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A general synthetic strategy for N, P co-doped graphene supported metal-rich noble metal phosphides for hydrogen generation

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Green Energy & Environment 2024年第1期9卷 152-162页

作者： Jingwen Ma xiang Li Guangyu Lei jun Wang Juan Wang Jian Liu Ming Ke Yang Li Chunwen Sun School of Chemical and Environmental Engineering China University of Mining and Technology(Beijing)Beijing100083China State Key Laboratory of Heavy Oil Processing China University of PetroleumBeijing102249China Lab of Advanced Nano-structures&Transfer Processes Department of Chemical EngineeringTianjin UniversityTianjin300354China PetroChina Planning and Engineering Institute Beijing100083China

The exploitation of electrocatalysts with high activity and durability for HER is desirable for future energy systems,but it is still a *** have attracted increasing attentions,but the preparation process often needs toxic regents or dangerous reaction ***,we develop a general green method to fabricate metal-rich NMPs anchored on NPG through pyrolyzing DNA cross-linked *** obtained Ru_(2) P-NPG exhibits an ultrasmall overpotential of 7 mV at 10 mA cm^(2) and ultralow Tafel slope of 33 mV dec^(-1) in 1.0 mol L?1 KOH,even better than that of commercial Pt/*** addition,Ru 2 P-NPG also shows low overpotentials of 29 and 78 mV in 0.5 mol L^(-1) H_(2)SO_(4) and 1.0 mol L^(-1) PBS,*** superior activity can be attributed to the ultrafine dispersion of Ru 2 P nanoparticles for more accessible sites,more defects formed for abundant active sites,the two-dimensional plane structure for accelerated electron transfer and mass transport,as well as the regulation of electron distribution of the ***,the synthetic method can also be applied to prepare other metal-rich noble metal phosphides(Pd_(3)P-NPG and Rh_(2)P-NPG),which also exhibits high activity for *** work provides an effective strategy for designing NMP-based electrocatalysts.

关键词： Noble metal phosphides Electrocatalyst Deoxyribonucleic acid Hydrogen evolution pH universal

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含铝炸药能量释放的简化模型

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爆炸与冲击 2005年第4期25卷 309-312页

作者：周俊祥徐更光王廷增北京理工大学机械电子工程系北京100081

为了在水下爆炸效应中反映出非理想爆轰特性的影响,建立了含铝炸药非理想爆轰能量释放的简化模型。该模型以CJ爆轰理论和二次反应理论为基础,把含铝炸药化学反应划分为快速反应和慢速反应,以释放的化学能和慢反应速率常数作为非理想特... 详细信息

为了在水下爆炸效应中反映出非理想爆轰特性的影响,建立了含铝炸药非理想爆轰能量释放的简化模型。该模型以CJ爆轰理论和二次反应理论为基础,把含铝炸药化学反应划分为快速反应和慢速反应,以释放的化学能和慢反应速率常数作为非理想特征参数,并应用于一维数值模拟。计算结果与基本实验结果一致,冲击波峰值的计算误差不大于10%,衰减时间常数的误差小于5%,冲击波能与实验值也具有良好的一致性。简化模型合理地描述了含铝炸药非理想爆轰的主要过程及非理想特性,可应用于含铝炸药的设计和爆炸效应的分析。

关键词：爆炸力学简化模型二次反应理论含铝炸药数值分析爆轰

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肿瘤治疗靶点survivin及其分子拮抗剂的研究进展

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中国药理学通报 2005年第4期21卷 389-392页

作者：黄玮琳周向军王永祥上海交通大学药学院上海200030

survivin是IAP家族成员之一,分布于有丝分裂元件,具有调控细胞有丝分裂和抑制细胞凋亡的功能。survivin在大多数正常组织中未被检测,但在肿瘤组织中过量表达。survivin作为癌症治疗的一个重要靶点,针对survivin的多种分子拮抗剂的研究... 详细信息

survivin是IAP家族成员之一,分布于有丝分裂元件,具有调控细胞有丝分裂和抑制细胞凋亡的功能。survivin在大多数正常组织中未被检测,但在肿瘤组织中过量表达。survivin作为癌症治疗的一个重要靶点,针对survivin的多种分子拮抗剂的研究已经取得了一定成果。

关键词： survivin 肿瘤靶点分子拮抗剂

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Demonstration of safety characteristics and effects on gut microbiota of Lactobacillus gasseri HMV18

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Food Science and Human Wellness 2024年第2期13卷 611-620页

作者： Xianxian Jia Miaomiao Jia xiang Gao xiang Li Mengyuan Wang Shengqiang Du Rui Huang Xiaotong Li jun Zhang Shujin Li Chunling Ma Yan Zhang Bin Cong Department of Pathogen Biology Institute of basic MedicineHebei Medical UniversityShijiazhuang 050017China Research Unit of Digestive Tract Microecosystem Pharmacology and Toxicology Chinese Academy of Medical SciencesShijiazhuang 050017China Institute of Basic Medicine Hebei Medical UniversityShijiazhuang 050017China College of Forensic Medicine Hebei Key Laboratory of Forensic MedicineCollaborative Innovation Center of Forensic Medical Molecular IdentificationHebei Medical UniversityShijiazhuang 050017China Hebei Food Safety Key Laboratory Hebei Food Inspection and Research InstituteShijiazhuang 050227China

Human normal flora is a source of *** safety characteristics of a specific isolate determine its application in foods or *** food-borne-pathogen antagonist strain Lactobacillus gasseri HMV18 is one of the isolates from normal human *** this work,we assessed the in vitro pH tolerance,bile tolerance,biogenic amine production,mucin utilization,and safety of in vivo administration to mice to evaluate general health,organ-body weight index,organ histopathological change,whether *** HMV18 can colonize in the gut or modulate the gut microbiota after oral *** results suggest that *** HMV18 can tolerate pH 3 for 2 h,3%bile for 3 h,biogenic amine negative,mucin usage negative,does not encode verified toxins,and cause no visible change in mice's *** HMV18 might not colonize in mice's gut,but can significantly affect the structure of gut microbiota.A bibliographical survey suggested that there were as few as 8 opportunistic infection cases from 1984 to 2022 and that the possibility for *** to cause infection is relatively ***,this work provides a basis for the foods or drugs application of *** HMV18 and gives a map of experiments for the safety assessment of probiotics.

关键词： Probiotics Lactobacillus gasseri Safety assessment Gut microbiota

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Anomalous{1012}tensile twinning and subsequent detwinning in a friction stir processed carbon fiber-reinforced Mg composite

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Journal of Magnesium and Alloys 2024年第4期12卷 1511-1517页

作者： Wei Zhao Zhihao Jiang xiang Wu Yujing Liu Haokun Yang jun Wang Qi Liu Xiaochun Liu Institute of Metals College of Materials Science and EngineeringChangsha University of Science&TechnologyChangsha 410114China Department of Mechanical Engineering City University of Hong KongHong KongChina Smart manufacturing division Hong Kong Productivity CouncilHong Kong SAR 999077China Institute for Frontier Materials Deakin UniversityGeelongVIC 3216Australia Department of Industrial and Systems Engineering The Hong Kong Polytechnic UniversityHong KongChina

*** text Owing to their low density and high specific strength,magnesium alloys and magnesium-based composites have great potential as structure metal materials in applications where lightweight matters[1–4].Deformation twins[5],especially the{1012}tension twins(also called tensile or extension twins)with a low critical resolved shear stress(CRSS)[6],are commonly observed in Mg *** can provide the much-needed deformation along the c-axis in their hcp structure resulting from the very few easily activated slip systems in this crystal structure[7].The tensile twinning activation usually follows the macroscopic Schmid factor law[2],i.e.,the twin variant with the highest Schmid factor occurs,and it only appears when its Schmid factor is positive.

关键词： friction deformation magnesium

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A nano-sheet graphene-based enhanced thermal radiation composite for passive heat dissipation from vehicle batteries

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Nano Materials Science 2024年第4期6卷 443-455页

作者： Ji-xiang Wang Christopher Salmean Jiaxin Li Chaojie Lei jun Li Mingliang Zhong Bo Qi Yufeng Mao Hebei Key Laboratory of Man-machine Environmental Thermal Control Technology and Equipment Hebei Vocational University of Technology and Engineering College of Electrical Energy and Power EngineeringYangzhou University Department of Mechanical and Aerospace Engineering The Hong Kong University of Science and Technology Taizhou Wavexploration Energy Ltd. Department of Electrical and Computer Engineering University of Toronto China Academy of Launch Vehicle Technology Beijing Sino-Spark Technology Co. Ltd. School of Environmental Science and Engineering Suzhou University of Science and Technology Institute of Optics and Electronics Chinese Academy of Sciences National Key Laboratory of Optical Field Manipulation Science and Technology Chinese Academy of Sciences

In response to thermal runaway(TR) of electric vehicles, recent attention has been focused on mitigation strategies such as efficient heat dredging in battery thermal management. Thermal management with particular focus on battery cooling has been becoming increasingly significant. TR usually happened when an electric vehicle is unpowered and charged. In this state, traditional active battery cooling schemes are disabled, which can easily lead to dangerous incidents due to loss of cooling ability, and advanced passive cooling strategies are therefore gaining importance. Herein, we developed an enhanced thermal radiation material, consisting of ～1 μm thick multilayered nano-sheet graphene film coated upon the heat dissipation surface, thereby enhancing thermal radiation in the nanoscale. The surface was characterized on the nanoscale, and tested in a battery-cooling *** found that the graphene-based coating's spectral emissivity is between 91 % and 95 % in the mid-infrared region, and thermal experiments consequently illustrated that graphene-based radiative cooling yielded up to15.1 % temperature reduction when compared to the uncoated analogue. Using the novel graphene surface to augment a heat pipe, the temperature reduction can be further enlarged to 25.6 %. The new material may contribute to transportation safety, global warming mitigation and carbon neutralization.

关键词： Battery thermal management Nano-sheet graphene Functional material Passive cooling Thermal radiation

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CCDC181 is required for sperm flagellum biogenesis and male fertility in mice

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Zoological Research 2024年第5期45卷 1061-1072页

作者： xiang-jun Zhang Xiao-Ning Hou Jian-Teng zhou Bao-Lu Shi Jing-Wei Ye Meng-Lei Yang Xiao-Hua Jiang Bo Xu Li-Min Wu Qing-Hua Shi Division of Reproduction and Genetics First Affiliated Hospital of University of Science and Technology of China(USTC)Hefei National Laboratory for Physical Sciences at MicroscaleSchool of Basic Medical SciencesDivision of Life Sciences and MedicineBiomedical Sciences and Health Laboratory of Anhui ProvinceInstitute of Health and MedicineHefei Comprehensive National Science CenterUniversity of Science and Technology of ChinaHefeiAnhui 230001China

The structural integrity of the sperm flagellum is essential for proper sperm *** defects can result in male infertility,yet the precise mechanisms underlying this relationship are not fully ***181,a coiled-coil domain-containing protein,is known to localize on sperm flagella and at the basal regions of motile *** this knowledge,the specific functions of CCDC181 in flagellum biogenesis remain *** this study,Ccdc181 knockout mice were *** absence of CCDC181 led to defective sperm head shaping and flagellum ***,the Ccdc181 knockout mice exhibited extremely low sperm counts,grossly aberrant sperm morphologies,markedly diminished sperm motility,and typical multiple morphological abnormalities of the flagella(MMAF).Additionally,an interaction between CCDC181 and the MMAF-related protein LRRC46 was identified,with CCDC181 regulating the localization of LRRC46 within sperm *** findings suggest that CCDC181 plays a crucial role in both manchette formation and sperm flagellum biogenesis.

关键词： Male infertility CCDC181 MMAF Spermiogenesis Flagellum biogenesis

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Fermi Rubik's Cube in High-Pressure Induced Chlorine-Rich Compounds

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Chinese Physics Letters 2024年第10期41卷 78-83页

作者： jun Kong Lei Su Haixu Cui Hairui Ding Jingyu Hou Chunxia Chi Shiyang Liu xiang-Feng zhou Hui-Tian Wang Xiao Dong Key Laboratory of Weak-Light Nonlinear Photonics and School of Physics Nankai UniversityTianjin 300071China Center for High Pressure Science and Technology Advanced Research Beijing 100093China Key Laboratory of Photochemistry Institute of ChemistryUniversity of Chinese Academy of SciencesChinese Academy of SciencesBeijing 100190China College of Physics and Materials Science Tianjin Normal UniversityTianjin 300387China Center for High Pressure Science State Key Laboratory of Metastable Materials Science and TechnologySchool of ScienceYanshan UniversityQinhuangdao 066004China National Laboratory of Solid State Microstructures School of Physicsand Collaborative Innovation Center of Advanced MicrostructuresNanjing UniversityNanjing 210093China

In the quasi-free electron model,the Fermi surface spreads into a sphere in the Brillouin zone,i.e.,the Fermi *** Fermi sphere exists widely in metal systems,no matter whether the crystal is in a body-center cubic,face-center cubic,or hexagonal close-packed ***,we report a class of compounds stabilized at high pressure with Rubik’s cubic Fermi surface.

关键词： surface. Fermi cubic

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Oxidation resistant low-alloyed Ti alloys with good ductility

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Rare Metals 2024年第8期43卷 3921-3936页

作者： Meng Li Zhang-Zhi Shi jun-Yi Xu Fu-Zhi Dai xiang-Min Li Zi-Lin Li Lu-Ning Wang Beijing Advanced Innovation Center for Materials Genome Engineering State Key Laboratory for Advance Metals and MaterialsSchool of Materials Science and EngineeringUniversity of Science and Technology BeijingBeijingBeijing 100083China Institute of Materials Intelligent Technology Liaoning Academy of MaterialsShenyang 110004China

Oxidation resistance enhancement of pure Ti often comes at the cost of reduced ductility,which is frequently the problem through alloying with sole Al,Si,W,Mo and *** overcome the short coming of single element alloying,this paper proposes a multi-element low-alloying strategy to take advantage of synergistic effects and resolve the conflict between oxidation resistance and *** demonstrates that the addition of a small quantity of Ta(0.51wt%)can boost both oxidation resistance and ductility in comparison to pure ***,the combined addition of a small amount(0.54 wt%)of Ta,Nb and Si not only preserves good ductility of pure Ti,but also reduces mass gains to 14%-67%of pure Ti during 100 h oxidation at 650-850℃in *** indicates even better oxidation resistance than that obtained through the use of Ta,Nb,or Nb+Ta *** Ta+Nb+Si alloying creates an oxide layer that is less porous and more resistant to stratification and ***,a 3-μm N-rich layer can form in the Ti substrate beneath the oxide scale,in which phase transformation generates coherent Ti_(2)N with(0001)_(Ti)as the habit plane,with N atoms prefers to diffuse along■than along[0001]_(Ti).The completely transformed Ti_(2)N region or partially transformed Ti+Ti_(2)N region can effectively impede oxygen ***,the multielement low-alloying strategy is promising for enhancing both oxidation resistance and mechanical properties of metallic materials in the future.

关键词： Ti alloys Multi-element Co-alloying Oxidation resistance Mechanical properties

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Physics of cavitation near particles

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Journal of Hydrodynamics 2024年第1期36卷 102-118页

作者： Jia-xin Yu Xiao-yu Wang jun-wei Shen Jin-sen Hu xiang-qing Zhang Da-qing He Yu-ning Zhang Key Laboratory of Power Station Energy Transfer Conversion and System(Ministry of Education) School of Energy Power and Mechanical EngineeringNorth China Electric Power UniversityBeijing102206China

The combined effect of cavitation and silt abrasion presents a great challenge and threat to secure the operation and the efficiency of hydraulic machineries working in sediment-laden *** present paper critically reviews the current research progress on the interaction mechanisms of the bubbles and the ***,the analytical models including boundary treatment methods for predicting the jet dynamics of the bubble collapse near particles are ***,the bubble collapsing dynamics,jet dynamics and shock wave characteristics near particles are revealed both experimentally and ***,the bubble-particle-wall system is investigated with a focus on microjets.

关键词： Cavitation bubble particle jet shock wave

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