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Journal of Thermal Science 2024年第3期33卷 1216-1230页

作者： YU Haoyang GAO Mingming zhang Hongfu CHEN Jiyu LIU Jizhen YUE Guangxi The State Key Laboratory of Alternate Electrical Power System with Renewable Energy Sources School of Control and Computer EngineeringNorth China Electric Power UniversityBeijing102206China CHN Energy New Energy Technology Research Institute Co. Ltd.Beijing102209China Department of Energy and Power Engineering Tsinghua UniversityBeijing100084China

To address the pressing need for intelligent and efficient control of circulating fluidized bed(CFB)units,it is crucial to develop a dynamic model for the key operating parameters of supercritical circulating fluidized bed(SCFB)***,data-knowledge-driven dynamic model of bed temperature,load,and main steam pressure of the SCFB unit has been ***,a knowledge-driven method is employed to develop a dynamic model for key operating parameters of SCFB *** model parameters are determined based on the operating data of the unit and continuously optimized in real ***,Bidirectional Long Short-Term Memory combined with Convolutional Neural Network and Attention Mechanism is utilized to build the dynamic model of bed temperature,load,and main steam ***,a collaboration and integration method based on the critic weight method and the variation coefficient method is proposed to establish data-knowledge-driven model of key operating parameters for SCFB *** model displays great accuracy and fitting ability compared with other methods and effectively captures the dynamic characteristics,which can provide a research basis for the design of intelligent flexible control mode of SCFB unit.

关键词： circulating fluidized bed dynamic model data-knowledge-driven method deep learning power plant

Identifying the Hydrochemical Characteristics,Genetic Mechanisms and Potential Human Health Risks of Fluoride and Nitrate Enriched Groundwater in the Tongzhou District,Beijing,North China

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Acta Geologica Sinica(English Edition) 2024年第2期98卷 468-476页

作者： zhang Shouchuan LIU Kai MA Yan WANG Luyao SUN Junliang Chinese Academy of Geological Sciences Beijing 100037China School of Water Resources and Environment China University of Geosciences(Beijing)Beijing 100083China

Fluoride and nitrate enriched groundwater are potential threats to the safety of the groundwater supply that may cause significant effects on human health and public safety,especially in aggregated population areas and economic *** study focuses on the high F^(−)and NO_(3)^(−)concentration groundwater in Tongzhou District,Beijing,North China.A total of 36 groundwater samples were collected to analyze the hydrochemical characteristics,elucidate genetic mechanisms and evaluate the potential human health *** results of the analysis indicate:Firstly,most of the groundwater samples are characterized by Mg-HCO_(3) and Na-HCO_(3) with the pH ranging from 7.19 to 8.28 and TDS with a large variation across the range 471-2337 mg/*** NO_(3)^(−)concentration in 38.89%groundwater samples and the F^(−)concentration in 66.67%groundwater samples exceed the permissible limited ***,F^(−)in groundwater originates predominantly from water-rock interactions and the fluorite dissolution,which is also regulated by cation exchange,competitive adsorption of HCO_(3)−and an alkaline ***,the effect of sewage disposal and agricultural activities have a significant effect on high NO3-concentration,while the high F^(−)concentration is less influenced by anthropogenic *** alkaline environment favors nitrification,thus being conducive to the production of NO_(3)^(−).Finally,the health risk assessment is evaluated for different population *** results indicate that high NO_(3)^(−)and F^(−)concentration in groundwater would have the largest threat to children’s *** findings of this study could contribute to the provision of a scientific basis for groundwater supply policy formulation relating to public health in Tongzhou District.

关键词： fluoride concentration nitrate pollution genetic mechanism health risk assessment Tongzhou District

Analysis of the interaction between bolt-reinforced rock and surface support in tunnels based on convergence-confinement method

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第6期16卷 1936-1951页

作者： Zhenyu Sun Dingli zhang Qian Fang Yanjuan Hou Nanqi Huangfu Key Laboratory for Urban Underground Engineering of Ministry of Education Beijing Jiaotong UniversityBeijing100044China

To investigate the interaction of the bolt-reinforced rock and the surface support,an analytical model of the convergence-confinement type is proposed,considering the sequential installation of the fully grouted rockbolts and the surface *** rock mass is assumed to be elastic-brittle-plastic material,obeying the linear Mohr-Coulomb criterion or the non-linear Hoek-Brown *** to the strain states of the tunnel wall at bolt and surface support installation and the relative magnitude between the bolt length and the plastic depth during the whole process,six cases are categorized upon solving the *** case is divided into three stages due to the different effects of the active rockbolts and the passive surface *** fictitious pressure is introduced to quantify the threedimensional(3D)effect of the tunnel face,and thus,the actual physical location along the tunnel axis of the analytical section can be *** using the bolt-rock strain compatibility and the rocksurface support displacement compatibility conditions,the solutions of longitudinal tunnel displacement and the reaction pressure of surface support along the tunnel axis are *** proposed analytical solutions are validated by a series of 3D numerical *** parametric studies are conducted to examine the effect of the typical parameters of rockbolts and surface support on the tunnel displacement and the reaction pressure of the surface support under different rock *** results show that the rockbolts are more effective in controlling the tunnel displacement than the surface support,which should be installed as soon as possible with a suitable *** tunnels excavated in weak rocks or with restricted displacement control requirements,the surface support should also be installed or closed timely with a certain *** proposed method provides a convenient alternative approach for the optimization of rockbolts and surface support

关键词： Analytical model Longitudinal tunnel displacement Fictitious pressure Active rockbolts Surface support reaction pressure Tunnel design

Multiscale modeling of gas-induced fracturing in anisotropic clayey rocks

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第6期16卷 2091-2110页

作者： Jianxiong Yang Jianfeng Liu Zhengyuan Qin Xuhai Tang Houquan zhang State Key Laboratory of Hydraulics and Mountain River Engineering College of Water Resource and HydropowerSichuan UniversityChengdu610042China School of Resources and Safety Engineering Wuhan Institute of TechnologyWuhan430073China School of Civil Engineering Wuhan UniversityWuhan430072China State Key Laboratory of Intelligent Construction and Healthy Operation and Maintenance of Deep Underground Engineering China University of Mining and TechnologyXuzhou221116China

In the context of repositories for nuclear waste,understanding the behavior of gas migration through clayey rocks with inherent anisotropy is crucial for assessing the safety of geological disposal *** primary mechanism for gas breakthrough is the opening of micro-fractures due to high gas *** occurs at gas pressures lower than the combined strength of the rock and its minimum principal stress under external loading *** investigate the mechanism of microscale mode-I ruptures,it is essential to incorporate a multiscale approach that includes subcritical microcracks in the modeling *** this contribution,we derive the model from microstructures that contain periodically distributed microcracks within a porous *** damage evolution law is coupled with the macroscopic poroelastic system by employing the asymptotic homogenization method and considering the inherent hydro-mechanical(HM)anisotropy at the *** resulting permeability change induced by fracture opening is implicitly integrated into the gas flow *** examples are presented to validate the developed model step by *** analysis of local macroscopic response is undertaken to underscore the influence of factors such as strain rate,initial damage,and applied stress,on the gas migration *** examples of direct tension tests are used to demonstrate the model’s efficacy in describing localized failure ***,the simulation results for preferential gas flow reveal the robustness of the two-scale model in explicitly depicting gas-induced fracturing in anisotropic clayey *** model successfully captures the common behaviors observed in laboratory experiments,such as a sudden drop in gas injection pressure,rapid build-up of downstream gas pressure,and steady-state gas flow following gas breakthrough.

关键词： Deep geological repositories Mode-I microcracks Time-dependent damage Fracturing process Anisotropic rock

Designing metal-organic framework fiber network reinforced polymer electrolytes to provide continuous ion transport in solid state lithium metal batteries

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Nano Research 2024年第4期17卷 2719-2727页

作者： Wanqing Fan Ying Huang Meng Yu Kaihang She Jingren Gou Zheng zhang MOE Key Laboratory of Material Physics and Chemistry Under Extraordinary Conditions School of Chemistry and Chemical EngineeringNorthwestern Polytechnical UniversityXi’an 710072China Beijing Key Laboratory of Membrane Materials and Engineering Department of Chemical EngineeringTsinghua UniversityBeijing 100084China

Polyethylene oxide(PEO)-based solid-state electrolytes are considered ideal for electrolyte materials in solid-state lithium metal batteries(SSLMBs).However,practical applications are hindered by the lower conductivity and poor interfacial ***,we propose a strategy to construct a three-dimensional(3D)fiber network of metal-organic frameworks(MOFs).Composite solid electrolytes(CSEs)with continuous ion transport pathways were fabricated by filling a PEO polymer matrix in fibers containing interconnected *** 3D fiber network provides a fast Li+transport path and effectively improves the ionic conductivity(1.36×10^(-4) S·cm^(-1),30℃).In addition,the network of interconnected MOFs not only effectively traps the anions,but also provides sufficient mechanical strength to prevent the growth of Li *** from the advantages of structural design,the CSEs stabilize the Li/electrolyte interface and extend the cycle life of the Li-symmetric cells to 3000 *** assembled SSLMBs exhibit excellent cycling performance at both room and high *** addition,the constructed pouch cells can provide an areal capacity of 0.62 mA·h·cm^(-2),which can still operate under extreme *** work provides a new strategy for the design of CSEs with continuous structure and stable operation of SSLMBs.

关键词： polyethylene oxide(PEO) solid-state lithium metal batteries(SSLMBs) three-dimensional fiber network composite solid electrolytes(CSEs)

Evaluating the tumor stratification with a lysosomal pH sensitive-probe by fluorescence lifetime imaging

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Chinese Chemical Letters 2024年第3期35卷 262-267页

作者： Jun Yan Xing Liang Qian zhang Luolin Wang Weiying Lin Guangxi Key Laboratory of Electrochemical Energy Materials Institute of Optical Materials and Chemical BiologySchool of Chemistry and Chemical EngineeringGuangxi UniversityNanning 530004China

Owing to the anaerobic metabolism in the tumor,abundant acidic metabolites are produced and accumulated in the ***,the cells in different tumor layers are directly linked to the pH ***,due to the lack of robust tools,the high-efficient evaluation of the acidic micro-environment of tumor stratification faces the challenge of accurate *** designed a new pH sensitive fluorescent lifetime probe target to *** we expected,the fluorescence lifetime of PLN possesses a good linear fit to the pH value,which could detect the pH change at a single lysosome level in real time,and then evaluate the different acidity of tumor *** probe PLN is successfully used to evaluate the tumor stratification by fluorescence lifetime imaging microscopy(FLIM)for the first time,which is of great significance in the preoperative diagnosis of clinical tumor treatment or evaluation of drug delivery effect.

关键词： FLIM pH Fluorescence imaging Lysosome Tumor imaging

Flow resistance in the channel-bar landscape of large alluvial rivers

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Frontiers of Earth Science 2024年第2期18卷 412-421页

作者： Yong HU Congcong LIU Jinyun DENG Wei zhang Yitian LI State Key Laboratory of Water Resources and Hydropower Engineering Science Wuhan UniversityWuhan 430072China CCCC Second Harbor Engineering Company Ltd Wuhan 430040China Key Laboratory of Large-span Bridge Construction Technology Wuhan 430040China Research and Development Center of Transport Industry of Intelligent Manufacturing Technologies of Transport Infrastructure Wuhan 430040China CCCC Highway Bridge National Engineering Research Centre Co.Ltd Wuhan 430040China

Accurate approaches for estimating flow resistance in large alluvial rivers are fundamental for simulating discharge,sediment transport,and flood ***,methods for estimating riverbed resistance and additional resistance in the channel-bar landscapes remain poorly *** this study,we used in situ river bathymetry,sediment,and hydraulic data from the Shashi Reach in the Yangtze River to develop a semi-empirical approach for calculating flow *** method quantitatively separates flow resistance into riverbed resistance and additional resistance and shows high accuracy in terms of deviation ratio(~20%),root-mean-square error(~0.008),and geometric standard deviation(~3).Additional resistance plays a dominant role under low-flow conditions but a secondary role under high flows,primarily due to the reduction in momentum exchange in channel-bar regions as discharge *** resistance first decreases and then increases,which might be attributed to bedform changes in the lower and transitional flow regimes as flow velocity ***,our findings further the understanding of dynamic changes in flow resistance in the channel-bar landscapes of large river systems and have important implications for riverine ecology and flood management.

关键词： flow resistance channel-bar landscape interaction region large river bedform

Research Progress in the Fabrication of Covalent Organic Framework Membranes for Chemical Separations

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Chinese Journal of Polymer Science 2024年第2期42卷 141-158,I0005页

作者： Cui-Ting Ding Jin-Qiu Yuan Meng-Ying Xie Qing-Yuan Liu Zeng-Guang Yao Shi-Yu zhang Run-Nan zhang Hong Wu Zhong-Yi Jiang Key Laboratory for Green Chemical Technology of Ministry of Education School of Chemical Engineering and TechnologyTianjin UniversityTianjin300072China Zhejiang Institute of Tianjin University NingboZhejiang315201China Haihe Laboratory of Sustainable Chemical Transformations Tianjin300192China Tianjin Key Laboratory of Membrane Science and Desalination Technology Tianjin UniversityTianjin300072China Joint School of National University of Singapore and Tianjin University International Campus of Tianjin UniversityBinhai New CityFuzhou350207China

Membrane technology has become one of the most promising separation technologies for its energy saving, high separation efficiency, environmental friendliness, and economic feasibility. Covalent organic frameworks(COFs) with intrinsically high porosity, controllable pore size, uniform pore size distribution and long-range ordered channel structure, have emerged as next-generation materials to fabricate advanced separation membranes. This feature article summarizes some latest studies in the development of pure COF membranes in our lab, including their fabrication and applications in chemical separations. Finally, current challenges facing high-performance COF separation membranes are discussed.

关键词： Covalent organic frameworks Covalent organic framework membranes Water treatment Organic solvent nanofiltration Gas separation

Wheat morphological and biochemical responses to copper oxide nanoparticles in two soils

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Pedosphere 2024年第4期34卷 814-825页

作者： Qian YANG Haipeng LI Yuqing zhang Yinghao LIU Helian LI School of Water Conservancy and Environment University of JinanJinan 250022China

The widespread application of copper oxide nanoparticles(CuO NPs)in agricultural production has caused growing concerns about their impact on *** this study,wheat root elongation was used to evaluate the toxic effect concentrations of CuO NPs in two soils with differing properties,collected from farmlands in Guangdong(GD)and Shandong(SD)provinces,*** morphological and biochemical properties were also assessed to explore the toxicity mechanism of CuO NPs on wheat *** root elongation results revealed lower toxic effect concentration values in the plants grown in GD soil than in SD ***,the treatment with CuO NPs at 200 mg Cu kg^(-1) significantly reduced wheat root and shoot biomass by 35.8%and 15.8%,respectively,in GD *** microscopy showed that CuO NPs deformed wheat roots and entered leaf cells,causing deformation and damaging the cell *** CuO NP treatments also decreased chlorophyll content,increased antioxidant enzyme activity,and increased membrane lipid peroxidation in wheat *** addition of CuO NPs significantly reduced the Zn(by 17.3%)and Fe(by 26.9%)contents in the leaves of plants grown in GD and SD soils,***,the contents of Cu,Mg,and Mn were increased by 27.4%–52.5%in GD soil and by 17.9%–71.6%in SD *** results suggested that CuO NPs showed greater toxicity to wheat plants grown in acidic soil than in alkaline soil and that the adverse effects of CuO NP treatments on wheat seedlings were due to a combination of CuO NPs and released Cu^(2+).

关键词： antioxidant enzyme activity chlorophyll content CuO nanoparticles element accumulation membrane lipid peroxidation root elongation toxic effectconcentration

Roof collapse mechanism of weak surrounding rock for deep-buried tunnels under high geostress conditions

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Journal of Mountain Science 2024年第7期21卷 2408-2426页

作者： zhang Qi GUO Xiaokang YAN Zhiguo LEI Zhongdai SHEN Yixin School of Civil Engineering Southeast UniversityNanjing 211189China Department of Geotechnical Engineering Tongji UniversityShanghai 200092China

High geostress,a typical attribute of tunnels located at significant depths,is crucial in causing stress-induced failure and influencing the stability of the tunnel *** study developed an analytical method for the failure mechanism that occurs in deep-buried tunnel roofs,taking into account the influence of *** limit analysis theory was utilized for deriving analytical solutions about the geometry of the collapsing surface and the limit supporting *** collapsing surface obtained by the analytical solution was validated by the findings of the physical model test,which shows a high level of agreement with the actual *** extensive investigation was done to explore the effects of the lateral pressure coefficients,the tunnel buried depth,the geological conditions of the surrounding rock,the long-short axis ratio,and the size of the tunnel *** findings indicate that an increase in the lateral pressure coefficient from 0.5 to 1.5 results in a reduction in the height of the collapsing zone by 2.08 m and the width of the collapsing zone by 1.15 m,while simultaneously increases the limit supporting pressure by 18.9%.The proposed upper bound method accurately determines the limit supporting pressure and the geometry of the collapsing surface,which aligns well with the results acquired through numerical modelling and on-site monitoring in actual engineering *** proposed analytical method can serve as a reference for similar crown failure issues of deep-buried tunnels.

关键词： Geostress Deep-buried tunnels Collapse mechanism Pressure arch Limit analysis HoekBrown criterion