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Chinese Journal of Chemical Engineering 2024年第7期71卷 91-101页

作者： Yuting zhang Yuwei Tang Ruiping yan Shuang liang Zhongmou Liu Yadong yang Key Laboratory of Songliao Aquatic Environment Ministry of EducationJilin Jianzhu UniversityChangchun 130118China School of Environmental Science and Engineering Yancheng Institute of TechnologyYancheng 224051China

A biochar-supported green nZVI(G-nZVI@MKB)composite was synthesized using mango kernel waste with“dual identity”as reductant and biomass of *** G-nZVI@MKB with a Fe/C mass ratio of 2.0(G-nZVI@MKB2)was determined as the most favorable composite for hexavalent chromium(Cr(VI))*** influencing parameters were discussed,and 99.0%of Cr(VI)removal occurred within 360 min under these optimized ***-second order kinetic model and intra-particle diffusion model well depicted Cr(VI)removal *** XRD,FTIR,SEM,and XPS analyses verified the key roles of G-nZVI and functional groups,as well as the primary removal mechanisms involving electrostatic attraction,reduction,and complexation.G-nZVI@MKB2 exhibited good stability and reusability with only a 16.4%decline in Cr(VI)removal after five *** study offered evidence that mango kernel could be recycled as a beneficial resource to synthesize green nZVI-loaded biochar composite for efficient Cr(VI)elimination from water.

关键词： Synthesis Biochar-supported nZVI Hexavalent chromium Reduction Regeneration

Experimental Study on Impingement Processes of Fuel Sprays on Biomimetic Structured Surfaces

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Journal of Bionic Engineering 2024年第1期21卷 362-373页

作者： yanling Chen liang Guo Wanchen Sun Yuying yan Rong Xuan Junfeng zhang State Key Laboratory of Automotive Simulation and Control Jilin UniversityChangchun 130025China Faculty of Engineering University of NottinghamNottingham NG72RDUK

To improve the controllability of the wall-wetting process after the fuel spray-wall impingement in internal combustion engines,the methods of laser etching,chemical etching and surface free energy modification are used to prepare biomimetic structured surfaces with different *** impingement processes of diesel and n-butanol sprays on the walls under different conditions are experimentally *** the surface oleophilicity increases,the spreading radius of wall-impinging sprays *** about 5 s after the fuel injections,the fuel spray droplets hit the walls for the first time,and the secondary breakup and rebound *** mixture concentrations of different fuels hitting the various walls reach the peak *** a higher surface temperature,the peak value of the mixture concentration is mainly related to the heat flux to the fuel droplets in different boiling regimes from the metal *** concentration of the air–fuel mixture in the near wall region increases with increasing surface oleophilicity,increasing wall temperature and decreasing ambient *** with diesel,n-butanol presents a higher air–fuel mixture concentration in the near wall region.

关键词： Spray-wall impingement Morphological development Air-fuel mixture concentration Surface wettability Wall temperature:Ambient pressure

Behaviors analysis of on-coming cluster based on knowledge under cluster security requirements

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Chinese Journal of Aeronautics 2024年第9期37卷 448-462页

作者： Huixia zhang yan liang Ying SHI Yuedong WANG Chaoxiong MA Ran WANG School of Automation Northwestern Polytechnical UniversityXi'an 710129China Key Laboratory of Information Fusion Technology Ministry of EducationXi'an 710129China

Analysis of cluster behaviors of the on-coming cluster is an essential measure for high value locations on the *** target tracking and clustering analysis,cluster behaviors analysis under cluster security requirements remains an open issue,which is a joint analysis of clus-tering,intent reasoning and activity *** address this issue,a framework for cluster behav-iors analysis is proposed by incorporating expert knowledge and domain knowledge,and a knowledge-assisted score function with is designed to improve the accuracy of intent reasoning net-work,overcoming the effects of possible knowledge *** framework consists of three mod-ules for cluster analysis,intent reasoning and activity region analysis for typical tasks,in which an intent reasoning network is constructed to obtain cluster intents by using a hybrid knowledge and data driven ***,considering the complexity of the battlefield environment,dif-ferent tasks and corresponding activity region optimization functions are designed for cluster activ-ity region analysis,which are vital elements of cluster behaviors *** demonstrate the effectiveness of the proposed cluster behaviors analysis framework.

关键词： Cluster analysis Intent reasoning,Activity region analysis Cluster behavior Battlefield environment

基于改进附着能量模型的TNBA晶体在二元溶剂中的形貌预测

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原子与分子物理学报 2025年第5期42卷 143-148页

作者：都吉航王保国陈亚芳李鑫懿赵文虎张彦亮中北大学环境与安全工程学院山西北方晋东化工有限公司

TNBA作为一种新型含能材料，其具有高爆速，低敏感性的特点，为了研究TNBA在二元溶剂中的生长形貌，本研究采用附着能（AE）模型来预测TNBA在真空中的晶体形貌，同时采用改进附着能（MAE）模型和分子动力学（MD）方法，预测了TNBA晶体... 详细信息

TNBA作为一种新型含能材料，其具有高爆速，低敏感性的特点，为了研究TNBA在二元溶剂中的生长形貌，本研究采用附着能（AE）模型来预测TNBA在真空中的晶体形貌，同时采用改进附着能（MAE）模型和分子动力学（MD）方法，预测了TNBA晶体在四种不同二元溶剂中二甲基甲醇（IPA）/丙酮（AC）、IPA/二甲基亚砜（DMSO）、IPA/乙酸乙酯（EA）和IPA/水（H2O）的晶体形貌.结果表明，TNBA晶体在真空中的形态为不规则的多面体，由六个重要的主生长晶面构成，分别为（1 0 0）、（1 1 0）、（0 1 1）、（1 1-1）、（1 0-2）和（0 0 2），其中（1 0 0）面所占比例最大，达到33.766%.在IPA/DMSO和PA/EA溶剂中重结晶得到的晶体为块状，在IPA/AC和IPA/H2O为棒状.总而言之，IPA/DMSO和IPA/EA溶剂更适合TNBA晶体重结晶选择.

关键词： TNBA晶体改进附着能量模型二元溶剂形貌预测分子动力学模拟

Enhancing CO2 cycloaddition through ligand functionalization:A case study of UiO-66 metal-organic frameworks

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Double Fano resonances in disk-nonconcentric ring plasmonic nanostructures

结构化学 2024年第2期43卷 9-12页

作者： Ruowen liang Chao zhang Guiyang yan Fujian Province Key Laboratory of Featured Biochemical and Chemical Materials Ningde Normal UniversityNingde352100PR China State Key Laboratory of Photocatalysis on Energy and Environment Fuzhou University Fuzhou350002PR China State Key Laboratory of Photocatalysis on Energy and Environment Fuzhou University Fuzhou350002PR China

The synthesis of cyclic carbonates from CO2 and epoxides offers a remarkable 100％atomic *** literature describes the CO2 cycloaddition mechanism predominantly as an"epoxide activation"pathway[1].This process can be effectively facilitated by heterogeneous catalysts possessing Lewis acidity,potentially optimising the capture and activation of the epoxide via metal-oxygen ***-organic frameworks(MOFs)have recently garnered attention as new catalysts,credited to their structural adaptability and multifunctional ***,MOFs with exposed metal sites function as Lewis acid sites,thus enhancing the cycloaddition *** numerous researchers emphasize the pivotal role of epoxide activation in the CO2 cycloaddition process,the challenge of activating inherently stable CO2 molecules often remains *** CO2 activation can potentially reduce the energy barriers of the reaction,thereby enhancing the overall *** prior studies on MOFs'catalytic activities for CO2 cycloaddition primarily emphasise their Lewis acidity sites[2,3],with scant attention to the syn-ergistic effects between the Lewis acid and base sites.

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Optoelectronics Letters 2024年第1期20卷 1-6页

作者： zhang Xingfang LIU Fengshou liang Lanju yan Xin School of Opt-Electronic Engineering Zaozhuang UniversityZaozhuang 277160China Laboratory of Optoelectronic Information Processing and Display of Shandong Zaozhuang 277160China

The plasmonic properties of gold nanostructures composed of a disk outside a nonconcentric ring are numerically studied by the finite difference time domain(FDTD)*** results show that two Fano resonances are formed as a result of the coupling of the octupolar and quadrupolar modes of the ring with the dipolar mode of the *** reduction in structural symmetry causes a red shift of the Fano resonances and distinct changes in spectral lineshape by offsetting the center of the inner surface of the ring to different *** effects of several geometric parameters on the characteristics of Fano resonances are also *** addition,the refractive index(RI)sensitivities for the two Fano resonances can be up to 581 nm/RIU and 780 nm/RIU with the corresponding figure of merits(FOMs)as large as 12.7 and 10.2,*** properties render the structures useful for potential applications in multi-wavelength sensors.

关键词： method resonance render

Missing Value Imputation for Radar-Derived Time-Series Tracks of Aerial Targets Based on Improved Self-Attention-Based Network

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Computers, Materials & Continua 2024年第3期78卷 3349-3376页

作者： Zihao Song yan Zhou Wei Cheng Futai liang Chenhao zhang Department of Early Warning Intelligence Early Warning AcademyWuhan430019China

The frequent missing values in radar-derived time-series tracks of aerial targets(RTT-AT)lead to significant challenges in subsequent data-driven ***,the majority of imputation research focuses on random missing(RM)that differs significantly from common missing patterns of *** method for solving the RM may experience performance degradation or failure when applied to RTT-AT *** autoregressive deep learning methods are prone to error accumulation and long-term dependency *** this paper,a non-autoregressive imputation model that addresses the issue of missing value imputation for two common missing patterns in RTT-AT is *** model consists of two probabilistic sparse diagonal masking self-attention(PSDMSA)units and a weight fusion *** learns missing values by combining the representations outputted by the two units,aiming to minimize the difference between the missing values and their actual *** PSDMSA units effectively capture temporal dependencies and attribute correlations between time steps,improving imputation *** weight fusion unit automatically updates the weights of the output representations from the two units to obtain a more accurate final *** experimental results indicate that,despite varying missing rates in the two missing patterns,our model consistently outperforms other methods in imputation performance and exhibits a low frequency of deviations in estimates for specific missing *** to the state-of-the-art autoregressive deep learning imputation model Bidirectional Recurrent Imputation for Time Series(BRITS),our proposed model reduces mean absolute error(MAE)by 31%~50%.Additionally,the model attains a training speed that is 4 to 8 times faster when compared to both BRITS and a standard Transformer model when trained on the same ***,the findings from the ablation experiments demonstrate that the PSDMSA,the weight fusion unit,cascade network design

关键词： Missing value imputation time-series tracks probabilistic sparsity diagonal masking self-attention weight fusion

New Insights into Microplastic Contamination in Different Types of Leachates: Abundances, Characteristics, and Potential Sources

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Engineering 2024年第6期37卷 62-68页

作者： Lei zhang Wentao Zhao liang zhang Zhenxiao Cai Ruiqi yan Xia Yu Damià Barceló Qian Sui State Environmental Protection Key Laboratory of Environmental Risk Assessment and Control on Chemical Process School of Resources and Environmental EngineeringEast China University of Science and TechnologyShanghai 200237China State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and EngineeringTongji UniversityShanghai 200092China Shanghai Institute of Pollution Control and Ecological Security Shanghai 200092China PerkinElmer Inc.Shanghai 201203China Maihai Environmental Protection Technology Co. Ltd.SuzhouJiangsu 215000China Department of Environmental Chemistry Institute of Environmental Assessment and Water ResearchSpanish Council for Scientific Research(IDAEA-CSIC)Barcelona 08034Spain

Municipal solid waste(MSW)is an important destination for abandoned *** the waste disposal process,large plastic debris is broken down into microplastics(MPs)and released into the ***,current research only focuses on landfill leachates,and the occurrence of MPs in other leachates has not been ***,herein,the abundance and characteristics of MPs in three types of leachates,namely,landfill leachate,residual waste leachate,and household food waste leachate,were studied,all leachates were collected from the largest waste disposal center in *** results showed that the average MP abundances in the different types of leachates ranged from(129±54)to(1288±184)MP particles per liter(particlesL1)and the household food waste leachate exhibited the highest MP abundance(p80%)of small MPs(20–100 lm)in landfill leachates compared to other *** the best of our knowledge,this is the first study discussing the sources of MPs in different leachates,which is important for MP pollution control during MSW disposal.

关键词： Microplastics Landfill leachate Residual waste leachate Household food waste leachate Source

Research on Bast Fiber Extracted from the White Bark of Three Species in the Genus Broussonetia

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Chinese Journal of Polymer Science 2024年第6期42卷 729-738页

作者： Shan-Shan Jin Si-Nong Wang yan-yan Huang Jing-Yu zhang Peng Liu Hui Yu Hong-Dong zhang Yu-liang yang Institute for Preservation and Conservation of Chinese Ancient Books Fudan University LibraryFudan UniversityShanghai200433China State key laboratory of Molecular Engineering of polymers Department of Macromolecular ScienceFudan UniversityShanghai200433China

Against the backdrop of a global paper resource shortage,there is a growing need to identify fast-growing tree species capable of producing long-lasting *** plant species namely Broussonetia kazinoki,Broussonetia papyrifera and hybrid paper mulberry,belong to the Broussonetia genus,were collected from China to study their white bark suitability for pulp and *** chemical composition revealed that the holocellulose content in Broussonetia kazinoki and Broussonetia papyrifera was more than 80%.The molecular weight distribution of several holocellulose/α-cellulose is observed by GPC,which allows us to better observe the changes of various components on the molecular *** yield,lignin,whiteness,and molecular weight of the pulps obtained by NaOH treatment were *** microscope was used to characterize the fiber length-width ratio and ***,the improvement of the fiber rigidity method based on the Kratky-Porod chain model makes it more theoretical and further reveals the influencing factors of fiber *** study demonstrates the high potentiality of these three species for papermaking applications.

关键词： Broussonetia genus Cellulose Alkaline pulping Kratky-Porod chain model Fiber rigidity

Boron nitride nanofibers enhanced composite PEO-based solid-state polymer electrolytes for lithium metal batteries

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Chinese Chemical Letters 2024年第6期35卷 216-221页

作者： Qianqian Song Yunting zhang Jianli liang Si Liu Jian Zhu Xingbin yan School of Materials Science and Engineering Sun Yat-Sen UniversityGuangzhou 510275China College of Physics and Materials Science Tianjin Normal UniversityTianjin 300387China Department of Chemistry&Center of Super-Diamond and Advanced Films(COSDAF) City University of Hong KongHong Kong 999077China Guangdong-Hong Kong-Macao Joint Laboratory for Intelligent Micro-Nano Optoelectronic Technology School of Physics and Optoelectronic EngineeringFoshan UniversityFoshan 528225China

Polyethylene oxide(PEO)-based solid-state polymer electrolytes(SPEs)are limited by their poor cyclic stability and inferior ionic conductivity for applicating in high-safety,long-cycling and high-energy-density lithium metal ***,porous boron nitride nanofibers(BNNFs)are filled into PEO-based SPE,which significantly suppresses Li dendrites growth and enhances the electrochemical performance of Li metal *** with high porosity have more active sites to connect with PEO,which can effectively reduce the crystallinity of the PEO matrix and enhance its ionic ***,owing to the hardness and good stability of BNNFs,BNNFs/PEO/Li TFSI electrolyte exhibits a wider electrochemical window,better mechanical property and higher thermal stability compared with PEO/Li TFSI ***,the Li symmetric cell composed of 1%BNNFs/PEO/Li TFSI performs good cyclic stability(>1800 h),and the Li||1%BNNFs/PEO/Li TFSI||LFP full battery shows obviously improved performances in charge-discharge polarization voltage,discharge specific capacity,rate performance and cyclic stability than the Li||PEO/Li TFSI||LFP battery.

关键词： Solid-state polymer electrolyte Boron nitride nanofibers Lithium metal battery Ionic conductivity Li dendrite