different positions of blast furnace tuyere coal powder injection lance (coaxial and cross-axis) on key parameters such as temperature distribution, gas flow, and combustion efficiency. The results demonstrate that adjusting the angle of the injection lance significantly modifies the average and peak temperatures in the raceway, while the composition of gas components remains relatively stable. When the injection lance angle is 10°, the average temperature and peak temperature in the raceway are 2294 K and 2747 K, respectively. When the injection lance angle is 12°, the combustion efficiency of the PC reaches 80.8%. This study reveals the significant impact of the injection lance angle on the combustion process. Especially at an angle of 12°, the combustion efficiency of the blast furnace significantly improves. With coaxial injection, the combustion rate increases as the distance between the injection lance tip and the tuyere increases. This paper is instructive for the optimization of the blast furnace combustion system, which improve fuel utilization efficiency and reduce environmental emissions. This paper provides practical recommendations for adjusting blast furnace operational parameters, offering insights for achieving more efficient and environmentally friendly industrial production.

关键词： Pulverized coal combustion Tuyere raceway Blast furnace CFD simulation

Crystal structure and optical performance analysis of a new type of persistent luminescence material with multi-functional application prospects

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Journal of Energy Chemistry 2022年第6期31卷 150-160,I0005页

作者： Songsong Ding Pohua Chen Haijie Guo Peng Feng yunpeng zhou Yuhua Wang Junliang Sun National and Local Joint Engineering Laboratory for Optical Conversion Materials and Technology of National Development and Reform Commission Department of Materials ScienceSchool of Materials and EnergyLanzhou UniversityLanzhou 730000GansuChina College of Chemistry and Molecular Engineering Beijing National Laboratory for Molecular SciencesPeking UniversityBeijing 100871China

Persistent luminescence (PersL) materials,as environmentally friendly and energy-saving materials,have broad application prospects in many fields such as lighting,chemistry and even ***,studies on the types,performances and mechanism of PersL materials are still insufficient,which significantly restricts their development and *** this consideration,we successfully synthesized a yellow PersL material CaSrGa_(4)O_(8)(CSG).The crystal structure was studied in detail through Rotation Electron Diffraction (RED) and Powder X-ray Diffraction (PXRD).What’s more,by co-doping Mn^(2+) and Yb^(3+),the afterglow brightness of CSG could be increased by nearly 20 times,and the afterglow duration could reach more than 6 *** is worth mentioning that the samples also have excellent performances in mechanical luminescence (ML),photostimulated luminescence (PSL) and cathodoluminescence (CL),which was also investigated ***,an anti-counterfeiting label was designed by the samples to reveal the potential of their application in *** results showed that our research not only provided a new candidate PersL material for multifunctional applications,but also gave good help for studying the physical and chemical properties of CSG.

关键词： Persistent luminescence Multifunctional materials Mechanoluminescence Anti-counterfeiting Cathodoluminescence

Direct Conversion of Methane to Propylene

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Research 2024年第2期2023卷 463-472页

作者： yunpeng Hou Yuxiang Lan Chao Qian Shaodong zhou College of Chemical and Biological Engineering Zhejiang Provincial Key Laboratory of Advanced Chemical Engineering Manufacture TechnologyZhejiang University310027 HangzhouP.R.China Zhejiang Provincial Innovation Center of Advanced Chemicals Technology Institute of Zhejiang University-Quzhou324000 QuzhouP.R.China

Nonoxidative coupling of methane exhibits promising prospect in that it affords value-added hydrocarbons and hydrogen with high atom ***,challenge remains in direct,selective conversion of methane to more valuable hydrocarbons like *** current work presents a catalyst with well-dispersed Ta atoms anchored by graphitic C_(3)N_(4)-supported *** a catalyst is able to convert methane selectively to ethylene and propylene at a relatively low temperature(350℃).The conception of the active center and construction of the catalyst have been described,and the origins of the catalytic performance are discussed.

关键词： methane catalyst hydrocarbons