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Electron delocalization-enhanced sulfur reduction kinetics on an MXene-derived heterostructured electrocatalyst

Nano Research 2024年第8期17卷 7153-7162页

作者： Yunmeng Li yinze Zuo Xiang Li Yongzheng zhang Cheng {2. Xiaomin Cheng Jian wang Jitong wang Hongzhen Lin Licheng Ling State key laboratory of Chemical Engineering Key Laboratory of Specially Functional Polymeric Materials and Related Technology(Ministry of Education)East China University of Science and TechnologyShanghai 200237China Institute of New Energy materials and Engineering College of Materials Science and EngineeringFuzhou UniversityFuzhou 350108China key laboratory of Specially Functional Polymeric {2. and Related Technology(Ministry of Education) School of Materials Science and EngineeringEast China University of Science and TechnologyShanghai 200237China i-Lab&CAS key laboratory of Nanophotonic {2. and Device Suzhou Institute of Nano-Tech and Nano-Bionics Chinese Academy of SciencesSuzhou 215123China Helmholtz Institute Ulm(HIU) D89081 UlmGermany

Lithium-sulfur(Li-S)batteries mainly rely on the reversible electrochemical reaction of between lithium ions(Li^(+))and sulfur species to achieve energy storage and conversion,therefore,increasing the number of free Li^(+)and improving the Li^(+)diffusion kinetics will effectively enhance the cell ***,Mo-based MXene heterostructure(MoS_(2.@Mo_(2.C)was developed by partial vulcanization of Mo_(2.C MXene,in which the introduction of similar valence S into Mo-based MXene(Mo_(2.C)can create an electron delocalization *** theoretical simulations and electrochemical characterisation,it is demonstrated that the MoS_(2.@Mo_(2.C heterojunction can effectively promote ion desolvation,increase the amount of free Li^(+),and accelerate Li^(+)transport for more efficient polysulfide *** addition,the MoS_(2.@Mo_(2.C material is also capable of accelerating the oxidation and reduction of polysulfides through its sufficient defects and vacancies to further enhance the catalytic ***,the Li-S battery with the designed MoS_(2.@Mo_(2.C electrocatalyst performed for 500 cycles at 1 C and still maintained the ideal capacity(664.7 mah·g^(−1)),and excellent rate performance(567.6 mah·g^(−1)at 5 C).Under the extreme conditions of high loading,the cell maintained an excellent capacity of 775.6 mah·g^(−1)after 100 *** also retained 838.4 mah·g^(−1)for 70 cycles at a low temperature of 0℃,and demonstrated a low decay rate(0.063%).These results indicate that the delocalized electrons effectively accelerate the catalytic conversion of lithium polysulfide,which is more practical for enhancing the behaviour of Li-S batteries.

关键词： delocalized electron lithium sulfur batteries MXene-based heterostructures catalytic desolvation multi-catalytic sites

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Photo-induced effect in the layered perovskite manganite La_(1.2.Sr_(1.8)Mn_(1.8)Co_(0.2.O_(7)

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Science China(Physics,Mechanics & Astronomy) 2004年第1期47卷 113-120页

作者： zhang Ruili1, DAI Jianming1, SONG Wenhai1, ma Yongqing1, YANG Jie1 & SUN Yuping1,{2.. key laboratory of Internal Friction and Defects in Solids, Institute of Solid State Physics, Chinese Academy of Sciences, Hefei 2.0031, China 2. National laboratory of Solid State Microstructures, nanjing university, nanjing 2.0008, China Correspondence should be addressed to zhang Ruili (email: rlzhang@***) Received September 1, 2.03 key laboratory of Internal Friction and Defects in Solids Institute of Solid State Physics Chinese Academy of Sciences Hefei 230031 China National laboratory of Solid State Microstructures Nanjing University Nanjing 210008 China

It is helpful to study the photo-induced effect in the perovskite manganites not only for elucidating the mechanism of colossal magnetoresistance (CMR) effect but also for potential applications in technology. The laser-induced effect in the Co doping layered perovskite manganites La1.2.r1.8Mn1.8Co0.2.7 is studied in this paper and the obtained results are also compared with that gained in the Nd-doping manganites with cubic perovskite structure.

关键词： laser, layered perovskite manganites, photo-induced effect, spin-state.

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Structure-based design of pan-coronavirus inhibitors targeting host cathepsin L and calpain-1

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Signal Transduction and Targeted Therapy 2024年第4期9卷 1651-1664页

作者： Xiong Xie Qiaoshuai Lan Jinyi Zhao Sulin zhang {2. Liu Yumin zhang Wei Xu maolin Shao Jingjing Peng Shuai Xia Yan Zhu Keke zhang Xianglei zhang Ruxue zhang jian Li Wenhao Dai Zhen Ge Shulei Hu Changyue Yu Jiang wang Dakota ma Mingyue Zheng Haitao Yang Gengfu Xiao Zihe Rao {2. {2. Leike zhang Fang Bai Yao Zhao Shibo Jiang Hong Liu Drug Discovery and Design Center State Key Laboratory of Drug ResearchCAS Key Laboratory of Receptor ResearchShanghai Institute of Materia MedicaChinese Academy of SciencesShanghai 201203China university of Chinese Academy of Sciences Beijing 100049China key laboratory of Medical Molecular Virology(MOE/NHC/CAMS) School of Basic Medical SciencesShanghai Institute of Infectious Disease and BiosecurityFudan UniversityShanghai 200032China Shanghai Institute for Advanced Immunochemical Studies and School of Life Science and Technology ShanghaiTech UniversityShanghai 201210China State key laboratory of Virology Wuhan Institute of VirologyCenter for Biosafety Mega-ScienceChinese Academy of SciencesWuhan 430071China School of Chinese materia Medica Nanjing University of Chinese Medicine138 Xian Lin RoadJiangsu 210023 NanjingChina School of Pharmaceutical Science and Technology Hangzhou Institute for Advanced StudyUCASHangzhou 310024China National Clinical Research Center for Infectious Disease Shenzhen Third People's HospitalShenzhen 518112China

Respiratory disease caused by coronavirus infection remains a global health *** several SARS-CoV-2.specific vaccines and direct-acting antivirals are available,their effcacy on emerging coronaviruses in the future,including SARS-CoV-2.variants,might be ***-targeting antivirals provide preventive and therapeutic strategies to overcome resistance and manage future outbreak of emerging *** L(CTSL)and calpain-1(CAPN1)are host cysteine proteases which play crucial roles in coronaviral entrance into cells and infection-related immune ***,two peptidomimetic a-ketoamide compounds,14a and 14b,were identified as potent dual target inhibitors against CTSL and *** X-ray crystal structures of human CTSL and CAPN1 in complex with 14a and 14b revealed the covalent binding of a-ketoamide groups of 14a and 14b to C2. of CTSL and C115 of *** showed potent and broad-spectrum anticoronaviral activities in vitro,and it is worth noting that they exhibited low nanomolar potency against SARS-CoV-2.and its variants of concern(VOCs)with ECso values ranging from 0.80 to 161.7 nM in various *** mechanistic exploration indicated that they exhibited anticoronaviral activity through blocking viral ***,14a and 14b exhibited good oral pharmacokinetic properties in mice,rats and dogs,and favorable safety in *** addition,both 14a and 14b treatments demonstrated potent antiviral potency against SARS-CoV-2.XBB 1.16 variant infection in a K18-hACE2.transgenic mouse *** 14b also showed effective antiviral activity against HCoV-OC43 infection in a mouse model with a final survival rate of 60%.Further evaluation showed that 14a and 14b exhibited excellent antiinflammatory effects in Raw 2.4.7 mouse macrophages and in mice with acute *** together,these results suggested that 14a and 14b are promising drug candidates,providing novel insight into developing pan-coronavirus inhibitors with anti

关键词： calpain overcome entrance

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Degeneration Directory:a multi-omics web resource for degenerative diseases

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Protein & Cell 2024年第5期15卷 385-392页

作者： Haoteng Yan Changfa lu Chenyang Lan Si wang Weiqi {2. Zan He Jinghao Hu Jiaqi Ai Guang-Hui Liu Shuai ma Yuanchun Zhou Jing Qu State key laboratory of Membrane Biology Institute of ZoologyChinese Academy of SciencesBeijing 100101China State key laboratory of Stem Cell and Reproductive Biology Institute of ZoologyChinese Academy of SciencesBeijing 100101China key laboratory of Organ Regeneration and Re{2. Institute of ZoologyChinese Academy of SciencesBeijing 100101China Advanced Innovation Center for Human Brain Protection and National Clinical Research Center for Geriatric DisordersXuanwu Hospital Capital Medical UniversityBeijing 100053China Aging Translational Medicine Center International Center for Aging and CancerBeijing Municipal Geriatric Medical Research CenterXuanwu HospitalCapital Medical UniversityBeijing 100053China Computer Network Information Center Chinese Academy of SciencesBeijing 100190China The Fifth People’s Hospital of Chongqing Chongqing 400062China Aging Biomarker Consortium Beijing 100101China CAS key laboratory of Genomic and Precision Medicine Beijing Institute of GenomicsChinese Academy of Sciences and China National Center for BioinformationBeijing 100101China university of Chinese Academy of Sciences Beijing 100049China Sino-Danish College University of Chinese Academy of SciencesBeijing 101408China Beijing Institute for Stem Cell and Regenerative Medicine Beijing 100101China Institute for Stem Cell and Regeneration Chinese Academy of SciencesBeijing 100101China

Background of *** degeneration refers to the gradual decline in organ function and structure deterioration that occurs during aging,which represents the greatest risk factor for various degenerative diseases,including cardiovascular diseases,neurodegenerative diseases,and osteoarthritis,etc.(Aging Biomarker et al.,2.2.;Becker et al.,{2.8;Cai et al.,2.2.).

关键词： Directory web Becker

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Preparation and properties of ZrO_(2.-strengthened porous mullite insulation materials using Y_(2.O_(3) additive

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Journal of Iron and Steel Research International 2024年第6期31卷 1514-1521页

作者： wang-zhi Yu yi-hong Shi Ping Liu Yong-wan Wu Cheng-hao Song Xian-gong Deng Xiang Ding Song-lin Ran yi zhang Hai-jun zhang Hai-liang Deng Advanced Ceramics Research Center School of Materials Science and EngineeringAnhui University of TechnologyMa'anshan 243002AnhuiChina The State key laboratory of Refractories and Metal{2.rgy Wuhan University of Science and TechnologyWuhan 430081HubeiChina

ZrO_(2.-strengthened porous mullite insulation materials were prepared by foaming technology utilizing ZrSiO_(4) and Al_(2.O_(3) as primary materials and Y_(2.O_(3) as an *** effects of Y_(2.O_(3) contents on the phase composition,microstructure,mechanical properties,and heat conductivity of the porous mullite insulation materials were investigated.A suitable Y_(2.O_(3) content could promote phase transition of monoclinic ZrO_(2.(m-ZrO_(2.)to tetragonal ZrO_(2.(t-ZrO_(2.),reduce pore size,and improve the strengths of as-prepared *** cold crushing strength and bending strength of as-prepared specimens with a 119µm spherical pore size using 6 wt.%Y_(2.O_(3) were 35.2.and 13.0 MPa,respectively,with a heat conductivity being only 0.2.8 W/(m K).

关键词： Porous mullite insulation material Zirconium oxide Y_(2.O_(3) Mechanical property Heat conductivity

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Frontiers in high entropy alloys and high entropy functional materials

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Rare Metals 2024年第10期43卷 4639-4776页

作者： Wen-Tao zhang Wen Huang Fu-Jie Yu Qi Zhao Xin-Dong Zhu Tao Feng Yao Jiang Xiao-Ming Li Xue-Fei Miao He Zhu Si Lan Xue-Qian wang Bao-Long Shen Zhe Jia Feng-Qi zhang Wei wang Qi Liu Yang Ren Xun-Li wang Xiao-Ya Cui Xiao-Yang wang Ya-Nan Chen Bing-Bing Fan Meng-Ru Li Qi-Long Gao Jia-Ming Guo Zeng-Bao Jiao Zhi-Min Guo Yu-Ping Zhao Qian Yu Rui Huang Ling-Kun zhang yi-Ping lu Xu-Bo Li Huai-Jun Lin Yan ma Wei-Ming Yang Zhi-Hua Shen Hai-Yan He Yong-Gang Sun Yong-Jiang Huang De-Zhuang wang Qing-Feng Liu Fei-Yang wang Hui Liu Hong-Hui Wu Li-Qiang wang Yang lu Nan wang Tian-Li wang Wei-Bing Liao yi-Han wang Yuan Wu Yu-Zhen yin Jie Pan yi zhang Qing wang Jian-Yang zhang Tao Yang Yasir Sohail Jin-Yu zhang Hua Ji Qiang Li Wei-Di Liu Zhi-Gang Chen Xiong-Jun Liu Wen ma Liang mao Zhen-Duo Wu School of materials Science and Engineering Nanjing University of Science and Technology jiangsu key {2. for Advanced Metallic {2. School of Materials Science and Engineering Southeast University Department of Physics City University of Hong Kong School of materials Science and Engineering Tianjin University School of Physics and Microelectronics Zhengzhou University Department of Mechanical Engineering Research Institute for Advanced Manufacturing The Hong Kong Polytechnic University Center of Electron Microscopy and State key laboratory of Silicon {2. School of Materials Science and Engineering Zhejiang University key laboratory of Solidification Control and Digital Preparation Technology (Liaoning Province) School of Materials Science and Engineering Dalian University of Technology Institute of Advanced Wear & Corrosion Resistance and Functional materials Jinan University School of Mechanics and Civil Engineering China University of Mining and Technology School of Physical Sciences Great Bay University School of materials Science andEngineering Harbin Institute of Technology State key laboratory of {2.-Oriented Chemical Engineering College of Chemical Engineering Nanjing Tech University Beijing Advanced Innovation Center for materials Genome Engineering Research Institute for Carbon Neutrality University of Science and Technology Beijing Department of Mechanical Engineering The University of Hong Kong School of Computing Macquarie University key laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong Province College of Physics and Optoelectronic Engineering Shenzhen University State key laboratory for Advanced Metals and {2. University of Science and Technology Beijing State key laboratory of {2. Processing and Die & Mould Technology School of Materials Science and Engineering Huazhong University of Science and Technology Institute of materials Shanghai University Department of materials Science and Engineering C

Owing to their exceptional properties, high-entropy alloys(HEAs) and high-entropy materials have emerged as promising research areas and shown diverse applications. Here,the recent advances in the field are comprehensively reviewed,organized into five sections. The first section introduces the background of HEAs, covering their definition, significance,application prospects, basic properties, design principles, and microstructure. The subsequent section focuses on cutting-edge high-entropy structural materials, highlighting developments such as nanostructured alloys, grain boundary engineering,eutectic systems, cryogenic alloys, thin films, micro-nano-lattice structures, additive {2.nufacturing, high entropy metallic glasses, nano-precipitate strengthened alloys, composition modulation, alloy fibers, and refractory systems. In the following section, the emphasis shifts to functional materials, exploring HEAs as catalysts, {2.gneto-caloric materials, corrosion-resistant alloys, radiation-resistant alloys, hydrogen storage systems, and materials for biomedicine. Additionally, the review encompasses functional high-entropy materials outside the realm of alloys, including thermoelectric, quantum dots, nanooxide catalysts, energy storage materials, negative ther{2.l expansion ceramics,and high-entropy wave absorption materials. The paper concludes with an outlook, discussing future directions and potential growth areas in the field. Through this comprehensive review,researchers, engineers, and scientists {2.y gain valuable insights into the recent progress and opportunities for further exploration in the exciting do{2.ins of high-entropy alloys and functional materials.

关键词： Cutting-edge structural materials Cutting-edgefunctional materials High entropy alloys

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Free-Standing Multiscale Porous High Entropy NiFeCoZn Alloy as the Highly Active Bifunctional Electrocatalyst for Alkaline Water Splitting

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Chinese Journal of Chemistry 2024年第13期42卷 1465-1473页

作者： Qiuping zhang Xu wang Tianzhen Jian Wenqing {2. Caixia Xu Qiuxia Zhou Hong Liu Institute for Advanced Interdisciplinary Research(iAIR) Collaborative Innovation Center of Technology and Equipment for Biological Diagnosis and Therapy in Universities of ShandongSchool of Chemistry and Chemical EngineeringUniversity of JinanJinanShandong 250022China School of Medical Information and Engineering Southwest Medical UniversityLuzhouSichuan 646000China State key laboratory of Crystal {2. Shandong UniversityJinanShandong 250100China

In the endeavor of searching for highly active and stable electrocatalysts toward overall water splitting,high-entropy-alloys have been the intense subjects owing to their advanced physicochemical *** non-noble metal free-standing multiscale porous NiFeCoZn high-entropy-alloy is in situ constructed on the surface layer of NiZn intermetallic and Ni heterojunction over nickel foam(NiFeCoZn/NiZn-Ni/NF)by one scalable dealloying protocal to fulfill the outstanding bifunctional electrocatalytic performances toward overall water *** of the high-entropy effects and specific hierarchical porous architecture,the as-made NiFeCoZn/NiZn-Ni/NF displays high intrinsic catalytic activities and durability toward both hydrogen evolution reaction(HER)and oxygen evolution reaction(OER)in alkaline *** particular,the in-situ construction of bimodal porous NiFeCoZn high-entropy-alloy results in the small overpotentials(η1000=2.4/409 mV for HER and OER),low Tafel slopes,and exceptional long-term catalytic durability for 400 ***,the electrolyzer constructed with NiFeCoZn/NiZn-Ni/NF as both cathode and anode exhibits a low cell voltage of 1.72.V to deliver the current density of 500 ma·cm^(–2. for overall water *** work not only provides a facile and scalable protocol for the preparation of self-supporting high-entropy-alloy nanocatalysts but also enlightens the engineering of high performance bifunctional electrocatalysts toward water splitting.

关键词： High-entropy-alloys Bifunctional electrocatalyst Dealloying/Electrocatalysis Oxygen evolution reaction Hydrogen evolution reaction

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CD97 inhibits osteoclast differentiation via Rap1a/ERK pathway under compression

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International Journal of Oral Science 2024年第1期16卷 134-144页

作者： Xuan Zhou Xinjia Cai Fengyang Jing Xuefen Li Jianyun zhang Heyu zhang Tiejun Li Department of Oral Pathology Peking University School and Hospital of Stomatology&National Center of Stomatology&National Clinical Research Center for Oral Diseases&National Engineering Laboratory for Digital and Material Technology of Stomatology&Beijing Key Laboratory of Digital Stomatology&Research Center of Engineering and Technology for Computerized Dentistry Ministry of Health&NMPA Key Laboratory for Dental MaterialsBeijingChina Research Unit of Precision Pathologic Diagnosis in Tumors of the Oral and maxillofacial Regions Chinese Academy of Medical Sciences(2019RU034)BeijingChina Central laboratory Peking University School and Hospital of StomatologyBeijingChina

Acceleration of tooth movement during orthodontic treatment is challenging, with osteoclast-mediated bone resorption on the compressive side being the rate-limiting step. Recent studies have demonstrated that mechanoreceptors on the surface of monocytes/macrophages, especially adhesion G protein-coupled receptors (aGPCRs), play important roles in force ***, its role in the regulation of osteoclast differentiation remains unclear. Herein, through single-cell analysis, we revealed that CD97, a novel mechanosensitive aGPCR, was expressed in macrophages. Compression upregulated CD97 expression and inhibited osteoclast differentiation;while knockdown of CD97 partially rescued osteoclast differentiation. It suggests that CD97 may be an important mechanosensitive receptor during osteoclast differentiation. RNA sequencing analysis showed that the Rap1a/ERK signalling pathway mediates the effects of CD97 on osteoclast differentiation under compression. Consistently, we clarified that administration of the Rap1a inhibitor GGTI2.8 increased osteoclast activity, thereby accelerating tooth movement. In conclusion,our results indicate that CD97 suppresses osteoclast differentiation through the Rap1a/ERK signalling pathway under orthodontic compressive force.

关键词： CD97 osteoclast inhibited

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Biochar regulates biogeochemical cycling of iron and chromium in a soil-rice system by stimulating Geobacter and Clostridium

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Pedosphere 2024年第5期34卷 929-940页

作者： Min XU Yang LIN Jing ma lulu LONG chao CHEN Gang YANG Chun SONG Jun WU Xiaohong zhang Peng GAO College of Environmental Science Sichuan Agricultural University Soil Water and Ecosystem Sciences Department University of Florida College of Water Conservancy and Hydropower Engineering Sichuan Agricultural University Department of Environmental and Occupational Health University of Pittsburgh School of Public Health

In soil-rice systems,microbial reduction of iron （Fe） has been recognized as a crucial biogeochemical process that regulates Fe and chromium （Cr）translocation;however,the underlying processes are *** investigate the impacts of biochar on the biochemical cycling of Fe and Cr and their toxicity to rice,maize straw biochar was applied at 1%（weight/weight） to a paddy soil spiked with 300 mg kg-1Cr under two phosphorus （P） levels (0 or 90 mg kg-1) in a pot *** {2. microbial groups affecting Fe dissimilatory reduction and their environmental drivers were *** inhibited root Cr uptake by 36%,owing to the promoted iron plaque （IP） formation on the rice root *** analysis showed that Fe concentration in pore water was strongly linked to the abundances of Geobacter （r=0.81–0.94,P2. determinants influencing Fe-reducing bacterial abundances,accounting for 42.and 32.of the variation in community composition,***,biochar increased Fe and P concentrations in root cell walls,which retained more ***,Cr stress in rice under biochar treatment was relieved through increasing IP formation and altering subcellular *** mechanistic insights had important implications for reducing Cr uptake by rice.

关键词： chromium translocation iron plaque iron reduction maize straw biochar microbial reduction paddy soil phosphorus fertilization subcellular distribution

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construction and performance test of charged particle detector array for maTE

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Nuclear Science and Techniques 2024年第8期35卷 92-100页

作者： Xiao‑Bin Li Long‑Hui Ru Zhi‑chao zhang Bing‑Feng Lv Ning‑Tao zhang Jin‑Long zhang Chen‑Gui lu Bing‑Shui Gao Jun‑Bing ma Fu‑Shuai Shi Satoru Terashima Xiao‑Dong Xu Zhen Bai Shi‑Wei Xu Yan‑Yun Yang Hooi‑Jin Ong Xiao‑Dong Tang Institute of Modern Physics(IMP) Chinese Academy of SciencesLanzhou 730000China School of Nuclear Science and Technology University of Chinese Academy of SciencesBeijing 100049China Research Center for Nuclear Physics Osaka UniversityIbarakiOsaka 567‑0047Japan RIKEN Nishina Center WakoSaitama 351‑0198Japan Joint Department for Nuclear Physics Lanzhou University and Institute of Modern PhysicsChinese Academy of SciencesLanzhou 730000China

A charged particle array named maTE-PA,which serves as an auxiliary detector system for a Multi-purpose Active-target Time projection chamber used in nuclear astrophysical and exotic beam Experiments(maTE),was *** array comprised of 2. single-sided strip-silicon detectors covering approximately 10%of the solid *** detectors facilitated the detection of reaction-induced charged particles that penetrate the active volume of the *** performance of maTE-PA has been experimentally studied using an alpha source and a 36-MeV 14 N beam injected into the maTE chamber on the radioactive ion beam line in Lanzhou(RIBLL).The chamber was filled with a gas mixture of 95%4 He and 5%CO_(2. at a pressure of 500 *** results indicated good separation of light-charged particles using the forward double-layer silicon detectors of *** energy resolution of the Si detectors was deduced to be approximately 1%(σ)for an energy loss of approximately 10 MeV caused by theα*** inclusion of maTE-PA improves particle identification and increases the dynamic range of the kinetic energy of charged particles,particularly that of theαparticles,up to approximately 15 MeV.

关键词： Silicon detector array Active target Time projection chamber

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