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Characteristics of vertical ozone distribution in the lower troposphere in the Yangtze River Delta at Lin'an in the spring of 2001

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Science china Earth sciences 2005年第9期48卷 1519-1528页

作者： zheng xiangdong1, chan chuenyu2. cui hong2. qin yu3, chan loyan2. zheng yongguang3 & lee yusiang2.1. chinese academy of meteorological sciences, beijing 100081, china 2. Department of Civil and Structural Engineering, hong Kong Polytechnic University, Hung Hom, hong Kong, china 3. Department of Atmospheric sciences, Peking University, beijing 100871, china 1. chinese academy of meteorological sciences 100081 Beijing China 2. Department of Civil and Structural Engineering Hong Kong Polytechnic University Hung Hom Hong Kong China 3. Department of Atmospheric sciences Peking University 100871 Beijing China

We analyzed vertical distributions of ozone (O3) in the lower troposphere (< 5 km above ground) at Lin’an (119.75°E, 30.30°N), Zhejiang Province using electrochemical concen- tration cell (ECC) ozonesonde data obta... 详细信息

We analyzed vertical distributions of ozone (O3) in the lower troposphere (119.75°E, 30.30°N), Zhejiang Province using electrochemical concen- tration cell (ECC) ozonesonde data obtained from February 21 to April 13, 2001. The results showed that the vertical O3 distributions are controlled by metrological conditions and the char- acteristics of O3 profiles are related to those of wet bulb potential temperature and wind field. O3 below 2 km showed that the strongest variability and enhanced O3 mixing ratios were associated with easterly winds that blow pollutants from the upwind source region of the Yangtze River Delta (YRD) region. Vertical O3 profiles below 5 km can be grouped into 5 categories: (1) peak mixing ratio type, (2) well-mixed type, (3) layered-structure type, (4) episodic pollution type and (5) alti- tudinal increasing type. Vertical distributions of O3 affected by regional transport of polluted air masses were investigated. Transport of polluted air from high latitudes of northern china, ac- companying subsiding motion of air and stagnant atmospheric conditions are important factors that lead to high mixing ratios of O3 at Lin’an. The stagnant atmospheric conditions associated with a continental high pressure system and pollution plume transported from the YRD and cen- tral-eastern china also lead to regional accumulation of O3 and high O3 mixing ratio at Lin’an. Long-range transport of O3 and pollutants from the Pearl River Delta in South china and in-situ O3 formation also resulted in elevated O3 mixing ratios at around 1 km altitudes and layered O3 distribution in the lower troposphere.

关键词： vertical ozone distribution, lower troposphere, Yangtze River Delta, Lin'an.

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