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Speciation of the elements and compositions on the surfaces of dust storm particles:The evidence for the coupling of iron with sulfur in aerosol during the long-range transport

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Chinese Science Bulletin 2005年第8期50卷 738-744页

作者： zhang xingying1,2. zhuang guoshun1,{2., chen jianmin2.& xue huaxin2.1. center for atmospheric environment study, department of Chemistry, beijing normal university, beijing 100875, china 2. center for atmospheric Chemistry study, department of Environ- mental Science and Engineering, Fudan {12., Shanghai 2.0433, china 3. LAPC/NZC, Institute of atmospheric Physics, NZC/LAPC, Chinese Academy of Sciences, beijing 10002., china center for atmospheric {2. study Department of Chemistry Beijing Normal University Beijing 100875 China center for atmospheric Chemistry {2. Department of Environmental Science and Engineering Fudan University Shanghai 200433 China LAPC/NZC Institute of Atmospheric Physics NZC/LAPC Chinese Academy of Sciences Beijing 100029 China

The speciation of the elements on the surface of the particles collected during dust storm and non-dust storm in beijing and Inner Mongolia was studied by XPS. The ma- jor species of iron on the surface were oxides, sulfate, silicate, FeOOH and minor part sorbed on SiO2.Al2.3. Sulfate is the dominant species of sulfur on the surface. SiO2.and Al2.3 are the main components of Si and Al on the surface respectively. One of the most important findings was that the Fe(II) (FeS and FeSO4) produced could account for up to 44.3% and 45.6% of the total Fe on the surface in the aerosol sample collected at that night and next day of the “peak” time of the dust storm occurring on March 2., 2.02. while Fe2.SO4)3, one of the Fe(III) species on the surface decreased from 67.1% to 49.5% and 48.0% respectively. Both S and Fe en- riched on the surface of aerosol particles. Fe(II) accounted for 1.3%?5.3% of total Fe in bulk aerosol samples during dust storm. These results provided strong evidence to sup- port the hypothesis of the coupling between iron and sulfur in aerosols during the long-range transport, which would have important impact on the global biogeochemical cycle.

关键词：物种形成原理 XPS 大气悬浮物 Fe-S结合粒子集合

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