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Inkjet-Printing Controlled Phase Evolution Boosts the Efficiency of Hole Transport Material Free and Carbon-Based CsPbBr_(3) Perovskite Solar Cells Exceeding 9%

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Energy & Environmental Materials 2024年第2期7卷 209-220页

作者： lihua zhang Shi Chen Jie Zeng Zhengyan Jiang Qian Ai Xianfu zhang Bihua Hu Xingzhu Wang Shihe Yang Baomin Xu Department of Materials Science and Engineering and Shenzhen Engineering Research and Development Center for Flexible Solar Cells Southern University of Science and TechnologyShenzhen 518055China Department of Chemistry The Hong Kong University of Science and TechnologyClear Water BayHong KongChina Henan Key Laboratory of Photovoltaic Materials Henan UniversityKaifeng 475004China Guangdong Key Lab of Nano-Micro Material Research School of Chemical Biology and BiotechnologyShenzhen Graduate SchoolPeking UniversityShenzhen 518055China Key University Laboratory of Highly Efficient Utilization of Solar Energy and Sustainable Development of Guangdong Southern University of Science and TechnologyShenzhen 518055China Guangdong-Hong Kong-Macao Joint Laboratory for Photonic-Thermal-Electrical Energy Materials and Devices Southern University of Science and TechnologyShenzhen 518055China

Hole transport material free carbon-based all-inorganic CsPbBr_(3)perovskite solar cells(PSCs)are promising for commercialization due to its low-cost,high open-circuit voltage(V_(oc))and superior *** to the different solubility of PbBr_(2)and CsBr in conventional solvents,CsPbBr_(3)films are mainly obtained by multi-step spin-coating through the phase evolution from PbBr_(2)to CsPb_(2)Br_(5)and then to CsPbBr_(3).The scalable fabrication of high-quality CsPbBr_(3)films has been rarely ***,an inkjet-printing method is developed to prepare high-quality CsPbBr_(3)*** formation of long-range crystalline CsPb_(2)Br_(5)phase can effectively improve phase purity and promote regular crystal stacking of CsPbBr_(3).Consequently,the inkjet-printed CsPbBr_(3)C-PSCs realized PCEs up to 9.09%,8.59%and 7.81%with active areas of 0.09,0.25,and 1 cm^(2),respectively,demonstrating the upscaling potential of our fabrication method and *** high performance is mainly ascribed to the high purity,strong crystal orientation,reduced surface roughness and lower trap states density of the as-printed CsPbBr_(3)*** work provides insights into the relationship between the phase evolution mechanisms and crystal growth dynamics of cesium lead bromide halide films.

关键词： all-inorganic perovskite solar cells CsPbBr_(3) inkjet-printing phase evolution

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Combined application of organic fertilizer and chemical fertilizer alleviates the kernel position effect in summer maize by promoting post-silking nitrogen uptake and dry matter accumulation

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Journal of Integrative Agriculture 2024年第4期23卷 1179-1194页

作者： Lichao Zhai lihua zhang Yongzeng Cui Lifang Zhai Mengjing Zheng Yanrong Yao Jingting zhang Wanbin Hou Liyong Wu Xiuling Jia Institute of Cereal and Oil Crops Hebei Academy of Agriculture and Forestry Sciences/Key Laboratory of Crop Cultivation Physiology and Green Production of Hebei ProvinceShijiazhuang 050035China Hebei Science and Technology Innovation Service Center Shijiazhuang 050051China Yongnian Agricultural Technology Extension Center Handan 057150China Ningjin Agricultural Technology Extension Center Xingtai 055550China

Adjusting agronomic measures to alleviate the kernel position effect in maize is important for ensuring high *** order to clarify whether the combined application of organic fertilizer and chemical fertilizer(CAOFCF)can alleviate the kernel position effect of summer maize,field experiments were conducted during the 2019 and 2020 growing seasons,and five treatments were assessed:CF,100%chemical fertilizer;OFCF1,15%organic fertilizer+85%chemical fertilizer;OFCF2,30%organic fertilizer+70%chemical fertilizer;OFCF3,45%organic fertilizer+55%chemical fertilizer;and OFCF4,60%organic fertilizer+40%chemical *** with the CF treatment,the OFCF1 and OFCF2 treatments significantly alleviated the kernel position effect by increasing the weight ratio of inferior kernels to superior kernels and reducing the weight gap between the superior and inferior *** effects were largely due to the improved filling and starch accumulation of inferior ***,there were no obvious differences in the kernel position effect among plants treated with CF,OFCF3,or OFCF4 in most *** area indexes,post-silking photosynthetic rates,and net assimilation rates were higher in plants treated with OFCF1 or OFCF2 than in those treated with CF,reflecting an enhanced photosynthetic capacity and improved postsilking dry matter accumulation(DMA)in the plants treated with OFCF1 or *** with the CF treatment,the OFCF1 and OFCF2 treatments increased post-silking N uptake by 66.3 and 75.5%,respectively,which was the major factor driving post-silking photosynthetic capacity and ***,the increases in root DMA and zeatin riboside content observed following the OFCF1 and OFCF2 treatments resulted in reduced root senescence,which is associated with an increased post-silking N *** showed that post-silking N uptake,DMA,and grain yield in summer maize were negatively correlated with the kernel position *** conclusion,the combined application of

关键词： chemical fertilizer dry mater accumulation kernel position effect N uptake organic fertilizer

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The Enlightenment of Tai Chi Philosophical World View on Human Peace

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International Relations and Diplomacy 2024年第3期12卷 91-97页

作者： zhang lihua Tsinghua University BeijingChina

This paper discusses the worldview of classical Chinese Tai Chi philosophy:the holistic view,the view of Yin and Yang,view of change,view of no change,and view of harmony and their enlightenment to human *** holistic view inspires people to look at human society from the height of the whole earth,and consider not only national interests,but also the interests of all *** view of yin-yang tells people that when analyzing problems,they should look at the two aspects of yin-yang integration,not only to consider their own national interests,but also the interests of other countries,not only to see the contradictions and conflicts between countries,but also to see mutual benefits,to develop positive factors and to overcome negative factors;The view of change tells people that national leaders should adjust their foreign relations according to the changes of the times and the situation on the premise of abiding by objective laws;The view of no change tells us to act in accordance with the laws of nature and society,and that countries should respect each other,benefit each other,and cooperate for win-win *** view of harmony enlightens us that in international relations,we should advocate the idea of living in harmony,harmony in diversity and harmonious coexistence,and oppose hegemonism and power politics.

关键词： Taiji philosophy the worldview the enlightenment positive significance human peace

A Pt/CeO_(2)Hybrid Nanozyme with Stable Peroxidase Activity for the Detection of Acetylcholine

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Chemical Research in Chinese Universities 2024年第2期40卷 268-271页

作者： CUI Xulian MA Baofu PAN Hui XIA Yu LIU Li ZHAO Baofeng LIANG Zhen zhang lihua zhang Yukui State Key Laboratory of Medical Proteomics Dalian Institute of Chemical PhysicsChinese Academy of ScienceDalian116023P.R.China The Research Center for Medical Genomics Key Laboratory of Medical Cell BiologyMinistry of EducationSchool of Life ScienceChina Medical UniversityShenyang110001P.R.China River Fisheries Research Institute Chinese Academy of Fishery SciencesGuangzhou510000P.R.China

Acetylcholine(ACh)is a common neurotransmitterl)that is secreted by cholinergic neurons[2]and is found mainly in the peripheral and central nervous systems.[3]ACh transmits nerve signals from presynaptic to postsynapt... 详细信息

关键词： Acetylcholine/choline Nanozyme Hydrogen peroxide Alzheimer’s disease

Glycerol Electrooxidation over Precision-Synthesized Gold Nanocrystals with Different Surface Facets

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Precision Chemistry 2024年第3期2卷 103-111页

作者： Hansen Mou Fang Lu Zechao Zhuang Qiaowan Chang lihua zhang Xiaobo Chen Yugang zhang Jingguang G.Chen Department of Chemical Engineering Columbia UniversityNew YorkNew York 10027United States School of Chemical Engineering and Bioengineering Washington State UniversityPullmanWashington 99164United States Center for Functional Nanomaterials Brookhaven National LaboratoryUptonNew York 11973United States Materials Science and Engineering Program State University of New York at BinghamtonBinghamtonNew York 13902United States Chemistry Division Brookhaven National LaboratoryUptonNew York 11973United States

Electrochemical glycerol oxidation(EGO)emerges as a promising route to valorize glycerol,an underutilized byproduct from biodiesel production,into value-added *** study employed three types of gold(Au)nanocrystals with controlled shapes to elucidate the facet-dependent electrocatalytic behavior in ***,rhombic dodecahedral,and cubic Au nanocrystals with{111},{110},and{100}facets,respectively,were precisely synthesized with uniform size and *** dodecahedra exhibited the lowest onset potential for EGO due to facile AuOH formation,while octahedra showed enhanced electrochemical activity for glycerol oxidation and resistance to ***-situ FTIR analysis revealed that Au{111}surfaces selectively favored C_(2) products,whereas Au{100}surfaces promoted C_(3) product formation,highlighting the significant effect of facet orientation on EGO performance and informing catalyst design.

关键词： Electrochemical glycerol oxidation Precision synthesis Shaped nanocrystals Au nanocrystals SAXS In-situ FTIR

Tunable off-resonant Rydberg microwave frequency comb spectroscopy based on metawaveguide coupled Rydberg atoms

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Chinese Optics Letters 2024年第8期22卷 1-6页

作者： lihua zhang Zongkai Liu Bang Liu Qifeng Wang Yu Ma Tianyu Han Zhengyuan zhang Hanchao Chen Shiyao Shao Qing Li Jun zhang Dongsheng Ding Baosen Shi Key Laboratory of Quantum Information University of Science and Technology of ChinaHefei 230026China Synergetic Innovation Center of Quantum Information and Quantum Physics University of Science and Technology of ChinaHefei 230026China

Studying Rydberg microwave frequency comb(MFC)spectroscopy helps increase the working bandwidth of the Rydberg *** Letter demonstrates off-resonant Rydberg MFC spectroscopy in a meta-waveguide-coupled Rydberg atomic *** off-resonant MFC field couples with the Rydberg atoms through a *** system can receive the microwave field in the working band from 0.5 GHz to 13.5 GHz,and the MFC spectroscopy covers a span of 36 MHz at three different arbitrarily-chosen frequencies of 2 GHz,3 GHz,and 5.8 *** MFC spectrum that covers a wide range of 125 MHz is also *** work is significant for tunable wide-band instant microwave signal detection in the Rydberg atomic system,which is useful in microwave frequency metrology,communication,and radar.

关键词： Rydberg atoms microwave frequency comb spectroscopy metawaveguide tunability

Efficient photocatalytic reduction of COto formate by a molecular noble metal-free system

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Science China Chemistry 2024年

作者： lihua zhang Lingjing Chen Huatian Shi Yue Wei Gui Chen Tai-Chu Lau School of Environment and Civil Engineering Research Center for Eco-environmental Engineering Dongguan University of Technology Department of Chemistry and Institute of Molecular Functional Materials City University of Hong Kong

Reducing CO2to carbon-neutral solar fuels can not only alleviate the energy demand but also mitigate the greenhouse *** present,developing an efficient non-noble metal photo/electrocatalytic system for converting CO2to a specific product beyond CO is still a big ***,we report a new cobalt complex bearing 2,2′-bi-1,10-phenanthroline ligand that can photocatalytically reduce CO2to formate （HCOO-）.Turnover number （TON） for HCOO-up to 677 with 99%selectivity can be achieved using organic dyes purpurin as photosensitizer and 1,3-dimethyl-2-phenyl-2,3-dihydro-1H-benzo[d]imidazole （BIH） as sacrificial reductant in a CO2-saturated NMP/TEA （v/v,3:1） solution under visible light *** potential electrolysis at-1.41 V （***/AgCl） in the presence of 12 mM Et3NHBF4also produced HCOO-with Faradaic efficiency of39%.Spectroscopic and electrochemical studies suggest that a[CoI-H]species is the key intermediate for CO2reduction.

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反思历史主义:文学批评对文学史的拯救

南方文坛 2024年第2期 128-129页

作者：张丽华北京大学中文系

黄子平老师提出的“同时代人”概念出自阿甘本。这个词的含义与我们通常从字面引起的联想——作为代际关系的“同代人”的意涵十分不同。它不是一个社会学概念,而是指向人文学者对自我与时代以及对一种新的时间哲学和历史哲学的思考。... 详细信息

黄子平老师提出的“同时代人”概念出自阿甘本。这个词的含义与我们通常从字面引起的联想——作为代际关系的“同代人”的意涵十分不同。它不是一个社会学概念,而是指向人文学者对自我与时代以及对一种新的时间哲学和历史哲学的思考。在阿甘本看来,“真正同时代的人,真正属于其时代的人,也是那些既不与时代完全一致,也不让自己适应时代要求的人”(阿甘本:《何谓同时代人?》)。所谓的同时代性,指的是一种自我与时代既依附又保持距离的奇特关系,确切地说,是一种通过疏离、脱节乃至时代错位而让自己与时代产生关联的辩证法。

关键词：同时代人黄子平文学批评阿甘本人文学者社会学概念历史主义同时代性

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System design and validation of Queqiao-2 lunar relay communication satellite

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中国空间科学技术(中英文) 2024年第5期44卷 23-39页

作者： zhang lihua XIONG Liang SUN Ji CHEN Luojing XIAO Chuan ZHOU Wenyan WANG Yong LIU Wangwang GUAN Yifeng CHEN Tao YU Xiaochuan XU Jin CHEN Guohui CAO Xiaoping DFH Satellite Co. Ltd. Beijing Institute of Spacecraft System Engineering Beijing Institute of Control Engineering Academy of Space Information Systems

In order to provide relay communication supports for future Chinese lunar exploration program, Queqiao-2 relay communication satellite was ***-2 can perform scientific observations with three kinds of scientific instruments on *** system design of Queqiao-2,including mission orbit and transfer orbit design, configuration and layout design, housekeeping and information flow design, power supply and distribution design, GNC and propulsion system design, communication links design, etc.,was accomplished through comprehensive tradeoff and evaluation on technical maturity, availability, schedule, cost, and so *** a view to reducing development risk, both the platform and relay communication payloads were developed based on significant heritage from previous Queqiao relay satellite and other relevant ***-2 features flexible system architecture to support multiple frequencies, modulations, data rates and software reconfigurations to meet new user *** to a successful launch on March 20,2024,by means of 5 orbit maneuvers, Queqiao-2 was inserted into a highly elliptical frozen mission orbit around the moon with a 24h period on *** on-orbit tests and calibrations, Queqiao-2 has possessed the capacity to provide reliable relay communication services to multiple lunar exploration missions, as well as the capacity to perform scientific *** the support of Queqiao-2,Chang′e-6 achieved its ambitious mission goal to collect and return samples from the moon′s mysterious far *** the meanwhile, Queqiao-2 has also paved the way for the following Chinese lunar exploration missions including Chang′e-7 and Chang′*** design life time of Queqiao-2 is more than 8 *** from flexibility and extensibility of relay communication system design, it is convenient to provide relay communication services for future lunar exploration missions of both China and other *** addition, innovative

关键词： lunar explorations relay communication Queqiao system design test validation