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Ultrahigh energy storage performance realized in AgNbO_(3)-based antiferroelectric materials via multiscale engineering

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Journal of Advanced Ceramics 2023年第6期12卷 1166-1177页

作者： mingyuan zhao Jing Wang Ji Zhang Li-Feng Zhu Lei zhao Key Laboratory of High-Precision Computation and Application of Quantum Field Theory of Hebei Province College of Physics Science&TechnologyHebei UniversityBaoding 071002China State Key Laboratory of Mechanics and Control of Mechanical Structures College of Aerospace EngineeringNanjing University of Aeronautics and AstronauticsNanjing 210016China School of Materials Science and Engineering Nanjing University of Science&TechnologyNanjing 210094China School of Materials Science and Engineering University of Science and Technology BeijingBeijing 100083China

Antiferroelectric(AFE)materials are promising for the applications in advanced high-power electric and electronic *** them,AgNbO_(3)(AN)-based ceramics have gained considerable attention due to their excellent energy storage ***,multiscale synergistic modulation is proposed to improve the energy storage performance of AN-based materials,whereby the multilayer structure is employed to improve the breakdown strength(Eb),and Sm/Ta doping is utilized to enhance the AFE *** a result,ultrahigh recoverable energy storage density(Wrec)up to 15.0 J·cm^(-3) and energy efficiency of 82.8%are obtained at 1500 kV·cm^(-3) in Sm/Ta co-doped AN multilayer ceramic capacitor(MLCC),which are superior to those of the state-of-the-art AN-based ceramic ***,the discharge energy density(Wa)in direct-current charge-discharge performance reaches 9.1 J·cm^(-3),which is superior to that of the reported lead-free energy storage *** synergistic design of composition and multilayer structure provides an applicable method to optimize the energy storage performance in all dielectric energy storage systems.

关键词： antiferroelectric(AFE) AgNbO_(3)(AN)-based ceramics energy storage multilayer structure

Energy storage performance and phase transition under high electric field in Na/Ta co-doped AgNbO_(3)ceramics

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Journal of Materiomics 2023年第1期9卷 19-26页

作者： mingyuan zhao Jing Wang Hao Yuan Zehan Zheng Lei zhao Key Laboratory of High-precision Computation and Application of Quantum Field Theory of Hebei Province College Physics Science and TechnologyHebei UniversityBaoding071002China State Key Laboratory of Mechanics and Control of Mechanical Structures College of Aerospace EngineeringNanjing University of Aeronautics and AstronauticsNanjing210016China

Lead-free antiferroelectric ceramics with high energy storage performance show great potential in pulsed power ***,poor breakdown strength and antiferroelectric stability are the two main drawbacks that limit the energy storage performance of antiferroelectric ***,highquality(Ag_(1-x)Na_(x))(Nb_(1-x)Ta_(x))O_(3)ceramics were prepared by the tape casting *** breakdown strength was greatly improved as a result of the high density and fine grains,while the antiferroelectric stability was enhanced owning to the M2 *** from the synergistic improvement in breakdown strength and antiferroelectric stability,(Ag_(0.80)Na_(0.20))(Nb_(0.80)Ta_(0.20))O_(3)ceramic reveals a benign energy storage performance of W_(rec)=5.8 J/cm^(3)and h=61.7%with good temperature stability,frequency stability and cycling *** is also found that the high applied electric field can promote the M2-M3 phase transition,which may provide ideas to improve the thermal stability of the energy storage performance in AgNbO_(3)-based ceramics.

关键词： Antiferroelectric ceramics AgNbO_(3)-based ceramics Phase transition Tape casting process

The separation single-wall carbon nanotubes on length by sepharose gel

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Science China(Physics,Mechanics & Astronomy) 2012年第7期55卷 1178-1182页

作者： REN LingLing zhao mingyuan WANG ZhiHua National Institute ofMetrology Beijing 100013 China Department of Applied Chemistry Beijing University of Chemical Technology Beijing 100013 China

The separations of single-wall carbon nanotubes on length by sepharose gel were investigated in this work. The solutions of sodium dodecyl sulfate and sodium deoxycholate were applied as the eluent in sequence. SEM and Raman were used to characterize the length of nanotube bundles. The results show that the longer nanotubes were eluted out first, and then the shorter tubes were followed by the sodium dodecyl sulfate. However, the separated order was totally reversed by the sodium deoxycholate. By this method, the process generated nanotube fractions not only were narrower in length distributions, but also could control the separation orders by changing the eluents. Moreover, the separation principle was also discussed.

关键词： single-wall carbon nanotubes length separation sepharose gel sodium dodecyl sulfate sodium deoxycholate

Phase transition and piezoelectric property of (Ag,K)NbO_(3) ceramics

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Journal of Materiomics 2022年第4期8卷 863-872页

作者： Lin Chen mingyuan zhao Jing Wang Suwei Zhang Fuhua Sun Lei zhao Key Laboratory of High-precision Computation and Application of Quantum Field Theory of Hebei Province College Physics Science and TechnologyHebei UniversityBaoding071002China Key Laboratory of Mechanics and Control of Mechanical Structures College of Aerospace EngineeringNanjing University of Aeronautics and AstronauticsNanjing210016China Center for Advanced Measurement Science National Institute of MetrologyBeijing100029China Institute for Advanced Materials Hubei Normal UniversityHuangshi435002China

AgNbO_(3) is an antiferroelectric (AFE) material with double hysteresis loop. Both the antiferroelectricityand ferroelectricity can be enhanced by doping. Herein, the ferroelectricity of AgNbO_(3) ceramics wasenhanced via K-doping and the phase diagram of the (Ag_(1-x)K_(x))NbO_(3) ceramics was upgraded. In details,(Ag_(1-x)K_(x))NbO_(3) ceramics are ferrielectric (FIE) M1 phase as x=5.00-5.50 mol% and ferroelectric (FE) Ophase as x=5.75-6.00 mol% before poling, and FE O phase as x=5.00-6.00 mol% after poling at roomtemperature. With increasing temperature, (Ag_(1-x)K_(x))NbO_(3) ceramics show the phase evolutions from FIEM1, AFE M2 to paraelectric (PE) T phase at x=5.00-5.50 mol% and from FE O, FE T to PE T phase at x=5.75-6.00 mol% before poling, and from FE O, FE T to PE T phase at x=5.00-6.00 mol% after *** d33 values of 180 pC/N and 285 pC/N are obtained at the FE O-FE T and FE T-PE T phase *** work sheds light on a novel and promising lead-free piezoelectric system.

关键词： (Ag_(1-x)K_(x))NbO_(3)ceramics Phase diagram Piezoelectric property

Dual-responsive fiber-reinforced hydrogel actuators by direct ion patterning

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Nano Research 2023年第12期16卷 13381-13391页

作者： mingyuan zhao Dong Han Yuan Meng Jing Liu Yuting Zhu Zhongxian Li Kai Li Wentao Liu Zhuo Ao CAS Center for Excellence in Nanoscience National Center for Nanoscience and TechnologyBeijing 100190China School of Future Technology University of Chinese Academy of SciencesBeijing 100049China College of Life Sciences Beijing University of Chinese MedicineBeijing 100029China

Nature inspired deformable heterogeneous smart hydrogels have attracted much attention in many fields such as biomedicine devices and soft ***,normal spatial heterogeneous hydrogel structures can only respond to single factor and take one action as set in ***,we report a pre-stretched metal-liganded shape memory hydrogel with fiber reinforced,P(AAc-co-AAm)/CCNFs-Fe3+(CCNFs:carboxylated cellulose nanofibers,AAc:acrylic acid,AAm:acrylamide),which can conduct shape deformation by solvent induction and ultraviolet(UV)*** deformation pattern could be programmed by the deposing of ferroin ***,the pre-stretched shape memory hydrogels could effectively produce cyclic actuation or complex shape actuation by UV *** importantly,combining the solvent response with the light response enabled complex reversible actuations,such as simulating the bending and unfolding of *** addition of CCNFs significantly enhanced the mechanical properties of the *** hydrogels with 3 wt.%CCNFs showed an elongation at break of about 500%and a significant increase in tensile strength of 8.7-fold to 1.55 MPa after coordination with metal ions,which was able to meet the mechanical requirements of the bionic actuated *** work demonstrated that combining light-programmed and light-responsive shape-memory hydrogels,complemented by another independent response property,could achieve complex and reversible programmed actuations.

关键词： dual responsive hydrogel shape deformation metal ion pattern carboxylated cellulose nanofibers(CCNFs) light induction

Light field depth estimation:A comprehensive survey from principles to future

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High-Confidence Computing 2024年第1期4卷 92-107页

作者： Tun Wang Hao Sheng Rongshan Chen Da Yang Zhenglong Cui Sizhe Wang Ruixuan Cong mingyuan zhao State Key Laboratory of Virtual Reality Technology and Systems School of Computer Science and EngineeringBeihang UniversityBeijing 100191China Zhongfa Aviation Institute Beihang UniversityHangzhou 311115China Faculty of Applied Sciences Macao Polytechnic UniversityMacao 999078China State Key Laboratory of Software Development Environment School of Computer Science and EngineeringBeihang UniversityBeijing 100191China

Light Field(LF)depth estimation is an important research direction in the area of computer vision and computational photography,which aims to infer the depth information of different objects in threedimensional scenes by capturing LF *** this new era of significance,this article introduces a survey of the key concepts,methods,novel applications,and future trends in this *** summarize the LF depth estimation methods,which are usually based on the interaction of radiance from rays in all directions of the LF data,such as epipolar-plane,multi-view geometry,focal stack,and deep *** analyze the many challenges facing each of these approaches,including complex algorithms,large amounts of computation,and speed *** addition,this survey summarizes most of the currently available methods,conducts some comparative experiments,discusses the results,and investigates the novel directions in LF depth estimation.

关键词： Light field Depth estimation Deep learning Sub-aperture image Epipolar-plane image

A survey for light field super-resolution

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High-Confidence Computing 2024年第1期4卷 118-129页

作者： mingyuan zhao Hao Sheng Da Yang Sizhe Wang Ruixuan Cong Zhenglong Cui Rongshan Chen Tun Wang Shuai Wang Yang Huang Jiahao Shen State Key Laboratory of Virtual Reality Technology and Systems School of Computer Science and EngineeringBeihang UniversityBeijing 100191China Key Laboratory of Data Science and Intelligent Computing International Innovation InstituteBeihang UniversityHangzhou 311115China State Key Laboratory of Software Development Environment School of Computer Science and EngineeringBeihang UniversityBeijing 100191China

Compared to 2D imaging data,the 4D light field(LF)data retains richer scene’s structure information,which can significantly improve the computer’s perception capability,including depth estimation,semantic segmentation,and LF ***,there is a contradiction between spatial and angular resolution during the LF image acquisition *** overcome the above problem,researchers have gradually focused on the light field super-resolution(LFSR).In the traditional solutions,researchers achieved the LFSR based on various optimization frameworks,such as Bayesian and Gaussian *** learning-based methods are more popular than conventional methods because they have better performance and more robust generalization *** this paper,the present approach can mainly divided into conventional methods and deep learning-based *** discuss these two branches in light field spatial super-resolution(LFSSR),light field angular super-resolution(LFASR),and light field spatial and angular super-resolution(LFSASR),***,this paper also introduces the primary public datasets and analyzes the performance of the prevalent approaches on these ***,we discuss the potential innovations of the LFSR to propose the progress of our research field.

关键词： Light field super-resolution Convolutional neural network Transformer Sub-aperture image Epipolar-plane image

Cloning and Expression of Anthocyanin Biosynthesis Related Gene RrMYB6 in Rosa rugosa

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Agricultural Sciences 2018年第3期9卷 374-383页

作者： Kai Zou Yang Wang mingyuan zhao Lanyong zhao Zongda Xu Forestry College of Shandong Agricultural University Tai’an China

R2R3-MYB transcription factor plays an important role in plant anthocyanin synthesis. Based on the transcriptional database of Rosa rugosa, one MYB transcription factor related to floral color, RrMYB6, was cloned. By using bioinformatics analysis method, cloning MYB gene and analyzing its function in anthocyanin biosynthesis regulation, we hope to lay a solid foundation for new color variety breeding of R. rugosa. Using the R. rugosa “Zi zhi” as the material, we obtained the total length of cDNA of RrMYB6 by RT-PCR and RACE. By analyzing its bioinformatics, we found that the formula of the protein was C1491H2368N452O470S17, molecular weight was 34690.97 Da, the theoretical pI was 8.74. In addition, it belonged to unstable protein with an unstable index at 50.59, and it was also a hydrophilic protein with the total average hydrophobic index at -0.847. In the secondary structure of RrMYB6 protein, the Alpha helix accounted for 32.35%, random coil was 47.39%, extended strand was 11.11%, and beta turn was 9.15%. The sequence analysis showed that RrMYB6 had a typical R2R3-MYB domain and bHLH binding domain, and it also had an N1, C1, C2 inhibitory motif, belonging to the Sg4 subfamily MYB protein. What’s more, evolutionary analysis indicated that the RrMYB6 protein was closely related with the MYB protein in Rosacea family, while it was far from those in other families. The expression analysis showed that RrMYB6 protein decreased with the color of petals deeping, and its expression was the lowest in the petals while the highest in stamens. According to the above results, it was speculated that RrMYB6 was involved in regulating the anthocyanin synthesis of R. rugosa, which belonged to negative regulatory mechanism.

关键词： Rosa rugosa Anthocyanin R2R3-MYB Gene Expression

Cloning and Expression Analysis of TTG1 Gene Related to Rosa rugosaTrichomes Formation

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American Journal of Plant Sciences 2019年第2期10卷 265-275页

作者： Yu Wang mingyuan zhao Zongda Xu Lanyong zhao Xu Han College of Forestry Shandong Agricultural University Tai’an China

The TTG1 transcription factor plays an important role in the formation of plant trichomes. Based on the R. rugosa transcriptome data, this study cloned a R. rugosa TTG1 gene, named RrTTG1, and carried out bioinformatics analysis and fluorescence quantitative analysis to explore the relationship between TTG1 gene and R. rugosa trichomes formation, in order to lay a good foundation to cultivate a thornless plant in the family Rosaceae. In this experiment, six hybrid cultivars of R. rugosa “Zizhi”, R. rugosa “Xizi”, R. rugosa “Tang fen”, R. rugosa “Hun chun”, R. rugosa “Zi long wo chi” and R. rugosa “Tian e huang” were used as experimental materials, and the cDNA full length of this gene was obtained by RT-PCR and RACE, and the full length of the cDNA was 1348 bp. After bioinformatics analysis, it is predicted that its molecular formula is C1723H2661N465O529S12, the molecular weight is 38.71 KB, and the isoelectric point is 5.00. Its instability index is 54.30, which belongs to unstable protein;and its hydrophilic amino acid distribution is relatively uniform, and the amount is larger than hydrophobic amino acid, which belongs to hydrophilic protein. Phylogenetic tree was constructed for the TTG1 gene. Evolutionary analysis indicated that RrTTG1 is closely related to the TTG1 protein of Rosaceae family, and has a close relationship with other families. The expression analysis showed that the expression of RrTTG1 protein was negatively correlated with the trichome content of R. rugosa stems and leaves. The expression levels of the three spiny varieties of R. rugosa “Hun chun”, R. rugosa “Xizi” and R. rugosa “Zi long wo chi” were lower, and the expressions of the three less thorn varieties of R. rugosa “Zizhi”, R. rugosa “Tian e huang” and R. rugosa “Tang fen” were higher. According to the above results, it was speculated that RrTTG1 is involved in the synthesis of R. rugosa trichomes and belongs to the negative regulation mechanism.

关键词： R. rugosa Trichome RrTTG1 Gene Expression