检索结果-南通市图书馆

Chinese Chemical Letters 2024年第3期35卷 149-152页

作者： Yujie zhang Siyi Liu Dongdong Chen xing Xu School of Environmental Science and Engineering Shandong UniversityQingdao 266237China

Fabrication of single atom catalysts(SACs)by a green and gentle method is important for their practical Fenton-like *** this work,a high effective iron-based catalyst was prepared from the iron-rich Enteromorpha for NPX degradation via peroxymonosulfate(PMS).Both Fe-SACs and iron-clusters was fabricated from the intrinsic iron element in Enteromorpha after the urea *** Fe-SACs/clusters can achieve 100%of NPX oxidation within 20 min with the k_(obs)of 0.282 min^(-1).Quenching tests indicated that the radical pathways were not dominated in the catalytic systems,and strong electron transfer process can be induced in the Fe-SACs/clusters+PMS system by using the NPX as electron donor and FeSACs/clusters/PMS^*complexes as electron *** result was consistent with the phenomenon observed in the galvanic oxidation *** addition,the Fe-SACs/clusters was deposited onto the ceramic membrane(CM)by the spraying-crosslinking process to form a Fe-SACs/clusters@CM,which showed an effective and continuous NPX degradation in a heterogeneous PMS system.

关键词： SACs Iron Clusters Fenton-like reaction Enteromorpha

Intrinsic lithiophilic carbon host derived from bacterial cellulose nanofiber for dendrite-free and long-life lithium metal anode

在线全文

学校读者我要写书评

暂无评论

Nano Research 2024年第5期17卷 4203-4210页

作者： Gangyi Xiong Jiayu Yu Yalan xing Puheng Yang Shichao zhang School of Materials Science and Engineering Beihang UniversityBeijing 100191China School of Physics Science and Nuclear Energy Engineering Beihang UniversityBeijing 100191China

Although lithium metal is considered a promising anode for advanced Li-S and Li-air batteries,the uncontrolled dendrite growth and infinite volume change impede its practical ***,we report an ideal framework composed of carbonized bacterial cellulose(CBC)nanofibers,which shows intrinsic lithiophilicity to molten lithium without any lithiophilic surface *** wetting behavior of molten lithium can be significantly improved because its surface functional groups provide thermodynamical driving force,and the high surface roughness derived from nanocracks leads to rapid infusion in *** hybrid anode exhibits long cycle life up to 2000 h and excellent deep stripping-platting capacity up to 20 mAh·cm^(-2).When the anode is assembled with LiFePO_(4) cathode,the full cell delivers a good cycling stability up to 700 *** is attributed to the intrinsic lithiophilic scaffold,which can not only lower the nucleation barrier of Li and provide uniform nucleation sites for stable Li stripping/plating,but also offer interspace to accommodate volume fluctuation of lithium during long *** work provides a new manner to achieve a series of intrinsic lithiophilic carbon skeletons based on the large family of biomass materials and organic materials.

关键词： intrinsic lithiophilicity lithium metal anode bacterial cellulose lithium dendrite long cycling life

First-Arrival Picking Method for Active Source Data with Ocean Bottom Seismometers Based on Spatial Waveform Variation Characteristics

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Journal of Ocean University of China 2024年第4期23卷 970-980页

作者： LIU Hongwei xing Lei ZHU Henghua zhang Jin zhang Jing LIU Huaishan Key Laboratory of Submarine Geosciences and Prospecting Techniques Ministry of EducationCollege of Marine GeosciencesOcean University of ChinaQingdao 266100China Laboratory for Marine Mineral Resources Qingdao Marine Science and Technology CenterQingdao 266071China College of Underwater Acoustic Engineering Harbin Engineering UniversityHarbin 150001China Shandong Institute of Geological Survey Jinan 250014China

The precision and reliability of first-arrival picking are crucial for determining the accuracy of geological structure inversion using active source ocean bottom seismometer(OBS)refraction *** methods for first-arrival picking based on sample points are characterized by theoretical errors,especially in low-sampling-frequency OBS data because the travel time of seismic waves is not an integer multiple of the sampling *** this paper,a first-arrival picking method that utilizes the spatial waveform variation characteristics of active source OBS data is ***,the distribution law of theoretical error is examined;adjacent traces exhibit variation characteristics in their ***,a label cross-correlation superposition method for extracting highfrequency signals is presented to enhance the first-arrival picking *** from synthetic and field data verify that the proposed approach is robust,successfully overcomes the limitations of low sampling frequency,and achieves precise outcomes that are comparable with those of high-sampling-frequency data.

关键词： first-arrival picking spatial waveform variation label cross-correlation superposition method

Heat dissipation of carbon shell in ZrC-SiC/TaC coating to improve protective ability against ultrahigh temperature ablation

在线全文

学校读者我要写书评

暂无评论

Journal of Advanced Ceramics 2024年第7期13卷 1080-1091页

作者： Yuyu zhang Xuemeng zhang Hongkang Ou Bozhe Wang Jia Sun Qiangang fu Science and Technology on Thermostructural Composite Materials Laboratory Shaanxi Key Laboratory of Fiber Reinforced Light-Weight CompositesNorthwestern Polytechnical UniversityXi’an 710072China System Design Institute of Hubei Aerospace Technology Academy Wuhan 430040China

To efficiently decrease ablation heat accumulation and improve the ability of ZrC-SiC/TaC coatings to protect carbon/carbon(C/C)composites,a thermally conductive nanonetwork with a ceramic@carbon core-shell structure was designed and ***-derived SiC/TaC with a graphene carbon shell was synthesized and introduced into a ZrC coating by supersonic atmospheric plasma spraying(SAPS).Graphene shell paths increased the heat transfer capability by lowering the surface temperature to approximately 200℃during oxyacetylene *** heat dissipation of the graphene shell in the ZrC-SiC/TaC@C coating reduced the volatilization of low-melting-point phases and delayed the sintering of ZrO_(2) ***,the graphene shell in ZrC-SiC/TaC@C coating decreased the mass and linear ablation rates by 91.4%and 93.7%compared to ZrC-SiC/TaC coating,*** work provided a constructive idea for improving the ablation resistance of the coatings by incorporating carbon nanomaterials as a function of heat dissipation.

关键词： carbon/carbon(C/C)composites carbon nanomaterials core-shell structure polymer-derived ceramic(PDC) ablation resistance

New speckle pattern interferometry for precise in situ deformation measurements

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Chinese Optics Letters 2024年第1期22卷 34-40页

作者：章如月 Yu fu 缪泓 CAS Key Laboratory of Mechanical Behavior and Design of Materials Department of Modern MechanicsUniversity of Science and Technology of ChinaHefei 230027China Shenzhen Key Laboratory of Intelligent Optical Measurement and Detection College of Physics and Optoelectronic EngineeringShenzhen UniversityShenzhen 518060China

A new electronic speckle pattern interferometry method is proposed to realize in situ deformation *** feature of the method is the combination of a high-speed camera and multiple laser Doppler vibrometers(LDVs)for synchronous *** high-speed camera is used to record and select effective interferograms,while the LDVs are used to measure the rigid body displacement caused by vibrations.A series of effective interferograms with known shifted phase values are obtained to calculate the deformation *** experimental results show that the method performs well in measuring static and dynamic deformations with high accuracy in vibrating environments.

关键词： speckle pattern interferometry laser Doppler vibrometers in situ deformation measurements

Exploring Trade-offs in Thermal Interface Materials:The Impact of Polymer-Filler Interfaces on Thermal Conductivity and Thixotropy

在线全文

学校读者我要写书评

暂无评论

Chinese Journal of Polymer Science 2024年第7期42卷 916-925,I0006页

作者： Bin zhang Zheng-Li Dou Yong-Zheng zhang Qiang fu Kai Wu College of Polymer Science and Engineering State Key Laboratory of Polymer Materials EngineeringSichuan UniversityChengdu610065China

Effective thermal transport across solid-solid interfaces which is essential in thermal interface materials(TIMs),necessitates both optimal thixotropy and high thermal *** role of filler surface modification,a fundamental aspect of TIM fabrication,in the influence of these properties is not fully *** study employs the use of a silane coupling agent(SCA)to modify alumina,integrating experimental approaches with molecular dynamics simulations,to elucidate the interface effects on thixotropy and thermal conductivity in polydimethylsiloxane(PDMS)-based *** findings reveal that the variations of SCAs modify both interface binding energy and transition layer *** interface binding energy restricts macromolecular segmental relaxation near the interface,hindering desirable thixotropy and bond line *** the contrary,the thickness of the transition layer at the interface positively influences thermal conductivity,facilitating the transport of phonons between the polymer and ***,selecting an optimal SCA allows a balance between traditionally conflicting goals of high thermal conductivity and minimal bond line thickness,achieving an impressively low interface thermal resistance of just 2.45-4.29 K·mm^(2)·W^(-1)at275.8 kPa.

关键词： Thermal interface material Surface modification Thermal conductivity Thixotropy Interface thermal resistance

Effect of low-speed waterjet pressure on the rock-breaking performance of unsubmerged cavitating abrasive waterjet

在线全文

学校读者我要写书评

暂无评论

Petroleum Science 2024年第4期21卷 2638-2649页

作者： Chen-xing Fan Deng Li Yong Kang Hai-Tao zhang Hubei Key Laboratory of Waterjet Theory and New Technology Wuhan University School of Power and Mechanical Engineering Wuhan University

Unsubmerged cavitating abrasive waterjet(UCAWJ) has been shown to artificially create a submerged environment that produces shear cavitation, which effectively enhances rock-breaking performance. The shear cavitation generation and collapse intensity depend on the pressure difference between the intermediate high-speed abrasive waterjet and the coaxial low-speed waterjet. However, the effect of the pressure of the coaxial low-speed waterjet is pending. For this purpose, the effect of low-speed waterjet pressure on rock-breaking performance at different standoff distances was experimentally investigated,and the effects of erosion time and ruby nozzle diameter on erosion performance were discussed. Finally,the micromorphology of the sandstone was observed at different locations. The results show that increased erosion time and ruby nozzle diameter can significantly improve the rock-breaking performance. At different standoff distances, the mass loss increases first and then decreases with the increase of low-speed waterjet pressure, the maximum mass loss is 10.4 g at a low-speed waterjet pressure of0.09 MPa. The surface morphology of cavitation erosion was measured using a 3D profiler, the increase in both erosion depth and surface roughness indicated a significant increase in the intensity of the shear cavitation collapse. At a low-speed waterjet pressure of 0.18 MPa, the cavitation erosion surface depth can reach 600 μm with a roughness of 127 μm.

关键词： Rock-breaking Coaxial low-speed waterjet pressure Abrasive waterjet Cavitation Unsubmerged environment

The Effect of Blending Ratio on the Structure and Properties of the PPR/PS In situ Fiber Reinforced System Prepared by Multi-Flow Vibration Injection Molding

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

Chinese Journal of Polymer Science 2024年第6期42卷 851-863页

作者： Yan-Jiang Li Meng-Long Hu Jun-Wen zhang Qiang fu Jie zhang College of Polymer Science and Engineering State Key Laboratory of Polymer Materials EngineeringSichuan UniversityChengdu610065China

To enhance the mechanical properties of polypropylene random copolymer(PPR),polystyrene(PS)with four different contents were added to the PPR matrix through melt ***,using the Multi-Flow Vibration Injection Molding(MFVIM)technology,PPR/PS in situ microfiber composites(MFC)with different blending ratios were *** results indicated that blending ratio had a great impact on the phase morphology and crystal structure of MFVIM samples,which was different from those of conventional injection molding(CIM)*** ultrafine fibers could be formed under the shear field and could absorb the PPR molecular chains to form hybrid shish-kebab ***,the PPR matrix could also form shish-kebab structures under the effect of strong *** the PS content reached 20%,under the combined action of PS in situ microfibers and highly oriented crystal structure,the tensile strength and Young’s modulus of the sample were obviously improved and the impact strength remained at a relatively high *** a strong and tough balanced PPR based material was *** results provide valuable insights for expanding the industrial and daily-life applications of PPR and show promising development prospects.

关键词： PPR MFVIM In situ microfibers Shearfield Hybrid shish-kebab structures

Cage-confinement synthesis of MoC nanoclusers as efficient sulfiphilic and lithiophilic regulator for superior Li–S batteries

在线全文

学校读者我要写书评

暂无评论

Rare Metals 2024年第2期43卷 624-634页

作者： xing-Yuan zhang Mei-Na Lei Shan Tian Jian-Gan Wang State Key Laboratory of Solidification Processing Center for Nano Energy MaterialsSchool of Materials Science and EngineeringNorthwestern Polytechnical University and Shaanxi Joint Laboratory of Graphene(NPU)Xi’an710072China

High-energy-density Li-S batteries are subjected to serious sulfur deactivation and short cycle lifetime caused by undesirable polysulfide shuttle effect and frantic lithium dendrite *** this work,a controllable cage-confinement strategy to fabricate molybdenum carbide(MoC)nanoclusters as a high-efficient sulfiphilic and lithiophilic regulator to mitigate the formidable issues of Li-S batteries is *** sub-2 nm MoC nanoclusters not only guarantee robust chemisorption and fast electrocatalytic conversion of polysulfides to enhance the sulfur electrochemistry,but also homogenize Li^(+) flux to suppress the lithium dendrite *** a consequence,the MoC-modified separator endows the batteries with boosted reaction kinetics,promoted sulfur utilization,and improved cycling stability.A reversible capacity of 701 mAh·g^(−1) at a high rate of 5.0C and a small decay rate of 0.076%per cycle at 1.0C over 600 cycles are *** study offers a rational route for design and synthesis of bifunctional nanoclusers with both sulfiphilicity and lithiophilicity for high-performance Li-S batteries.

关键词： Li-S batteries Nanocluster Electrocatalyst Polysulfide shuttle Li dendrites

Controllable nucleation and deformation of skyrmions on surface of magnetic nanotubular monolayer

在线全文

学校读者我要写书评

暂无评论

Rare Metals 2024年第7期43卷 3250-3259页

作者： Xin-Xin zhang Chen-Yu zhang Yi-Xin xing Chao Man Jiao Liu Yong Hu Department of Physics College of SciencesNortheastern UniversityShenyang 110819China School of Materials and Mineral Resources Engineering Universiti Sains MalaysiaEngineering Campus14300 Nibong TebalPenangMalaysia State Key Laboratory of Rolling and Automation Northeastern UniversityShenyang110819China

Magnetic skyrmions emerge when the energy of ferromagnetic exchange interaction promoting parallel alignment of spins enters in competition with energies favoring non-collinear alignment of spins such as Dzy aloshinskii-Moriya interaction(DMI),long-rang dipole-dipole interaction(DDI),or higher-order exchange *** perform an unbiased Monte Carlo simulation to study the DMI-based skyrmion nucleation and stabilization on the surface of magnetic nanotubular monolayer controlled by tuning constants of DDI(g) and next-nearest-neighbor antiferromagnetic exchange interaction(j') with appropriate *** g and j',the loosely distributed skyrmions initially nucleate on the surface of nanotube approaching to the magnetic field(h) direction with increasing h in the intermediate ***,the skyrmion size,shape,density,distribution and crystal structure,as well as its driven field range,are tailored by g and j'.This work demonstrates the skyrmion nucleation mechanisms in three-dimensional magnetic nanostructures with curvature effect and multiple interactions,serving as a benchmark for a guide to experimentalists for preparation of samples in magnetic skyrmion states.

关键词： Magnetic nanotube Magnetic skyrmion Dzyaloshinskii-Moriya interaction Dipole-dipole interaction Monte Carlo simulation