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Laser-rewritable room temperature phosphorescence based on in-situ polymerized tartaric acid

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Science China Chemistry 2024年第9期67卷 3029-3038页

作者： Tuo-Yu Zhou Tai-Wen Li Hai-Fu Zhang rui-Lin Chai Qian Zhao Penglin Zhang Guang-Yue Li Qian-Wen Wang Chang Li Yu Shu zhi Fan Sheng-Hua Li College of Chemical Engineering and Materials Science College of SciencesTianjin University of Science&TechnologyTianjin 300457China College of Chemical Engineering North China University of Science and TechnologyTangshan 063210China Tianjin Key Laboratory of Multiplexed Identification for Port Hazardous Chemicals Tianjin University of Science&TechnologyTianjin 300457China

Organic room temperature phosphorescence(RTP)materials have potential applications in information technology and ***,the precise control of the afterglow in reversible manners remains challenging for organic ***,we report a kind of organic RTP material fabricated by simple heating mixtures of tartaric acid(TA)and aromatic acids,which can switch their phosphorescence by *** mixtures show tunable phosphorescence from indigo to orange with phosphorescence efficiency of up to 53.99% due to locking different organic luminogens by the TA-formed matrix through the noncovalent *** afterglow of those materials lasts a few seconds and disappears by water fumigation,which can be repeated in response to wet/heat *** drop-casting those materials on glass slides,a laser-repatternable phosphorescence is achieved by facile laser direct writing and quenched by water *** results open the opportunity for the design of smart stimuli-responsive phosphorescence materials from sustainable natural products.

关键词： room temperature phosphorescence tunable afterglows tartaric acid laser direct writing stimuli-response

Probing the Gamma-Ray Emission Region of Five TeV Flat Spectrum Radio Quasars

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Research in Astronomy and Astrophysics 2024年第6期24卷 156-169页

作者： Hu-Bing Xiao Hai-Tao Cao rui Xue Jin-Ting Cai Ge-Ge Wang Marina Manganaro Shao-Hua Zhang zhi-Hao Ouyang Li-Ping Fu Jun-Hui Fan Shanghai Key Lab for Astrophysics Shanghai Normal UniversityShanghai 200234China School of Information Engineering Guangzhou Panyu PolytechnicGuangzhou 511483China Department of Physics Zhejiang Normal UniversityJinhua 321004China College of Mathematics and Physics Guangxi Minzu UniversityNanning 530006China Key Laboratory of Cosmology and Astrophysics(Liaoning) College of SciencesNortheastern UniversityShenyang 110819China Department of Physics University of RijekaRijeka 51000Croatia Center for Astrophysics Guangzhou UniversityGuangzhou 510006China Key Laboratory for Astronomical Observation and Technology of Guangzhou Guangzhou 510006China Astronomy Science and Technology Research Laboratory of Department of Education of Guangdong Province Guangzhou 510006China

The location ofγ-ray emission of blazars remains a contested topic,inspiring the development of numerous investigative techniques to address this *** this work,we analyzed Fermiγ-ray light curves in the GeV and MeV bands,employing the discrete cross-correlation function method to discern time lags between the two *** 4C+21.35,Ton 599,B21420+32,and PKS 1510-089,we identified a time lag spanning several days,while for PKS 1441+25,the time lag was not statistically *** results imply that the soft photons necessary for inverse Compton scattering predominantly originate from the dusty torus in the first four sources,whereas for PKS1441+25,they seem to be sourced mainly from the broad-line *** analysis of the opacity(τγγ)and the GeV spectra study supports the conclusion that the location of the dissipation region must be beyond the BLR to avoid significant ***,for PKS 1441+25,the emission region is also posited to lie outside yet proximate to the *** parameters of describing the emission region were obtained by fitting broadband spectral energy distribution with contemporaneous observation *** findings suggest that for the five TeV FSRQs,during Te V flaring events,the jet appears to maintain an equilibrium between the energy density of the magnetic field and that of the particles for all investigated sources,with the exceptions of 4C+21.35 and PKS1441+*** terms of the overall jet power,particle energy is the dominant contributor,and the observed blazar radiation cannot be solely attributed to the magnetic field,except in the case of 4C+***,magnetic reconnection is unlikely to be the primary mechanism behind particle acceleration in these systems.

关键词： galaxies:active gamma-rays:galaxies galaxies:jets

Enhanced energy storage properties and good stability of novel(1-x)Na_(0.5)Bi_(0.5)TiO_(3)-xCa(Mg_(1/3)Nb_(2/3))O_(3) relaxor ferroelectric ceramics prepared by chemical modification

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Journal of Materiomics 2024年第4期10卷 770-782页

作者： Ying Zhang Meng-Han Yan zhi-Fei Zhang Hai-rui Bai Peng Li Wei-Fang Han Ji-Gong Hao Wei Li Yu-Chao Li Chun-Ming Wang Peng Fu School of Materials Science and Engineering Liaocheng UniversityLiaocheng252059China Shandong Laboratory of Yantai Advanced Materials and Green Manufacturing 300 Changjiang RoadYantai264006China School of Physics Shandong UniversityJinan250100China

The increase in energy consumption and its collateral damage on the environment has encouraged the development of environment-friendly ceramic materials with good energy storage *** this work,(1-x)Na_(0.5)Bi_(0.5)TiO_(3)-xCa(Mg_(1/3)Nb_(2/3))O_(3) ceramics were synthesized by the solid-state reaction *** 0.88Na_(0.5)Bi_(0.5)TiO_(3)-0.12Ca(Mg_(1/3)Nb_(2/3))O_(3) ceramic exhibited a high recoverable energy storage density of 8.1 J/cm3 and energy storage efficiency of 82.4% at 550 kV/*** introduction of Ca(Mg_(1/3)Nb_(2/3))O_(3) reduced the grain size and increased the band gap,thereby enhancing the breakdown field strength of the ceramic *** method also resulted in good temperature stability(20–140℃),frequency stability(1–200 Hz),and fatigue stability over 106 *** addition,an ultrahigh power density of 187 MW/cm^(3) and a fast charge-discharge rate(t0.9=57.2 ns)can be obtained *** element method analysis revealed that the decrease of grain size was beneficial to the increase of breakdown field ***,the 0.88Na_(0.5)Bi_(0.5)TiO_(3)-0.12Ca(Mg_(1/3)Nb_(2/3))O_(3) ceramics resulted in high energy storage properties with good stability and were promising environment-friendly materials for advanced pulsed power systems applications.

关键词： (1-x)Na_(0.5)Bi_(0.5)TiO_(3)-xCa(Mg_(1/3)Nb_(2/3))O_(3)ceramics Relaxor ferroelectrics Breakdown field strength Energy storage properties Stability

铁路路基动力响应的2.5D有限元方法研究现状及展望

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岩土力学 2024年第1期45卷 284-301页

作者：王瑞胡志平长安大学建筑工程学院陕西西安710061

作为一种频域计算方法,2.5D有限元具备计算效率高、内存占用小等优势,同时也存在诸多局限。经过20余年的发展,2.5D有限元方法已经具备了描述复杂土体本构关系和复杂路基几何特征条件下铁路路基动力响应的能力。荷载输入方法、建模策略... 详细信息

作为一种频域计算方法,2.5D有限元具备计算效率高、内存占用小等优势,同时也存在诸多局限。经过20余年的发展,2.5D有限元方法已经具备了描述复杂土体本构关系和复杂路基几何特征条件下铁路路基动力响应的能力。荷载输入方法、建模策略和波动吸收边界的持续优化使得2.5D有限元方法的精度不断提高,二维插值方法则为进一步提升计算效率提供了思路。目前,2.5D有限元已经成为铁路路基动力响应研究中的常用方法。为了理清铁路路基动力响应2.5D有限元方法的发展脉络,分别从荷载输入、路基系统、响应输出和计算精度及效率的提升方面总结了其发展现状,介绍了2.5D有限元在发展过程中遇到的瓶颈问题及解决对策。在此基础上,针对算法的精度和效率、研究的对象和内容进行了进一步的讨论和展望。

关键词： 2.5D有限元方法铁路路基动力响应建模吸收边界二维插值

Research progress on insomnia treated by traditional Chinese medicine and acupuncture based on microbial-gut-brain axis theory

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World Journal of Clinical Cases 2024年第18期12卷 3314-3320页

作者： Li-Min Pan zhi-Bo Hong rui-Qian Guan Department of Outpatient Deputy Chief Physician The First Affiliated Hospital of Heilongjiang University of Chinese MedicineHaerbin 150010Heilongjiang ProvinceChina School of Heilongjiang University of Chinese Medicine Graduate Heilongjiang University of Chinese MedicineHaerbin 150000Heilongjiang ProvinceChina Heilongjiang University of Chinese Medicine The Second Affiliated Hospital of Heilongjiang University of Chinese MedicineHaerbin 150010Heilongjiang ProvinceChina

Insomnia,as one of the emotional diseases,has been increasing in recent years,which has a great impact on people's life and ***,researchers are eager to find a more perfect *** microbiome-gut-brain axis is a new theory that has gradually become popular abroad in recent years and has a profound impact in the field of *** recent years,traditional Chinese medicine(TCM)has played an increasingly important role in the treatment of insomnia,especially acupuncture and Chinese herbal *** is the main method of TCM in the treatment of *** paper mainly reviews the combination degree of"microorganism-gut-brain axis"theory with TCM and acupuncture under the system of *** explore the mechanism of TCM and acupuncture in the treatment of insomnia under the guidance of"microorganismgut-brain axis"theory,in order to provide a new idea for the diagnosis and treatment of insomnia.

关键词： Insomnia Microorganism Intestine-brain axis Traditional Chinese medicine Acupuncture and moxibustion

HgS/CdS/HgS球状纳米系统电子的能量与寿命以及概率分布

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物理学报 2003年第9期52卷 2284-2289页

作者：郑瑞伦陈志谦张翠玲刘俊西南师范大学物理系重庆400715

建立了HgS CdS HgS球状纳米系统物理模型和电子状态满足的方程 .应用S矩阵理论 ,探讨了s态电子的能量和寿命以及概率分布随势垒和势阱宽度的变化规律 .结果表明 :电子能量和寿命随垒势宽度增大而增大 ;电子能量随阱宽增大而减小 ,而寿... 详细信息

建立了HgS CdS HgS球状纳米系统物理模型和电子状态满足的方程 .应用S矩阵理论 ,探讨了s态电子的能量和寿命以及概率分布随势垒和势阱宽度的变化规律 .结果表明 :电子能量和寿命随垒势宽度增大而增大 ;电子能量随阱宽增大而减小 ,而寿命随阱宽增大而增大 ;

关键词：球状纳米系统电子状态能量寿命电子概率分布势垒宽度势阱宽度 HgS/CdS/HgS系统硫化汞硫化镉

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沉积物总氮总磷同时消解分析方法

海洋通报 2009年第4期28卷 97-101页

作者：郑瑞芝陈然王鑫煌张钒福建海洋研究所福建厦门361012

对沉积物样品通过同时消解可分别测定总氮和总磷的方法作了探讨。总氮用次溴酸盐氧化比色法,比凯氏定氮法快速省时;总磷用钒钼酸铵比色法。采用同时消解沉积物样品,简化了分析操作流程,使分析条件与工作曲线酸度相同,因而取得较好的测... 详细信息

对沉积物样品通过同时消解可分别测定总氮和总磷的方法作了探讨。总氮用次溴酸盐氧化比色法,比凯氏定氮法快速省时;总磷用钒钼酸铵比色法。采用同时消解沉积物样品,简化了分析操作流程,使分析条件与工作曲线酸度相同,因而取得较好的测定效果:总氮回收率102%～105%,精密度3.6%;总磷精密度5.5%,测定值都在标准值范围之内,适用于批量测定。

关键词：沉积物总氮总磷同时消解测定

Mandarin fish von Hippel-Lindau protein regulates the NF-κB signaling pathway via interaction with IκB to promote fish ranavirus replication

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Zoological Research 2024年第5期45卷 990-1000页

作者： zhi-Min Li Xiao-Wei Qin Qi Zhang Jian He Min-Cong Liang Chuan-rui Li Yang Yu Weng-Hui Liu Shao-Ping Weng Jian-Guo He Chang-Jun Guo School of Marine Sciences State Key Laboratory for BiocontrolSouthern Marine Science and Engineering Guangdong Laboratory(Zhuhai)Guangdong Province Key Laboratory of Aquatic Economic Animals&Guangdong Provincial Observation and Research Station for Marine Ranching of the Lingdingyang BaySun Yat-sen UniversityGuangzhouGuangdong 510275China Guangdong Laboratory for Lingnan Modern Agriculture South China Agricultural UniversityGuangzhouGuangdong 510640China

The von Hippel-Lindau tumor suppressor protein(VHL),an E3 ubiquitin ligase,functions as a critical regulator of the oxygen-sensing pathway for targeting hypoxia-inducible *** evidence suggests that mammalian VHL may also be critical to the NF-κB signaling pathway,although the specific molecular mechanisms remain ***,the roles of mandarin fish(Siniperca chuatsi)VHL(scVHL)in the NF-κB signaling pathway and mandarin fish ranavirus(MRV)replication were *** transcription of scVHL was induced by immune stimulation and MRV infection,indicating a potential role in innate ***-luciferase reporter gene assays and reverse transcription quantitative PCR(RT-qPCR)results demonstrated that scVHL evoked and positively regulated the NF-κB signaling *** with NF-κB signaling pathway inhibitors indicated that the role of scVHL may be mediated through scIKKα,scIKKβ,scIκBα,or ***-immunoprecipitation(Co-IP)analysis identified scIκBαas a novel target protein of ***,scVHL targeted scIκBαto catalyze the formation of K63-linked polyubiquitin chains to activate the NF-κB signaling *** MRV infection,NF-κB signaling remained activated,which,in turn,promoted MRV *** findings suggest that scVHL not only positively regulates NF-κB but also significantly enhances MRV *** study reveals a novel function of scVHL in NF-κB signaling and viral infection in fish.

关键词： VHL NF-κB IκBα Ranavirus Mandarin fish

Disulfiram ameliorates STING/MITA-dependent inflammation and autoimmunity by targeting RNF115

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Cellular & Molecular Immunology 2024年第3期21卷 275-291页

作者： zhi-Dong Zhang Chang-rui Shi Fang-Xu Li Hu Gan Yanhong Wei Qianhui Zhang Xin Shuai Min Chen Yu-Lin Lin Tian-Chen Xiong Xiaoqi Chen Bo Zhong Dandan Lin Department of Gastrointestinal Surgery Medical Research InstituteFrontier Science Center of Immunology and MetabolismZhongnan Hospital of Wuhan UniversityWuhan UniversityWuhan430071China Department of Virology College of Life SciencesWuhan UniversityWuhan430072China TaiKang Center for Life and Medical Sciences Wuhan UniversityWuhan430071China Wuhan Research Center for Infectious Diseases and Cancer Chinese Academy of Medical SciencesWuhan430071China Department of Rheumatology and Immunology Zhongnan Hospital of Wuhan UniversityWuhan430071China Cancer Center Renmin Hospital of Wuhan UniversityWuhan430060China

STING(also known as MITA)is an adaptor protein that mediates cytoplasmic DNA-triggered signaling,and aberrant activation of STING/MITA by cytosolic self-DNA or gain-of-function mutations causes severe ***,we show that STING-mediated inflammation and autoimmunity are promoted by RNF115 and alleviated by the RNF115 inhibitor disulfiram(DSF).Knockout of RNF115 or treatment with DSF significantly inhibit systemic inflammation and autoimmune lethality and restore immune cell development in Trex1^(–/–)mice and STING^(N153S/WT) bone marrow chimeric *** addition,knockdown or pharmacological inhibition of RNF115 substantially downregulate the expression of IFN-α,IFN-γand proinflammatory cytokines in PBMCs from patients with systemic lupus erythematosus(SLE)who exhibit high concentrations of dsDNA in peripheral ***,knockout or inhibition of RNF115 impair the oligomerization and Golgi localization of STING in various types of cells transfected with cGAMP and in organs and cells from Trex1^(–/–)***,knockout of RNF115 inhibits the activation and Golgi localization of STINGN153S as well as the expression of proinflammatory cytokines in myeloid cells but not in endothelial cells or *** together,these findings highlight the RNF115-mediated cell type-specific regulation of STING and STINGN153S and provide potential targeted intervention strategies for STING-related autoimmune diseases.

关键词： STING/MITA Disulfiram RNF115 SLE Autoimmunity