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Ultrathin GaN Film Derived from Amorphous Ga_(2)O_(3) Film

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Journal of Wuhan University of Technology(Materials Science) 2024年第4期39卷 814-818页

作者：王鹏 zhang Binbin LIU Xiaofei zhang xin TU rong zhang Song 李宝文 State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China State Key Laboratory of Silicate Materials for Architectures School of Materials Science and EngineeringWuhan University of TechnologyWuhan 430070China

It remains a big challenge to synthesize two-dimensional(2D)GaN material for applications in power *** synthetic methods require complex equipment and processes and time ***,we reported a two-step route to prepare polycrystalline 2D GaN *** amorphous ultrathin Ga_(2)O_(3)film was first exfoliated from the surface of liquid *** a vapor phase reaction,2D Ga_(2)O_(3)film was then converted into 2D GaN film while maintaining the 2D *** and high-resolution transmission electron microscope(HRTEM)analysis implies the successful synthesis of wurtzite-type GaN ultrathin *** simple strategy proposed in this work will provide more opportunities for applications of GaN ultrathin film in many devices.

关键词： GaN Ga_(2)O_(3) liquid gallium

Surface iodine and pyrenyl-graphdiyne co-modified Bi catalysts for highly efficient CO_(2) electroreduction in acidic electrolyte

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Nano Research 2024年第4期17卷 2381-2387页

作者： Min zhang Juan Wang xin rong Xiu-Li Lu Tong-Bu Lu MOE International Joint Laboratory of Materials Microstructure Institute for New Energy Materials and Low Carbon TechnologiesSchool of Materials Science and EngineeringTianjin University of TechnologyTianjin 300384China

CO_(2) electroreduction to formic acid/formate would contribute to alleviating the energy and climate *** work reports a Bi-based catalyst derived from the in-situ electroreduction of Bi_(2)O_(2)CO_(3) modified with iodine and pyrenyl-graphdiyne(PGDY)on the surface for efficient electroreduction of CO_(2) in acidic electrolyte,with a high partial current density of 98.71 mA·cm^(-2) and high Faradaic efficiency(FE)>90%over the potential range from^(-1).2 to-1.5 V *** hydrogen electrode(RHE),as well as the long-term operational stability over 240 h without degradation in H-type *** results and density function theory calculations show that the synergistic effect of surface iodine and PGDY is responsible for this active and extremely stable process of CO_(2) electroreduction via lowering the energy barriers for formation of*OCHO intermediate,suppressing the competitive HER by enhancing the concentration of both K+and CO_(2) at reaction interface,as well as preventing the dissolution and re-deposition of active Bi atoms on surface during catalytic *** work provides new insight into designing highly active and stable electrocatalysts for CO_(2) reduction.

关键词： CO_(2) reduction electrocatalysis Bi-based catalysts acidic electrolyte

Dimethylamine oxalate manipulating CsPbI_(3) perovskite film crystallization process for high efficiency carbon electrode based perovskite solar cells

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Journal of Energy Chemistry 2024年第6期93卷 221-228,I0006页

作者： Wenran Wang xin Peng Jianxin zhang Jiage Lin rong Huang Guizhi zhang Huishi Guo Zhenxiao Pan xinhua Zhong Huashang Rao Key Laboratory for Biobased Materials and Energy of Ministry of Education College of Materials and EnergySouth China Agricultural UniversityGuangzhou 510642GuangdongChina College of Chemistry and Civil Engineering Shaoguan UniversityShaoguan 512005GuangdongChina Guangdong Provincial Key Laboratory of Utilization and Conservation of Food and Medicinal Resources in Northern Region Shaoguan UniversityShaoguan 512005GuangdongChina

Crystallization process determines the quality of perovskite films and the performances of resultant perovskite solar cells(PSCs).Dimethylamine oxalate has been proven as a multifunctional modulator,and is explored as an efficient additive in manipulating the crystallization process of CsPbI_(3) perovskite *** one hand,oxalate serves as the precipitator that facilitates the nucleation process of *** larger size of intermediate is conductive to the larger size and smaller grain boundaries of resultant *** the other hand,in subsequent annealing process,the phase conversion and growth process of transient perovskite can be decelerated due to the strong interactions of oxalate with both dimethylamine cation(DMA^(+))and Pb^(2+).Due to the optimized crystallization kinetics,the morphology and quality of CsPbI_(3) perovskite films are comprehensively improved with lower defect concentrations,and charge recombination loss is effectively *** from the optimized crystal quality of perovskite films,the carbon electrode-based CsPbI_(3) PSCs exhibit a champion efficiency of 18.48%.This represents one of the highest levels among all hole transport layer-free inorganic perovskite solar cells.

关键词： Solar cells Perovskite CsPbI_(3) Carbon electrodes Oxalate

A note on self-normalized Dickey-Fuller test for unit root in autoregressive time series with GARCH errors

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Applied Mathematics(A Journal of Chinese Universities) 2008年第2期23卷 197-201页

作者： YANG Xiao-rong zhang Li-xin Dept. of Math. Zhejiang Univ. Hangzhou 310027 China

In this article, the unit root test for AR（p） model with GARCH errors is considered. The Dickey-Fuller test statistics are rewritten in the form of self-normalized sums, and the asymptotic distribution of the test s... 详细信息

关键词： unit root AR (p)-GARCH (1,1) self-normalized Dickey-Fuller test statistic.

Species’ geographical range, environmental range and traits lead to specimen collection preference of dominant plant species of grasslands in Northern China

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Plant Diversity 2024年第3期46卷 353-361页

作者： Jingya zhang Cui Xiao Xiaoyu Duan xin Gao Hao Zeng rong'an Dong Gang Feng Keping Ma Ministry of Education Key Laboratory of Ecology and Resource Use of the Mongolian Plateau&Inner Mongolia Key Laboratory of Grassland Ecology School of Ecology and EnvironmentInner Mongolia UniversityHohhot 010021China State Key Laboratory of Vegetation and Environmental Change Institute of BotanyChinese Academy of SciencesBeijing 100093China

Many different factors,such as species traits,socio-economic factors,geographical and environmental factors,can lead to specimen collection *** study aims to determine whether grassland specimen collection in China is preferred by species traits(i.e.,plant height,flowering and fruiting period),environmental range(i.e.,the temperature and precipitation range)and geographical range(i.e.,distribution range and altitudinal range).Ordinary least squares models and phylogenetic generalized linear mixed models were used to analyze the relationships between specimen number and the explanatory *** Forest models were then used to find the most parsimonious multivariate *** results showed that interannual variation in specimen number between 1900 and 2020 was *** number of these species in southeast China was notably lower than that in northwest *** range and geographical range of species had significant positive correlations with specimen *** addition,there were relatively weak but significant associations between specimen number and species trait(i.e.,plant height and flowering and fruiting period).Random Forest models indicated that distribution range was the most important variable,followed by flowering and fruiting period,and altitudinal *** findings suggest that future floristic surveys should pay more attention to species with small geographical range,narrow environmental range,short plant height,and short flowering and fruiting *** correction of specimen collection preference will also make the results of species distribution model,species evolution and other works based on specimen data more accurate.

关键词： Biological specimen Collection preference Dominant plant species Environmental range Geographical range Species traits

基于FMEA和FTA的VLCC翼型风帆装置风险分析

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船海工程 2024年第1期53卷 16-20页

作者：陈海成张道坤张荣鑫樊付见中国船级社技术研究开发中心北京100007 中国船级社大连分社大连116013

为了保证VLCC翼型风帆装置的安全有效运行,开展基于FMEA和FTA方法的风帆系统风险分析,以设计工作流程为主线,分别判断风帆在各工况下机械、结构、电气、液压等方面潜在的失效模式、原因和后果,评估每个失效模式的可能性、严重性和探测... 详细信息

为了保证VLCC翼型风帆装置的安全有效运行,开展基于FMEA和FTA方法的风帆系统风险分析,以设计工作流程为主线,分别判断风帆在各工况下机械、结构、电气、液压等方面潜在的失效模式、原因和后果,评估每个失效模式的可能性、严重性和探测性水平,基于风险优先数RPN判定失效模式的风险程度,制定高风险项的安全防控措施。基于故障树方法,以“无法紧急降帆”为顶事件,逐层分析分析其故障原因,确定不同事件的逻辑关系,构建故障树,针对每个基本事件制定防控措施。

关键词：翼型风帆风险分析 FMEA方法 FTA方法