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Fast and Balanced Charge Transport Enabled by Solution-Processed Metal Oxide Layers for Efficient and Stable Inverted Perovskite Solar Cells

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Energy & Environmental Materials 2024年第2期7卷 240-248页

作者： Jing zhang James Mcgettrick Kangyu Ji Jinxin Bi Thomas Webb Xueping Liu Dongtao Liu Aobo Ren Yuren Xiang Bowei Li Vlad Stolojan Trystan Watson Samuel D.Stranks Wei zhang Advanced Technology Institute(ATI) University of SurreyGuildfordSurrey GU27XHUK SPECIFIC College of EngineeringSwansea UniversityBay Campus SA18ENSwansea UK Cavendish Laboratory University of CambridgeJ JThomson AvenueCambridge CB30HEUK Department of Chemical Engineering&Biotechnology University of CambridgePhilippa Fawcett DriveCambridge CB30ASUK

Metal oxide charge transport materials are preferable for realizing long-term stable and potentially low-cost perovskite solar cells(PSCs).However,due to some technical difficulties(e.g.,intricate fabrication protocols,high-temperature heating process,incompatible solvents,etc.),it is still challenging to achieve efficient and reliable all-metal-oxide-based ***,we developed efficient inverted PSCs(IPSCs)based on solution-processed nickel oxide(NiO_(x))and tin oxide(SnO_(2))nanoparticles,working as hole and electron transport materials respectively,enabling a fast and balanced charge transfer for photogenerated charge *** further understanding and optimizing the perovskite/metal oxide interfaces,we have realized an outstanding power conversion efficiency(PCE)of 23.5%(the bandgap of the perovskite is 1.62 eV),which is the highest efficiency among IPSCs based on all-metal-oxide charge transport *** to these stable metal oxides and improved interface properties,ambient stability(retaining 95%of initial PCE after 1 month),thermal stability(retaining 80%of initial PCE after 2 weeks)and light stability(retaining 90%of initial PCE after 1000 hours aging)of resultant devices are enhanced *** addition,owing to the low-temperature fabrication procedures of the entire device,we have obtained a PCE of over 21%for flexible IPSCs with enhanced operational stability.

关键词： fast and balanced charge transfer inverted perovskite solar cells long-term stability low-temperature processing metal oxides

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断控缝洞型碳酸盐岩立式板状油藏注采井网构建

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西南石油大学学报（自然科学版） 2024年第4期46卷 74-84页

作者：邓兴梁张仕帆汪鹏王彭张杰中国石油塔里木油田公司勘探开发研究院新疆库尔勒841000 中国石油天然气集团有限公司超深层复杂油气藏勘探开发技术研发中心新疆库尔勒841000 中国地质大学(武汉)未来技术学院湖北武汉430074

断控缝洞型碳酸盐岩油藏缝洞结构和连通关系复杂,传统井网部署易产生低产能井,需构建立体注采井网以提高产能。通过油藏数值模拟研究了不同因素对塔里木富满油田满深3和满深4井区立体注采井网波及系数的影响,并设计了先导试验方案预测... 详细信息

断控缝洞型碳酸盐岩油藏缝洞结构和连通关系复杂,传统井网部署易产生低产能井,需构建立体注采井网以提高产能。通过油藏数值模拟研究了不同因素对塔里木富满油田满深3和满深4井区立体注采井网波及系数的影响,并设计了先导试验方案预测产能。结果表明,满深3井区注气井与采油井单个交错排状分布时波及系数最大;采油井纵向深度越大,波及系数越大;平面注采井距在500~1000m波及系数相对稳定,井距增至1500m时,波及系数大幅度减小。满深4井区注气井、注水井与采油井单个交错排状分布时波及系数最大。先导试验中,满深3和满深4井区分别采取“浅部注N_(2),深部采油”和“顶部注N_(2),底部注水,中部采油”的井网构建方案,阶段末采出程度分别达到21.3%与22.4%,相比于基础衰竭式开发和注水开发方案有了显著提升。

关键词：富满油田断控缝洞型油藏碳酸盐岩立体注采井网井网构建波及系数

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Cobalt-nanoparticle catalysts derived from zeolitic imidazolate framework@MXene composites for efficient oxidative self-coupling of benzylamines

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Frontiers of Chemical Science and Engineering 2024年第1期18卷 95-106页

作者： Jie Chen Mingyuan Jian Deqiong Xie Kecan Dou Deli Chen Weidong Zhu Fumin zhang Key Laboratory of the Ministry of Education for Advanced Catalysis Materials Institute of Physical ChemistryZhejiang Normal UniversityJinhua 321004China

In this study,we synthesize a catalyst comprising cobalt nanoparticles supported on MXene by pyrolyzing a composite in a N2 ***,the composite comprises a bimetallic Zn/Co zeolitic imidazole framework grown in situ on the outer surface of *** catalytic efficiency of the catalyst is tested for the self-coupling of 4-methoxybenzylamine to produce value-added imine,where atmospheric oxygen(1 atm)is used as the *** on the results,the catalyst displayed impressive catalytic activity,achieving 95.4%yield of the desired imine at 383 K for 8 ***,the catalyst showed recyclability and tolerance toward benzylamine substrates with various functional *** outstanding performance of the catalyst is primarily attributed to the synergetic catalytic effect between the cobalt nanoparticles and MXene support,while also benefiting from the three-dimensional porous ***,a preliminary investigation of potential reaction mechanisms is conducted.

关键词： MXene sacrificial template oxidative self-coupling Co nanoparticles imine

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Experimental and numerical analyses of the effect of fibre content on the close-in blast performance of a UHPFRC beam

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Defence Technology（防务技术） 2024年第1期31卷 242-261页

作者： Junbo Yan Qiyue zhang Yan Liu yingliang Xu Zhenqing Shi Fan Bai Fenglei Huang State Key Laboratory of Explosion Science and Technology Beijing Institute of TechnologyBeijing 100081China Beijing Institute of Technology Chongqing Innovation Center Chongqing 401120China

Limited research has been conducted on the influences of fiber content on close-in blasting characteristics for ultrahigh-performance fiber-reinforced concrete(UHPFRC)*** paper aims to address this knowledge gap through experimental and mesoscale numerical *** were conducted on ten UHPFRC beams built with varying steel fiber volumetric fractions subjected to close-in explosive ***,this study considered other parameters,such as the longitudinal reinforcement type and *** the case of UHPFRC beams featuring normal-strength longitudinal reinforcement of diametersΦ12,Φ16,andΦ20,a reduction in maximum displacement by magnitudes of19.6%,19.5%,and 17.4%was observed,respectively,as the volumetric fractions of fiber increased from1.0%to 2.5%.In addition,increasing the longitudinal reinforcement ratio and using high-strength steel longitudinal reinforcement both significantly reduced the deformation characteristics and increase the blasting resistances of UHPFRC ***,the effects on the local crushing and spalling damage were not significant.A mesoscale finite element model,which considers the impacts of fiber parameters on UHPFRC beam behaviors,was also established and well correlated with the test ***,parametric analyses were further conducted to examine the impacts of the steel fiber content and length and the hybrid effects of various types of microfibers and steel fibers on the blasting performance of UHPFRC beams.

关键词： Blast performance Close-in blast Fiber content Mesoscale approach UHPFRC beams

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Identification of Fusarium wilt resistance gene SiRLK1 in Sesamum indicum L.

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The Crop Journal 2024年第1期12卷 252-261页

作者： yinghui Duan Wenwen Qu Shuxian Chang Ming Ju Cuiying Wang Cong Mu Hengchun Cao Guiting Li Qiuzhen Tian Qin Ma Zhanyou zhang Haiyang zhang Hongmei Miao The Shennong Laboratory Zhengzhou 450002HenanChina Henan Sesame Research Center Henan Academy of Agricultural SciencesZhengzhou 450002HenanChina Key Laboratory of Specific Oilseed Crops Genomics of Henan Province Henan Sesame Research CenterHenan Academy of Agricultural SciencesZhengzhou 450002HenanChina

Sesame Fusarium wilt(SFW),caused by Fusarium oxysporum ***(Fos),is one of the most devastating diseases affecting sesame *** the genetic control of SFW resistance is pivotal for effective disease management in *** inheritance study on a cross between the highly resistant variety Yuzhi 11 and the highly susceptible accession Sp1 using a Fos pathogenicity group 1 isolate indicated that resistance was conferred by a single dominant *** target locus was located in a 1.24 Mb interval on chromosome 3 using a combination of cross-population association mapping and bulked segregant *** genetic mapping further narrowed the interval between 21,350 and 21,401 *** locus Sindi_0812400 was identified as the SFW resistance gene and officially designated *** gene encodes a specific malectin/receptor-like protein kinase with three putative tandem kinase domains and is considered a kinase fusion *** analysis revealed that a high proportion(49.44%)of variants within the locus was located within the kinase domainⅢ,and several of which were evidently associated with the diversity in SFW response,indicating the critical role of kinase domainⅢin expression of disease *** findings provide valuable information for further functional analysis of SFW resistance genes and marker-assisted resistance breeding in sesame.

关键词： Breeding for resistance Genetic analysis Molecular analysis Tandem kinase domain

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大庆市蝶类多样性及其影响因素

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草业科学 2024年第4期41卷 845-855页

作者：袁改霞张大川张国发殷亚杰张奕婷李玥徐太海大庆师范学院生物工程学院黑龙江大庆163712 温州市洞头区气象局温州市台风监测预报技术重点实验室浙江温州325700

为明确大庆市蝶类多样性及其影响因素,2016-2019年利用样线法对大庆市不同生境类型中的蝴蝶开展了调查研究。共观测到蝴蝶5780只,隶属6科29属36种。灰蝶科的个体数最多,蛱蝶科的物种数最多,是当地的优势类群;凤蝶科仅1种,是当地的稀有... 详细信息

为明确大庆市蝶类多样性及其影响因素,2016-2019年利用样线法对大庆市不同生境类型中的蝴蝶开展了调查研究。共观测到蝴蝶5780只,隶属6科29属36种。灰蝶科的个体数最多,蛱蝶科的物种数最多,是当地的优势类群;凤蝶科仅1种,是当地的稀有类群。优势种7个,常见种5个,少见种4个,稀有种20个。不同的生境蝶类群落种类与数量存在一定的差异,人为干扰小、植物群落结构最为复杂的新华草原蝶类的属数和种数最多,而人为干扰较强、植物群落单一的大庆龙凤湿地自然保护区最少;新华草原的蝶类多样性指数最高,大庆龙凤湿地自然保护区最低;新华草原的丰富度指数最高,乘风湖岸边最低。蝶类物种数、个体数、多样性指数及丰富度指数月度变化基本一致,且与月均温显著正相关(P<0.05),而与月降水量无相关性。综上,蝶类多样性与植被类型、月均温有明显的相关性。而相同气象条件下,植被类型是影响蝶类分布的重要因素。为了保护与丰富蝶类资源,建议植被单一的区域,进行适度的植被异质化建设。

关键词：蝴蝶多样性指数人为干扰气象因子月动态丰富度指数数量特征

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Insight into structural degradation of NCMs under extreme fast charging process

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Rare Metals 2024年第1期43卷 41-50页

作者： Yu Tang Xing-Yu Wang Jin-Can Ren Bo-Wen Chen Zhi-Yong Huang Wei Wang Ya-Lan Huang Bing-Hao zhang Si Lan zhang-Long He Qi Liu Hao He Department of Physics City University of Hong KongHong Kong 999077China Shenzhen Research Institute City University of Hong KongShenzhen 518057China College of Materials Science and Engineering Changsha University of Science&TechnologyChangsha 410114China

Lithium-ion batteries(LIBs)with extreme fast charging(XFC)capability are considered an effective way to alleviate range anxiety for electric vehicle(EV)*** to the high ionic and electronic conductivity of LiNi_(x)Co_(y)Mn_zO_(2)(x+y+z=1,NCM)cathodes,the inevitable Li plating of graphite in NCM|graphite cell is usually identified as a key bottleneck for XFC ***,the capacity decay mechanism of cathode materials under XFC has not been fully *** this work,three typical NCM cathode materials with different Ni fractions were chosen and their electrochemical performances under XFC associated with structural evolution were investigated.A faster capacity decay of NCMs under XFC conditions is observed,especially for Ni-rich ***-situ X-ray diffraction(XRD)reveals that the multiple caxis parameters appear at the high-voltage regions in Nirich NCMs,which is probably triggered by the larger obstruction of Li(de)***,NCMs with moderate Ni fraction also present a similar trend under XFC *** phenomenon is more detrimental to the structural and morphological stability,resulting in a faster capacity decay than that under low current *** work provides new insight into the degradation mechanism of NCMs under XFC conditions,which can promote the development of NCM cathode materials with XFC capability.

关键词： Lithium-ion batteries Ni fraction Extreme fast charging Structural evolution

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Allelic reprogramming of chromatin states in human early embryos

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National Science Review 2024年第03期11卷 58-71页

作者： Shenli Yuan Lei Gao Wenrong Tao Jianhong Zhan Gang Lu Jingye zhang Chuanxin zhang Lizhi Yi Zhenbo Liu Zhenzhen Hou Min Dai Han Zhao Zi-Jiang Chen Jiang Liu Keliang Wu Center for Reproductive Medicine Shandong University CAS Key Laboratory of Genome Sciences and Information Collaborative Innovation Center of Genetics and Development Beijing Institute of Genomicsand China National Center for BioinformationChinese Academy of Sciences University of Chinese Academy of Sciences CUHK-SDU Joint Laboratory on Reproductive Genetics School of Biomedical Sciences the Chinese University of Hong Kong Key Laboratory of Reproductive Endocrinology of the Ministry of Education Shandong University Center for Reproductive Medicine Ren Ji Hospital School of Medicine Shanghai Jiao Tong University CAS Center for Excellence in Animal Evolution and Genetics Chinese Academy of Sciences

The reprogramming of parental epigenomes in human early embryos remains elusive. To what extent the characteristics of parental epigenomes are conserved between humans and mice is currently unknown. Here,we mapped parental haploid epigenomes using human parthenogenetic and androgenetic embryos. Human embryos have a larger portion of genome with parentally specific epigenetic states than mouse *** allelic patterns of epigenetic states for orthologous regions are not conserved between humans and mice. Nevertheless, it is conserved that maternal DNA methylation and paternal H3K27me3 are associated with the repression of two alleles in humans and mice. In addition, for DNA-methylation-dependent imprinting, we report 19 novel imprinted genes and their associated germline differentially methylated regions. Unlike in mice, H3K27me3-dependent imprinting is not observed in human early ***, allele-specific epigenomic reprogramming is different in humans and mice.

关键词： human embryo epigenetics reprogramming DNA methylation H3K27me3 chromatin accessibility

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Novel wood-plastic composite fabricated via modified steel slag:Preparation,mechanical and flammability properties

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International Journal of Minerals,Metallurgy and Materials 2024年第9期31卷 2110-2120页

作者： Ling Zhao Kai Zhao Zhenwei Shen Yifan Wang Xiaojie Xia Hao zhang Hongming Long School of Metallurgical Engineering Anhui University of TechnologyMa’anshan 243032China School of Civil Engineering and Architecture Anhui University of TechnologyMa’anshan 243032China School of Materials Science and Engineering Anhui University of TechnologyMa’anshan 243032China Key Laboratory of Metallurgical Emission Reduction and Resources Recycling(Anhui University of Technology) Ministry of EducationMa’anshan 243002China

A novel method was developed to enhance the utilization rate of steel slag(SS).Through treatment of SS with phosphoric acid and aminopropyl triethoxysilane(KH550),we obtained modified SS(MSS),which was used to prepare MSS/wood-plastic composites(MSS/WPCs)by replacing talcum powder(TP).The composites were fabricated through melting blending and hot *** mechanical and combustion properties,which comprise heat release,smoke release,and thermal stability,were systematically *** can improve the mechanical strength of the composites through grafting reactions between wood powder and ***,MSS/WPC#50(16wt%MSS)with an MSS-to-TP mass ratio of 1:1 exhibited optimal comprehensive *** with those of WPC#0 without MSS,the tensile,flexural,and impact strengths of MSS/WPC#50 were increased by 18.5%,12.8%,and 18.0%,***,the MSS/WPC#50 sample achieved the highest limited oxygen index of 22.5%,the highest vertical burning rating at the V-1 level,and the lowest horizontal burning rate at 44.2 mm/*** formation of a dense and stable char layer led to improved thermal stability and a considerable reduction in heat and smoke releases of MSS/WPC#***,the partial replacement of TP with MSS slightly compromised the mechanical and flame-retardant properties,possibly due to the weak grafting caused by SS powder *** findings suggest the suitability of MSS/WPCs for high-value-added applications as decorative panels indoors or outdoors.

关键词： modified steel slag wood–plastic composites preparation method mechanical property flame retardant

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Superior piezoelectric performance with high operating temperature in bismuth ferrite-based ternary ceramics

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Journal of Materials Science & Technology 2024年第2期169卷 172-181页

作者： Yunyao Huang Leiyang zhang Ruiyi Jing Yang Yang Vladimir Shur Xiaoyong Wei Li Jin Electronic Materials Research Laboratory Key Laboratory of the Ministry of EducationSchool of Electronic Science and EngineeringXi’an Jiaotong UniversityXi’an 710049China Faculty of Materials and Manufacturing Key Laboratory of Advanced Functional MaterialsEducation Ministry of ChinaBeijing University of TechnologyBeijing 100124China School of Natural Sciences and Mathematics Ural Federal UniversityEkaterinburg620000Russia

Due to the thermal depolarization effect,adequate piezoelectric performance with high operating temperature is regarded to be challenging to accomplish concurrently in piezoceramics for applications in specific piezoelectric *** this work,we synthesized(0.8−x)BiFeO_(3)-x PbTi_(3)-0.2Ba(Zr_(0.25)Ti_(0.75))O_(3)(abbreviated as BFO-x PT-BZT)ternary solid solutions with 0.15≤x≤0.30 by conventional solid-state reaction *** MPB composition with a coexisting state of rhombohedral-tetragonal phases exhibits enhanced electromechanical properties,including Curie temperature of 380℃,large-signal equivalent piezoelectric coefficient d^(∗)_(33)of 395 pm V^(-1),small-signal piezoelectric coefficient d_(33)of 302 pC N^(-1),and electromechanical coupling factor k_(p)of 50.2%,which is comparable to commercial PZT-5A ceramics,indicating potential in high-temperature ***,in-situ X-ray diffraction(XRD)and piezoelectric force microscopic(PFM)techniques demonstrate that multiphase coexistence and complex nanodomains promote piezoelectric response via *** x=0.24 composition exhibits the highest in-situ d_(33)of 577 pC N^(-1)and good temperature stability in 30−280℃,indicating that BZT-modified BFO-PT ceramics are promising candidates for high-temperature piezoelectric devices.

关键词： High-temperature piezoelectrics Morphotropic phase boundary In-situ technique Domain structure BFO

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