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Facile and efficient synthesis of quinoline-4-carboxylic acids under microwave irradiation

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Chinese Chemical Letters 2010年第1期21卷 35-38页

作者： Zhu, Hui Yang, Ri Fang yun, liu hong Li, Jin Beijing Inst Pharmacol & Toxicol Dept Med Chem Beijing 100850 Peoples R China

A facile and efficient method for the preparation of 2-non-substituted quinoline-4-carboxylic acids is described via the Pfitzinger reaction of isatins with sodium pyruvate following consequent decarboxylation under m... 详细信息

关键词： Quinoline-4-carboxylic acids Pfitzinger reaction Microwave irradiation

Isolation and Characterization of Copia-like Retrotransposons from 12 Sweet Orange （Citrus sinensis Osbeck） Cultivars

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Journal of Integrative Plant Biology 2005年第12期47卷 1507-1515页

作者： Neng-Guo TAO Juan XU yun-Jiang CHENG liu hong Wen-Wu GUO Hua-Lin YI Xiu-Xin DENG State Key Laboratory of Crop Genetic Improvement National Center of Crop Molecular Breeding Huazhong Agricultural University Wuhan 430070 China

As the largest transposable element in the plant genome, retrotransposons are thought to be involved in citrus genetic instability and genome evolution, especially in sweet orange, which is prone to bud mutation. In the present study, the presence of copia-like retrotransposons, their heterogeneity, genomic distribution, and transcriptional activities in Citrus were investigated in 12 sweet orange （Citrus sinensis Osbeck） cultivars using a PCR assay designed to detect copia-like reverse transcriptase （RT） sequences. Twelve amplification products from each cultivar were cloned and sequenced. The cloned sequences showed great heterogeneity, except “Dream” navel and “Hamlin”, both of which shared the same sequence. Frame shifting, termination, deletion, and substitution accounted for the heterogeneity of RT sequences. Southern blot hybridization using the RT1 clone from the “Cara Cara” navel as a probe showed that multiple copies were integrated throughout the sweet orange genomes, which made the retrotransposon possible an effective molecular marker to detect citrus evolution events and to reveal its relationship with bud mutation. No transcriptional activities of the retrotransposon were detected by RT-PCR and Northern analysis in the fruits and leaves of either “Cara Cara” or “Seike” navels.

关键词： bud mutation Citrus cloning PCR retrotransposons.

Ultra-large Scale Molecular Dynamics Simulation for Nano-engineering

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Chemical Research in Chinese Universities 2008年第3期24卷 367-370页

作者： ZHAO Jian-wei YIN Xing LIANG Shuai liu yun-hong WANG Dong-xu DENG Sheng-yuan HOU Jie School of Chemistry and Chemical Engineering Nanjing University Nanjing 210093 P. R. China

In light of the special need of nano-engineering, an ultra-large scale and high-performance molecular dynamics（MD） simulation program was implemented. In many nano-engineering processes, the free boundary condition should be adopted. To meet this particular requirement, a pointer link and dynamic array data structures were employed so that both reliability and accuracy of simulation could be ensured. Using this method, one could realize the MD simulation of the nano-engineering system consisting of several million atoms per single CPU.

关键词： Molecular dynamics Nano-engineering Dynamic array Verlet table Cell list

Parametric instability in the pure-quartic nonlinear Schrödinger equation

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Chinese Physics B 2024年第3期33卷 316-321页

作者：张云红刘冲 School of Physics Northwest UniversityXi'an 710127China Shaanxi Key Laboratory for Theoretical Physics Frontiers Xi'an 710127China Peng Huanwu Center for Fundamental Theory Xi'an 710127China

We study the nonlinear stage of modulation instability(MI)in the non-intergrable pure-quartic nonlinear Schrödinger equation where the fourth-order dispersion is modulated *** the three-mode truncation,we reveal the complex recurrence of parametric resonance(PR)breathers,where each recurrence is associated with two oscillation periods(PR period and internal oscillation period).The nonlinear stage of parametric instability admits the maximum energy exchange between the spectrum sidebands and central mode occurring outside the MI gain band.

关键词： modulation instability parametric resonance breather three-mode truncation energy exchange

Rudiments of Sexual Equality in China

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Women of China 1997年第12期 45-46页

作者： FU yun hong liu

CHINESE people’s earliest awakening to sexual equality occurred in the middle- and latestages of the Ming Dynasty (1368-1644). Although still a feudal society, China had seen the relation of production with capitalist economic systems at that time. Capitalist ideology also found a space in some people’s thinking. Feudal ideology, especially ethical codes discriminating against women, were being attacked then. One outstanding figure who attacked

关键词： Li Rudiments of Sexual Equality in China

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港珠澳大桥非通航孔桥钻孔平台施工方案比选

桥梁建设 2015年第2期45卷 6-11页

作者：刘运洪中铁大桥局集团有限公司湖北武汉430050

港珠澳大桥CB05标非通航孔桥为跨径85m的钢-混组合连续梁桥,采用钢管复合桩基础,每墩均由6根钢管复合桩组成,全桥共372根。针对该桥结构特点和施工难点,桩基础施工提出了"钢管桩+型钢"结构的普通钻孔平台(方案1)和"整体桁架式"结构的整... 详细信息

港珠澳大桥CB05标非通航孔桥为跨径85m的钢-混组合连续梁桥,采用钢管复合桩基础,每墩均由6根钢管复合桩组成,全桥共372根。针对该桥结构特点和施工难点,桩基础施工提出了"钢管桩+型钢"结构的普通钻孔平台(方案1)和"整体桁架式"结构的整体钻孔平台(方案2)施工方案,通过文明施工、安全环保、施工工效及经济性方面的比选,采用方案2施工。在工厂内将钻孔平台零散构件按标准化要求加工成型后,组焊成整体桁架式结构,利用船舶整体运输至墩位,再采用吊船整体安装或整体拆除倒用,完成钻孔平台施工。该方案有效地缩短了钻孔平台逐墩转换的间歇时间,具有高效、安全、环保、节能、快速等优势。

关键词：港珠澳大桥连续梁桥桩基础钢管复合桩整体桁架式钻孔平台方案比选桥梁施工

Detecting secondary spin with extreme mass ratio inspirals in scalar-tensor theory

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Chinese Physics C 2024年第9期48卷 210-224页

作者： hong Guo Chao Zhang yunqi liu Rui-hong Yue yun-Gui Gong Bin Wang Center for Gravitation and Cosmology College of Physical Science and TechnologyYangzhou UniversityYangzhou 225009China Escola de Engenharia de Lorena Universidade de São PauloLorenaSP 12602-810Brazil Shanghai Frontier Research Center for Gravitational Wave Detection Shanghai Jiao Tong UniversitySha nghai 200240 China 4 School of Aeronautics and AstronauticsShanghai Jiao Tong UniversityShanghai 200240China School of Physics Huazhong University of Science and TechnologyWuhan 430074China Department of Physics School of Physical Science and TechnologyNingbo UniversityNingbo 315211China

In this study,we investigate the detectability of the secondary spin in an extreme mass ratio inspiral(EMRI) system within a modified gravity model coupled with a scalar *** central black hole,which reduces to a Kerr one,is circularly spiralled by a scalar-charged spinning secondary body on the equatorial *** analysis reveals that the presence of the scalar field amplifies the secondary spin effect,allowing for a lower limit of the detectability and an improved resolution of the secondary spin when the scalar charge is sufficiently *** findings suggest that secondary spin detection is more feasible when the primary mass is not large,and TianQin is the optimal choice for detection.

关键词： Gravitational wave EMRI secondary spin scalar radiation

Optimized the vanadium electrolyte with sulfate-phosphoric mixed acids to enhance the stable operation at high-temperature

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Frontiers of Chemical Science and Engineering 2024年第2期18卷 13-26页

作者： Ling Ge Tao liu Yimin Zhang hong liu School of Resource and Environmental Engineering Wuhan University of Science and TechnologyWuhan 430081China State Environmental Protection Key Laboratory of Mineral Metallurgical Resources Utilization and Pollution Control Wuhan University of Science and TechnologyWuhan 430081China Hubei Collaborative Innovation Center for High Efficient Utilization of Vanadium Resources Wuhan University of Science and TechnologyWuhan 430081China Hubei Provincial Engineering Technology Research Center of High Efficient Cleaning Utilization for Shale Vanadium Resource Wuhan University of Science and TechnologyWuhan 430081China School of Resource and Environmental Engineering Wuhan University of TechnologyWuhan 430070China

Herein, the influence of the concentration design and comprehensive performance of the sulfate-phosphoric mixed acid system electrolyte is investigated to realize an electrolyte that maintains high energy density and stable operation at high temperatures. Static stability tests have shown that VOPO4 precipitation occurs only with vanadium(V) electrolyte. The concentration of vanadium ion of 2.0–2.2 mol·L^(–1), phosphoric acid of 0.10–0.15 mol·L^(–1), and sulfuric acid of 2.5–3.0 mol·L^(–1) are suitable for a vanadium redox flow battery in the temperature range from –20 to 50 ℃. The equations for predicting the viscosity and conductivity of electrolytes are obtained by the response surface method. The optimized electrolyte overcomes precipitation generation. It has 2.8 times higher energy density than the non-phosphate electrolyte, and a coulomb efficiency of 94.0% at 50 ℃. The sulfate-phosphoric mixed acid system electrolyte promotes the electrode reaction process, increases the current density, and reduces the resistance. This work systematically optimizes the concentrations of composition of positive and negative vanadium electrolytes with mixed sulfate-phosphoric acid. It provides a basis for the different valence states and comprehensive properties of sulfate-phosphoric mixed acid system vanadium electrolytes under extreme environments, guiding engineering applications.

关键词： all vanadium redox flow battery mixed-acid vanadium electrolyte concentration optimization response surface methodology high-temperature stability

Insights into photocatalytic mechanism over a novel Cu_(2)WS_(4)/MoS_(2) S-scheme heterojunction

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Rare Metals 2024年第7期43卷 3118-3133页

作者： Wei Zhao Ji-Hui Cao Jun-Jie Liao yun liu Xiao-Jun Zeng Jun-Yu Shen Xue-Kun hong Yang Guo He-Hua Zeng Ya-Zi liu School of Materials Engineering Jiangsu Key Laboratory of Advanced Functional MaterialsSchool of Electronic and Information EngineeringChangshu Institute of TechnologyChangshu215500China School of Chemistry and Chemical Engineering Changji UniversityChangji 831100China State Environmental Protection Key Laboratory of Soil Environmental Management and Pollution Control Ministry of Ecology and EnvironmentNanjing Institute of Environmental SciencesNanjing 210023China School of Environment Jiangsu Engineering Lab of Water and Soil Eco-RemediationNanjing Normal UniversityNanjing 210023China Department of Chemical Engineering Curtin UniversityPerthWA6845Australia

A novel efficient Cu_(2)WS_(4)/MoS_(2) step-scheme(S-scheme)heterojunction photocatalyst was constructed for the first time and applied in the removal of environmental *** the as-prepared photocatalysts,the Cu_(2)WS_(4)/MoS_(2)-8%heterojunc tion photoc atalyst demonstrates the optimal photocatalytic performance,with the catalytic oxidation efficiency of tetracycline(TC)and the catalytic reduction efficiency of Cr^(6+)reaching 93.3%and 82.1%,*** excellent catalytic properties of Cu_(2)WS_(4)/MoS_(2) heterojunction photocatalysts are attributed to the effective separation pathways of charges and the presence of S-scheme heterojunctions,together with stronger redox *** is speculated that the photogenerated carrier migration path of the Cu_(2)WS_(4)/MoS_(2) catalyst follows the typical S-scheme photocatalytic mechanism,which is verified by the in-depth experimental study and simulated calculations including the electron paramagnetic resonance(EPR)analysis,free radical quenching experiments,charge density distribution,and simulated built-in electric field formation at the interface,which acts as driving force to promote the separation of photoinduced electrons and ***,the photocatalytic mechanism of S-scheme photogenerated carrier migration for the Cu_(2)WS_(4)/MoS_(2) catalyst is revealed based on the systematic experimental techniques and simulated calculations,accounting for its superior photocatalytic oxidation and reduction *** study provides inspiring implications to develop high-efficient S-scheme photocatalytic systems for versatile applications in solarenergy conversion.

关键词： Cu_(2)WS_(4)/MoS_(2) S-scheme Heterojunction Photocatalysis