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Magnetic emission intensity enhancement for amorphous alloys by constructing a multi-phase structure withα-Fe nanocrystals

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Nano Research 2024年第7期17卷 6630-6637页

作者： Ke Liu zhi Qin Jie Shen zhi cheng Shiyue You Liang Ma Jing Zhou Wen Chen State Key Laboratory of Advanced Technology for Materials Synthesis and Processing School of Materials Science and EngineeringWuhan University of TechnologyWuhan 430070China Sanya Science and Education Innovation Park Wuhan University of TechnologySanya 572024China Hubei Longzhong Laboratory Wuhan University of Technology Xiangyang Demonstration ZoneXiangyang 441000China

The perturbation in the magnetic field generated by the rotation or oscillation of magnetic domains in magnetic materials can emit low-frequency electromagnetic waves,which are expected to be used in low-frequency ***,the magnetic emission intensity,defined by the perturbation ability,of current commercially applied amorphous alloys,such as Metglas,cannot meet the application requirements for low-frequency antennas due to the domain motion energy ***,a multi-phase Metglas amorphous alloy was constructed by incorporatingα-Fe nanocrystals using rapid annealing to manipulate the domain *** was found that 3.89 times higher magnetic emission intensity is obtained compared to the pristine due to the synergism of the deformation and displacement ***,the low-frequency magnetic emission performance verification was carried out by preparing magnetoelectric composites as the antenna vibrator by assembling the alloy and macro piezoelectric fiber composites(MFC).Enhancements of magnetic emission intensity are found at 93.3%and 49.2%at the first and second harmonic frequencies compared with the unmodified alloy ***,the approach leads to the development of high-performance communication with a novel standard for evaluation.

关键词： multi-phase amorphous alloys magnetic emission intensity enhancing mechanism magnetic domain pinning theory Jiles-Atherton model analysis

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Dual modification of LiNi_(0.83)Co_(0.11)Mn_(0.06)O_(2) cathode materials by K^(+) doping and Li_(3)PO_(4) coating for lithium ions batteries

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Rare Metals 2024年第7期43卷 3007-3018页

作者： Wei Xiao Jia-Le Wang zhi-cheng Yi cheng-Jin Liu Chang Miao Yu Xin Shu-Qing Nie College of Chemistry and Environmental Engineering Yangtze UniversityJingzhou 434023China

Li_(3)PO_(4)@Li_(0.99)K_(0.01)Ni_(0.83)Co_(0.11)Mn_(O.06)O_(2)(NCM-KP) cathode powders are synthesized via K^(+)doping in calcination processes and H_3PO_4 coating in sol-gel processes.K^(+) precisely enters into the lattice to widen the(003) plane to 0.4746 nm with a lower cationic disordered degree of 1.87%.Moreover,the surface residual lithium salts are treated by H_3PO_4 to generate a uniform Li_(3)PO_(4) coating layer of approximately 11.41 nm,which completely covers on the surface of secondary spherical particles to improve the interfacial *** 25℃,the NCM-KP electrode delivers a discharge specific capacity of 148.9 mAh·g^(-1) with a remarkable capacity retention ratio of 84.1% after 200 cycles at 1.0C and retains a high reversible specific capacity of 154.4 mAh·g^(-1) at *** at 1.0C and 60℃,it can maintain a reversible discharge specific capacity of 114.6 mAh·g^(-1) with 0.21% of capacity decay per cycle after 200 cycles,which is significantly lower than 0.40% for the pristine NCM ***,the charge transfer resistance of 238.89 Ω for the NCM-KP electrode is significantly lower than 947.41 Ω for the pristine NCM one by restricting the interfacial side ***,combining K+doping and Li_(3)PO_(4) coating is an effective strategy to enable the significant improvement of the electrochemical property of high-nickel cathode materials,which may be mainly attributed to the widened diffusion pathway and the formed Li_(3)PO_(4) protective layer,thus promoting Li~+diffusion rate and preventing the erosion of HF.

关键词： High-nickel cathode material Residual lithium K^(+)doping Li_(3)PO_(4)coating Lithium ions battery

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Theoretical insights into efficient oxygen evolution reaction using non-noble metal single-atom catalysts on W2CO2 MXene

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Rare Metals 2024年第10期43卷 5082-5094页

作者： Jing-Yu Zhou zhi-cheng Han Shu Zhao Tao Yang Da-Zhou Yan Hai-Jun Yu Institute of Advanced Battery Materials and Devices College of Materials Science and EngineeringBeijing University of Technology Key Laboratory of Advanced Functional Materials Ministry of EducationBeijing University of Technology China ENFI Engineering Corporation National Engineering Research Center of Silicon-Based Materials Manufacturing Technology

The pursuit of highly active oxygen evolution reaction （OER） catalysts,especially those free of noble metals,is a focal point in fuel cell *** extensive density functional theory calculations,this study designed and evaluated the activity and stability of singleatom catalysts （SACs） composed of 3d,4d and 5d transition metals supported on tungsten-based MXene for OER *** highlighted the exceptional OER performance of Ni@W2CO2,Rh@W2CO2and Pt@W2CO2,displaying remarkably low overpotentials The catalytic activity of TM@W2CO2SACs exhibited a robust correlation with surface properties,particularly the d-band center index and surface work *** Ni@W2CO2,Rh@W2CO2and Pt@W2CO2emerged as promising candidates for OER and oxygen reduction reaction （ORR） bifunctional catalysis,while Pt@W2CO2and Rh@ W2CO2showed high potential for OER and hydrogen evolution reaction （HER） bifunctional catalysis The effectiveness of tungsten-based MXene as a substrate for non-noble-metal SACs marks a breakthrough in OER catalyst design,driving advancements towards sustainable energy solutions and addressing critical challenges in energy conversion and storage.

关键词： Density functional theory MXene Non-noble metal Oxygen evolution reaction Single-atom catalysts

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Multimorbidity and mortality among older patients with coronary heart disease in Shenzhen,China

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Journal of Geriatric Cardiology 2024年第1期21卷 81-89页

作者： Fu-Rong LI Shuang WANG Xia LI zhi-Yuan cheng cheng JIN Chun-Bao MO Jing ZHENG Feng-Chao LIANG Dong-Feng GU Shenzhen Key Laboratory of Cardiovascular Health and Precision Medicine Southern University of Science and TechnologyShenzhenGuangdongChina School of Public Health and Emergency Management Southern University of Science and TechnologyShenzhenGuangdongChina Shenzhen Health Development Research and Data Management Center ShenzhenChina School of Medicine Southern University of Science and TechnologyShenzhenGuangdongChina

BACKGROUND The current understanding of the magnitude and consequences of multimorbidity in Chinese older adults with coronary heart disease(CHD)is *** aimed to assess the association and population-attributable fractions(PAFs)between multimorbidity and mortality among hospitalized older patients who were diagnosed with CHD in Shenzhen,*** We conducted a retrospective cohort study of older Chinese patients(aged≥65 years)who were diagnosed with *** proportional hazards models were used to estimate the associations between multimorbidity and all-cause and cardiovascular disease(CVD)*** also calculated the *** The study comprised 76,455 older hospitalized patients who were diagnosed with CHD between January 1,2016,and August 31,*** them,70,217(91.9%)had multimorbidity,defined as the presence of at least one of the predefined 14 chronic *** with cancer,hemorrhagic stroke and chronic liver disease had the worst overall death risk,with adjusted HRs(95%CIs)of 4.05(3.77,4.38),2.22(1.94,2.53),and 1.85(1.63,2.11),*** CVD mortality,the highest risk was observed for hemorrhagic stroke,ischemic stroke,and chronic kidney disease;the corresponding adjusted HRs(95%CIs)were 3.24(2.77,3.79),1.91(1.79,2.04),and 1.81(1.64,1.99),***-cause mortality was mostly attributable to cancer,heart failure and ischemic stroke,with PAFs of 11.8,10.2,and 9.1,*** for CVD mortality,the leading PAFs were heart failure,ischemic stroke and diabetes;the corresponding PAFs were 18.0,15.7,and 6.1,*** Multimorbidity was common and had a significant impact on mortality among older patients with CHD in Shenzhen,***,heart failure,ischemic stroke and diabetes are the primary contributors to ***,prioritizing improved treatment and management of these comorbidities is essential for the survival prognosis of CHD patients from a holistic public health perspective.

关键词： patients morbidity mortality

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Room-temperature Self-healing and Recyclable PDMS Elastomers with Superior Mechanical Properties for Triboelectric Nanogenerators

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Chinese Journal of Polymer Science 2024年第10期42卷 1566-1577,I0014页

作者： Shu-Juan Wang Lu Wang Hong-Zhe Su zhi-cheng Wu Qiao-Gen Zhang Wei Fan Xin-Li Jing School of Chemistry Joint Innovation Center of Thermal Protection MaterialsXi’an Jiaotong UniversityXi’an710049China School of Electrical Engineering Xi’an Jiaotong UniversityXi’an710049China School of Textile Science and Engineering Xi’an Polytechnic UniversityXi’an710048China

Polydimethylsiloxane(PDMS)is an electron-withdrawing material that is widely used in triboelectric nanogenerators(TENGs).However,PDMS has poor mechanical properties after curing and is easily damaged when subjected to long-term ***,the long-term stable operation of TENGs under mechanical deformation cannot be *** this work,multiple hydrogen bonds and aromatic disulfide bonds were introduced into PDMS *** elastomers exhibited high toughness(a tensile strength of 1.91 MPa and an elongation at break of 340%),good recyclability,and room-temperature self-healing properties(healing efficiency of 96.4%in 24 h).Recyclable sandwich-like triboelectric nanogenerators with excellent electrical output performance(13.5 V)and room-temperature self-healing performance(24 h,98%recovery of self-generating performance)were prepared by utilizing the hydrogen bonding between the PDMS elastomer and *** work reported herein offers theoretical guidance and a compelling strategy for developing high-performance TENG negative friction layers.

关键词： Polydimethylsiloxane Aromatic disulfide bonds Hydrogen bonds Room temperature self-healing Triboelectric nanogenerator

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Dual-curvilinear beam enabled tunable manipulation of high-and low-refractive-index particles

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Photonics Research 2024年第7期12卷 1427-1436页

作者： ZHENG YUAN CHENCHEN ZHANG YUAN GAO WENXIANG YAN XIAN LONG zhi-cheng REN XI-LIN WANG JIANPING DING HUI-TIAN WANG National Laboratory of Solid State Microstructures and School of Physics Nanjing UniversityNanjing 210093China Collaborative Innovation Center of Advanced Microstructures Nanjing 210093China Collaborative Innovation Center of Solid-State Lighting and Energy-Saving Electronics Nanjing 210093China

We present an innovative approach for the simultaneous agile manipulation of high-refractive-index(HRI) and low-refractive-index(LRI) particles. Our method involves introducing a dual-curvilinear optical vortex beam(DC-OVB) generated by superimposing a pair of curved beams: HRI and LRI particles are controlled by the bright curve and the dark channel between the two curves, respectively. The proposed DC-OVB provides customizable motion paths and velocities for both LRI and HRI particles. Each curve of the DC-OVB can support a distinct orbital flow density(OFD), enabling the application of torques to HRI and LRI particles, guiding them to orbit along specified trajectories and prompting them to execute various curvilinear motions simultaneously,including curvilinear movement, revolution, and rotation.

关键词： tunable refractive beam

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Transition-Metal-Free Allylic Defluorination Cross-Electrophile Coupling Employing Rongalite

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Chinese Journal of Chemistry 2024年第12期42卷 1360-1366页

作者： Xiang-Long Chen Chun-Yan Wu Dong-Sheng Yang Bo-cheng Tang Huai-Yu Wang zhi-cheng Yu Anling Li Yan-Dong Wu An-Xin Wu National Key Laboratory of Green Pesticide International Joint Research Center for Intelligent Biosensor Technology and HealthCollege of ChemistryCentral China Normal UniversityWuhanHubei 430079China state Key Laboratory of Chemical Biology and Drug Discovery Department of Applied Biology and Chemical Technology The HongKong Polytechnic UniversityKowloonHong Kong SARChina Department of Clinical Laboratory Center for Gene Diagnosisand Program of Clinical Laboratory MedicineZhongnan Hospital of Wuhan UniversityWuhanHubei 430062China

Comprehensive Summary The conversion of CF3-alkenes to gem-difluoroalkenes using reductive cross-coupling strategy has received much attention in recent years,however,the use of green and readily available reducing salt to mediate these reactions remains to be *** this work,a concise construction of gem-difluoroalkenes,which requires neither a catalyst nor a metal reducing agent,was ***,a safe and inexpensive industrial product,was employed as both a radical initiator and *** procedure was compatible with both linear and cyclic diaryliodonium salts,enabling a wide variety of substrates(>70 examples).The utility of this approach was demonstrated through gram-scale synthesis and efficient late-stage functionalizations of anti-inflammatory drugs.

关键词： Defluoroarylation Transition metal free gem-Difluoroalkenes Rongalite Single electron transfer C-C coupling Redox reactions Cross-coupling

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I_(2)-DMSO-Mediated Multicomponent [2+1+1+1] Annulation Reaction via Ethyl Nitroacetate C-NO_(2), Bond Cleavage as a C1 Synthon: A Route to Multisubstituted 6-Pyrrolidinones Derivatives with a Quaternary Center

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Chinese Journal of Chemistry 2024年第17期42卷 2029-2034页

作者： zhi-cheng Yu Xi Shen You Zhou Xiang-Long Chen Li-Sheng Wang Yan-Dong Wu An-Xin Wu National Key Laboratory of Green Pesticide International Joint Research Centerfor Intelligent BiosensorTechnologyand HealthCollegeof ChemistryCentral ChinaNormal UniversityWuhanHubei 430079China

A[2+1+1+1]cyclization reaction has been developed for the synthesis of multisubstituted 6-pyrrolidinones from commercially available aryl methyl ketones,primary amines,and ethyl *** this I_(2)-DMSO-meditated process,the C-NO_(2) bond of ethyl nitroacetate is cleaved,affording a C1 synthon,and the formation of two C-C and two C-N bonds and a quaternary carbon center are constructed in one *** method has good substrate compatibility and permits the late-stage modification of pharmaceutical compounds.

关键词： Cyclization Multisubstituted 6-pyrrolidinones I_(2)-DMSO C1 building blocks Quaternary carbon center Late-stage modification Cracking

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Depositional process of hyperpycnal flow deposits:A case study on Lower Cretaceous Sangyuan outcrop in the Luanping Basin,Northeast China

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China Geology 2024年第3期7卷 505-516页

作者： De-zhi Yan Ru-kai Zhu Hao Shou Zhao-hui Xu Wei-hong Liu Si-cheng Zhu zhi-cheng Lei Jing-ya Zhang Chang Liu Yi Cai Huai-min Xu Research Institute of Petroleum Exploration and Development PetroChinaBeijing 100083China National Energy Tight Oil and Gas R&D Center Beijing 100083China PetroChina Key Laboratory of Oil and Gas Reservoir Beijing 100083China State Key Laboratory of Petroleum Resources and Prospecting China University of Petroleum(Beijing)Beijing 102249China College of Geosciences China University of Petroleum(Beijing)Beijing 102249China Jiangxi Engineering Laboratory on Radioactive Geoscience and Big Data Technology Department of Information and EngineeringEast China University of TechnologyNanchang 330013China

Sedimentary process research is of great significance for understanding the distribution and characteristics of *** the detailed observation and measurement of the Sangyuan outcrop in Luanping Basin,this paper studies the depositional process of the hyperpycnal flow deposits,and divides their depositional process into three phases,namely,acceleration,erosion and *** the acceleration phase,hyperpycnal flow begins to enter the basin nearby,and then speeds up *** developed in the acceleration phase are *** addition,the original deposits become unstable and are taken away by hyperpycnal flows under the eroding *** a result,there are a lot of mixture of red mud pebbles outside the basin and gray mud pebbles within the *** the erosion phase,the reverse deposits are eroded and become thinner or even ***,no reverse grading characteristic is found in the proximal major channel that is closer to the source,but it is still preserved in the middle branch channel that is far from the *** entering the deceleration phase,normally grading deposits appear and cover previous *** final deposits in the basin are *** are reverse,and others are *** are superimposed with each other under the action of hyperpycnal *** analysis of the Sangyuan outcrop demonstrates the sedimentary process and distribution of hyperpycnites,and reasonably explain the sedimentary characteristics of *** is helpful to the prediction of oil and gas exploration targets in gravity flow deposits.

关键词： Hyperpycnal flow Sedimentary characteristics Depositional process Gravity flow deposit Hyperpycnite Red mud pebble Gray mud pebble Oil and gas exploration engineering Luanping Basin

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Review on recent advances of inorganic electrode materials for potassium-ion batteries

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Tungsten 2024年第1期6卷 174-195页

作者： Jian-Zhen Xiong Ze-cheng Yang Xin-Liang Guo Xi-Ying Wang Chao Geng Zong-Fu Sun An-Yong Xiao Quan-Chao Zhuang Ya-Xin Chen zhi-cheng Ju School of Materials Science and Physics China University of Mining and TechnologyXuzhou 221116China

Rechargeable potassium-ion batteries(PIBs)have great potential in the application of electrochemical energy storage devices due to the low cost,the abundant resources and the low standard reduction potential of *** electrode materials are the key factors to determine the electrochemical performance of devices,relevant research is being carried out to build high-performance *** recent years,significant progress has been made in the study of the design of inorganic electrode ***,we review the cathode materials(Prussian blue and its analogues,layered oxides and poly anionic compounds)and the anode materials(antimony-based,selenium-based and bismuth-based compounds).On the basis of previous work,the structural design principles for improving the performance of electrode materials are reasonably *** the same time,the problems that need to be solved in the preparation of electrode materials and the direction of future research and improvement are pointed out.

关键词： Inorganic electrode materials Potassium-ion batteries Cathode materials Anode materials

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