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Multifunctional MOF@COF Nanoparticles Mediated Perovskite Films Management Toward Sustainable Perovskite Solar Cells

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Nano-Micro Letters 2024年第9期16卷 195-208页

作者： Yayu Dong Jian zhang hongyu zhang Wei Wang Boyuan Hu Debin Xia Kaifeng Lin Lin Geng Yulin Yang MIIT Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage School of Chemistry and Chemical EngineeringHarbin Institute of TechnologyHarbin 150001HeilongjiangPeople’s Republic of China School of Materials Science and Engineering East China Jiaotong UniversityNanchang 330013JiangxiPeople’s Republic of China School of Materials Science and Engineering Harbin Institute of TechnologyHarbin 150001HeilongjiangPeople’s Republic of China

Although covalent organic frameworks(COFs)with highπ-conjugation have recently exhibited great prospects in perovskite solar cells(PSCs),their further application in PSCs is still hindered by face-to-face stacking and aggregation ***,metal-organic framework(MOF-808)is selected as an ideal platform for the in situ homogeneous growth of a COF to construct a core-shell MOF@COF nanoparticle,which could effectively inhibit COF stacking and *** synergistic intrinsic mechanisms induced by the MOF@COF nanoparticles for reinforcing intrinsic stability and mitigating lead leakage in PSCs have been *** complementary utilization ofπ-conjugated skeletons and nanopores could optimize the crystallization of large-grained perovskite films and eliminate *** resulting PSCs achieve an impressive power conversion efficiency of 23.61%with superior open circuit voltage(1.20 V)and maintained approximately 90%of the original power conversion efficiency after 2000 h(30-50%RH and 25-30℃).Benefiting from the synergistic effects of the in situ chemical fixation and adsorption abilities of the MOF@COF nanoparticles,the amount of lead leakage from unpackaged PSCs soaked in water(<5 ppm)satisfies the laboratory assessment required for the Resource Conservation and Recovery Act Regulation.

关键词： Perovskite solar cells Covalent organic frameworks Metal-organic frameworks Lead leakage Stability

Identification and functional verification of Y-chromosome-specific gene typo-gyf in Bactrocera dorsalis

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Insect Science 2024年第4期31卷 1270-1284页

作者： Peipei Liu Shuning Yu Wenping Zheng Qiuyuan zhang Jiao Qiao Ziniu Li Zhurong Deng hongyu zhang National Key Laboratory for Germplasm Innovation and Utilization for Fruit and Vegetable Horticultural Crops Hubei Hongshan LaboratoryChina-Australia Joint Research Centre for Horticultural and Urban PestsInstitute of Urban and Horticultural EntomologyCollege of Plant Science and TechnologyHuazhong Agricultural UniversityWuhanChina

Genes on the Y chromosome play important roles in male sex determination and *** identification of Y-chromosome-specific genes not only provides a theoretical basis for the study of male reproductive development,but also offers genetic control targets for agricultural ***,Y-chromosome genes are rarely characterized due to their high repeatability and high heterochromatinization,especially in the oriental fruit *** this study,1011 Y-chromosome-specific candidate sequences were screened from 2 to 4 h Bactrocera dorsalis embryo datasets with the chromosome quotient method,6 of which were identified as Y-chromosome-specific sequences by polymerase chain reaction,including typo-gyf,a 19126-bp DNA sequence containing a 575-amino acid open reading *** deformation and a significant reduction in sperm number were observed after typo-gyf knockdown with RNA interference in *** typo-gyf knockout with clustered regularly interspaced palindromic repeats(CRISPR)/CRISPR-associated protein 9 in the embryonic stage,the sex ratio of the emergent adults was unbalanced,with far more females than males.A genotype analysis of these females with the Y-chromosome gene MoY revealed no sex ***-gyf knockout led to the death of XY individuals in the embryonic *** conclude that typo-gyf is an essential gene for male survival,and is also involved in testicular development and *** identification of typo-gyf and its functional verification provide insight into the roles of Y-chromosome genes in male development.

关键词： Bactrocera dorsalis spermatogenesis testis typo-gyf gene Y-specific gene

Potential impact of specific therapy on pregnant women with pulmonary arterial hypertension without cardiac shunt:a descriptive study in northern China

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Emergency and Critical Care Medicine 2024年第2期4卷 60-66页

作者： Weida Lu Min Li Fuqing Ji Hua Feng Guo Li Qiushang Ji hongyu zhang Xiaopei Cui Department of Geriatric Medicine&Shandong Key Laboratory Cardiovascular Proteomics Qilu Hospital of Shandong UniversityJinanShandongChina Intensive Care Unit of Cardiac Surgery Shandong Provincial Qianfoshan Hospitalthe First Hospital Affiliated with Shandong First Medical UniversityAffiliated Hospital of Shandong UniversityJinanShandongChina Department of Cardiology Linyi Central HospitalLinyiShandongChina Department of Gastroenterology Shandong Provincial Hospital Affiliated to Shandong First Medical UniversityJinanShandongChina Department of Pulmonary and Critical Care Medicine the Affiliated Hospital of Qingdao UniversityQingdaoShandongChina Department of Cardiology Qilu Hospital of Shandong UniversityJinanShandongChina

Background:Pregnancy in women with pulmonary arterial hypertension(PAH)is a fatal condition,despite the effectiveness of PAH-specific *** coverage status and effect of specific therapies in pregnant patients with PAH without cardiac shunts in China remain *** investigate this issue,we conducted a multicenter retrospective study in northern ***:The study included 85 patients who were admitted to 4 clinical centers in Shandong Province between October 2010 and August *** endpoint events included(1)maternal death and/or(2)major adverse cardiac events,both occurring during pregnancy or within 6 weeks ***:Although the overall mortality rate was encouraging(11.8%),the number of patients receiving PAH-specific therapies was extremely low(28.2%).Moreover,only 15.3%of patients received adequate duration of PAH-specific therapy(≥4 weeks)before delivery,and this subgroup showed the lowest major adverse cardiac events rate(7.7%)compared with that in the untreated(19.7%)and short-time treated groups(<4 weeks;54.5%).Conclusion:Pregnant patients with PAH without cardiac shunts face significantly increased mortality ***-term PAH-specific therapy does not guarantee favorable maternal *** screening,early identification,and timely intervention are expected to improve maternal outcomes in pregnant women with PAH.

关键词： Major adverse cardiac events Maternal mortality Pregnancy outcome Pulmonary arterial hypertension Specific therapy

The haplotype-resolved genome assembly of autotetraploid rhubarb Rheum officinale provides insights into its genome evolution and massive accumulation of anthraquinones

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Plant Communications 2024年第1期5卷 196-214页

作者： hongyu zhang Qiang He Longsheng Xing Ruyu Wang Yu Wang Yu Liu Qinghong Zhou Xuanzhao Li Zheng Jia Ze Liu Yuqing Miao Tao Lin Wei Li Huilong Du School of Life Sciences Institute of Life Sciences and Green DevelopmentBasic Science Center for Biotic Interaction in HebeiHebei UniversityBaoding 071000China College of Horticulture China Agricultural UniversityNo.2 Yuanmingyuan West RoadHaidian DistrictBeijing 100193China

Rheum officinale,a member of the Polygonaceae family,is an important medicinal plant that is widely used in traditional Chinese ***,we report a 7.68-Gb chromosome-scale assembly of *** with a contig N50 of 3.47 Mb,which was clustered into 44 chromosomes across four homologous *** genomics analysis revealed that transposable elements have made a significant contribution to its genome evolution,gene copy number variation,and gene regulation and expression,particularly of genes involved in metabolite biosynthesis,stress resistance,and root *** placed the recent autotetraploidization of *** at~0.58 mya and analyzed the genomic features of its homol-ogous *** no dominant monoploid genomes were observed at the overall expression level,numerous allele-differentially-expressed genes were identified,mainly with different transposable element insertions in their regulatory regions,suggesting that they functionally diverged after *** genomics,transcriptomics,and metabolomics,we explored the contributions of gene family amplification and tetraploidization to the abundant anthraquinone production of ***,as well as gene expression patterns and differences in anthraquinone content among *** report of-fers unprecedented genomic resources for fundamental research on the autopolyploid herb *** and guidance for polyploid breeding of herbs.

关键词： Rheum officinale genomics comparative genomics polyploid anthraquinone biosynthesis

交互主体性视阈下中国叙事传播的形塑——基于我国外宣译释知识体系构建的考察

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河南大学学报（社会科学版） 2024年第2期64卷 130-135,156页

作者：张宏雨张滟上海海事大学外国语学院上海201306

中国叙事语际传播是一种持之恒久的文化传播方式。目前它正从“译介世界”向兼具“译介中国”的交互向度转型,中译外逐年增加,“中语”深度西传,但仍存在理论构建的历史觉悟与系统性不足、理论话语的文化自我主体性意识内力不敷等问题... 详细信息

中国叙事语际传播是一种持之恒久的文化传播方式。目前它正从“译介世界”向兼具“译介中国”的交互向度转型,中译外逐年增加,“中语”深度西传,但仍存在理论构建的历史觉悟与系统性不足、理论话语的文化自我主体性意识内力不敷等问题。沿波讨源,深耕民族传统资源,强化中国外宣译释自主知识体系构建的战略意识,强调方法意识上中国价值深层格融的方法自觉、概念意识上以概念自觉为主导的概念自信、文献意识上写出文献应用的自信深度等,构筑体现开放包容的外宣译释话语及其学术阐释的体制与模式,为中国文化的译介与传播提供理论力量。

关键词：中国叙事语际传播外宣译释主体性自主知识体系

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基于特征增稳的混合固态激光雷达目标检测

汽车工程 2024年第6期46卷 1015-1024页

作者：金立生张洪瑜郭柏苍燕山大学车辆与能源学院秦皇岛066004 燕山大学起重机械关键技术全国重点实验室秦皇岛066004 燕山大学河北省特种运载装备重点实验室秦皇岛066004

稳定的点云特征提取对激光雷达三维目标检测至关重要。针对现有深度学习算法仅能处理机械旋转式激光雷达点云数据,而对混合固态激光雷达数据支持不足的问题,本文基于IA-SSD搭建了适用于混合固态激光雷达的目标检测模型。首先,在点云编... 详细信息

稳定的点云特征提取对激光雷达三维目标检测至关重要。针对现有深度学习算法仅能处理机械旋转式激光雷达点云数据,而对混合固态激光雷达数据支持不足的问题,本文基于IA-SSD搭建了适用于混合固态激光雷达的目标检测模型。首先,在点云编码前端添加了Cloth Simulation Filtering(CSF)用于地面次优点过滤;其次,利用局部特征融合和全局双线性正则化层组成的注意力机制,从局部和全局共同推动点云几何信息与特征信息融合;再次,利用GhostGConv替换原有低效的逐点卷积,通过通道混洗机制加强点云的特征交互,构建了增强型特征提取网络。最后,在点检测器IA-SSD中整合了上述模块完成模型构建。在混合固态激光雷达数据集SimoSet开展的验证结果表明,所提出的方法显著优于SimoSet数据集支持的其他算法精度指标;在KITTI数据集中等难度检测中,所提方法将IA-SSD三分类平均检测精度分别提升了1.17、1.47、0.5百分点。

关键词：车辆工程环境感知目标检测混合固态激光雷达特征增稳

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润滑水凝胶涂层研究进展

清华大学学报（自然科学版） 2024年第3期64卷 381-392页

作者：郭伟成廖元太张洪玉清华大学高端装备界面科学与技术全国重点实验室北京100084

随着医学技术进步,对医用材料在生物相容性和功能性方面的要求也日益提高。作为一种新型表面修饰技术,润滑水凝胶涂层近年来受到广泛关注。该文旨在从水凝胶润滑原理、水凝胶润滑改性方式和水凝胶涂层的修饰方法3方面综述润滑水凝胶涂... 详细信息

随着医学技术进步,对医用材料在生物相容性和功能性方面的要求也日益提高。作为一种新型表面修饰技术,润滑水凝胶涂层近年来受到广泛关注。该文旨在从水凝胶润滑原理、水凝胶润滑改性方式和水凝胶涂层的修饰方法3方面综述润滑水凝胶涂层的相关研究。首先,从关节软骨的润滑机理出发,引出水凝胶润滑原理相关研究;其次,基于已有润滑理论,介绍了几类典型的水凝胶润滑改性方式,并详细阐述了现有几种水凝胶涂层的修饰方法,为设计水凝胶涂层提供参考;最后,对润滑水凝胶涂层的研究进行总结与展望。

关键词：水凝胶涂层润滑改性修饰方法

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直接接触式膜蒸馏结晶回收沼液氨氮性能

农业工程学报 2024年第5期40卷 239-245页

作者：张军张鸿宇周婷晏水平贺清尧华中农业大学工学院武汉430070 农业农村部长江中下游农业装备重点实验室武汉430070

为解决现有沼液氨氮膜回收技术中氮肥浓度低和副产物价值低的问题,该研究提出采用膜蒸馏结晶技术实现沼液中氨氮的结晶回收。研究中,通过提升近饱和接收液的温度来平衡膜两侧的水蒸气分压,在保证氨氮传质通量的情况下最小化水分传质。... 详细信息

为解决现有沼液氨氮膜回收技术中氮肥浓度低和副产物价值低的问题,该研究提出采用膜蒸馏结晶技术实现沼液中氨氮的结晶回收。研究中,通过提升近饱和接收液的温度来平衡膜两侧的水蒸气分压,在保证氨氮传质通量的情况下最小化水分传质。操作结束后接收液中铵盐达到超饱和状态,冷却至常温即可回收铵盐晶体。结果表明,当进料侧沼液温度为40℃时,近饱和磷酸二氢铵温度需提高至47℃,而使用硫酸为吸收剂时,近饱和硫酸铵溶液温度需提高至65℃。酸液温度升高对氨通量也有促进作用,氨通量由40℃时的10.70 g/(m^(2)·h)小幅提升至70℃时的14.90 g/(m^(2)·h)。进料侧氨氮质量浓度的提升可显著增加氨氮回收通量。磷酸二氢铵为吸收剂时,试验6 h后晶体中的氨氮回收率为77.60%,采用硫酸为吸收剂时可提高至92.20%。继续延长处理时间,晶体中的氨氮回收率甚至超过100%。显然,采用膜蒸馏结晶技术回收沼液氨氮具一定的可行性,研究结果可为沼液氨氮的高价值回收提供一定参考。

关键词：沼液结晶膜蒸馏水分传质高价值回收

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全站仪自动目标识别测定真北方位角

导航定位学报 2024年第5期12卷 164-170页

作者：张宏宇许皓瑞河南理工大学测绘与国土信息工程学院河南焦作454000

为了进一步提升导弹预设阵地建设、航空航天器发射、陀螺仪标校等领域中真北方位测定的精度和准确度,提出一种真北方位角测定方法:通过研究多种真北方位角测定方法,在分析现有方法特点及测量精度的基础上,提出并实现一种利用具备自动目... 详细信息

为了进一步提升导弹预设阵地建设、航空航天器发射、陀螺仪标校等领域中真北方位测定的精度和准确度,提出一种真北方位角测定方法:通过研究多种真北方位角测定方法,在分析现有方法特点及测量精度的基础上,提出并实现一种利用具备自动目标识别(ATR)功能的全站仪来实现真北方位角测量的方法;并运用2种方法对所测得的4个真北方位角的精度及准确度进行分析。实验结果表明,不符值绝对值最大为0.38″,对于短边真北方位角其真实准确度可以做到优于±0.5″,能够证明其可行性及准确性,为确定方位基准的外符精度提供参考。

关键词：真北方位自动目标识别(ATR) 全站仪天文方位角精度分析