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Complete multiple round quantum dense coding with quantum logical network

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Chinese Science Bulletin 2007年第9期52卷 1162-1165页

作者： LI ChunYan1,2.LI XiHan1,2.DENG FuGuo1,2.3,zhou Ping1,2.& zhou hongyu1,2.3 1 key laboratory of beam technology and material modification of ministry of {12.,beijing normal university,beijing 100875,china 2.18},and Department of material Science and Engineering,beijing normal university,beijing 100875,china 3 beijing Radiation Center,beijing 100875,china key laboratory of {2. technology and material modification of ministry ofeducation Beijing Normal University Beijing 100875 China

We present a complete multiple round quantum dense coding scheme for improving the source ca-pacity of that introduced recently by zhang et al. The receiver resorts to two qubits for storing the four local unitary ope... 详细信息

关键词：量子通信多重量子紧凑编码量子逻辑网络量子纠缠

Effect of Microstructural Characteristics on Fracture Toughness in Direct energy Deposited Novel Ti-6Al-4V-1Mo Alloy

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Acta Metallurgica Sinica(English Letters) 2024年第1期37卷 119-131页

作者： Chao Xia Kexin zhao Xin zhou Yuqi He Panpan Gao Hengxin {2. Guangrui Gao Fengying {2. Hua Tan School of material Science and Engineering Chang’an UniversityXi’an710064China Science and technology on Plasma Dynamics laboratory Air Force Engineering UniversityXi’an710038China State key laboratory of Solidification Processing Northwestern Polytechnical UniversityXi’an710072China Surface material Protection Co. LtdXi’an710018China

Meeting the damage tolerance requirements for engineering-grade titanium alloys pose a significant challenge in achieving high fracture toughness in direct energy deposition(DED)titanium *** work primarily investigated the relationship between the microstructure and the fracture toughness of DED new Ti-6Al-4V-1Mo *** types of microstructures were designed via two process strategies:high-line energy density(HE)and {2.-line energy density(LE).Relative to LE samples,HE samples possess larger-sized microstructural characteristics(coarser grain boundaryα(α_(GB)),largerαcolonies,and coarserαlaths).Lessα/βphase boundaries were formed by coarserαlaths in the HE samples,increasing the movement of dislocations,resulting in tensile strength decreasing from 1007.1 MPa(LE)to 930.8 MPa(HE)and elongation increasing from 10.8%(LE)to 15.7%(HE).Also,HE samples exhibited an excellent fracture toughness of 114.0 MPa m^(1/2.,significantly higher than that of LE samples(76.8 MPa m^(1/2.).An analysis of crack propagation paths was conducted to investigate the factors contributing to *** primary factor enhancing toughness is the frequent obstruction of cracks by coarseαGB and largeαcolonies in HE ***,the pretty large-angle deflections induced by the superposition effect of coarseαGB and largeαcolonies play a vital of significant *** factors induced the long and tortuous high-energy pathways,which resulted in ultimately improved fracture *** discovered microstructural toughening mechanisms can serve as a reference for future studies involving titanium alloys,offering insights on how to enhance fracture toughness by achieving similar characteristics.

关键词： Direct energy deposition Ti-6Al-4V-1Mo Tensile properties Fracture toughness Crack propagation

Designing Tough,Printable,and Adaptable Eutectogels with Multinetworks via Synergy of Rapid Orthogonal Photopolymerizations and Solvent Effect in Seconds

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CCS Chemistry 2024年第2期6卷 390-402页

作者： Jupen Liu Lijun zhou Ping zhang Yanxia {2. Hongqiu Wei You Yu key laboratory of Synthetic and Natural Functional Molecule Chemistry of the {2. of education College of Chemistry and Materials ScienceNorthwest UniversityXi’an 710069

Achieving a straightforward design of tough,printable,and adaptable polymeric eutectogels is still challenging in related fields due to the uncontrollable polymerization and solvent-exchanging processes,and inherent contrasting multiple ***,we report a one-step synergistic strategy based on ruthenium chemistry-catalyzed photopolymerization and solvent effect for preparing high-performance *** orthogonal ruthenium photochemistry helps multinetworks formation via phenol-coupling of gelatin and copolymerization of acrylamide(AAm)and[2.(methacryloyloxy)ethyl]trimethylammonium tetrafluoroborate(META)monomers in *** obvious difference in the supramolecular interactions of free AAm monomers and polymerized units in P(AAm-co-META)with deep eutectic solvents(DESs)significantly promotes the microphase-separation behavior in ***,the in situ polymerization and microphase-separation behavior enable the as-prepared eutectogel materials to have excellent mechanical properties(stress of∼1.2.MPa),toughness(∼4.0 MJ m^(−3)),elasticity,adaptivity,and conductivity(∼0.5 S m^(−1)at room temperature).Also,the critical strength of the resultant eutectogels can be modulated by varying the DES *** rapid and well-controlled synergistic approach is compatible with extrusion printing techniques to make flexible sensors with high sensitivities and response times to detect pressure in a range of 0–500 *** a general and simple strategy has application potential in biological,engineering,and material sciences.

关键词： orthogonal chemistry visible-light photopolymerization solvent effect microphase separation adaptable polymers printable eutectogels

Phase reconfiguration of heterogeneous CoFeS/CoNiS nanoparticles for superior battery-type supercapacitors

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Journal of energy Chemistry 2024年第9期96卷 217-225页

作者： Lina Ma Fan Li Min zhou Jidong Dong Hao Luo Wei zhang Wenchao {2. Xinliang Li Zaixing Jiang Yudong Huang College of Chemistry and Chemical Engineering Qingdao UniversityQingdao 266071ShandongChina School of materials Science and Engineering Xiamen University of TechnologyXiamen 361024FujianChina Co-Innovation Center of Efficient Processing and Utilization of Forest Resources College of Materials Science and EngineeringNanjing Forestry UniversityNanjing 210037JiangusChina key laboratory of {2. physics Ministry of EducationSchool of Physics and MicroelectronicsZhengzhou UniversityZhengzhou 450052HenanChina MIIT key laboratory of Critical {2.s technology for New energy Conversion and Storage State Key Laboratory of Urban Water Resource and EnvironmentSchool of Chemistry and Chemical EngineeringHarbin Institute of TechnologyHarbin 150001HeilongjiangChina material Science and Engineering College Northeast Forestry UniversityHarbin 150040HeilongjiangChina

Developing advanced battery-type materials with abundant active sites,high conductivity,versatile morphologies,and hierarchically porous structures is crucial for realizing high-quality hybrid ***,heterogeneous FeS@NiS is synthesized by cationic Co doping via surface-structure *** density functional theory(DFT)theoretical calculations are firstly performed to predict the advantages of Co dopant by improving the OH^(−)adsorption properties and adjusting electronic structure,benefiting ions/electron *** dynamic surface evolution is further explored which demonstrates that CoFeS@CoNiS could be quickly reconstructed to Ni(Co)Fe_(2.O_(4)during the charging process,while the unstable structure of the amorphous Ni(Co)Fe_(2.O_(4)results in partial conversion to Ni/Co/FeOOH at high potentials,which contributes to the more reactive active site and good structural ***,the free-standing electrode reveals excellent electrochemical performance with a superior capacity(335.6 mA h g^(−1),2.84 F g^(−1))at 3 A g^(−1).Furthermore,the as-fabricated device shows a quality energy density of 78.1 W h kg^(−1)at a power density of 750 W kg^(−1)and excellent cycle life of 9{2.%capacitance retention after 5000 *** work offers a facile strategy to construct versatile morphological structures using electrochemical activation and holds promising applications in energy-related fields.

关键词： In-situ reconfiguration Heterogeneous design Battery-type supercapacitors Superior performance Sulphide

Effect of Thermal Fatigue Loading on Tensile Behavior of H13 Die Steel with Biomimetic Surface

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Journal of Bionic Engineering 2010年第4期7卷 390-396页

作者： Zhihui zhang~1,Luquan Ren~1,Hong zhou~2,Zhiwu Han~1,Xin Tong~3,Yu zhao~1,Li Chen~1 1.key laboratory of Bionic Engineering (ministry of education,china),Jilin university,Changchun 130022,P.R.china 2.key laboratory of Automobile materials (ministry of education,china),Jilin university,Changchun 130022,P.R.china 3.The Department of materials Surface Engineering,Guangzhou Research institute of Non-Ferrous Metals,Guangzhou 510651,P.R.china [a] key laboratory of Bionic Engineering ({2. of education China) Jilin University Changchun 130022 P. R. China [b] Key Laboratory of Automobile Materials (Ministry of Education China) Jilin University Changchun 130022 P. R. China [c] The Department of Materials Surface Engineering Guangzhou Research Institute of Non-Ferrous Metals Guangzhou 510651 P. R. China

Biomimetic surface is an effective ways to promote the performance grade and applied range of materials without alteringtheir *** improved properties such as resisting fatigue,enduring wear,etc,have been achieved by applyingbiomimetic morphology or structure to some engineering material *** this paper,aiming to reveal the relationshipbetween thermal cracking behavior and mechanical properties of engineering materials with biomimetic surface,biomimeticspecimens were fabricated using laser technique by imitating the heterogeneous structure on the surface of plant *** of thermal fatigue cycling on the tensile properties of H13 die steel specimens with different surfaces (several types ofbiomimetic surfaces and a smooth surface) was compared and *** a result,due to the coupling effects of themorphological features on the surface and the microstructure characteristics within unit zone,these specimens with biomimeticsurface exhibit remarkably enhanced Ultimate Tensile Strength (UTS) and 0.2. Yield Strength (YS) compared with referencespecimens while corresponding ductility remains largely unaffected even heightened,whether the thermal fatigue loads or *** relative mechanisms leading to these improvements have been discussed.

关键词： biomimetic surface coupling thermal fatigue tensile property H13 steel

Transforming waste particles into valuable adsorbents via amyloid-mediated molecular engineering

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Science china Chemistry 2024年

作者： Qingmin Yang Jian zhao Yujia zhang Xingyu {2. Hao Ren Bowen Hu Zhongli Lei Lixin Chen Peng Yang School of material and Chemical Engineering Bengbu University Anhui Provincial Engineering laboratory of Silicon-Based materials School of Chemistry and Chemical Engineering Northwestern Polytechnical University key laboratory of Applied Surface and Colloid Chemistry Ministry of Education School of Chemistry and Chemical EngineeringShaanxi Normal University Xi'an key laboratory of Polymeric Soft Matter School of Chemistry and Chemical Engineering Shaanxi Normal University International Joint Research Center on Functional Fiber and Soft Smart Textile School of Chemistry and Chemical EngineeringShaanxi Normal University

The high-value utilization of industrial solid waste using a facile and eco-friendly process is of great interest and significance in reducing environmental pollution and developing a green circular economy. Herein, we propose an amyloid-mediated molecular engineering strategy to transform particulate waste into valuable adsorbents for metal ions. Our method has the advantage of aqueous solution fabrication under mild conditions without the use of high-temperature hydrothermal methods and toxic chemical reagents. Amyloid-mediated molecular engineering manipulates the phase transition of bovine serum albumin（BSA）on particulate waste surfaces, resulting in a remarkable ～3.1 times improvement in the adsorption capacity of fly ash, a typical industrial solid waste for gold ions after modification with the phase-transitioned BSA（PTB）. The resultant adsorption ability was 69–1,980 times higher than those of conventional and emerging adsorbent materials such as ion exchange resins, activated carbon（AC）, covalent organic frameworks（COFs）, and metal-organic frameworks（MOFs）. We further demonstrated the application of our PTB-modified materials in the recovery of precious metals from low-grade gold ore and electronic waste leachates. Consequently, this strategy could increase the value of waste materials nearly 2. times. In addition, this method is generally extendable to other conventional industrial adsorbents such as resin, clay, and Al2.3, and enhances their adsorption capabilities at least twofold. Overall, this work provides a simple and green approach for improving the adsorption performance of solid particles, and is expected to develop into a universal strategy for transforming waste particles into high-value-added products.

关键词：

Boosting rate performance of layered lithium-rich cathode materials by oxygen vacancy induced surface multicomponent integration

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Journal of energy Chemistry 2024年第5期92卷 250-262页

作者： Youyou Fang Yuefeng Su Jinyang Dong Jiayu zhao Haoyu Wang Yun Lu Bin zhang Hua Yan Feng Wu Lai Chen beijing key {2. of Environmental Science and Engineering School of Material Science and EngineeringBeijing Institute of TechnologyBeijing 100081China Chongqing Innovation Center Beijing Institute of TechnologyChongqing 401120China Yibin Libode New materials Co. Ltd.Yibin 64400SichuanChina School of Metallurgy and Environment Central South UniversityChangsha 410083HunanChina Engineering Research Center of the ministry of education for Advanced Battery {2.s Central South UniversityChangsha 410083HunanChina

The rapid development of electric vehicles and portable energy storage systems demands improvements in the energy density and cost-effectiveness of lithium-ion batteries,a domain in which Lithium-rich layered cathode(LLO){2.s inherently ***,these {2.s face practical challenges,such as low initial Coulombic efficiency,inferior cycle/rate performance,and voltage decline during cycling,which limit practical *** study introduces a surface multi-component integration strategy that incorporates oxygen vacancies into the pristine LLO {2. Li1.2.n_(0.6)Ni_(0.2.O_(2..This process involves a brief citric acid treatment followed by calcination,aiming to explore rate-dependent degradation *** induced surface oxygen vacancies can reduce surface oxygen partial pressure and diminish the generation of O_(2.and other highly reactive oxygen species on the surface,thereby facilitating the activation of Li ions trapped in tetrahedral sites while overcoming transport ***,the formation of a spinel-like phase with 3D Li+diffusion channels significantly improves Li^(+)diffusion kinetics and stabilizes the surface *** optimally modified sample boasts a discharge capacity of 2.9.5 mA h g^(-1)at a 0.1 C and 2.1.6 mA h g^(-1)at a 1 C during the initial activation cycle,with an impressive capacity of 2.2.1 mA h g^(-1)at a 5 *** notably,it retained nearly 70%of its capacity after 300 cycles at this elevated *** straightforward,effective,and highly viable modification strategy provides a crucial resolution for overcoming challenges associated with LLO {2.s,making them more suitable for practical application.

关键词： Lithium-ion battery Layered lithium rich cathode Surface multicomponent integration Rate-dependent degradation and Li^(+) diffusion kinetics

Measurement of solar pp neutrino flux using electron recoil data from PandaX-4T commissioning run

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Chinese physics C 2024年第9期48卷 1-7,300页

作者： Xiaoying Lu Abdusalam Abdukerim Zihao Bo Wei Chen Xun Chen Yunhua Chen Chen Cheng zhaokan Cheng Xiangyi Cui Yingjie Fan Deqing Fang Lisheng Geng Karl Giboni Xuyuan Guo Chencheng Han Ke Han Changda He Jinrong He Di Huang Junting Huang zhou Huang Ruquan Hou Yu Hou Xiangdong Ji Yonglin Ju Chenxiang Li Jiafu Li Mingchuan Li Shuaijie Li Tao Li Qing Lin Jianglai Liu Congcong Lu Lingyin Luo Yunyang Luo Wenbo Ma Yugang Ma Yajun Mao Yue Meng Xuyang Ning Binyu Pang Ningchun Qi Zhicheng Qian Xiangxiang Ren Nasir Shaheed Xiaofeng Shang Xiyuan Shao Guofang Shen Manbin Shen Lin Si Wenliang Sun Yi Tao Anqing Wang Meng Wang Qiuhong Wang Shaobo Wang Siguang Wang Wei Wang Xiuli Wang Xu Wang zhou Wang Yuehuan Wei Mengmeng Wu Weihao Wu Yuan Wu Mengjiao Xiao Xiang Xiao Kaizhi Xiong Binbin Yan Xiyu Yan Yong Yang Chunxu Yu Ying Yuan Zhe Yuan Youhui Yun Xinning Zeng Minzhen zhang Peng zhang Shibo zhang Shu zhang Tao zhang Wei zhang Yang zhang Yingxin zhang Yuanyuan zhang Li zhao Jifang zhou Ning zhou Xiaopeng zhou Yubo zhou Zhizhen zhou Research Center for Particle Science and technology Institute of Frontier and Interdisciplinary ScienceShandong UniversityQingdao 266237China key laboratory of Particle {2. and Particle Irradiation of ministry of education Shandong UniversityQingdao 266237China School of physics and Astronomy Shanghai Jiao Tong UniversityKey Laboratory for Particle Astrophysics and Cosmology(MoE)Shanghai Key Laboratory for Particle Physics and CosmologyShanghai 200240China New Cornerstone Science laboratory Tsung-Dao Lee InstituteShanghai Jiao Tong UniversityShanghai 200240China Shanghai Jiao Tong university Sichuan Research institute Chengdu 610213China Jinping Deep Underground Frontier Science and Dark Matter key laboratory of Sichuan Province Liangshan 615000China Yalong River Hydropower Development Company Ltd.288 Shuanglin RoadChengdu 610051China School of physics Sun Yat-Sen UniversityGuangzhou 510275China Sino-French institute of nuclear Engineering and {2. Sun Yat-Sen UniversityZhuhai 519082China Department of physics Yantai UniversityYantai 264005China key laboratory of {2. physics and Ion-beam Application(MOE) Institute of Modern PhysicsFudan UniversityShanghai 200433China School of physics Beihang UniversityBeijing 102206China beijing key {2. of Advanced nuclear materials and physics Beihang UniversityBeijing 102206China Peng Huanwu Collaborative Center for Research and education Beihang UniversityBeijing 100191China Southern Center for nuclear-Science Theory(SCNT) Institute of Modern PhysicsChinese Academy of SciencesHuizhou 516000China School of Mechanical Engineering Shanghai Jiao Tong UniversityShanghai 200240China Department of physics University of MarylandCollege ParkMaryland 20742USA State key laboratory of Particle Detection and Electronics University of Science and Technology of ChinaHefei 230026China Department of Modern physics University of Science and Technology of ChinaHefei 230026China School of physics Peking UniversityBeijing 100871Ch

The proton-proton(pp)fusion chain dominates the neutrino production in the *** uncertainty of the predicted pp neutrino flux is at the sub-percent level,whereas that of the best measurement is O(10%).In this study,for the first time,we measure solar pp neutrinos in the electron recoil energy range from 2. to 144 keV using the PandaX-4T commissioning data with 0.63 tonne×year *** pp neutrino flux is determined as(8.0±3.9(stat)±10.0(syst))×1010 s^(-1)cm^(-2.,which is consistent with the Standard Solar Model and existing measurements,corresponding to an upper flux limit of 2..3×10^(10)s^(-1)cm^(-2.at 90%C.L..

关键词： solar pp neutrino flux PandaX-4T electron recoil spectrum

High-repetition-rate and high-power efficient picosecond thin-disk regenerative amplifier

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High Power Laser Science and Engineering 2024年第2期12卷 16-23页

作者： Sizhi Xu Yubo Gao Xing Liu Yewang Chen Deqin Ouyang Junqing zhao Minqiu Liu Xu Wu Chunyu Guo Cangtao zhou Qitao Lue Shuangchen Ruan key laboratory of Advanced Optical Precision Manufacturing {2. of Guangdong Higher education institutes Sino-German College of Intelligent ManufacturingShenzhen Technology UniversityShenzhenChina Han’s Laser technology Industry Group Co. Ltd.ShenzhenChina Shenzhen key laboratory of Laser Engineering College of Physics and Optoelectronic EngineeringShenzhen UniversityShenzhenChina Shenzhen key laboratory of Ultraintense Laser and Advanced {2. technology College of Engineering PhysicsShenzhen Technology UniversityShenzhenChina

We present an effective approach to realize a highly efficient,high-power and chirped pulse amplification-free ultrafast ytterbium-doped yttrium aluminum garnet thin-disk regenerative amplifier pumped by a zero-phonon line 969 nm laser *** amplifier delivers an output power exceeding 154 W at a pulse repetition rate of 1 MHz with custom-designed 48 pump *** exceptional thermal management on the thin disk through high-quality bonding,efficient heat dissipation and a fully locked spectrum collectively contributes to achieving a remarkable optical-to-optical efficiency of 61%and a near-diffraction-limit beam quality with an M2.factor of *** the best of our knowledge,this represents the highest conversion efficiency reported in ultrafast thin-disk regenerative ***,the amplifier operates at room temperature and exhibits exceptional stability,with root mean square stability of less than 0.33%.This study significantly represents advances in the field of laser amplification systems,particularly in terms of efficiency and average *** advantageous combination of high efficiency and diffraction limitation positions the thin-disk regenerative amplifier as a promising solution for a wide range of scientific and industrial applications.

关键词： high efficiency high power picosecond laser regenerative amplifier thin-disk laser