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The Crop Journal 2024年第1期12卷 102-109页

作者： Gousi li Jingluan Han Chen Yi Hao Luo yuzhu Wang Fengpin Wang Xiaoyu Wang Letian Chen Yaling Zhang State Key Laboratory for Conservation and Utilization of Subtropical Agro-Bioresources College of Life SciencesSouth China Agricultural UniversityGuangzhou 510642GuangdongChina Guangdong Laboratory for lingnan Modern Agriculture Guangzhou 510642GuangdongChina National Key Laboratory of Plant Molecular Genetics Shanghai Center for Plant Stress BiologyCAS Center for Excellence in Molecular Plant SciencesShanghai Institute of Plant Physiology and EcologyChinese Academy of SciencesShanghai 200032China

Plasma membrane intrinsic proteins(PIPs)are conserved plant aquaporins that transport small molecules across the plasma membrane to trigger instant stress responses and maintain cellular homeostasis under biotic and abiotic stress.To elucidate their roles in plant immunity to pathogen attack,we characterized the expression patterns,subcellular localizations,and H_(2)O_(2)-transport ability of 11 OsPIPs in rice(Oryza sativa),and identified OsPIP2;6 as necessary for rice disease resistance.OsPIP2;6 resides on the plasma membrane and facilitates cytoplasmic import of the immune signaling molecule H_(2)O_(2).Knockout of OsPIP2;6 increases rice susceptibility to Magnaporthe oryzae,indicating a positive function in plant immunity.OsPIP2;6 interacts with OsPIP2;2,which has been reported to increase rice resistance to pathogens via H_(2)O_(2)transport.Our findings suggest that OsPIP2;6 cooperates with OsPIP2;2 as a defense signal transporter complex during plant–pathogen interaction.

关键词： Aquaporin Plant immunity Rice blast H_(2)O_(2)transport

Boron promoted Fe^(3+)/peracetic acid process for sulfamethazine degradation:Efficiency,role of boron,and identification of the reactive species

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Journal of Environmental Sciences 2024年第1期135卷 72-85页

作者： Yanhong Zhang Guangbing liu yuzhu Xue lichun Fu Yawei Qian Minhui Hou Xiang li Chen ling Ying Zhang Yuwei Pan Jiangsu Provincial Key Laboratory of Environmental Engineering Jiangsu Provincial Academy of Environmental ScienceNanjing 210036China College of Biology and the Environment Nanjing Forestry UniversityNanjing 210037China School of Iron and Steel Soochow UniversitySuzhou 215000China School of the Environment Nanjing UniversityNanjing 210023China SUMEC Complete Equipment&Engineering Co. LTD.Nanjing 211500China Key Laboratory of Pollution Process and Environmental Criteria Ministry of EducationCollege of Environmental Science and EngineeringNankai UniversityTianjin 300350China School of Environment Key Laboratory for Yellow River and Huai River Water Environmental and Pollution ControlMinistry of EducationHenan Key Laboratory for Environmental Pollution ControlHenan Normal UniversityXinxiang 453007China

In this work,boron(B)was used to promote Fe^(3+)/peracetic acid(Fe^(3+)/PAA)for the degradation of sulfamethazine(SMT).An SMT degradation efficiency of 9.1%was observed in the Fe^(3+)/PAA system over 60 min,which was significantly increased to 99.3%in the B/Fe^(3+)/PAA system over 10 min.The B/Fe^(3+)/PAA process also exhibited superior resistance to natural substances,excellent adaptability to different harmful substances,and good removal of antibiotics in natural fresh water samples.The mechanism of action of boron for Fe^(3+)reduction was determined using scanning electron microscopy(SEM),X-ray photoelectron spectroscopy(XPS),Fourier transform infrared(FT-IR)spectroscopy,density functional theory(DFT)calculations,and electrochemical tests.The dominant role of^(·)OH was confirmed using quenching experiments,electron spin resonance(EPR)spectroscopy,and quantitative tests.Organic radicals(R-O^(·))and Fe(IV)also significantly contribute to the removal of SMT.DFT calculations on the reaction between Fe^(2+)and the PAA were conducted to further determine the contribution from ^(·)OH,R-O^(·),and Fe(IV)from the perspective of thermodynamics and the reaction pathways.Different boron dosages,Fe^(3+)dosages,and initial pH values were also investigated in the B/Fe^(3+)/PAA system to study their effect of SMT removal and the production of the reactive species.Fe(IV)production determined the k_(R-O·+Fe(IV))value suggesting that Fe(IV)may play a more important role than R-O^(·).A comparison of the results with other processes has also proved that the procedure described in this study(B/Fe^(3+)/PAA)is an effective method for the degradation of antibiotics.

关键词： Boron Peracetic acid Sulfamethazine DFT Reactive species

Micelle-directed self-assembly of single-crystal-like mesoporous stoichiometric oxides for high-performance lithium storage

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National Science Review 2024年第4期11卷 195-205页

作者： Yanhua Wan Changyao Wang Xingmiao Zhang Yang Yin Mengmeng liu Bing Ma linlin Duan yuzhu Ma Wei Zhang Changlin Zheng Dongliang Chao Fei Wang Yongyao Xia Wei li Department of Chemistry Laboratory of Advanced Materials Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials State Key Laboratory of Molecular Engineering of Polymers College of Chemistry and Materials ScienceFudan University State Key Laboratory of Surface Physics and Department of Physics Fudan University

Due to their uncontrollable assembly and crystallization process,the synthesis of mesoporous metal oxide single crystals remains a formidable challenge.Herein,we report the synthesis of single-crystal-like mesoporous li2TiSiO5by using soft micelles as templates.The key lies in the atomic-scale self-assembly and step-crystallization processes,which ensure the formation of single-crystal-like mesoporous li2TiSiO5microparticles via an oriented attachment growth mechanism under the confinement of an in-situ formed carbon matrix.The mesoporous li2TiSiO5anode achieves a superior rate capability(148 mAh g-1at5.0 A g-1) and outstanding long-term cycling stability(138 mAh g-1after 3000 cycles at 2.0 A g-1) for lithium storage as a result of the ultrafast li+diffusion caused by penetrating mesochannels and nanosized crystal frameworks（5-10 nm）.In comparison,bulk li2TiSiO5exhibits poor rate capability and cycle performance due to micron-scale diffusion lengths.This method is very simple and reproducible,heralding a new way of designing and synthesizing mesoporous single crystals with controllable frameworks and chemical functionalities.

关键词： mesoporous materials micelles single-crystal-like li2TiSiO5 lithium-ion batteries

Design and experiment of concentrated flexibility-based variable camber morphing wing

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Chinese Journal of Aeronautics 2022年第5期35卷 455-469页

作者： yuzhu li Wenjie GE Jin ZHOU Yonghong ZHANG Donglai ZHAO Zhuo WANG Dianbiao DONG School of Mechanical Engineering Northwestern Polytechnical UniversityXi’an 710072China School of Aeronautic Science and Engineering Beihang UniversityBeijing 100083China

The morphing wing has a significant positive effect on the aerodynamic performance of the aircraft.This paper describes a leading-edge of variable camber wing with concentrated flexibility based on the geared five-bar mechanism.The driving points of morphing skin formed by the glass fibre composite sheet were optimized to make the skin deformation smooth.A geared fivebar kinematic mechanism rigidly connected to the skin was proposed to drive the leading-edge deformation.Besides,a new kind of concentrated flexure hinge was designed using the pseudorigid-body method and applied to the joint between the rigid mechanism and the skin.Finally,the leading-edge prototypes with traditional hinges and flexure hinges were produced,respectively.The feasibility of the concentrated flexibility leading-edge was verified through the comparative experiments of ground deformation.Simultaneously,aerodynamic analysis was carried out to compare the concentrated flexure leading-edge wing with the original airfoil.

关键词： Aircraft Concentrated flexure hinge Leading-edge Morphing wing Pseudo-rigid-body model

Effects of daily light integral on tomato(Solanum lycopersicon L.)grafting and quality in a controlled environment

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International Journal of Agricultural and Biological Engineering 2022年第6期15卷 44-50页

作者： Jinxiu Song Yulong Fan Xingqun li yuzhu li Hanping Mao Zhiyu Zuo Zhirong Zou College of Agricultural Engineering Jiangsu UniversityZhenjiang 212013JiangsuChina Key Laboratory of Modern Agricultural Equipment and Technology Ministry of EducationZhenjiang 212013JiangsuChina College of Horticulture Northwest A&F UniversityYangling 712100ShaanxiChina

As the source of energy and biological signals,light can influence the healing process of grafted seedlings by regulating the synthesis of the endogenous hormone,regeneration of wound-healing tissue,and connection of vascular tissue in grafted seedlings.The effect of daily light integral(Dli)on the healing process and seedling quality of tomato(Solanum lycopersicum L.)was analyzed in this study,with the comparison of grafted seedlings treated in dark for 7 d after grafting.The results showed that the height increment of scion and rootstock,adhesion of graft union,stem flow,total chlorophyll content,and net photosynthesis rate increased gradually with increasing light intensity,and no longer increased significantly when the Dli was higher than 5.04 mol/m^(2)·d.The contents of auxin(IAA)and gibberellin(GA)in tomato leaves increased and abscisic acid(ABA)decreased with the increase of Dli.However,there was no significant difference between the treatments with Dli higher than 6.48 mol/m^(2)·d.Both the biomass and energy use efficiency(EUE)of grafted seedlings increased with Dli in a certain range and then decreased.The biomass was the largest when Dli was 5.04 mol/m^(2)·d.However,EUE was highest when Dli was 7.46 mol/m^(2)·d.In conclusion,a suitable Dli is beneficial to cultivate high-quality grafted tomato seedlings,and increasing Dli within a certain range can promote biomass accumulation,connection of vascular tissue,and endogenous hormone biosynthesis in tomato grafted seedlings during the healing period.The lighting environment with Dli of 5.04 mol/m^(2)·d(light intensity of 100μmol/m^(2)·s and light time of 14 h/d)is recommended for the healing treatment in high-quality production,which also improves EUE during the healing period of tomato grafted seedlings.

关键词： stress resistance endogenous hormones stem flow energy use efficiency seedling index

High-rate metal-free MXene microsupercapacitors on paper substrates

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Carbon Energy 2024年第5期6卷 94-104页

作者： Han Xue Po‐Han Huang Lee‐Lun Lai Yingchun Su Axel Strömberg Gaolong Cao yuzhu Fan Sergiy Khartsev Mats Göthelid Yan‐Ting Sun Jonas Weissenrieder Kristinn BGylfason Frank Niklaus Jiantong li School of Electrical Engineering and Computer Science KTH Royal Institute of TechnologyStockholmSweden School of Engineering Sciences KTH Royal Institute of TechnologyStockholmSweden

MXene is a promising energy storage material for miniaturized microbatteries and microsupercapacitors(MSCs).Despite its superior electrochemical performance,only a few studies have reported MXene-based ultrahigh-rate(>1000 mV s^(−1))on-paper MSCs,mainly due to the reduced electrical conductance of MXene films deposited on paper.Herein,ultrahigh-rate metal-free on-paper MSCs based on heterogeneous MXene/poly(3,4-ethylenedioxythiophene)-poly(styrenesulfonate)(PEDOT:PSS)-stack electrodes are fabricated through the combination of direct ink writing and femtosecond laser scribing.With a footprint area of only 20 mm^(2),the on-paper MSCs exhibit excellent high-rate capacitive behavior with an areal capacitance of 5.7 mF cm^(−2)and long cycle life(>95%capacitance retention after 10,000 cycles)at a high scan rate of 1000 mV s^(−1),outperforming most of the present on-paper MSCs.Furthermore,the heterogeneous MXene/PEDOT:PSS electrodes can interconnect individual MSCs into metal-free on-paper MSC arrays,which can also be simultaneously charged/discharged at 1000 mV s^(−1),showing scalable capacitive performance.The heterogeneous MXene/PEDOT:PSS stacks are a promising electrode structure for on-paper MSCs to serve as ultrafast miniaturized energy storage components for emerging paper electronics.

关键词： direct ink writing femtosecond laser scribing MXene on-paper microsupercapacitors PEDOT:PSS ultrahigh rate capability

Facile synthesis of the Mn_(3)O_(4)polyhedron grown on N-doped honeycomb carbon as high-performance negative material for lithium-ion batteries

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International Journal of Minerals,Metallurgy and Materials 2023年第6期30卷 1152-1161页

作者： Dan Zhang Chunyan Zhang Xuan Zheng Yizhuo Zhao Xinyu Shi Baomin Luo yuzhu li Guangyin liu Xiaodi liu Chuang Yu College of Chemistry and Pharmaceutical Engineering Nanyang Normal UniversityNanyang 473061China State Key Laboratory of Advanced Electromagnetic Engineering and Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074China

Because of their large volume variation and inferior electrical conductivity,Mn_(3)O_(4)-based oxide anode materials have short cyclic lives and poor rate capability,which obstructs their development.In this study,we successfully prepared a Mn_(3)O_(4)/N-doped honeycomb carbon composite using a smart and facile synthetic method.The Mn_(3)O_(4)nanopolyhedra are grown on N-doped honeycomb carbon,which evidently mitigates the volume change in the charging and discharging processes but also improves the electrochemical reaction kinetics.More importantly,the Mn-O-C bond in the Mn_(3)O_(4)/N-doped honeycomb carbon composite benefits electrochemical reversibility.These features of the Mn_(3)O_(4)/N-doped honeycomb carbon(NHC)composite are responsible for its superior electrochemical performance.When used for li-ion batteries,the Mn_(3)O_(4)/N-doped honeycomb carbon anode exhibits a high reversible capacity of 598 mAh·g^(−1)after 350 cycles at 1 A·g^(−1).Even at 2 A·g^(−1),the Mn_(3)O_(4)/NHC anode still delivers a high capacity of 472 mAh·g^(−1).This work provides a new prospect for synthesizing and developing manganese-based oxide materials for energy storage.

关键词： Mn_(3)O_(4) polyhedron nitrogen-doped honeycomb carbon anode lithium-ion battery

Highly Efficient Aligned Ion‑Conducting Network and Interface Chemistries for Depolarized All‑Solid‑State lithium Metal Batteries

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Nano-Micro Letters 2024年第5期16卷 102-119页

作者： Yongbiao Mu Shixiang Yu yuzhu Chen Youqi Chu Buke Wu Qing Zhang Binbin Guo lingfeng Zou Ruijie Zhang Fenghua Yu Meisheng Han Meng lin Jinglei Yang Jiaming Bai lin Zeng Shenzhen Key Laboratory of Advanced Energy Storage Southern University of Science and TechnologyShenzhen 518055People’s Republic of China Department of Mechanical and Energy Engineering Southern University of Science and TechnologyShenzhen 518055People’s Republic of China SUSTech Energy Institute for Carbon Neutrality Southern University of Science and TechnologyShenzhen 518055People’s Republic of China Department of Mechanical and Aerospace Engineering Hong Kong University of Science and TechnologyKowloon 997077Hong Kong Special Administrative Region of ChinaPeople’s Republic of China HKUST Shenzhen-Hong Kong Collaborative Innovation Research Institute FutianShenzhenPeople’s Republic of China

Improving the long-term cycling stability and energy density of all-solid-state lithium(li)-metal batteries(ASSLMBs)at room temperature is a severe challenge because of the notorious solid–solid interfacial contact loss and sluggish ion transport.Solid electrolytes are generally studied as two-dimensional(2D)structures with planar interfaces,showing limited interfacial contact and further resulting in unstable li/electrolyte and cathode/electrolyte interfaces.Herein,three-dimensional(3D)architecturally designed composite solid electrolytes are developed with independently controlled structural factors using 3D printing processing and post-curing treatment.Multiple-type electrolyte films with vertical-aligned micro-pillar(p-3DSE)and spiral(s-3DSE)structures are rationally designed and developed,which can be employed for both li metal anode and cathode in terms of accelerating the li+transport within electrodes and reinforcing the interfacial adhesion.The printed p-3DSE delivers robust long-term cycle life of up to 2600 cycles and a high critical current density of 1.92 mA cm^(−2).The optimized electrolyte structure could lead to ASSLMBs with a superior full-cell areal capacity of 2.75 mAh cm^(−2)(LFP)and 3.92 mAh cm^(−2)(NCM811).This unique design provides enhancements for both anode and cathode electrodes,thereby alleviating interfacial degradation induced by dendrite growth and contact loss.The approach in this study opens a new design strategy for advanced composite solid polymer electrolytes in ASSLMBs operating under high rates/capacities and room temperature.

关键词： All-solid-state lithium metal batteries Composite solid electrolyte 3D printing Areal capacity Interfacial degradation

Clinical characteristics and north-south differences of inflammatory bowel disease in China: A cross-sectional study and meta-analysis

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Frigid Zone Medicine 2024年第1期4卷 23-30页

作者： Qi liang Bo Qu Chunye li Yue Hu Chunyi Yang Tingting Yang yuzhu Di Hui li Harbin Medical University Harbin 150086China Digestive Department the 2nd Affiliated Hospital of Harbin Medical UniversityHarbin 150086China Huangshi Hospital of Traditional Chinese Medicine Huangshi 435000China

Objective:This study aimed to estimate the incidence rate and clinical characteristics of inflammatory bowel disease(IBD)in the Chinese population,specially comparing the North and South regions.Methods:We designed a questionnaire survey for patients diagnosed with IBD and conducted a systematic literature search in PubMed,China National Knowledge Internet,and Wanfang digital database,covering studies published between 2012 and 2022.Meta-analysis was performed to determine the overall incidence rate and prevalence of clinical manifestations of Crohn's disease(CD)and ulcerative colitis(UC)in China's Mainland.Clinical phenotypes and demographic characteristics were calculated with 95%confidence intervals(CI).A comparison between the northern and southern regions was also conducted.Results:The questionnaire survey included 440 patients,and 64 publications were included for Meta-analysis.The overall incidence rates of IBD,CD,and UC were 1.36(95%CI:0.79-2.33)per 100,000 person-years,0.23(95%CI:0.09-0.58)per 100,000 person-years,and 1.12(95%CI:0.69-1.80)per 100,000 person-years,respectively.The incidence rates of IBD,CD,and UC were all higher in southern China compared to the North.Clinical characteristics of 440 IBD patients from the questionnaire and 2,821 CD patients and 12,809 UC patients from the literature were analyzed.There were more male patients compared to female patients.CD cases in the North exhibited earlier disease diagnosis(Plizations rates(P<0.01)compared to the South.UC cases in the North had higher severity(P<0.01),anemia rates(P<0.01),and weight loss(P<0.01)compared to the South.Conclusions:The incidence rates of IBD,CD,and UC were higher in southern China than in the North.Northern patients exhibited more severe symptoms compared to their southern counterparts.

关键词： inflammatory bowel disease Crohn's disease ulcerative colitis epidemiology clinical characteristics

Deep learning-enabled virtual histological staining of biological samples

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light(Science & Applications) 2023年第3期12卷 335-354页

作者： Bijie Bai Xilin Yang yuzhu li Yijie Zhang Nir Pillar Aydogan Ozcan Electrical and Computer Engineering Department University of CaliforniaLos AngelesCA 90095USA Bioengineering Department University of CaliforniaLos Angeles 90095USA California NanoSystems Institute(CNSi) University of CaliforniaLos AngelesCAUSA

Histological staining is the gold standard for tissue examination in clinical pathology and life-science research,which visualizes the tissue and cellular structures using chromatic dyes or fluorescence labels to aid the microscopic assessment of tissue.However,the current histological staining workflow requires tedious sample preparation steps,specialized laboratory infrastructure,and trained histotechnologists,making it expensive,time-consuming,and not accessible in resource-limited settings.Deep learning techniques created new opportunities to revolutionize staining methods by digitally generating histological stains using trained neural networks,providing rapid,cost-effective,and accurate alternatives to standard chemical staining methods.These techniques,broadly referred to as virtual staining,were extensively explored by multiple research groups and demonstrated to be successful in generating various types of histological stains from label-free microscopic images of unstained samples;similar approaches were also used for transforming images of an already stained tissue sample into another type of stain,performing virtual stain-to-stain transformations.In this Review,we provide a comprehensive overview of the recent research advances in deep learning-enabled virtual histological staining techniques.The basic concepts and the typical workflow of virtual staining are introduced,followed by a discussion of representative works and their technical innovations.We also share our perspectives on the future of this emerging field,aiming to inspire readers from diverse scientifc fields to further expand the scope of deep learning-enabled virtual histological staining techniques and their applications.

关键词： Deep generating consuming