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Construction of 2D/2D Ti_(3)C_(2)T_(x)MXene/CdS heterojunction with photothermal effect for efficient photocatalytic hydrogen production

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Journal of Materials Science & Technology 2024年第4期171卷 1-9页

作者： T.y.Huang z.y.ng S.y.yang z.H.Dai y.J.Liu J.H.Liao G.y.zhong z.J.Xie y.P.Fang S.S.zhang Key Laboratory for Biobased Materials and Energy of Ministry of Education Guangdong Laboratory for Lingnan Modern AgricultureCollege of Materials and EnergySouth China Agricultural UniversityGuangzhou 510643China School of Physics and Optoelectronics South China University of TechnologyGuangzhou 510640China School of Chemical Engineering and Energy Technology Guangdong Provincial Key Laboratory of Distributed Energy SystemsDongguan University of TechnologyDongguan 523808China

The insensitivity of semiconductors to visible and infrared light is a key constraint on the utilization of light energy in photocatalytic *** photocatalysts with full-spectrum absorption through surface engineering is an effective approach to fully harnessing light energy in semiconductor ***,a novel stable Ti_(3)C_(2)T_(x)MXene/CdS heterojunction catalyst is obtained by in-situ epitaxial growth of two-dimensional(2D)CdS nanosheets on 2D MXene interface via a solvothermal *** exceptional light absorption properties of MXene confer outstanding full-spectrum driven photocat-alytic hydrogen evolution capability upon the heterogeneous *** unique 2D/2D structure effectively mitigated the recombination of photogenerated carriers,enhancing the photocatalytic performance of the ***,the composite catalyst exhibits a significantly higher surface temperature of 80.4℃under visible light irradiation at an intensity of 0.1 W/cm^(2),which is 1.84 times higher than that of *** irradiation of visible and near infrared light,the composite catalyst with photothermal ef-fect demonstrates a remarkable hydrogen evolution rate of 65.4 mmol g^(-1)h^(-1),which is 7.2 times higher than that of CdS *** study introduces a novel approach for constructing full-spectrum absorption catalysts and expands the application of the photothermal effect in photocatalytic hydrogen evolution research.

关键词： Two-dimensional structure Heterostructure Photothermal effect Photocatalyst Hydrogen evolution

Precipitation of multi-type nano-quasicrystals in a Mg-zn-y alloy

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Journal of Magnesium and Alloys 2024年第3期12卷 997-1008页

作者： W.z.Wang X.z.zhou L.F.zhang H.Q.ye z.Q.yang Shenyang National Laboratory for Materials Science Institute of Metal ResearchChinese Academy of ScienceShenyang 110016China Ji Hua Laboratory Foshan 528251China Foshan University Foshan 528231China

Mg-6zn-1y(at.%)ribbons with strengthening precipitates of multi-type nanoquasicrystals were prepared by melt-spinning followed by aging *** evolution of the rapidly solidified ribbons during isothermal aging was comprehensively studied using various electron microscopy *** new kinds of decagonal quasicrystals were formed in aged ribbons,in addition to precipitation of nanometer icosahedral ***-resolution observations reveal that both decagonal quasicrystals can be modeled by quasiperiodic tiling with decagonal clusters of 2.5 nm in diameter,but overlap of neighboring clusters in both decagonal quasicrystals is different from the Gummelt model observed in other quasicrystals.A shell composed of complex Laves Mg-zn domains was formed surrounding each decagonal quasicrystal precipitate upon prolonged *** addition,all kinds of nanoprecipitates exhibit excellent structure and size stability at 573 *** findings may have implications for not only fundamental studies about quasicrystals,but also microstructural manipulation of high-performance Mg alloys.

关键词： Quasicrystal Mg alloys Rapid solidification Scanning-transmission electron microscopy.

Rational design of AgGaS/znS/znS quantum dots with a near-unity photoluminescence quantum yield via double shelling scheme

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Journal of Materials Science & Technology 2024年第2期169卷 235-242页

作者： H.X.Lu H.Liu z.z.Fu y.y.Chen H.Q.Dai z.Hu W.L.zhang R.Q.Guo Institute for Electric Light Sources School of Information Science and TechnologyFudan UniversityShanghai 200433China Institute of Future Lighting Academy for Engineering and TechnologyFudan UniversityShanghai 200433China yiwu Research Institute of Fudan University YiwuZhejiang 322000China zhongshan-Fudan Joint Innovation Center Zhongshan 528437China

In this study,a two-step method was used to synthesize highly luminescent AgGaS/znS/znS quantum dots(QDs).In the first step,an inner znS shell was formed via a one-pot method,which resulted in a smaller lattice mismatch between the AgGaS core and the outer znS shell,thereby facilitating the formation of a thick outer *** the two-step shelling process,the synthesized AgGaS/znS/znS QDs showed an excellent photoluminescence quantum yield(PLQy)of 96.4%with a peak wavelength of 508 nm,repre-senting the highest PLQy reported thus far for AgGaS ***,the effect of halogen ions in zn precursors on the shelling process was *** was proposed that the capacity of halogen ions to coordinate with the QDs influenced the balance between zn cation diffusion and znS shelling ***,the znS shelling reaction was dominant when znCl_(2)was employed,while zn cation diffusion was the dominant process under the I^(−)-rich *** work provides insights into the interfacial restructuring during the znS shelling and offers a clear map for the tailored synthesis of core/shell QDs.

关键词： AgGaS Quantum dots Photoluminescence Core/shell Alloyed core/shell interface

Distinct Electrical and Mechanical Responses of a Cu-10Fe Composite Prepared by Hot-Pressed Sintering and Post Treatment

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Acta Metallurgica Sinica(English Letters) 2024年第2期37卷 255-265页

作者： X.y.yue S.y.Peng X.zhang C.N.He y.z.Tian Key Laboratory for Anisotropy and Texture of Materials(Ministry of Education) School of Materials Science and EngineeringNortheastern UniversityShenyang110819China School of Materials Science and Engineering and Tianjin Key Laboratory of Composite and Functional Materials Tianjin UniversityTianjin300350China Research Centre for Metallic Wires Northeastern UniversityShenyang110819China

A Cu-10wt%Fe composite was prepared through hot-pressed sintering,and the material was subsequently solution *** hot-pressed sintered and solution treated materials were rolled and *** precipitation behavior and performance changes were systematically studied by using scanning electron microscopy and transmission electron *** contrast to the hot-pressed sintered specimen,the solution treatment significantly affects the thermal stability and properties of the Cu-10wt%Fe *** Cu-10wt%Fe composite was prepared after solid solution,cold rolling and aging at 773 K for 1 h,and it obtained excellent tensile strength of 494 MPa,uniform elongation of 16.3%,electrical conductivity of 51.1%IACS and softening temperature of 838 *** for the distinct difference in thermal stability and properties between hot-pressed sintered and solution treated specimens were *** findings provide a theoretical basis for designing high-performance Cu-based in-situ composites by post treatment.

关键词： Cu-Fe composite Hot-pressed sintering Thermal stability Strength Electrical conductivity

Quantification of CO2 Emissions from Three Power Plants in China Using OCO-3 Satellite Measurements

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Advances in Atmospheric Sciences 2024年第11期41卷 2276-2288页

作者： yang y. zhou M. Wang W. Ning z. zhang F. Wang P. College of Data Science Jiaxing University Jiaxing 314000 China LAGEO Institute of Atmospheric Physics Chinese Academy of Sciences Beijing 100029 China Shanghai Ecological Forecasting and Remote Sensing Center Shanghai 200030 China CNRC Institute of Atmospheric Physics Chinese Academy of Sciences Beijing 100029 China Key Laboratory of Atmospheric Environment and Extreme Meteorology Institute of Atmospheric Physics Chinese Academy of Sciences Beijing 100029 China Department of Atmospheric and Oceanic Sciences / Institute of Atmospheric Sciences Fudan University Shanghai 200082 China

Coal-fired power plants are a major carbon source in China. In order to assess the evaluation of China’s carbon reduction progress with the promise made on the Paris Agreement, it is crucial to monitor the carbon flux intensity from coal-fired power plants. Previous studies have calculated CO2 emissions from point sources based on Orbiting Carbon Observatory-2 and -3 (OCO-2 and OCO-3) satellite measurements, but the factors affecting CO2 flux estimations are uncertain. In this study, we employ a Gaussian Plume Model to estimate CO2 emissions from three power plants in China based on OCO-3 XCO2 measurements. Moreover, flux uncertainties resulting from wind information, background values, satellite CO2 measurements, and atmospheric stability are discussed. This study highlights the CO2 flux uncertainty derived from the satellite measurements. Finally, satellite-based CO2 emission estimates are compared to bottom-up inventories. The satellite-based CO2 emission estimates at the Tuoketuo and Nongliushi power plants are ∼30 and ∼10 kt d−1 smaller than the Open-Data Inventory for Anthropogenic Carbon dioxide (ODIAC) respectively, but ∼10 kt d−1 larger than the ODIAC at Baotou. © Institute of Atmospheric Physics/Chinese Academy of Sciences, and Science Press 2024.

关键词： CO2 emission Gaussian Plume Model OCO-3 power plant

Multi-population particle swarm optimization algorithm for automatic design of steel frames

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Frontiers of Structural and Civil Engineering 2024年第1期18卷 89-103页

作者： Wenchen SHAN Jiepeng LIU yao DING y.Frank CHEN Junwen zhou Institute of Smart City and Intelligent Transportation Southwest Jiaotong UniversityChengdu 610000China School of Civil Engineering Chongqing UniversityChongqing 400045China Department of Civil Engineering the Pennsylvania State UniversityMiddletownPA 17057USA

Steel structures are widely used;however,their traditional design method is a trial-and-error procedure which is neither efficient nor cost ***,a multi-population particle swarm optimization(MPPSO)algorithm is developed to optimize the weight of steel frames according to standard design *** are made to improve the algorithm performances including the constraint-based strategy,piecewise mean learning strategy and multi-population cooperative *** proposed method is tested against the representative frame taken from American standards and against other steel frames matching Chinese design *** related parameter influences on optimization results are *** the representative frame,MPPSO can achieve greater efficiency through reduction of the number of analyses by more than 65% and can obtain frame with the weight for at least 2.4%lighter.A similar trend can also be observed in cases subjected to Chinese design *** addition,a migration interval of 1 and the number of populations as 5 are recommended to obtain better MPPSO *** purpose of the study is to propose a method with high efficiency and robustness that is not confined to structural scales and design *** aims to provide a reference for automatic structural optimization design problems even with dimensional *** proposed method can be easily generalized to the optimization problem of other structural systems.

关键词： steel frame multi-population particle swarm optimization automatic structural optimization design

Four Late-type Galaxies with Double Radio Lobes and Properties of Such Galaxies

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Research in Astronomy and Astrophysics 2024年第4期24卷 84-90页

作者： z.S.yuan X.y.Gao z.L.Wen J.L.Han National Astronomical Observatories Chinese Academy of SciencesBeijing 100101China CAS Key Laboratory of FAST National Astronomical ObservatoriesChinese Academy of SciencesBeijing 100101China School of Astronomy and Space Sciences University of Chinese Academy of SciencesBeijing 100049China

The triggering mechanism for radio lobes from late-type galaxies is not fully *** samples are desired for a thorough investigation and *** utilizing the optical data from the newly released Dark Energy Spectroscopic Instrument imaging surveys and the radio sources from the NRAO VLA Sky Survey and the Faint Images of the Radio Sky at Twenty-centimeter,we identify four Late-type Galaxies with double Radio Lobes(La GRLs):J0217-3645,J0947+6220,J1412+3723 and J1736+*** previously known La GRLs,we confirm the correlation between radio power P_(1.4GHz)and stellar mass M_(*)of host ***(25/35)La GRLs belong to the blue cloud galaxies,while the newly identified cases in this work are located within the region of the red *** find a clear correlation between the differential radio power,i.e.,the offset from the P_(1.4GHz)-M_(*)relation,and the galaxy color,indicating that bluer galaxies at a fixed M_(*)tend to host more powerful radio ***,the majority(31/36)of La GRLs are either located in a galaxy group or displaying a disturbed *** suggest that all of the galaxy mass,color and surrounding environment could play important roles in triggering radio lobes in late-type galaxies.

关键词： galaxies:active galaxies:jets galaxies:spiral radio continuum:galaxies

A New Method for Deriving High-Vertical-Resolution Wind Vector Data from the L-Band Radar Sounding System in China

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Advances in Atmospheric Sciences 2024年第11期41卷 2192-2202页

作者： yuan F. zhou z. Liao J. National Meteorological Information Center China Meteorological Administration Beijing 100081 China

High-vertical-resolution radiosonde wind data are highly valuable for describing the dynamics of the meso- and microscale atmosphere. However, the current algorithm used in China’s L-band radar sounding system for calculating high-vertical-resolution wind vectors excessively smooths the data, resulting in significant underestimation of the calculated kinetic energy of gravity waves compared to similar products from other countries, which greatly limits the effective utilization of the data. To address this issue, this study proposes a novel method to calculate high-vertical-resolution wind vectors that utilizes the elevation angle, azimuth angle, and slant range from L-band radar. In order to obtain wind data with a stable quality, a two-step automatic quality control procedure, including the RMSE-F (root-mean-square error F) test and elemental consistency test are first applied to the slant range data, to eliminate continuous erroneous data caused by unstable signals or radar malfunctions. Then, a wind calculation scheme based on a sliding second-order polynomial fitting is utilized to derive the high-vertical-resolution radiosonde wind vectors. The evaluation results demonstrate that the wind data obtained through the proposed method show a high level of consistency with the high-resolution wind data observed using the Vaisala Global Positioning System and the data observed by the new Beidou Navigation Sounding System. The calculation of the kinetic energy of gravity waves in the recalculated wind data also reaches a level comparable to the Vaisala observations. © Institute of Atmospheric Physics/Chinese Academy of Sciences, and Science Press 2024.

关键词： high-vertical-resolution radiosonde wind vectors L-band radar sounding system polynomial fitting quality control upper air

Structural basis for polyuridine tract recognition by SARS-CoV-2 Nsp15

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Protein & Cell 2024年第7期15卷 547-552页

作者： Fumiaki Ito Hanjing yang z.Hong zhou Xiaojiang S.Chen Molecular and Computational Biology Department of Biological SciencesUniversity of Southern CaliforniaLos AngelesCA 90089United States Department of Microbiology Immunology and Molecular GeneticsUniversity of CaliforniaLos AngelesCA 90095United States California NanoSystems Institute University of CaliforniaLos AngelesCA90095United States Genetic Molecular and Cellular Biology ProgramKeck School of MedicineUniversity of Southern CaliforniaLos AngelesCA 90089United States Norris Comprehensive Cancer Center University of Southern CaliforniaLos AngelesCA 90089United States Center of Excellence in NanoBiophysics University of Southern CaliforniaLos AngelesCA 90089United States

Dear Editor,Coronaviruses have evolved a wide array of tactics to evade host antiviral *** host cells detect invading foreign nucleic acids including viral genome and viral replication intermediates,they activate interferon(IFN)signaling via cytoplasmic pattern recognition receptors(Kang et al.,2002;Kato et al.,2006).Remarkable stealth activities exhibited by coronaviruses are facilitated by a series of non-structural proteins(Nsps),such as Nsp15(Deng and Baker,2018;Deng et al.,2019;Hackbart et al.,2020),which is a uridine-specific endoribonuclease that mediates evasion of host detection of viral double-stranded RNA(dsRNA)(Bhardwaj et al.,2004;Deng et al.,2017;Frazier et al.,2021;Ivanov et al.,2004).Nsp15 targets a polyuridine[poly(U)]tract on the coronavirus negative strand RNA(Hackbart et al.,2020).Nsp15 limits the abundance and length of poly(U)within the negative strand RNA 5ʹ-extension by trimming down the initially synthesized poly(U)lead sequence to the optimal length that can suppress dsRNA formation but still serves as a template for poly(A)tail of the positive strand genome of the coronaviruses(Hofmann and Brian,1991).

关键词： p15 interferon template

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