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Design and Optimization of Communication System Based on Superconducting Three-Energy-Level System

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Journal of Communications and Information Networks 2023年第1期8卷 57-70页

作者： zhang junyu Gong Chen Li Shangbin Zhu Jinkang Key Laboratory of WirelessOptical Communications Chinese Academy of Sciencesthe School of Information Science and TechnologyUniversity of Science and Technology of ChinaHefei 230000China.

We propose aΛ-type superconducting three-energy-level device-based communication system for extremely weak microwave communication scenarios,for example,long-distance deep-space *** provide a system diagram and propose the frame synchronization and power estimation approaches based on pre-defined synchronization *** on the microwave response characteristics of the superconducting three-energy-level system,we further investigate the optimization of synchronization sequence and information symbol *** show that three-energy-level systems with weak Markovianity can be approximated using independent identical distribution methods to obtain optimal synchronization sequences,and the optimal modulation is *** proposed system design and optimization approaches are evaluated by numerical ***,we investigate the performance of the three-energy-level communication system in the presence of *** results show that the three-energy-level communication system can tolerate more than 10 dB interference compared to long term evolution(LTE)systems and achieve the same communication rate for the same bandwidth and temperature.

关键词： microwave photon detection Λ-type threeenergy-level system superconducting devices energy-level transition

Tracking the atomic pathways of Pt3Ni-Ni(OH)2 core-shell structures at the gas-liquid interface by in-situ liquid cell TEM

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Science China Chemistry 2020年第4期63卷 513-518页

作者： junyu zhang Gen Li Hong-Gang Liao Shi-Gang Sun State Key Lab of Physical Chemistry of Solid Surfaces Collaborative Innovation Center of Chemistry for Energy MaterialsCollege of Chemistry and Chemical EngineeringXiamen UniversityXiamen 361005China

Using the in-situ liquid cell transmission electron microscopy, the three-stage growth of Pt3Ni-Ni(OH)2 core-shell structures at the gas-liquid interfaces was clearly observed, which consists of(1) a thermodynamically driven Pt3Ni alloy core by the monomer attachment,(2) a nickel(Ni) shell formation due to the depletion of the Pt salt precursor, and(3) the oxidation and of the Ni shell into Ni(OH)2 flakes. We also further observed the nucleation and growth of the Ni(OH)2 flakes on an existing layer either at the middle part or at the step edge. More interestingly, the dynamic transformation among a Pt3Ni alloy, Ni clusters and Ni(OH)2 flakes was also imaged even at a high electron dose rate.

关键词： Pt3Ni-Ni(OH)2 core-shell structure liquid cell electron microscopy gas-liquid interface dynamic transformation

An average-value-at-risk criterion for Markov decision processes with unbounded costs

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Frontiers of Mathematics in China 2022年第4期17卷 673-687页

作者： Qiuli LIU Wai-Ki CHING junyu zhang Hongchu WANG School of Mathematical Sciences South China Normal UniversityGuangzhou510631China Advanced Modeling and Applied Computing Laboratory Department of MathematicsThe University of Hong KongHong KongChina School of Mathematics Sun Yat-Sen UniversityGuangzhou510275China

We study the Markov decision processes under the average-value-at-risk *** state space and the action space are Borel spaces,the costs are admitted to be unbounded from above,and the discount factors are state-action *** suitable conditions,we establish the existence of optimal deterministic stationary ***,we apply our main results to a cash-balance model.

关键词： Markov decision processes average-value-at-risk(AVaR) state-action dependent discount factors optimal policy

Active molecule-based theranostic agents for tumor vasculature normalization and antitumor efficacy

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Chinese Chemical Letters 2024年第8期35卷 229-234页

作者： Jin Wang Xiaoyan Pan junyu zhang Qingqing zhang Yanchen Li Weiwei Guo Jie zhang School of Pharmacy Health Science CenterXi’an Jiaotong UniversityXi’an 710061China Center of Advanced Pharmaceuticals and Biomaterials State Key Laboratory of Natural MedicineChina Pharmaceutical UniversityNanjing 210009China

Tumor vascular normalization has emerged as a promising strategy for synergistic therapy *** on the strategy of“fluorescence turn on-controllable release”,a novel bifunctional candidate was con-structed based on previous developed vascular normalization inducer QDAU5,which could self-assemble to form functional enzyme infrared QDAU5 nanoparticles(FEIRQ NPs).Subsequently,biological evaluation demonstrated that the FEIRQ NPs could induce ferroptosis,endoplasmic reticulum stress,and antigen pre-conditioning and maturation of dendritic cells and CD8^(+)T cells,leading to excellent antitumor efficacy in the absence of cytotoxic ***,FEIRQ NPs show high fluorescence intensity upon expo-sure to theβ-galactosidase(β-Gal)enzyme expressed in ovarian cancer,enabling real-time monitoring of therapeutic ***,our findings suggest a prospering strategy to early diagnosis and efficient therapy for ovarian cancer without cytotoxicity.

关键词： Tumor vasculature normalization Diagnosis and treatment Cytotoxicity Depleting glutathione Ferroptosis Immune activation

Deactivation of Cu-SAPO-34 by urea-related deposits at low temperatures and the regeneration

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Journal of Environmental Sciences 2019年第7期31卷 43-51页

作者： Yue Ma Xiaodong Wu junyu zhang Rui Ran Zhichun Si Duan Weng The Key Laboratory of Advanced Materials of Ministry of Education School of Materials Science and Engineering Tsinghua University School of Environment Tsinghua University Graduate School at Shenzhen Tsinghua University

Selective catalytic reduction(SCR) with urea catalyzed by Cu-SAPO-34 is an effective method to eliminate NO_x from diesel exhaust. However, urea-related deposits may form during cold-start and urban driving due to low exhaust temperatures. The activity of CuSAPO-34 at 175°C is significantly degraded by urea exposure, and 300°C is required for regeneration. Through in-situ diffuse reflectance infrared Fourier transform spectroscopy(DRIFTS) and temperature-programmed hydrolysis studies, the dominant stable deposit at 175°C is identified as biuret, which can be eliminated at 300°C. The urea-derived deactivation and regeneration mechanisms of Cu-SAPO-34 were compared with those of anatase-supported catalysts.

关键词： SCR Urea Biuret Cu-SAPO-34 Deactivation

Structural Origins for Enhanced Thermal Stability and Glass‑Forming Ability of Co–B Metallic Glasses with Y and Nb Addition

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Acta Metallurgica Sinica(English Letters) 2023年第6期36卷 962-972页

作者： Shuang Ma junyu zhang Xudong Wang Rie Y.Umetsu Li Jiang Wei zhang Man Yao Key Laboratory of Materials Modification by Laser Ionand Electron Beams(Ministry of Education)School of Materials Science and EngineeringDalian University of TechnologyDalian 116024China Institute for Materials Research Tohoku UniversitySendai 980‑8577Japan

The effects of Y and Nb addition on thermal stability,glass-forming ability(GFA),and magnetic softness of Co75B25 metallic glass(MG)were comprehensively *** experimental results indicated that the thermal stability,GF... 详细信息

关键词： Co-based metallic glasses Thermal stability Glass-forming ability Soft magnetic property Ab initio molecular dynamics simulations Local atomic structure

Ultrasmall AuPd nanoclusters on amine-functionalized carbon blacks as high-performance bi-functional catalysts for ethanol electrooxidation and formic acid dehydrogenation

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Journal of Energy Chemistry 2022年第5期31卷 556-563页

作者： Yuhuan Cui Ming Zhao Yining Zou junyu zhang Jiuhui Han Zhili Wang Qing Jiang Key Laboratory of Automobile Materials Ministry of EducationSchool of Materials Science and EngineeringJilin UniversityChangchun 130022JilinChina Frontier Research Institute for Interdisciplinary Sciences(FRIS) Tohoku UniversitySendai 980-8578Japan

The synthesis of ultrasmall metal nanoclusters(NCs) with high catalytic activities is of great importance for the development of clean and renewable energy technologies but remains a challenge. Here we report a facile wet-chemical method to prepare ~1.0 nm Au Pd NCs supported on amine-functionalized carbon blacks. The Au Pd NCs exhibit a specific activity of 5.98 mA cm_(AuPd)^(-2)and mass activity of 5.25 A mg_(auPd)^(-1) for ethanol electrooxidation, which are far better than those of commercial Pd/C catalysts(1.74 mAcm_(AuPd)^(-2) and 0.54 A mg_(Pd)^(-1) ). For formic acid dehydrogenation, the Au Pd NCs have an initial turn over frequency of 49339 h^(-1) at 298 K without any additive, which is much higher than those obtained for most of reported Au Pd catalysts. The reported synthesis may represent a facile and low-cost approach to prepare other ultrasmall metal NCs with high catalytic activities for various applications.

关键词： Ethanol electrooxidation Formic acid dehydrogenation AuPd Nanoclusters Bi-functional catalyst

Synergistic Combination of Biodegradable Peptide Polymer and Curcumin as Promising Antibiotic Substitution in Aquaculture to Alleviate the Global Challenge of Antimicrobial Resistance

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Chinese Journal of Chemistry 2022年第24期40卷 2947-2955页

作者： Pengcheng Ma Yuan Chen Ning Shao junyu zhang Yueming Wu Runhui Liu State Key Laboratory of Bioreactor Engineering East China University of Science and TechnologyShanghai200237 China Key Laboratory for Ultrafine Materials of Ministry of Education Frontiers Science Center for Materiobiology and Dynamic ChemistryShanghai Frontiers Science Center of Optogenetic Techniques for Cell MetabolismResearch Center for Biomedical Materials of Ministry of EducationSchool of Materials Science and EngineeringEast China University of Science and TechnologyShanghai200237 China

The massive use of antibiotics in aquaculture and resulted antibacterial resistance problem urgently need antibiotic substitutions. Herein, we report a promising substitution of aquaculture antibiotics using a synergistic combination of biodegradable peptide polymers and curcumin, a natural compound from plant. The synergistic combination shows strong antibacterial activity against V. fluvialis and some other common bacteria in aquaculture. The membrane-damaging antibacterial mechanism echoes our finding that the synergistic combination will not induce bacteria to develop resistance after continuous use. The synergistic combination also displays effective cure on V. fluvialis-infected zebrafish. The biodegradability of the peptide polymer enables the combination to lose antibacterial activity and will not cause selective pressure on bacterial in the environment. Our study indicates potential application of synergistic composition, biodegradable peptide polymer and curcumin, as promising antibiotic substitution in aquaculture, which represents a promising strategy to address the global challenge of antimicrobial resistance.

关键词： Antimicrobial polymer Aquaculture Peptides Antibiotics Biological activity

Advances in intelligent mass spectrometry data processing technology for in vivo analysis of natural medicines

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Chinese Journal of Natural Medicines 2024年第10期22卷 900-913页

作者： CHEN Simian DAI Binxin zhang Dandan YANG Yuexin zhang Hairong zhang junyu LU Di WU Caisheng Fujian Provincial Key Laboratory of Innovative Drug Target Research and State Key Laboratory of Cellular Stress Biology School of Pharmaceutical SciencesXiamen UniversityXiamen 361102China Xiamen Key Laboratory for Clinical Efficacy and Evidence-Based Research of Traditional Chinese Medicine Xiamen UniversityXiamen 361102China

Natural medicines(NMs)are crucial for treating human *** characterizing their bioactive components in vivo has been a key focus and challenge in NM ***-performance liquid chromatography-high-resolution mass spectrometry(HPLC-HRMS)systems offer high sensitivity,resolution,and precision for conducting in vivo analysis of ***,due to the complexity of NMs,conventional data acquisition,mining,and processing techniques often fail to meet the practical needs of in vivo NM *** the past two decades,intelligent spectral data-processing techniques based on various principles and algorithms have been developed and applied for in vivo NM ***,improvements have been achieved in the overall analytical performance by relying on these techniques without the need to change the instrument *** improvements include enhanced instrument analysis sensitivity,expanded compound analysis coverage,intelligent identification,and characterization of nontargeted in vivo compounds,providing powerful technical means for studying the in vivo metabolism of NMs and screening for pharmacologically active *** review summarizes the research progress on in vivo analysis strategies for NMs using intelligent MS data processing techniques reported over the past two *** discusses differences in compound structures,variations among biological samples,and the application of artificial intelligence(AI)neural network ***,the review offers insights into the potential of in vivo tracking of NMs,including the screening of bioactive components and the identification of pharmacokinetic *** aim is to provide a reference for the integration and development of new technologies and strategies for future in vivo analysis of NMs.

关键词： High-performance liquid chromatography–High-resolution mass spectrometry Data-acquisition Data-processing Artificial Intelligence Metabolomics