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In situ regeneration of catalyst for Fenton-like degradation by photogenerated electron transportation:Characterization,performance and mechanism comparison

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Chinese Chemical Letters 2025年第1期36卷 529-533页

作者： Ming-Zhen Li Yang zhang Kun Li Ya-Nan Shang yi-Zhen zhang Yu-jiao Kan Zhi-Yang jiao Yu-Yuan Han Xiao-Qiang Cao College of Safety and Environmental Engineering Shandong University of Science and TechnologyQingdao 266590China Engineering Research Center of Groundwater Pollution Control and Remediation Ministry of Education of ChinaBeijing Normal UniversityBeijing 100875China Environment Research Institute Shandong UniversityQingdao 266237China Institute of Yellow River Delta Earth Surface Processes and Ecological Integrity Shandong University of Science and TechnologyQingdao 266590China

Inactivation of carbon-based transition metal catalysts,which was caused by electron loss,limited their application in advanced oxidation ***,Co and TiO_(2) double-loaded carbon nanofiber material(Co@CNFs-TiO_(2))was synthesized in this *** and chemical catalytic systems were synergized *** was eliminated within 15 *** degradation rate remained above 90%after five cycles,and the 50%promotion proved the high stability of Co@CNFs-TiO_(2).The main reactive oxygen species in this system were sulfate radicals,whereas Co and TiO_(2) represented the active sites of the catalytic *** generated from TiO_(2) during the photocatalytic process were transferred to Co,which promoted the Co(Ⅲ)/Co(Ⅱ)cycle and maintained Co in a low-valence state,thereby stimulating the generation of sulfate *** this study,the effective regulation of reactive oxygen species in the reaction system was *** results provided a guidance for in situ electron replenishment and regeneration of carbon-based transition metal catalysts,which will expand the practical application of advanced oxidation processes.

关键词： Electron transportation Catalyst regeneration Peroxymonosulfate Co Photocatalytic

A review of functions and mechanisms of clay soil conditioners and catalysts in thermal remediation compared to emerging photo-thermal catalysis

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Journal of Environmental Sciences 2025年第1期147卷 22-35页

作者： Juan zhang Shuo Wang Xin Wang Wentao jiao Minghua zhang Fujun Ma State Key Laboratory of Advanced Metallurgy School of Metallurgical and Ecological EngineeringUniversity of Science and Technology BeijingBeijing 100083China Research Center for Eco-Environmental Sciences Chinese Academy of SciencesBeijing 100085China College of Agricultural and Environmental Sciences University of CaliforniaDavisCA 95616USA State Key Laboratory of Environmental Criteria and Risk Assessment Chinese Research Academy of Environmental SciencesBeijing 100012China

High temperatures and providing sufficient time for the thermal desorption of persistent organic pollutants(POPs)from contaminated clay soils can lead to intensive energy ***,this article provides a critical review of the potential additives which can improve soil texture and increase the volatility of POPs,and then discusses their enhanced mechanisms for contributing to a green ***-based additives have been used to reduce plasticity of bentonite clay,absorb water and replenish system *** contrast,non-Ca-based additives have been used to decrease the plasticity of kaolin *** soil structure and soil plasticity can be changed through cation exchange and flocculation *** transitionmetal oxides and alkalimetal oxides can be applied to catalyze and oxidize polycyclic aromatic hydrocarbons,petroleum and emerging *** this system,reactive oxygen species(•O_(2)^(-)and•OH)are generated fromthermal excitation without strong chemical ***,multiple active ingredients in recycled solid wastes can be controlled to reduce soil plasticity and enhance thermal ***,the alkali,nano zero-valent iron and nano-TiN can catalyze hydrodechlorination of POPs under reductive ***,photo and photo-thermal catalysis are discussed to accelerate replacement of fossil fuels by renewable energy in thermal remediation.

关键词： Persistent organic contaminants Clay soils Thermal remediation Soil conditioning Synergistic catalysis

Advances in the Development of Gradient Scaffolds Made of Nano‑Micromaterials for Musculoskeletal Tissue Regeneration

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Nano-Micro Letters 2025年第3期17卷 455-500页

作者： Lei Fang Xiaoqi Lin Ruian Xu Lu Liu Yu zhang Feng Tian jiao jiao Li Jiajia Xue Beijing Laboratory of Biomedical Materials Beijing University of Chemical TechnologyBeijing 100029People’s Republic of China State Key Laboratory of Organic‑Inorganic Composites Beijing University of Chemical TechnologyBeijing 100029People’s Republic of China School of Biomedical Engineering Faculty of Engineering and ITUniversity of Technology SydneySydneyNSW 2007Australia

The intricate hierarchical structure of musculoskeletal tissues,including bone and interface tissues,necessitates the use of complex scaffold designs and material structures to serve as tissue-engineered *** has led to growing interest in the development of gradient bone scaffolds with hierarchical structures mimicking the extracellular matrix of native tissues to achieve improved therapeutic *** on the anatomical characteristics of bone and interfacial tissues,this review provides a summary of current strategies used to design and fabricate biomimetic gradient scaffolds for repairing musculoskeletal tissues,specifically focusing on methods used to construct compositional and structural gradients within the *** latest applications of gradient scaffolds for the regeneration of bone,osteochondral,and tendon-to-bone interfaces are ***,the current progress of testing gradient scaffolds in physiologically relevant animal models of skeletal repair is discussed,as well as the challenges and prospects of moving these scaffolds into clinical application for treating musculoskeletal injuries.

关键词： Gradient scaffolds Musculoskeletal tissues Advanced manufacturing Biomaterials Tissue regeneration

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跨流域调水之水权制度探析

生态经济 2007年第10期23卷 127-130页

作者：章群张义佼西南财经大学法学院成都610074 四川省社科院人力资源研究所成都610071

跨流域调水乃21世纪我国水利系统工程的一大特点。在现实层面,我国跨流域调水确乎存在水资源的掠夺性开发和浪费现象。按国务院《关于做好建设节约型社会近期重点工作的通知》的要求,我国节水型社会建设的首选路径应是"推进国家水权制... 详细信息

跨流域调水乃21世纪我国水利系统工程的一大特点。在现实层面,我国跨流域调水确乎存在水资源的掠夺性开发和浪费现象。按国务院《关于做好建设节约型社会近期重点工作的通知》的要求,我国节水型社会建设的首选路径应是"推进国家水权制度建设"。因此,欲实现符合国情的节水型社会的理想化建构,首要前提应是对我国跨流域调水的水权制度予以探讨。

关键词：跨流域调水水权制度节水型社会

Chronic oleoylethanolamide treatment attenuates diabetes-induced mice encephalopathyby activating peroxisome proliferator-activatedreceptor alpha in hippocampus

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中国药理学与毒理学杂志 2018年第9期32卷 680-681页

作者： REN Tong LIU Jin-feng ZHUO Ren-gong XU Lan-xi zhang yi-jiao zhang Hui-jun PENG Lu CHEN Cai-xia ZHOU Yu ZHAO Yun LI Wen-jun LI ying JIN Xin YANG Li-chao Medical College Xiamen University Xiamen 361102 China Xiamen Hospital of Traditional Chinese Medicine Xiamen 361102 China Xiamen Medical College Xiamen 361000 China

OBJECTIVE Oleoylethanolamide(OEA) is an endogenous peroxisome proliferatoractivated receptor alpha(PPARα) agonist that acts on the peripheral control of energy *** studies have shown that OEA exerts neuroprotection after cerebral ***,whether OEA affects the outcomes of diabetes-induced encephalopathy(DE) requires further *** The chronic effects of OEA on DE were evaluated in C57BL/6 and PPARαknockout mice,*** cognitive function was assessed with Morris water *** expression of receptor for advanced glycation end products(RAGE) and phosphorylation of Tau in mice hippocampus were determined using Western *** influence of OEA in neuron loss and neuroplasticity were assessed with immunofluorescent staining and Western *** OEA markedly ameliorated performance in the Morris water maze,which was correlated with its capabilities of suppressing glycometabolism and phosphorylation of Tau in the *** offered protection from diabetes-induced impairments in hippocampal ***,the changes in Morris water maze performance and neuron loss could not be observed in PPARα knockout mouse models with OEA *** The ability of OEA to control PPARα signaling can serve as a novel neuroprotective approach for the treatment of diabetes-induced encephalopathy.

关键词： oleoylethanolamide diabeticencephalopathy spatial cognitive function neuroprotection peroxisome proliferator-activated receptor alpha

High-energy-density lithium manganese iron phosphate for lithium-ion batteries:Progresses,challenges,and prospects

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Journal of Energy Chemistry 2025年第1期100卷 1-17页

作者： Bokun zhang Xiaoyun Wang Shuai Wang Yan Li Libo Chen Handong jiao Zhijing Yu Jiguo Tu State Key Laboratory of Advanced Metallurgy University of Science and Technology BeijingBeijing 100083China Research Institute for Intelligent Wearable Systems The Hong Kong Polytechnic University Hong Kong 9977China Institute of Advanced Structure Technology Beijing Institute of TechnologyBeijing 100081China

The soaring demand for smart portable electronics and electric vehicles is propelling the advancements in high-energy–density lithium-ion *** manganese iron phosphate(LiMn_(x)Fe_(1-x)PO_(4))has garnered significant attention as a promising positive electrode material for lithium-ion batteries due to its advantages of low cost,high safety,long cycle life,high voltage,good high-temperature performance,and high energy *** LiMn_(x)Fe_(1-x)PO_(4)has made significant breakthroughs in the past few decades,there are still facing great challenges in poor electronic conductivity and Li-ion diffusion,manganese dissolution affecting battery cycling performance,as well as low tap *** review systematically summarizes the reaction mechanisms,various synthesis methods,and electrochemical properties of LiMn_(x)Fe_(1-x)PO_(4)to analyze reaction processes accurately and guide material ***,the main challenges currently faced are concluded,and the corresponding various modification strategies are discussed to enhance the reaction kinetics and electrochemical performance of LiMn_(x)Fe_(1-x)PO_(4),including multi-scale particle regulation,heteroatom doping,surface coating,as well as microscopic morphology ***,in view of the current research challenges faced by intrinsic reaction processes,kinetics,and energy storage applications,the promising research directions are *** importantly,it is expected to provide key insights into the development of high-performance and stable LiMn_(x)Fe_(1-x)PO_(4)materials,to achieve practical energy storage requirements.

关键词： Lithiummanganese iron phosphate High energydensity Lithium-ionbatteries Reactionmechanism Tap density

SensFL:Privacy-Preserving Vertical Federated Learning with Sensitive Regularization

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Computer Modeling in Engineering & Sciences 2025年第1期142卷 385-404页

作者： Chongzhen zhang Zhichen Liu Xiangrui Xu Fuqiang Hu jiao Dai Baigen Cai Wei Wang School of Automation and Intelligence Beijing Jiaotong UniversityBeijing100044China Shuohuang Railway Development Co. Ltd.National Energy GroupCangzhou062350China Beijing Key Laboratory of Security and Privacy in Intelligent Transportation School of Computer Science and TechnologyBeijing Jiaotong UniversityBeijing100044China

In the realm of Intelligent Railway Transportation Systems,effective multi-party collaboration is crucial due to concerns over privacy and data *** Federated Learning(VFL)has emerged as a promising approach to facilitate such collaboration,allowing diverse entities to collectively enhance machine learning models without the need to share sensitive training ***,existing works have highlighted VFL’s susceptibility to privacy inference attacks,where an honest but curious server could potentially reconstruct a client’s raw data from embeddings uploaded by the *** vulnerability poses a significant threat to VFL-based intelligent railway transportation *** this paper,we introduce SensFL,a novel privacy-enhancing method to against privacy inference attacks in ***,SensFL integrates regularization of the sensitivity of embeddings to the original data into the model training process,effectively limiting the information contained in shared *** reducing the sensitivity of embeddings to the original data,SensFL can effectively resist reverse privacy attacks and prevent the reconstruction of the original data from the *** experiments were conducted on four distinct datasets and three different models to demonstrate the efficacy of *** results show that SensFL can effectively mitigate privacy inference attacks while maintaining the accuracy of the primary learning *** results underscore SensFL’s potential to advance privacy protection technologies within VFL-based intelligent railway systems,addressing critical security concerns in collaborative learning environments.

关键词： Vertical federated learning privacy defenses

Lipid droplets in the nervous system:involvement in cell metabolic homeostasis

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Neural Regeneration Research 2025年第3期20卷 740-750页

作者： Yuchen zhang yiqing Chen Cheng Zhuang Jingxuan Qi Robert Chunhua Zhao jiao Wang School of Life Sciences Shanghai UniversityShanghaiChina School of Medicine Shanghai UniversityShanghaiChina Institute of Basic Medical Sciences Chinese Academy of Medical Sciences School of Basic MedicinePeking Union Medical CollegeBeijingChina Center of Excellence in Tissue Engineering Chinese Academy of Medical SciencesBeijingChina Beijing Key Laboratory of New Drug Development and Clinical Trial of Stem Cell Therapy BeijingChina

Lipid droplets serve as primary storage organelles for neutral lipids in neurons,glial cells,and other cells in the nervous *** droplet formation begins with the synthesis of neutral lipids in the endoplasmic ***,lipid droplets were recognized for their role in maintaining lipid metabolism and energy homeostasis;however,recent research has shown that lipid droplets are highly adaptive organelles with diverse functions in the nervous *** addition to their role in regulating cell metabolism,lipid droplets play a protective role in various cellular stress ***,lipid droplets exhibit specific functions in neurons and glial *** of lipid droplet formation leads to cellular dysfunction,metabolic abnormalities,and nervous system *** review aims to provide an overview of the role of lipid droplets in the nervous system,covering topics such as biogenesis,cellular specificity,and ***,it will explore the association between lipid droplets and neurodegenerative *** the involvement of lipid droplets in cell metabolic homeostasis related to the nervous system is crucial to determine the underlying causes and in exploring potential therapeutic approaches for these diseases.

关键词： Alzheimer's disease lipid droplet biogenesis lipid droplets lipid metabolism nervous system neurodegenerative disorders oxidative stress Parkinson's disease

Phonon-mediated superconductivity in orthorhombic XS(X=Nb,Ta or W)

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Chinese Physics B 2025年第2期34卷 419-423页

作者： Guo-Hua Liu Kai-Yue Jiang yi Wan Shu-Xiang Qiao Jin-Han Tan Na jiao Ping zhang Hong-Yan Lu School of Physics and Physical Engineering Qufu Normal UniversityQufu 273165China Institute of Applied Physics and Computational Mathematics Beijing 100088China

The unique three-dimensional orthorhombic NbS(o-NbS)compound synthesized in 1969 has recently been experimentally confirmed to be a superconductor[***.B 108174517(2023)].However,there is currently no theoretical research on its superconducting *** this work,we investigate the superconducting properties of o-Nb S from first-principles *** on the Eliashberg equation,it is found that the superconductivity mainly originates from the coupling between the electrons of Nb-4d orbitals and the vibrations of Nb atoms in the low-frequency region and those of S atoms in the high-frequency region.A superconducting transition temperature(T_c)of 10.7 K is obtained,which is close to the experimental value and higher than most transition metal chalcogenides(TMCs).The calculated thermodynamic properties in the superconducting state,such as specific heat,energy gap,isotope coefficient,etc.,also indicate that o-NbS is a conventional phonon-mediated *** results are consistent with recent experimental reports and provide a good understanding of the superconducting mechanism of o-Nb ***,the TMCs of o-TaS and o-WS are also investigated;these belong to the same and neighboring groups of Nb,and we find that o-TaS and o-WS are also phonon-mediated superconductors with T_c of 8.9 K and 7.2 K,respectively.

关键词： first-principles calculations phonon-mediated superconductivity orthorhombic transition metal chalcogenides