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High‑Energy and High‑Power Pseudocapacitor–Battery Hybrid Sodium‑Ion Capacitor with Na^(+) Intercalation Pseudocapacitance Anode

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Nano-Micro Letters 2021年第3期13卷 209-221页

作者： Qiulong Wei Qidong Li Yalong Jiang yunlong zhao Shuangshuang Tan Jun Dong Liqiang Mai Dong‑Liang Peng Department of Materials Science and Engineering Fujian Key Laboratory of Materials GenomeCollege of MaterialsXiamen UniversityXiamen 361005People’s Republic of China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070People’s Republic of China Shenzhen Geim Graphene Center Tsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055People’s Republic of China Advanced Technology Institute University of SurreyGuildford Surrey GU27XHUK

High-performance and low-cost sodium-ion capacitors(SICs)show tremendous potential applications in public transport and grid energy ***,conventional SICs are limited by the low specific capacity,poor rate capability,and low initial coulombic efficiency(ICE)of anode ***,we report layered iron vanadate(Fe5V15O39(OH)9·9H2O)ultrathin nanosheets with a thickness of~2.2 nm(FeVO UNSs)as a novel anode for rapid and reversible sodium-ion *** to in situ synchrotron X-ray diffractions and electrochemical analysis,the storage mechanism of FeVO UNSs anode is Na+intercalation pseudocapacitance under a safe potential *** FeVO UNSs anode delivers high ICE(93.86%),high reversible capacity(292 mAh g^−1),excellent cycling stability,and remarkable rate ***,a pseudocapacitor–battery hybrid SIC(PBH-SIC)consisting of pseudocapacitor-type FeVO UNSs anode and battery-type Na3(VO)2(PO4)2F cathode is assembled with the elimination of presodiation *** PBH-SIC involves faradaic reaction on both cathode and anode materials,delivering a high energy density of 126 Wh kg^−1 at 91 W kg^−1,a high power density of 7.6 kW kg^−1 with an energy density of 43 Wh kg−1,and 9000 stable *** tunable vanadate materials with high-performance Na+intercalation pseudocapacitance provide a direction for developing next-generation highenergy capacitors.

关键词： Sodium-ion capacitors Pseudocapacitance Hybrid capacitors Two-dimensional materials Iron vanadate

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产科常见易错手术操作编码案例分析

中国病案 2024年第3期25卷 38-41页

作者：黄娜萍徐倩成财达赵云龙中山大学附属第六医院广东省广州市510000

在ICD-9-CM-3中产科系统的手术操作因临床书写相同,手术操作过程相似,但编码往往不同,编码员在编码时常有误编。列举某院病案质控发现的产科手术操作编码错误较多的几种编码,例如催产素静滴、人工破膜引产术、会阴切开术、会阴裂伤修补... 详细信息

在ICD-9-CM-3中产科系统的手术操作因临床书写相同,手术操作过程相似,但编码往往不同,编码员在编码时常有误编。列举某院病案质控发现的产科手术操作编码错误较多的几种编码,例如催产素静滴、人工破膜引产术、会阴切开术、会阴裂伤修补术、剖宫产术、子宫球囊置入术等,探讨分析其编码要点及查找方法,总结产科中催产素静滴编码时需要注意是否药物增强分娩;人工破膜引产术根据操作时是否进入产程编码于73.01、73.09;会阴切开术根据是否伴有产钳或真空吸引操作编码于73.6、72.1、72.21、72.31、72.71;会阴裂伤修补术根据疾病性质编码于71.71、75.69、71.79;剖宫产术根据目的不同编码于74.1、74.91;子宫球囊置入术根据置入球囊目的不同编码于69.91、73.1、75.8;分娩后清宫术根据术式编码于69.02、69.52。编码员需提升临床基础知识和病案专业技能,熟练掌握产科手术操作编码规则,并与临床保持良好沟通,才能提高编码准确性。

关键词：产科手术手术操作编码编码分析

Sisyphus effects in hydrogen electrochemistry on metal silicides enabled by silicene subunit edge

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Science Bulletin 2019年第9期64卷 617-624页

作者： Zechao Zhuang Yong Li Jiazhao Huang Zilan Li Kangning zhao yunlong zhao Lin Xu Liang Zhou Lyudmila V. Moskaleva Liqiang Mai State Key Laboratory of Advanced Technology for Materials Synthesis and Processing International School of Materials Science and EngineeringWuhan University of Technology Institute of Applied and Physical Chemistry and Center for Environmental Research and Sustainable Technology University of Bremen Advanced Technology Institute University of Surrey Department of Chemistry University of the Free State

Nonmetal elements strictly govern the electrochemical performance of molybdenum ***,the exact role played by nonmetals during electrocatalysis remains largely *** intermetallic MoSi_2comprising silicene subunits,we present an unprecedented hydrogen evolution reaction(HER)behavior in aqueous alkaline *** continuous operation,the HER activity of MoSi_2shows a more than one order of magnitude improvement in current density from 1.1 to 21.5 mA cm^(à2)at 0.4 V ***,this activation behavior is highly reversible,such that voltage withdrawal leads to catalyst inactivation but another operation causes ***,the system shows dynamics strikingly analogous to the legendary Sisyphus’labor,which drops and recovers in a stepwise manner repeatedly,but never succeeds in reaching the top of the *** WSi_2behaves almost the same as MoSi_2,whereas other metal silicides with silicyne subunits,including CrSi_2and TaSi_2,do not exhibit any anomalous behavior.A thin amorphous shell of MoSi_2is observed after reaction,within which the Si remains partially oxidized while the oxidation state of Mo is basically ***-principles calculations further reveal that the adsorption of hydroxide ions on silicene subunit edges and the subsequent Si vacancy formation in MoSi_2jointly lead to the anomalous HER kinetics of the adjacent Mo active *** work demonstrates that the role of nonmetal varies dramatically with the electronic and crystallographic structures of silicides and that silicene structural subunit may serve as a promoter for boosting HER in alkaline media.

关键词： Sisyphus effect Electrochemistry Metal silicides Silicene subunit Hydrogen evolution reaction

香椿精油提取方法、成分分析及生物活性研究进展

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中国食品添加剂 2024年第4期35卷 289-294页

作者：刘雨辰曲梦锐赵云龙王东营河南工业大学粮油食品学院郑州450001

香椿在中国分布广泛,历史悠久。香椿精油是从香椿茎叶或香椿籽中提取出来的一种带有浓烈芳香气味的挥发油。其成分复杂,具有抗癌、抗肿瘤、抗氧化、抗菌、抗病毒等多种生物活性,在果蔬保鲜的应用中有一定的潜力。虽然香椿精油具有潜在... 详细信息

香椿在中国分布广泛,历史悠久。香椿精油是从香椿茎叶或香椿籽中提取出来的一种带有浓烈芳香气味的挥发油。其成分复杂,具有抗癌、抗肿瘤、抗氧化、抗菌、抗病毒等多种生物活性,在果蔬保鲜的应用中有一定的潜力。虽然香椿精油具有潜在的食品和医药应用价值,但应用尚处于探索阶段,相关研究较少。本文综述了香椿精油提取方法,化学成分,生物活性等方面的研究调查,以期为香椿精油的应用发展提供理论支持与参考,并促进相关研究的深入开展。

关键词：香椿精油提取方式成分分析生物活性

Towards Practical Application of Li-S Battery with High Sulfur Loading and Lean Electrolyte:Will Carbon-Based Hosts Win This Race?

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Nano-Micro Letters 2023年第9期15卷 384-422页

作者： Yi Gong Jing Li Kai Yang Shaoyin Li Ming Xu Guangpeng Zhang Yan Shi Qiong Cai Huanxin Li yunlong zhao Advanced Technology Institute University of SurreyGuildfordSurrey GU27XHUK Department of Chemical and Process Engineering University of SurreyGuildford GU27XHUK Department of Chemistry Physical and Theoretical Chemistry LaboratoryUniversity of OxfordOxford OX13QZUK Department of Engineering University of Cambridge9 JJ Thomson AvenueCambridge CB30FAUK State Key Laboratory for Chemo/Biosensing and Chemometrics College of Chemistry and Chemical EngineeringHunan UniversityChangsha 410082HunanPeople’s Republic of China College of Materials and Metallurgy Guizhou UniversityGuiyang 550025People’s Republic of China

As the need for high-energy–density batteries continues to grow, lithium-sulfur(Li–S) batteries have become a highly promising next-generation energy solution due to their low cost and exceptional energy density compared to commercially available Li-ion batteries. Research into carbon-based sulfur hosts for Li–S batteries has been ongoing for over two decades, leading to a significant number of publications and ***, the commercialization of Li–S batteries has yet to be realized. This can be attributed, in part, to the instability of the Li metal anode. However, even when considering just the cathode side, there is still no consensus on whether carbon-based hosts will prove to be the best sulfur hosts for the industrialization of Li–S batteries. Recently, there has been controversy surrounding the use of carbon-based materials as the ideal sulfur hosts for practical applications of Li–S batteries under high sulfur loading and lean electrolyte conditions. To address this question, it is important to review the results of research into carbon-based hosts, assess their strengths and weaknesses, and provide a clear perspective. This review systematically evaluates the merits and mechanisms of various strategies for developing carbon-based host materials for high sulfur loading and lean electrolyte conditions. The review covers structural design and functional optimization strategies in detail, providing a comprehensive understanding of the development of sulfur hosts. The review also describes the use of efficient machine learning methods for investigating Li–S batteries. Finally, the outlook section lists and discusses current trends, challenges, and uncertainties surrounding carbon-based hosts, and concludes by presenting our standpoint and perspective on the subject.

关键词： Li-S batteries Carbon materials Structural design Functional modification Machine learning

Monazite U-Th-Pb and sericite Rb-Sr dating of the Xiajiadian black shale-hosted gold deposit in the Qinling orogen,central China:Implications for regional gold metallogeny

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Science China Earth Sciences 2024年第8期67卷 2478-2494页

作者： Xueling YU Jianwei LI Xiaoye JIN Shaorui zhao Chongguo HE yunlong ZHU State Key Laboratory of Geological Processes and Mineral Resources China University of GeosciencesWuhan 430074China School of Earth Resources China University of GeosciencesWuhan 430074China

The Qinling orogen in central China contains several black shale-hosted gold deposits,but the age of their formation and a possible relation between gold mineralization and regional tectonism remain *** we present results of in situ monazite U-Th-Pb dating and sericite Rb-Sr dating of the Xiajiadian black shale-hosted gold deposit to provide tight constraints on the time of gold deposition and information on the tectonic setting under which the deposit *** Xiajiadian gold deposit is mainly hosted in black shales of the Lower Cambrian Shuigoukou formation,with minor ores contained in sandy conglomerate of the Lower Devonian Xichahe *** ores in the black shales have been intensively oxidized and consist mainly of hematite,goethite,gypsum,quartz,calcite,native gold,and unrecognized iron ***,gold ores in the sandy conglomerate are free of oxidation and thus provide an opportunity to date the formation of the Xiajiadian gold *** ores consist of pyrite,marcasite,sericite,and quartz,which are associated with a variety of accessory minerals,including monazite,apatite,and *** is mainly present as structure-bound ions or nanoparticles in pyrite and marcasite,but minor native gold grains also occur as inclusions in *** is well developed in the ores,and has close textural association with Au-bearing pyrite and *** monazite grains have zoned textures consisting of a core area(Mnz1)and an overgrowth zone(Mnz2).Mnz1 contains 4.8–13 wt.%ThO_(2)and shows large variations in HREE and prominent negative Eu anomalies in the chondrite-normalized REE *** yields common lead-corrected^(208)Pb/^(232)Th dates ranging from 910±10 to416±4 Ma(2σ).These dates are interpreted in terms of a detrital origin for monazite in the core ***2 has much lower ThO_(2)contents of 0.8–1.7 wt.%and shows weak negative Eu anomalies in the chondrite-normalized REE *** yields common lead-corrected^(208)Pb/^(232

关键词： Monazite U-Th-Pb dating Sericite Rb-Sr dating Late Triassic(Norian) Orogenic gold deposit Xiajiadian

An Extended Application form of Mobile Computing ── Augmented Reality

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High Technology Letters 2001年第2期7卷 39-41页

作者：杨孝宗 Sch. of Computer Sci. and Technol. Harbin Institute of Technology Harbin 150001 China

With the rapid developments of wireless communication and microelectronic technology, the bandwidth of wireless communication is becoming wider than ever, up to 100Gbps and the computer can be designed as small as a match with powerful computing and controlling capability. These rapid developments have extended the mobile computing. There are many application forms of mobile computing, such as mobile databases, mobile data management, wearable computing etc. A great branch of mobile computing, Augmented Reality (AR), which is the combination of mobile computing and wearable computers was discussed.

关键词： Mobile computing Wireless communication Wearable computer Augmented reality Contextual awareness Bluetooth HomeRF

Industrial-scale investigations on effects of tertiary-air declination angle on combustion and steam temperature characteristics in a 350-MW supercritical down-fired boiler

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Frontiers in Energy 2021年第1期15卷 132-142页

作者： Xiaoguang LI Lingyan ZENG Hongye LIU Yao LI Yifu LI yunlong zhao Bo JIAO Minhang SONG Shaofeng ZHANG Zhichao CHEN Zhengqi LI School of Energy Science and Engineering Harbin Institute of TechnologyHarbin 150001China Guizhou Wanfeng Electric Power Co. Ltd.Xingyi 562400China Guizhou Xingyi Project Department Huadian United(Beijing)Power Engineering Co.Ltd.Xingyi 562400China

Industrial-scale experiments were conducted to study the effects of tertiary air declination angle(TDA)on the coal combustion and steam temperature characteristics in the first 350-MW supercritical down-fired boiler in China with the multiple-injection and multiple-staging combustion(MIMSC)technology at medium and high *** experimental results indicated that as the TDA increased from 0°to 15°,the overall gas temperature in the lower furnace rose and the symmetry of temperature field was *** ignition distance of the fuel-rich coal/air flow *** near-burner region,the concentration of O2 decreased while the concentrations of CO and NO *** concentration of NO decreased in near-tertiary-air *** carbon in fly ash decreased significantly from 8.40%to 6.45%at a load of 260 *** a TDA of 15°,the ignition distances were the shortest(2.07 m and 1.73 m)at a load of 210 MW and 260 MW,*** main and reheat steam temperatures were the highest(557.2℃ and 559.4℃ at a load of 210 MW,558.4℃ and 560.3℃ at a load of 260 MW).The carbon in fly ash was the lowest(4.83%)at a load of 210 *** changing the TDA from 15°to 25°,the flame kernel was found to move downward and the main and reheat steam temperatures dropped *** change of TDA has little effect on NO_(x) emissions(660–681 mg/m^(3) at 6%O_(2)).In comprehensive consideration of the pulverized coal combustion characteristics and the unit economic performance,an optimal TDA of 15°is recommended.

关键词： supercritical down-fired boiler industrialscale experiment tertiary air declination angle coal combustion steamtemperature

Effect of annealing temperature on magnetic properties of a sintered Nd-Fe-B magnet after grain boundary diffusion with Dy_(70)Cu_(30) alloy

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Journal of Rare Earths 2024年第1期42卷 116-120,I0004页

作者： Ruipeng Qian Yuxuan Ma Fugang Chen Hui Sun Yong zhao yunlong Chen School of Materials Science and Engineering Jiangsu University of Science and TechnologyZhenjiang212003China School of Energy and Power Engineering Jiangsu University of Science and TechnologyZhenjiang212003China

Grain boundary diffusion process(GBDP)has been developed as an effective approach to increase the coercivity of sintered Nd-Fe-B magnets by regulating the compositions and phase distributions near grain *** work aims to explore how to select the optimum annealing temperature after *** this work GBDP was performed on a sintered Nd-Fe-B magnet using Dy_(70)Cu_(30) *** GBDP the low eutectic temperature of the grain boundary phases decreases from the initial 492 to 451℃.The magnetic property dependent on different annealing temperatures near the low eutectic temperature was *** magnetic properties,especially the squareness factor of demagnetization curve show a strong dependence on the annealing *** GBDP the optimal magnetic properties can be obtained after annealing just above the low eutectic temperature of the grain boundary *** mechanism is discussed based on the microstructure analysis.

关键词： Nd-Fe-B magnet Grain boundary diffusion Annealing Dy_(70)Cu_(30)alloy Rare earths