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Ground-state mass of ^(22)Al and test of state-of-the-art ab initio calculations

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Chinese Physics C 2024年第3期48卷 72-78页

作者：孙铭泽于越王新鹏王猛李健国张玉虎 K.Blaum 陈祖毅陈瑞九邓涵宇付超义葛文文黄文嘉焦红扬李红蕙李宏福罗胤芳廖挺 YuALitvinov 司敏帅鹏史金阳王茜邢元明徐星徐瑚珊许甫荣袁琪 T.Yamaguchi 颜鑫亮杨建成原有进周小红周旭张敏曾奇 CAS Key Laboratory of High Precision Nuclear Spectroscopy Institute of Modern PhysicsChinese Academy of SciencesLanzhou 730000China School of Nuclear Science and Technology University of Chinese Academy of SciencesBeijing 100049China Max-Planck-Institut für Kernphysik Saupfercheckweg 169117 HeidelbergGermany GSI Helmholtzzentrum für Schwerionenforschung Planckstraße 164291 DarmstadtGermany Advanced Energy Science and Technology Guangdong Laboratory Huizhou516007China State Key Laboratory of Nuclear Physics and Technology School of PhysicsPeking UniversityBeijing 100871China Department of Physics Saitama UniversitySaitama 338-8570Japan School of Nuclear Science and Engineering East China University of TechnologyNanchang 330013China

The ground-state mass excess of the T_(z)=−2 drip-line nucleus ^(22)Al is measured for the first time as 18103(10)keV using the newly-developed Bρ-defined isochronous mass spectrometry method at the cooler storage ring in *** new mass excess value allowed us to determine the excitation energies of the two low-lying 1+states in ^(22)Al with significantly reduced uncertainties of 51 *** compared to the analogue states in its mirror nucleus ^(22)F,the mirror energy differences of the two 1^(+)states in the ^(22)Al-^(22)F mirror pair are determined to be−625(51)keV and−330(51)*** excitation energies and mirror energy differences are used to test the state-of-the-art ab initio valence-space in-medium similarity renormalization group calculations with four sets of interactions derived from the chiral effective field *** mechanism leading to the large mirror energy differences is investigated and attributed to the occupation of theπs_(1/2) orbital.

关键词： nuclear mass Bρ-defined IMS mirror energy difference ab initio VS-IMSRG calculations chiral interactions

Hot deformation behavior and microstructure evolution of GH3536-TiB_(2) composites fabricated by powder metallurgy

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Science China(Technological Sciences) 2024年第7期67卷 2107-2124页

作者： zHOU ShiPeng wang Shuai HUANG LuJun zHANG Rui CHEN xin MENG FanChao CHEN Run SUN FengBo wang CunYu GENG Lin School of Materials Science and Engineering Harbin Institute of TechnologyHarbin 150001China Waikato Centre for Advanced Materials and Manufacturing School of EngineeringUniversity of WaikatoHamilton 3240New Zealand State Key Laboratory of Advanced Welding and Joining Harbin Institute of TechnologyHarbin 150001China

The hot deformation behavior and microstructure evolution of GH3536-TiB2composites fabricated by powder metallurgy(PM)were examined in the temperature range of 950–1150℃ and strain rate range of 0.001–1 s^(-1). The hot compression stress-strain curves and the constitutive equation were obtained. In addition, the hot processing map was drawn, which indicated that the appropriate hot working window was 950–1050℃/0.001–0.1 s^(-1)and 1050–1100℃/0.001–0.01 s^(-1). The microstructure analysis showed that the splitting and spheroidization of M3B2led to a decrease in size and volume fraction at 950–1100℃. At 1150℃,the eutectic microstructure of M_(3)B_(2)+ γ was formed due to the dissolution of M_(3)B_(2), which caused macroscopic cracking of the deformed sample. Additionally, the deformation temperature and the strain rate had little effect on the size and volume fraction of M_(3)B_(2). Besides, discontinuous dynamic recrystallization(DDRx) and continuous dynamic recrystallization(CDRx) were found in the deformed microstructure, while the former was dominant. Within the test range of this work, the dynamic recrystallization(DRx) fraction of the deformed composites was high due to the bulging nucleation of numerous interfaces. The DRx grain size increased with increasing deformation temperature or decreasing strain rate. Texture analysis showed that the deformation texture of //compression direction RD existed in the matrix when the deformation temperature was below 1100℃, and the texture type became //RD at 1100℃. Additionally, it was also found that the //RD texture was formed in M3B2under the strain rates of 0.1 and 0.01 s^(-1).

关键词： GH3536 alloy matrix composites powder metallurgy hot deformation behavior microstructure evolution

Enhancing electrolyte ion diffusion via direct ink writing pillar array structure of graphene electrodes for high-performance microsupercapacitors

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Nano Research 2024年第7期17卷 6203-6211页

作者： Yan zhang Huandi zhang xiaoxiao wang Cheng Tang xiaowei Shi zehua zhao Jiamei Liu Guolong wang Jianfeng Shen Lei Li State Key Laboratory for Mechanical Behavior of Materials School of Materials Science and EngineeringXi’an Jiaotong University28 Xianning West RoadXi’an 710049China Center for Materials Chemistry Frontier Institute of Science and TechnologyXi’an Jiaotong UniversityXi’an 710049China Instrument Analysis Center of xi'an Jiaotong University Xi’an Jiaotong University28 Xianning West RoadXi’an 710049China Institute of special materials and technology Fudan UniversityShanghai 200433China

The graphene-based microsupercapacitors(MSCs)suffer from graphene aggregation issue in *** reduces the electrolyte ions transportation in the electrodes to degrade the charge storage ability of MSCs,hampering their practical *** the electrolyte ions transportation in the electrodes can boost the charge storage ability of ***,we design and experimentally realize pillar array structure of graphene electrodes for MSCs by direct ink writing *** graphene electrodes with pillar array structure increase the contact area with electrolyte and short the electrolyte ions transport path,facilitating electrolyte ions transport in *** MSCs exhibit high areal capacitance of 25.67 mF·cm^(−2),high areal energy density of 20.54μWh·cm^(−2),and high power density of 1.45 mW·cm^(−2).One single MSCs can power timer for 10 min and pressure sensor more than 160 min,showing high practical application *** work provides a new avenue for developing high performance MSCs.

关键词： microsupercapacitors pillar array structure direct ink writing areal energy density ion transport

Boosted photocatalytic removal of NO using direct z-scheme UiO-66-NH_(2)/Bi_(2)MoO_(6) nanoflowers heterojunction:mechanism insight and humidity effect

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Rare Metals 2024年第8期43卷 3758-3770页

作者： Jiang-Yu-Shan Liang Hai-Tao Ren Abdelkader Labidi Qiu-Hui zhu Qi-Bing Dong Ahmed A.Allam Ahmed Rady Chuan-Yi wang School of Environmental Science and Engineering Shaanxi University of Science and TechnologyXi'an 710021China zoology Department Faculty of ScienceBeni-Suef UniversityBeni-Suef 6251lEgypt Department of zoology College of ScienceKing Saud University11451 RiyadhSaudi Arabia

In practical applications,relative humidity in the air is a key factor affecting the photocatalytic removal of NO,which is often overlooked in previous ***,we developed a direct z-scheme UiO-66-NH_(2)/Bi_(2)MoO_(6)heterojunction with a nanoflower-like structure to systematically investigate the effect of relative humidity on photocatalytic removal of *** optimized heterojunction for the removal efficiency of NO was 71.6%at1.07 mg·m^(-3)NO concentration(relative humidity=10%),and the generation of NO_(2) was only 1.1%.Interestingly,with the increase in relative humidity,it showed a higher inhibition effect on NO_(2),while the removal of NO decreased slightly(8%),which might be attributed to the affinity effect of NO_(2) with water molecules and the competitive adsorption of H_(2)O and NO on the surface of the heterojunction ***,the reaction pathways of NO removal at the developed heterojunctions were revealed by in situ DRIFTS *** work provides a novel vision for the development of direct z-scheme heterojunction photocatalysts to effectively remove NO and inhibit the formation of toxic intermediate NO_(2) under different humidities.

关键词： NO removal Relative humidity Direct z-scheme Bismuth molybdate Visible-light photocatalysis

A ratiometric fluorescent probe for hypoxanthine detection in aquatic products based on the enzyme mimics and fluorescence of cobalt-doped carbon nitride

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Food Science and Human Wellness 2024年第2期13卷 879-884页

作者： xin wang Chengyi Hong zhengzhong Lin zhiyong Huang College of Ocean Food and Biological Engineering Jimei UniversityXiamen 361021China

A ratiometric fluorescent probe for hypoxanthine(Hx)detection was established based on the mimic enzyme and fluorescence characteristics of cobalt-doped graphite-phase carbon nitride(Co doped g-C_(3)N_(4)).In addition to emitting strong fluorescence,the peroxidase activity of Co doped g-C_(3)N_(4)can catalyze the reaction of O-phenylenediamine and H_(2)O_(2)to produce diallyl phthalate which can emit yellow fluorescence at 570 *** the decomposition of Hx by xanthine oxidase,Hx can be indirectly detected by the generating hydrogen peroxide based on the measurement of fluorescent ratio I(F_(570)/F_(370)).The linear range was 1.7-272.2 mg/kg(R^(2)=0.997),and the detection limit was 1.52 mg/kg(3σ/K,n=9).The established method was applied to Hx detection in bass,grass carp,and shrimp,and the data were verified by *** result shows that the established probe is sensitive,accurate,and reliable,and can be used for Hx detection in aquatic products.

关键词： Co doped g-C_(3)N_(4) Ratiometric fluorescent probe Hypoxanthine Freshness Aquatic products

Outage Analysis of Optimal UAV Cooperation with IRS via Energy Harvesting Enhancement Assisted Computational Offloading

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Computer Modeling in Engineering & Sciences 2024年第2期138卷 1885-1905页

作者： Baofeng Ji Ying wang Weixing wang Shahid Mumtaz Charalampos Tsimenidis School of Information Engineering Henan University of Science and TechnologyLuoyang471000China Research and Innovation Center of Intelligent System Longmen LaboratoryLuoyang471000China State Key Laboratory of Complex Electromagnetic Environment Effects on Electronics and Information System(CEMEE) Luoyang471000China Sustainable Digital Communications and Energy Systems(DIGCOM)Group Nottingham Trent UniversityNottinghamUK

The utilization of mobile edge computing(MEC)for unmanned aerial vehicle(UAV)communication presents a viable solution for achieving high reliability and low latency *** study explores the potential of employing intelligent reflective surfaces(IRS)andUAVs as relay nodes to efficiently offload user computing tasks to theMEC server system ***,the user node accesses the primary user spectrum,while adhering to the constraint of satisfying the primary user peak interference ***,the UAV acquires energy without interrupting the primary user’s regular communication by employing two energy harvesting schemes,namely time switching(TS)and power splitting(PS).The selection of the optimal UAV is based on the maximization of the instantaneous signal-to-noise ***,the analytical expression for the outage probability of the system in Rayleigh channels is derived and *** study investigates the impact of various system parameters,including the number of UAVs,peak interference power,TS,and PS factors,on the system’s outage performance through *** proposed system is also compared to two conventional benchmark schemes:the optimal UAV link transmission and the IRS link *** simulation results validate the theoretical derivation and demonstrate the superiority of the proposed scheme over the benchmark schemes.

关键词： Unmanned aerial vehicle(UAV) intelligent reflective surface(IRS) energy harvesting computational offloading outage probability

Quantitative geochemical reconstruction of Eocene paleoenvironment in Fushun Basin,northeast China

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Acta Geochimica 2024年第3期43卷 571-587页

作者： Yuanji Li Pingchang Sun Qiang zhang Junxian wang Department of Safety Engineering Heilongjiang University of Science and TechnologyHarbin 150022China National Professional Center Lab of Safety Basic Research for Hydrocarbon Gas Pipeline Transportation Network Harbin 150022China College of Earth Sciences Jilin UniversityChangchun 130061JilinChina Beijing Research Institute of Uranium Geology Beijing 100029China

The quantitative estimation of key parameters of paleotemperature and paleoprecipitation is crucial for paleoclimate *** data from mod-ern sediments are highly consistent with climate data,and their relationship can provide an important reference for the quantitative reconstruction of the *** this study,detailed inorganic geochemical analysis was carried out using high-precision sampling of the Paleogene(LFD-1 well)Guchengzi,Jijuntun and xiloutian Formations in the Fushun Basin located in the mid-latitudes of the Northern *** Eocene Guchengzi Formation(54.51–47.8 Ma)and Jijuntun Formation(47.8–41.2 Ma)in the Fushun Basin were found to have been deposited under a humid *** lower(41.2–40.1 Ma)and upper(40.1–37.8 Ma)parts of the xiloutian Formation were character-ized by semiarid and semihumid–semiarid climates,respec-tively,which is very similar to the paleoclimatic information reflected by organic carbon *** Eocene Thermal Maximum 2(ETM2,~53.7 Ma),Early Eocene Climatic Optimum(EECO,~53.1–46.5 Ma),Eocene Thermal Maxi-mum 3(ETM 3,~52.8 Ma),and Middle Eocene Climatic Optimum(MECO,~40.7–40.1 Ma)events significantly enhanced chemical weathering during these *** rapid increase in pCO_(2)concentration leads to an increase in temperature,precipitation,and surface runoff,exhibiting strong chemical *** mean annual temperature(MATa)and mean annual precipitation(MAPa,MAPb,and MAPc)were estimated using parameters,such as the corrosion index without potassium(CIA-K),CaO/Al_(2)O_(3),and(Na_(2)O+K_(2)O)/Al_(2)O_(3).Comparing MAPa,MAPb,and MAPc with the MAP estimated using pollen data,MAPa and MAPb were found to be more sensitive to the climate during high precipitation periods(precipitation>1000 mm,Guchengzi Formation),and the recovered average precipi-tation was similar to *** contrast,MAPc was more sensitive to the climate during low precipitation periods(precipitationxilouti

关键词： Eocene Fushun Basin Major element Paleoclimate Geochemical reconstruction

Rational Design of Plasmonic Nanoparticle-Molecule Complexes for Chirality Sensing

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Chinese Journal of Chemistry 2024年第8期42卷 903-919页

作者： Chen wang Dandan Lu Lichao Sun Qingfeng zhang College of Chemistry and Molecular Sciences Wuhan UniversityWuhanHubei430072 China

Comprehensive Summary,Sensing the chirality of molecules is of great importance to fields such as enantioselective synthesis,pharmaceutical industry,and *** nanoparticles are ideal candidates for molecular sensing due to their inherent plasmonic properties that significantly enhance their sensitivity to surrounding *** plasmonic nanoparticle-molecule complexes for chirality sensing has drawn enormous attention in recent years due to their intriguing properties and potential ***,in this review,we believe it is timely to circumnavigate the rational design of plasmonic nanoparticle-molecule complexes and widen the scope of their emerging applications in chirality ***,we present different fundamental mechanisms for plasmon-based chirality that are built on the system of plasmonic nanoparticle-molecule ***,we review the typical applications of plasmonic nanoparticle-molecule complexes in chirality ***,we discuss the emerging biomedical applications that the plasmon-based chirality has attracted enormous ***,we provide an outlook on the challenges and opportunities in the field of plasmonic approaches for chirality sensing.

关键词： Chirality Surface plasmon resonance Nanoparticles Chiral molecules Chirality sensing

Area Operators on Bergman Spaces

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Acta Mathematica Sinica,English Series 2024年第5期40卷 1161-1176页

作者： xiao Fen LV Jordi PAU Mao Fa wang Department of Mathematics Huzhou UniversityHuzhou 313000P.R.China Departament de Matemàtiques i Informàtica Universitat de Barcelona08007 BarcelonaCataloniaSpain School of Mathematics and Statistics Wuhan UniversityWuhan 430072P.R.China

We completely characterize the boundedness of area operators from the Bergman spaces A_(α)^(p)(Bn)to the Lebesgue spaces L^(q)(S_(n))for all 0 详细信息

We completely characterize the boundedness of area operators from the Bergman spaces A_(α)^(p)(Bn)to the Lebesgue spaces L^(q)(S_(n))for all 0z.:Volterra operator,area integral and Carleson measures,*** Math.,54,2487–2500(2011)].Especially,in the case qzations for the area operators to be *** solve the cases left open there and extend the results to n-complex dimension.

关键词： Area operator Bergman space tent space area formula