检索结果-南通市图书馆

Adsorption and Vibration of Cl Atoms on Ni Low-index Surfaces

在线全文

学校读者我要写书评

暂无评论

Chemical Research in Chinese Universities 2006年第4期22卷 488-492页

作者： zhang jing diao zhao-yu wang ze-xin Department of Chemistry Shandong Normal University Jinan 250014 P. R. China

The 5-parameter Morse potential（5-MP） of the interactions between Cl atoms and Ni surfaces was constructed. The adsorption and diffusion of Cl atoms on Ni low index-surfaces were investigated with 5-MP in detail. All the critical characteristics of the system, such as adsorption site, adsorption geometry, binding energy, eigenvalues for vibration, etc. were obtained. The calculated results show that chlorine atoms are likely to be adsorbed on the high symmetry- sites. Cl atoms locate on the four-fold hollow sites of the intact Ni（100） surface, while they tend to occupy threefold sites on the Ni（ 111 ） surface. The four-fold hollow sites are the most stable adsorption sites on the Ni （110） surface for Cl, although the three-fold sites and the long-bridge sites are stable adsorption sites on the Ni（110） surface for the atoms of the first and second periods. For the Cl-Ni surface adsorption system, the surface binding energy of a Cl atom is relevant to the coarse degree of the cluster surface, and the binding energies have an order of Ni （ 111 ）〈 Ni（100）〈Ni（100）.

关键词： Cl-Ni system 5-MP Surface adsorption Surface vibration

Dielectric-ion-conductive ZnNb2O6 layer enabling rapid desolvation and diffusion for dendrite-free Zn metal batteries

在线全文

学校读者我要写书评

暂无评论

Journal of Energy Chemistry 2025年第1期100卷 693-701页

作者： Haifeng Yang Jian wang Panpan zhang Xiaomin Cheng Qinghua Guan jing Dong Bixian Chen Lujie Jia jing zhang Yongzheng zhang yunjian Liu Hongzhen Lin School of Materials Science and Engineering Jiangsu University i-Lab & CAS Key Laboratory of Nanophotonic Materials and Devices Suzhou Institute of Nano-Tech and Nano-Bionics Chinese Academy of Sciences Helmholtz Institute Ulm (HIU) Karlsruhe Institute of Technology (KIT) School of Materials Science and Engineering Xi'an University of Technology State Key Laboratory of Chemical Engineering East China University of Science and Technology

Rechargeable aqueous zinc-metal batteries （AZMBs） are promising candidates for large-scale energy storage systems due to their low cost and high ***,their performance and sustainability are significantly hindered by the sluggish desolvation kinetics at the electrode/electrolyte interface and the corresponding hydrogen evolution reaction where active water molecules tightly participate in the Zn（H2O）62+solvation ***,learnt from self-generated solid electrolyte interphase （SEI） in anodes,the dielectric but ion-conductive zinc niobate nanoparticles artificial layer is constructed on metallic Zn surface （ZNB@Zn）,acting as a rapid desolvation *** zincophilic and dielectric-conductive properties of ZNB layer accelerate interfacial desolvation/diffusion and suppress surface corrosion or dendrite formation,achieving uniform Zn plating/stripping behavior,as confirmed by electronic/optical microscopies and interface spectroscopical measurements together with theoretical ***,the as-prepared ZNB@Zn electrode exhibits excellent cycling stability of over 2000 h and robust reversibility （99.54%） even under high current density and depth of discharge ***,the assembled ZNB@Zn-based full cell displays high capacity-retention rate of 80.21%after 3000 cycles at 5 A g-1and outstanding rate performance up to 10 A *** large-areal pouch cell is stabilized for hundreds of cycles,highlighting the bright prospects of the dielectric but ion-conductive layer in further application of AZMBs.

关键词： Zn metal battery Dielectric artificial layer Rapid ion diffusion Zincophilic diffusion Active water inhibition

Repetitive traumatic brain injury–induced complement C1–related inflammation impairs long-term hippocampal neurogenesis

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

Neural Regeneration Research 2025年第3期20卷 821-835页

作者： jing wang Bing zhang Lanfang Li Xiaomei Tang Jinyu zeng Yige Song Chao Xu Kai zhao Guoqiang Liu Youming Lu xinyan Li Kai Shu Department of Neurosurgery Tongji HospitalTongji Medical CollegeHuazhong University of Science and TechnologyWuhanHubei ProvinceChina Department of Neurosurgery Shanxi Bethune HospitalShanxi Academy of Medical SciencesTongji Shanxi HospitalThird Hospital of Shanxi Medical UniversityTaiyuanShanxi ProvinceChina Department of Pathophysiology School of Basic Medicine and Tongji Medical CollegeHuazhong University of Science and TechnologyWuhanHubei ProvinceChina Institute for Brain Research Wuhan Center of Brain ScienceHuazhong University of Science and TechnologyWuhanHubei ProvinceChina Department of Graduate Student Chongqing Medical UniversityChongqingChina Department of Basic Medicine School of Medical ScienceHubei University for NationalitiesEnshiHubei ProvinceChina Department of Anatomy School of Basic Medicine and Tongji Medical CollegeHuazhong University of Science and TechnologyWuhanHubei ProvinceChina

Repetitive traumatic brain injury impacts adult neurogenesis in the hippocampal dentate gyrus,leading to long-term cognitive ***,the mechanism underlying this neurogenesis impairment remains *** this study,we established a male mouse model of repetitive traumatic brain injury and performed long-term evaluation of neurogenesis of the hippocampal dentate gyrus after repetitive traumatic brain *** results showed that repetitive traumatic brain injury inhibited neural stem cell proliferation and development,delayed neuronal maturation,and reduced the complexity of neuronal dendrites and *** with repetitive traumatic brain injuryalso showed deficits in spatial memory ***,following repetitive traumatic brain injury,neuroinflammation was enhanced in the neurogenesis microenvironment where C1q levels were increased,C1q binding protein levels were decreased,and canonical Wnt/β-catenin signaling was *** inhibitor of C1 reversed the long-term impairment of neurogenesis induced by repetitive traumatic brain injury and improved neurological *** findings suggest that repetitive traumatic brain injury–induced C1-related inflammation impairs long-term neurogenesis in the dentate gyrus and contributes to spatial memory retrieval dysfunction.

关键词： complement C1 dendrite dentate gyrus hippocampus neural stem cell neurogenesis neuroinflammation neurological function neuron traumatic brain injury

Adsorption and Diffusion of O Atoms on Ag(210) Stepped Surface

在线全文

学校读者我要写书评

暂无评论

Chemical Research in Chinese Universities 2007年第4期23卷 456-459页

作者： diao zhao-yu zhang Xue-na wang ze-xin zhang jing Deoartment of Chemistry Shandonx Normal University Jinan 250014 P. R. China School of Chemical and Biological Engineer Taiyuan Science and Technology Untverstty Taiyuan 030012 P. R. China

The O-Ag（210） surface adsorption system was studied via the five-parameter Morse potential theory. Mean- while, the 20-Ag （ 210） system was investigated v/a the extended London-Eyring-Polanyi-Sato （LEPS） potential theo- ry to learn the interaction between the adsorption states. Calculated results demonstrate that there are two stable on- surface adsorption sites（B and H） for 0 atoms on Ag（210） stepped surface. And the perpendicular vibrations are 30. 3 and 42.9 meV, which are close to that observed in high resolution electron energy loss spectroscopy （HREELS）. Also, there exists an octabedral subsurface adsorption state with a high vibrational frequency, and the interaction between the on-surface and subsurface 0 species is slight. The mode at 54.6 meV, which is close to that observed in HREELS（54-56 meV）, is because of the vibration of the 0 atom on B site under the influence of that on H site.

关键词： 5-MP LEPS Surface adsorption Vibration O-Ag(210) system

Unraveling brain aging through the lens of oral microbiota

在线全文

学校读者我要写书评

暂无评论

Neural Regeneration Research 2025年第7期20卷 1930-1943页

作者： Qinchao Hu Si wang Weiqi zhang jing Qu Guang-Hui Liu State Key Laboratory of Membrane Biology Institute of ZoologyChinese Academy of SciencesBeijingChina Hospital of Stomatology Guanghua School of StomatologyGuangdong Provincial Key Laboratory of StomatologySun Yat-sen UniversityGuangzhouGuangdong ProvinceChina Advanced Innovation Center for Human Brain Protection and National Clinical Research Center for Geriatric Disorders Xuanwu HospitalCapital Medical UniversityBeijingChina Aging Translational Medicine Center International Center for Aging and CancerBeijing Municipal Geriatric Medical Research CenterXuanwu HospitalCapital Medical UniversityBeijingChina CAS Key Laboratory of Genomic and Precision Medicine Beijing Institute of GenomicsChinese Academy of Sciences and China National Center for BioinformationBeijingChina University of Chinese Academy of Sciences BeijingChina Institute for Stem Cell and Regeneration Chinese Academy of SciencesBeijingChina Aging Biomarker Consortium BeijingChina State Key Laboratory of Stem Cell and Reproductive Biology Institute of ZoologyChinese Academy of SciencesBeijingChina Beijing Institute for Stem Cell and Regenerative Medicine BeijingChina

The oral cavity is a complex physiological community encompassing a wide range of *** of oral microbiota can lead to various oral infectious diseases,such as periodontitis and tooth decay,and even affect systemic health,including brain aging and neurodegenerative *** studies have highlighted how oral microbes might be involved in brain aging and neurodegeneration,indicating potential avenues for intervention *** this review,we summarize clinical evidence demonstrating a link between oral microbes/oral infectious diseases and brain aging/neurodegenerative diseases,and dissect potential mechanisms by which oral microbes contribute to brain aging and *** also highlight advances in therapeutic development grounded in the realm of oral microbes,with the goal of advancing brain health and promoting healthy aging.

关键词： Alzheimer's disease brain aging multiple sclerosis neurodegeneration neurodegenerative diseases oral microbiota Parkinson's disease periodontitis bacteria Porphyromonas gingivalis

Leader-follower: Human-centered intention-guided controller for novel SuperLimb with application to load-carrying scenarios

在线全文

学校读者我要写书评

暂无评论

Science China Technological Sciences 2025年第1期 325-338页

作者： Qinghua zhang Xianglong LI Hongwei jing Kerui SUN yuancheng LI Sikai zhao Lele LI Haotian JU Ziqi wang Rui WU Tianjiao ZHENG Jie zhao Yanhe ZHU The State Key Laboratory of Robotics and System Harbin Institute of Technology The Learning Algorithms and Systems Laboratory School of Engineeringécole Polytechnique Fédérale de Lausanne

Supernumerary robotic arms(SuperLimb) are a new type of wearable robot that works closely with humans as a third hand to augment human operation capability. Accurate conveyance of wearers' intentions, allocation of roles, and humancentered interaction considerations are the key points in the process of human–SuperLimb collaboration. This paper proposes a human-centered intention-guided leader–follower controller that relies on the dynamic modeling of SuperLimb with application to load-carrying scenarios. The proposed leader–follower controller takes the human as the leader and the SuperLimb as the follower, achieving effective information communication, autonomous coordination, and good force compliance between SuperLimb, humans, and the environment under human safety assurance. First, the human–SuperLimb dynamic system is modeled to achieve force interaction with the environment and wearer. Second, to achieve the precise intention extraction of humans, pose data from five visual odometry sensors are fused to capture the human state, the generalized position, the velocity of hands, and the surface electromyography signals from two myoelectric bracelets sensors are processed to recognize the natural hand gestures during load-carrying scenarios by a designed Swin transformer network. Then, based on the real-time distance detection between human and mechanical limbs, the security assurance and force-compliant interaction of the human–SuperLimb system are realized. Finally, the human hand muscle intention recognition, human–robot safety strategy verification,and comparative load-carrying experiments with and without the proposed method are conducted on the SuperLimb *** showed that the task parameters are well estimated to produce more reasonable planning trajectories, and SuperLimb could well understand the wearer's intentions to switch different SuperLimb actions. The proposed sensor-based human–robot communication framework motivates future studies of o

关键词：

Adsorption and Vibration of O Atoms on Fe Low-index and Fe(211) High-index Surfaces

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

Chemical Research in Chinese Universities 2007年第2期23卷 226-232页

作者： FENG Hui zhang Xue-na wang ze-xin diao zhao-yu QIAN zhao-sheng Department of Chemistry Shandong Normal University Jinan 250014 P. R. China Department of Chemistry Nanfing University Nanjing 210093 P. R. China

The 5-parameter Morse pntential（5-MP） of the interaction between oxygen atoms and iron surfaces was constructed. The adsorption and diffusion of O atoms on Fe low-index and Fe（211 ） high-index surfaces were investigated by using 5-MP. All the critical characteristics of the system, such as adsorption site, adsorption geometry, binding energy, and eigenvalues for vibration, were calculated. The calculation results show that O atoms are located at the fourfold hollow site of the Fe（100） surface with an eigenvibration at437 cm^-1. These results are in good agreement with the experimental and theoretical results obtained previously. With regard to the adsorption site of O-Fe（110） system, the authors of this study assume that the preferential adsorption state is the H3 site and not the LB site, which is not in agreement with the experimental inferences obtained earlier. However, on the Fe（ 111 ） and Fe（211 ） surfaces, O atoms predominantly occupy the quasi-3-fold site.

关键词： O-Fe system 5-MP Surface adsorption Vibration O-Fe(211 ) system

Adsorption Site and State of Nitrogen Atom on Ru(0001),(1010) Low-index and (1120),(1121) Stepped Surfaces

在线全文

学校读者我要写书评

暂无评论

Chemical Research in Chinese Universities 2009年第5期25卷 705-710页

作者： diao zhao-yu yu Hai-yan wang Zhong-ni zhang Xue-na wang ze-xin Department of Chemistry Shandong Normal University Jinan 250014 P. R. China

The adsorptions of nitrogen atoms on Ru（0001）, （1010） low index surfaces and （1120）, （1121） stepped surfaces were investigated by the five-parameter Morse potential（5-MP） method in details, Calculated results demonstrate that N atoms show a tendency to be adsorbed at threefold sites. No subsurface state was found for N atoms on Ru（1010） surface. There exist 6 stable adsorption sites for N atoms on Ru（1121） stepped surface which can be classified into 3 types： the on-surface adsorption state, the facet adsorption state and the subsurface state. Moreover, two new perpendicular vibrations at 97 and 98 meV are predicted. All calculated results are in good accord with HR-EELS experiments.

关键词： N-Ru system 5-MP Surface adsorption

Theoretical Studies on Adsorption Sites and States of O and N on Ni(311)

在线全文

学校读者我要写书评

暂无评论

Chemical Research in Chinese Universities 2009年第1期25卷 98-101页

作者： diao zhao-yu zhang yan zhang Xue-na wang ze-xin wang Zhong-ni Chemistry Department Shandong Normal University Jinan 250014 P. R. China

The adsorption of O and N atoms on the Ni（311） surface was investigated by the 5-parameter Morse potential（5-MP） method in detail. For the O-Ni（311） system, there are three surface adsorption states and the fcc-3-fold site is metastable; the frequency of 75 meV[67 meV in high resolution electron energy loss spectroscopy（HREELS） experiment] is attributed to the vibration at the hcp-3-fold site. For the N-Ni（311） system, however, there are only two surface adsorption states（no surface adsorption state was calculated atfcc-3-fold site）. In addition, subsurface states were predicted and all critical characteristics were obtained for the two systems.

关键词： 5-Parameter Morse potential O-Ni(311) system N-Ni(311) system Adsorption