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Nano Research 2024年第6期17卷 4994-5001页

作者： Xitong Ren Jiajie Sun yusen li Feng Bai Key Laboratory for Special Functional Materials of Ministry of Education National and Local Joint Engineering Research Center for High-Efficiency Display and Lighting TechnologySchool of Materials Science and Engineeringand Collaborative Innovation Center of Nano Functional Materials and ApplicationsHenan UniversityKaifeng 475004China School of Physics and Electronics Henan UniversityKaifeng 475004China

The combination of donor-acceptor(D-A)structures presents a viable strategy for fabricating covalent organic frameworks(COFs)with exceptional photocatalytic ***,the selection of functional groups on donor or acceptor building blocks and their effect on the macroscopic properties of COFs are *** this study,we tactfully synthesized a pair of Py-DBT-COFs from the same pyrene(Py)donor and 4,7-diphenylbenzo[c][1,2,5]thiadiazole(DBT)acceptor cores with distinct primitive functional *** primitive functional groups of building units determine the photocatalytic properties of corresponding ***,Py-C-DBT-COF synthesized from Py-4CHO and DBT-2NH_(2)showcases a splendid H_(2)evolution rate as high as 21,377.7μmol/(g·h)(with 5 wt.%Pt)originating from better charge transfer capacity,which is significantly superior to that of Py-N-DBT-COF constructed from Py-4NH_(2)and *** distinct photocatalytic performances of the two COFs are demonstrated to originate from the different charge separation and transfer *** work supplies a new avenue for optimizing the photocatalytic performance of D-A COFs from the perspective of primitive functional group selections.

关键词： covalent organic frameworks functional group donor-acceptor photocatalysis

An Overview on the Composition and Age of Upper Crust of Proto-Tethyan Lajishan Intra-oceanic Arc,NE Tibet Plateau

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Acta Geologica Sinica(English Edition) 2024年第2期98卷 285-302页

作者： FU Changlei HE Xiaohu YAN Zhen Jonathan CAITCHISON XIAO Wenjiao WANG Bingzhang li Wufu li yusen SinoProbe Laboratory Institute of GeologyChinese Academy of Geological SciencesBeijing 100037China Key Laboratory of the Northern Qinghai–Tibet Plateau Geological Processes and Mineral Resources Qinghai Geological Survey InstituteXining 810012China Department of Geology School of Earth SciencesYunnan UniversityKunming 650091China School of Earth and Environmental Sciences University of QueenslandBrisbane 4072Australia Xinjiang Institute of Ecology and Geography Chinese Academy of SciencesUrumqi 830011China State Key Laboratory of lithospheric Evolution Institute of Geology and GeophysicsChinese Academy of SciencesBeijing 100029China School of Earth Science and Resources China University of GeosciencesBeijing 100083China

Identification and anatomy of oceanic arcs within ancient orogenic belt are significant for better understanding the tectonic framework and closure process of paleo-ocean *** article summarizes the geological,geochemical,and geochronological characteristics of upper crust of Proto-Tethyan Lajishan intra-oceanic arc and provides new data to constrain the subduction evolution of the South Qilian *** intra-oceanic arc volcanic rocks,including intermediate-mafic lava,breccia,tuff,and minor felsic rocks,are distributed along southern part of the Lajishan ophiolite *** and isotopic compositions indicate that the intermediate-mafic lava were originated from depleted mantle contaminated by sediment melts or hydrous fluids,whereas the felsic rocks were likely generated by partial melting of juvenile mafic crust in intra-oceanic arc *** from felsic rocks yield consistent and concordant ages ranging from 506 to 523 Ma,suggesting these volcanic rocks represent the relicts of upper crust of the Cambrian intra-oceanic *** with the Cambrian forearc ophiolite and accretionary complex,we suggest that the Cambrian intra-oceanic arc in the Lajishan ophiolite belt is belonging to the intra-oceanic arc system which was generated by south-directed subduction in the South Qilian Ocean at a relatively short interval between approximately 530 and 480 Ma.

关键词： volcanic rocks intra-oceanic arc U-Pb age Lajishan ophiolite belt South Qilian Ocean Proto-Tethyan realm

Visualizing Wallerian degeneration in the corticospinal tract after sensorimotor cortex ischemia in mice

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Neural Regeneration Research 2024年第3期19卷 636-641页

作者： Jiao Mu liufang Hao Zijue Wang Xuyang Fu yusen li Fei Hao Hongmei Duan Zhaoyang Yang Xiaoguang li Beijing Key Laboratory for Biomaterials and Neural Regeneration School of Biological Science and Medical EngineeringBeihang UniversityBeijingChina Department of Neurobiology School of Basic Medical SciencesCapital Medical UniversityBeijingChina

Stroke can cause Wallerian degeneration in regions outside of the brain,particularly in the corticospinal *** investigate the fate of major glial cells and axons within affected areas of the corticospinal tract following stroke,we induced photochemical infarction of the sensorimotor cortex leading to Wallerian degeneration along the full extent of the corticospinal *** first used a routine,sensitive marker of axonal injury,amyloid precursor protein,to examine Wallerian degeneration of the corticospinal *** antibody to amyloid precursor protein mapped exclusively to proximal axonal segments within the ischemic cortex,with no positive signal in distal parts of the corticospinal tract,at all time *** improve visualization of Wallerian degeneration,we next utilized an orthograde virus that expresses green fluorescent protein to label the corticospinal tract and then quantitatively evaluated green fluorescent protein-expressing *** this approach,we found that axonal degeneration began on day 3 post-stroke and was almost complete by 7 days after *** addition,microglia mobilized and activated early,from day 7 after stroke,but did not maintain a phagocytic state over ***,astrocytes showed relatively delayed mobilization and a moderate response to Wallerian ***,no anterograde degeneration of spinal anterior horn cells was observed in response to Wallerian degeneration of the corticospinal *** conclusion,our data provide evidence for dynamic,pathogenic spatiotemporal changes in major cellular components of the corticospinal tract during Wallerian degeneration.

关键词： corticospinal tract green fluorescent protein microglia spinal anterior horn cells stroke virus trace Wallerian degeneration

2024年新疆乌什Ms 7.1地震InSAR同震形变探测与断层滑动分布反演

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成都理工大学学报（自然科学版） 2024年第4期51卷 641-653页

作者：李雨森李为乐许强许善淼地质灾害防治与地质环境保护国家重点实验室(成都理工大学) 成都610059 应急管理部滑坡灾害风险预警与防控实验室成都610059

2024年1月23日,新疆维吾尔自治区乌什县发生Ms 7.1地震,快速查明其同震形变场与发震断层滑动特征,有助于科学认识此次地震发震机理。利用Sentinel-1卫星升、降轨雷达影像,采用合成孔径雷达差分干涉测量技术获取了本次地震的同震形变场,... 详细信息

2024年1月23日,新疆维吾尔自治区乌什县发生Ms 7.1地震,快速查明其同震形变场与发震断层滑动特征,有助于科学认识此次地震发震机理。利用Sentinel-1卫星升、降轨雷达影像,采用合成孔径雷达差分干涉测量技术获取了本次地震的同震形变场,进而基于Okada弹性位错模型,确定了本次地震的震源参数,并基于分布式滑动模型反演了本次地震断层面上的滑动分布。结果表明,升、降轨同震形变场沿视线向最大形变量分别为75 cm和48 cm,断层最大滑动量为4.2 m,主要集中在地下3~20 km区域;模型正演结果表明,此次地震在垂直方向最大抬升约53 cm,最大沉降约12 cm;发震断层运动以逆冲为主,兼具少量左旋走滑,根据InSAR结果及地质资料综合判断,本次发震断层为迈丹断裂。

关键词：乌什地震合成孔径雷达差分干涉测量同震形变断层滑动分布反演

Morphology-controlled porphyrin nanocrystals with enhanced photocatalytic hydrogen production

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Nano Research 2022年第6期15卷 5719-5725页

作者： Ronghui Cao Jinghan Wang yusen li Jiajie Sun Feng Bai School of Physics and Electronics Henan UniversityKaifeng 475004China Key Laboratory for Special Functional Materials of Ministry of Education National and Local Joint Engineering Research Center for High-efficiency Display and Lighting TechnologySchool of Materials Science and Engineeringand Collaborative Innovation Center of Nano Functional Materials and ApplicationsHenan UniversityKaifeng 475004China Academy for Advanced Interdisciplinary Studies Henan UniversityKaifeng 475004China

Molecular self-assembly is a natured-inspired strategy to integrate individual functional molecules into supramolecular nanostructured materials through noncovalent bond interactions for solar to fuel ***,the design and engineering of the morphology,size,and orderly stacking of supramolecular nanostructures remain a great *** this study,regular porphyrin nanocrystals with different orderly stacked structures are synthesized through noncovalent self-assembly of Pt(II)meso-tetra(4-carboxyphenyl)porphine(PtTCPP),using surfactants with different *** synergy of noncovalent bond interactions between porphyrin molecules,and between porphyrin molecules and surfactants resulted in different molecular packing *** to the spatial ordering of PtTCPP molecules,the different nanocrystals exhibit both collective optical properties and morphology-dependent activities in photocatalytic hydrogen *** measurements of the photodeposition of dual cocatalysts showed that the photogenerated electrons and holes selectively aggregated at different active sites,revealing separation pathways and directional transfer of photogenerated electrons and holes in the *** study provides a new strategy to exert rational control over porphyrin self-assembly nanocrystals for highly efficient water splitting.

关键词： porphyrin self-assembly morphology-dependent photocatalytic activity directional transfer photogenerated electrons and holes

乌原鲤早期发育过程中生长及主要消化酶活性和肠道组织变化

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淡水渔业 2024年第4期54卷 85-92页

作者：陈礼龙吴伟军叶华李哲柯真林周康奇李育森林勇苏胜齐西南大学水产学院重庆400715 广西壮族自治区水产科学研究院广西水产遗传育种与健康养殖重点实验室南宁530021

本实验探究了乌原鲤(Procypris mera)1 DAH(Day after hatching,日龄)仔鱼到80 DAH幼鱼的生长过程中脂肪酶、淀粉酶、胰蛋白酶、碱性磷酸酶活性变化规律及其生长和肠道组织变化情况。结果显示,乌原鲤仔稚幼鱼阶段全长和体质量的拟合增... 详细信息

本实验探究了乌原鲤(Procypris mera)1 DAH(Day after hatching,日龄)仔鱼到80 DAH幼鱼的生长过程中脂肪酶、淀粉酶、胰蛋白酶、碱性磷酸酶活性变化规律及其生长和肠道组织变化情况。结果显示,乌原鲤仔稚幼鱼阶段全长和体质量的拟合增长方程分别为y=-0.00481x^(2)+1.00636x+3.33020(R^(2)=0.985,P<0.05)和y=0.1731x^(2)+3.76634x-40.61142(R^(2)=0.990,P<0.05),特定生长率为7.7402%/d。肠道组织8 DAH时出现大量的杯状细胞和黏膜褶皱,15 DAH时肠道组织分层明显,27 DAH时黏膜褶皱高度不一、肌肉层增厚,45 DAH时出现肠腺,标志发育趋于完善。脂肪酶、淀粉酶、胰蛋白酶、碱性磷酸酶在1 DAH时均已检测出活性,且这4种消化酶呈现出不同的变化趋势。脂肪酶活性在1~13 DAH时期是先上升后下降趋势并于13 DAH达到最小值(0.654±0.165)U/g,在17 DAH达到峰值(1.437±0.110)U/g后呈先波动下降后显著上升的趋势;淀粉酶活性在3 DAH达到最小值(0.039±0.002)U/g,随后显著上升,在7 DAH达到最大值(0.146±0.005)U/g后呈波动下降趋势;胰蛋白酶活性在6 DAH达到最小值(232.677±26.620)U/mg,在6~13 DAH时期显著上升,在17 DAH后总体呈上升趋势;碱性磷酸酶活性在1~4 DAH时期缓慢上升,在5~13 DAH时期显著上升,在13~35 DAH时期波动下降,在35 DAH后又呈显著上升趋势。由此可得出结论,乌原鲤早期发育过程中的主要消化酶活性随着生长发生显著变化,其消化功能逐渐完善;在5~15 DAH应投喂含有足量蛋白质和脂肪的饵料,在15~45 DAH需投喂充足蛋白质和脂肪的配合饲料,在45~80 DAH需投喂营养均衡并含有一定比例碳水化合物的配合饲料。

关键词：乌原鲤(Procypris mera) 生长早期发育消化酶活性

刚果(布)Mpassa-Moubiri铜多金属矿区多源遥感蚀变矿化异常提取

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矿产勘查 2024年第3期15卷 384-394页

作者：丁俊李玉森何长宇朱洹志湘潭大学土木工程学院湖南湘潭411105

刚果(布)Mpassa-Moubiri矿区铜、铅、锌等矿种找矿前景良好,运用多源遥感数据可提供丰富的找矿地质信息。本文选取Aster、Sentinel-2A、Worldview-2影像,采用主成分分析法分别提取白铅矿化、菱锌矿化、硅化、铁染、蓝铜矿化、孔雀石化... 详细信息

刚果(布)Mpassa-Moubiri矿区铜、铅、锌等矿种找矿前景良好,运用多源遥感数据可提供丰富的找矿地质信息。本文选取Aster、Sentinel-2A、Worldview-2影像,采用主成分分析法分别提取白铅矿化、菱锌矿化、硅化、铁染、蓝铜矿化、孔雀石化等蚀变矿化异常信息,光谱角监督分类方法提取浅表含矿黑土异常信息。运用GIS密度分割挖掘各类蚀变矿化信息空间分布规律,并将其作为评价指标构建层次分析模型,最终圈定异常强度阈值高于0.8、面积17.18 km^(2)的遥感综合异常区域。结果表明:遥感综合异常主要呈北东向展布,富集在碳酸盐岩与碎屑岩接触带的有利成矿部位,与地表调查、化探异常吻合较好,表明多源数据组合能有效提取该矿区蚀变矿化信息,可为后续大比例尺勘查工作部署提供依据。

关键词：多源遥感蚀变矿化异常信息主成分分析层次分析刚果(布)

2023年积石山Ms6.2级地震InSAR同震形变探测与断层滑动分布反演

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成都理工大学学报（自然科学版） 2024年第1期51卷 22-32,75页

作者：李雨森李为乐许强许善淼王运生地质灾害防治与地质环境保护国家重点实验室(成都理工大学) 成都610059 应急管理部滑坡灾害风险预警与防控实验室成都610059

2023年12月18日,甘肃省临夏回族自治州积石山县发生了Ms6.2级地震,地震灾害损失显著高于同震级地震,查明其同震形变场与断层滑动分布特征,有助于揭示此次地震灾害损失严重的原因。利用Sentinel-1卫星升、降轨雷达影像,采用合成孔径雷达... 详细信息

2023年12月18日,甘肃省临夏回族自治州积石山县发生了Ms6.2级地震,地震灾害损失显著高于同震级地震,查明其同震形变场与断层滑动分布特征,有助于揭示此次地震灾害损失严重的原因。利用Sentinel-1卫星升、降轨雷达影像,采用合成孔径雷达干涉技术获取了本次地震的同震形变场,进而基于Okada弹性位错模型,确定了本次地震的震源参数,并基于分布式滑动模型反演了本次地震断层面上的滑动分布。结果表明,积石山地震为逆冲型地震,升、降轨同震形变场沿视线向最大形变量分别为7.1 cm和7.8 cm,断层最大滑动量为0.31 m,主要集中在地下0~8 km。与2019年6月17日四川长宁Ms 6.0级地震对比发现,长宁地震地表最大形变量为8 cm,断层最大滑动量为0.38 m,均大于积石山地震,推测积石山地震灾害损失严重的主要原因为震区居民房屋相对集中、房屋抗震性能差和黄土区场地地震波放大效应等。

关键词：积石山地震合成孔径雷达干涉测量同震形变断层滑动震源机制反演

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红水河暗色唇鲮的年龄与生长研究

四川动物 2024年第1期43卷 65-72页

作者：孙扬言何佳洋李育森张雪玲柯真林吴志强黄亮亮桂林理工大学环境科学与工程学院广西桂林541004 广西遗传育种与健康养殖重点实验室广西水产科学研究院南宁530021 西南大学水产学院重庆402460 广西岩溶地区水污染控制与用水安全保障协同创新中心广西桂林541004 广西环境污染控制理论与技术重点实验室广西桂林541004

为了解广西壮族自治区红水河暗色唇鲮Semilabeo obscurus的年龄结构及生长特性,于2022年11月在红水河采集71尾样本。结果显示:样本群体由1~6龄组成,优势年龄组为3龄,占总数的39.44%;平均体长16.51 cm,平均体重122.35 g,体重(W)与体长(L... 详细信息

为了解广西壮族自治区红水河暗色唇鲮Semilabeo obscurus的年龄结构及生长特性,于2022年11月在红水河采集71尾样本。结果显示:样本群体由1~6龄组成,优势年龄组为3龄,占总数的39.44%;平均体长16.51 cm,平均体重122.35 g,体重(W)与体长(L)呈幂函数相关:♀:W=0.039L2.827;♂:W=0.025L2.963;群体:W=0.026L^(2.964),属匀速生长型;生长特性符合von Betalanffy生长方程:♀:Lt=24.74[1−e^(−0.4195(t+0.2438))],W_(t)=340.65[1−e^(−0.4195(t+0.2438))]2.827;♂:Lt=26.70[1−e^(−0.3103(t+0.6951))],Wt=427.98[1−e^(−0.3103(t+0.6951))]2.963;雌、雄体重生长的拐点年龄分别为2.38龄、2.85龄。本研究明确了红水河暗色唇鲮的生长特性,为其个体生物学提供了数据参考,有助于对其资源的评价和可持续利用。

关键词：暗色唇鲮年龄结构生长特性红水河

A quantum federated learning framework for classical clients

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Science China(Physics,Mechanics & Astronomy) 2024年第5期67卷 1-10页

作者： Yanqi Song yusen Wu Shengyao Wu Dandan li Qiaoyan Wen Sujuan Qin Fei Gao State Key Laboratory of Networking and Switching Technology Beijing University of Posts and TelecommunicationsBeijing 00876China Department of Physics The University of Western AustraliaPerthWA 6009Australia School of Computer Science(National Pilot Software Engineering School) Beijing University of Posts and TelecommunicationsBeijing100876China

Quantum federated learning(QFL)enables collaborative training of a quantum machine learning(QML)model among multiple clients possessing quantum computing capabilities,without the need to share their respective local ***,the limited availability of quantum computing resources poses a challenge for each client to acquire quantum computing *** raises a natural question:Can quantum computing capabilities be deployed on the server instead?In this paper,we propose a QFL framework specifically designed for classical clients,referred to as CC-QFL,in response to this *** each iteration,the collaborative training of the QML model is assisted by the shadow tomography technique,eliminating the need for quantum computing capabilities of ***,the server constructs a classical representation of the QML model and transmits it to the *** clients encode their local data onto observables and use this classical representation to calculate local *** local gradients are then utilized to update the parameters of the QML *** evaluate the effectiveness of our framework through extensive numerical simulations using handwritten digit images from the MNIST *** framework provides valuable insights into QFL,particularly in scenarios where quantum computing resources are scarce.

关键词： client server quantum

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