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Recent advances in the electrocatalytic oxidative upgrading of lignocellulosic biomass

ChemPhysMater 2024年第2期3卷 157-186页

作者： yufeng Qi hairui Guo Junting Li Li Ma Yang Xu Huiling Liu Cheng Wanga Zhicheng Zhang Institute for New Energy Materials and Low-Carbon Technologies School of Materials Science and EngineeringTianjin Key Laboratory of Advanced Functional Porous MaterialsTianjinUniversityof TechnologyTianjin 300384China Key Laboratory of Organic Integrated Circuit Minitry of Education&Tianjin Key Laboratoryof Molecular Optoelectronic Sciencespartment of ChemistrySchool of ScienceTianjin UniversityTianjin 300072China Collaborative Innovation Center of Chemical Science and Engineering(Tianjin) Tianjin 300072China

Lignocellulosic biomass is a critical renewable carbon resource,but most of its utilization is inefficient,and elec-trocatalytic oxidation is a promising method of upgrading lignocellulose into value-added fuels and chemicals under mild operating ***,efforts to enable conversion with a high efficiency and low energy con-sumption have been reported,but understanding the reaction mechanisms and realizing scaled-up applications of the electrooxidation of lignocellulosic biomass are still in their early stages.A timely overview of recently reported general reaction mechanisms,particularly the strategies developed for use in improving the reaction efficiencies,is necessary to inspire research regarding the highly efficient utilization of ***,we summa-rize the strategies developed to improve electrocatalytic performance in oxidative lignocellulose *** organized summary includes strategies ranging from designing efficient electrocatalysts and adding functional co-catalysts or electrolytes to employing advanced electrolyzers.A comprehensive overview of representative examples should provide universal principles to yield insight into the reaction processes and guide the design of efficient electrocatalytic ***,the challenges and opportunities in developing the electrocatalytic oxidative upgrading of lignocellulosic biomass in the near future are proposed.

关键词： Biomass conversion Lignocellulose Electrocatalysis Oxidative upgrading Electrocatalyst

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光纤时间频率同步技术及应用

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仪器仪表学报 2024年第2期45卷 47-62页

作者：陈雨锋王波清华大学精密仪器系北京100084 时空信息精密感知技术全国重点实验室北京100084 光子测控技术教育部重点实验室北京100084 中国兵器工业导航与控制技术研究所北京100089

时间是人类目前测量和复现不确定度指标最高的物理量,代表了人类科技发展的最高水平。光纤时频同步技术经过几十年的发展,目前已广泛应用于量子计量、射电干涉测量、定位导航、现代通信、电力电网、高能物理、大地测量等诸多领域,成为... 详细信息

时间是人类目前测量和复现不确定度指标最高的物理量,代表了人类科技发展的最高水平。光纤时频同步技术经过几十年的发展,目前已广泛应用于量子计量、射电干涉测量、定位导航、现代通信、电力电网、高能物理、大地测量等诸多领域,成为人类社会高效运行的重要支撑。得益于光纤时频同步技术的高可靠性和高稳定度,综合原子时“分布式”和“实时性”这一长期存在的矛盾得到了解决。文章介绍了光纤时频同步技术的发展历史、各技术路径的研究现状,以及基于北京地区光纤时频同步网生成的分布式实时综合原子时。在此基础上,指出光纤时频同步的发展重点正从技术研究转为大规模网络化应用,开展基于光网络的多功能、多应用融合研究,实现一体化通信、感知、计算、测量、控制,将是未来的重要发展趋势。

关键词：光纤网络时间同步频率同步光载射频综合原子时

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Decoding the fish genome opens a new era in important trait research and molecular breeding in China

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Science China(Life Sciences) 2024年第10期67卷 2064-2083页

作者： Qian Zhou Jialin Wang Jiongtang Li Zhangfan Chen Na Wang Ming Li Lei Wang yufeng Si Sheng Lu Zhongkai Cui Xuhui Liu Songlin Chen State Key Laboratory of Mariculture Biobreeding and Sustainable Goods Yellow Sea Fisheries Research InstituteChinese Academy of Fishery SciencesQingdaoShandong 266071China Laboratory for Marine Fisheries Science and Food Production Processes Qingdao Marine Science and Technology CenterQingdaoShandong 266237China Key Laboratory of Aquatic Genomics Ministry of Agriculture and Rural AffairsBeijing Key Laboratory of Fishery BiotechnologyChinese Academy of Fishery SciencesBeijing 100041China

Aquaculture represents the fastest-growing global food production sector,as it has become an essential component of the global food *** has the world's largest aquaculture industry in terms of production ***,the sustainable development of fish culture is hindered by several concerns,including germplasm degradation and disease *** practice of genomic breeding,which relies heavily on genome information and genotypephenotype relationships,has significant potential for increasing the efficiency of aquaculture *** 2014,the completion of the genome sequencing and annotation of the Chinese tongue sole signified the beginning of the fish genomics era in *** then,domestic researchers have made dramatic progress in functional genomic *** date,the genomes of more than 60 species of fish in China have been assembled and *** on these reference genomes,evolutionary,comparative,and functional genomic studies have revolutionized our understanding of a wide range of biologically and economically important traits of fishes,including growth and development,sex determination,disease resistance,metamorphosis,and ***,genomic tools and breeding techniques such as SNP arrays,genomic selection,and genome editing have greatly accelerated genetic improvement through the incorporation of functional genomic information into breeding *** review aims to summarize the current status,advances,and perspectives of the genome resources,genomic study of important traits,and genomic breeding techniques of fish in *** review will provide aquaculture researchers,fish breeders,and farmers with updated information concerning fish genomic research and breeding *** summary will help to promote the genetic improvement of production traits and thus will support the sustainable development of fish aquaculture.

关键词： fish genomics economic traits genomic selection genome editing genomic breeding

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Crucial role played by CK8^(+)cells in mediating alveolar injury remodeling for patients with COVID-19

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Virologica Sinica 2024年第3期39卷 390-402页

作者： yufeng Li Hengrui Hu Jia Liu Longda Ma Xi Wang Liang Liu Qian Liu Liang Ren Jiang Li Fei Deng Zhihong Hu Yiwu Zhou Manli Wang State Key Laboratory of Virology Wuhan Institute of VirologyCenter for Biosafety Mega-ScienceChinese Academy of SciencesWuhan430071China Department of Forensic Medicine Tongji Medical College of Huazhong University of Science and TechnologyWuhan430010China University of the Chinese Academy of Sciences Beijing100049China

The high risk of SARS-CoV-2 infection and reinfection and the occurrence of post-acute pulmonary sequelae have highlighted the importance of understanding the mechanism underlying lung repair after *** address this concern,comparative and systematic analyses of SARS-CoV-2 infection in COVID-19 patients and animals were *** the lungs of nine patients who died of COVID-19 and one recovered from COVID-19 but died of unrelated disease in early 2020,damage-related transient progenitor(DATP)cells expressing CK8 marker proliferated *** CK8^(+)DATP cells were derived from bronchial CK5^(+)basal ***,they showed different cell fate toward differentiation into type I alveolar cells in the deceased and convalescent patients,*** using a self-limiting hamster infection model mimicking the dynamic process of lung injury remodeling in mild COVID-19 patients,the accumulation and regression of CK8t cell marker were found to be closely associated with the disease ***,we examined the autopsied lungs of two patients who died of infection by the recent Omicron variant and found that they only exhibited mild pathological injury with no CK8^(+)cell *** results indicate a clear pulmonary cell remodeling route and suggest that CK8^(+)DATP cells play a primary role in mediating alveolar remodeling,highlighting their potential applications as diagnostic markers and therapeutic targets.

关键词： SARS-CoV-2 CK8t DATP cells Cell proliferation Lung injury-remodeling Autopsy Hamster infection model

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表面改性对铁基非晶合金微波吸收性能的影响

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表面技术 2024年第12期53卷 230-239页

作者：钟宇峰殷陶曾国勋吴起白张海舒畅广东工业大学材料与能源学院广州510000

目的旨在调节铁基非晶合金(IAA)粉体复合材料的微波吸收性能。方法先在铁基非晶合金粉体表面采用磁控溅射局部覆盖铝膜,再使用KH560硅烷偶联剂对粉体进行绝缘包覆。通过XRD、SEM和FT-IR分别对粉体进行材料表征,采用VSM和传输反射法分别... 详细信息

目的旨在调节铁基非晶合金(IAA)粉体复合材料的微波吸收性能。方法先在铁基非晶合金粉体表面采用磁控溅射局部覆盖铝膜,再使用KH560硅烷偶联剂对粉体进行绝缘包覆。通过XRD、SEM和FT-IR分别对粉体进行材料表征,采用VSM和传输反射法分别测试样品的电磁性能。结果镀铝后铁基非晶合金粉体的复介电常数实部εʹ提高了56.1%,复介电常数虚部εʺ提高了132.4%。绝缘包覆后铁基非晶合金粉体的εʹ降低变为铁基非晶合金的32.6%,εʺ变为铁基非晶合金的25.1%。镀铝再包覆KH560的铁基非晶合金粉体的εʹ和εʺ则分别变为铁基非晶合金的43.5%和36.6%,其复介电常数实部和虚部比镀铝后的样品低,比单纯用KH560包覆后的样品高,显示出镀铝可补偿因KH560绝缘包覆而带来的介电损耗能力下降,有利于调节KH560绝缘包覆的粉体材料的电磁性能。结论对铁基非晶合金粉体的绝缘包覆,改善了相应材料的高频吸收性能,但牺牲了其低频吸收性能,为了弥补这个不足,提出在铁基非晶合金粉体表面局部覆盖铝膜,再进行绝缘包覆,期望在绝缘包覆后,粉体仍有较高的介电损耗能力,达到调节材料中低频电磁波吸收能力的目的。样品模拟反射率曲线显示,样品厚度在2~3 mm时,铁基非晶合金/Al/KH560样品最低峰对应频率低于铁基非晶合金/KH560的相应峰位,铁基非晶合金粉体表面镀铝可明显改善其复合材料的低频微波吸收特性。

关键词：铁基非晶合金磁控溅射镀铝硅烷偶联剂微波吸收

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Bifunctional ZrO@ZIF-90 nanozyme with high phosphohydrolase activity for sensitive electrochemical detection of methyl parathion

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Food Science and Human Wellness 2024年

作者： Xiaomin Pang Geoffrey I.N.Waterhouse Ruiqiang Wang Xuguang Qiao yufeng Sun Zhixiang Xu Key Laboratory of Food Nutrition and Healthy in Universities of Shandong， College of Food Science and Engineering， Shandong Agricultural University School of Chemical Sciences， the University of Auckland Shandong Cayon Testing Co.， Ltd.

In this work， a novel bifunctional zirconium dioxide @ zeolitic imidazolate framework-90 (ZrO2@ZIF-90) nanozyme was successfully developed for the catalytic degradation and electrochemical detection of methyl parathion (MP). The ZrO2@ZIF-90 nanozyme with phosphatase hydrolysis activity can convert MP into p-nitrophenol (p-NP). The addition of ZrO2riched in Lewis acid Zr(IV) sites significantly enhanced the phosphatase hydrolysis activity of ZIF-90. ZrO2@ZIF-90 also displayed satisfactory electrocatalytic performance on account of the high surface area， high porosity and powerful enrichment ability of the ZIF-90 and the excellent ion transfer capacity of ZrO2. A ZrO2@ZIF-90 nanozyme modified glassy carbon electrode (ZrO2@ZIF-90/GCE) was then fabricated to analyze p-NP formed through MP degradation. Under the optimized conditions， the developed sensor displayed satisfactory analytical performance with a low limit of detection of 0.53 μmol L-1and two wide linear ranges (3-10 μmol L-1and 10-200 μmol L-1). ZrO2@ZIF-90 nanozyme accomplished to the degradation and electrochemical detection of MP in river water and spiked fruits. This study identifies a promising new strategy for the design of bifunctional nanozymes for the detection of environmental hazards.

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Corrigendum to“Bi-continuous Mg-Ti interpenetrating-phase composite as a partially degradable and bioactive implant material”[Journal of Materials Science&Technology 146(2023)211-220]

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Journal of Materials Science & Technology 2024年第3期170卷 255-257页

作者： Chenxi Dou Mingyang Zhang Dechun Ren haibin Ji Zhe Yi Shaogang Wang Zengqian Liu Qiang Wang yufeng Zheng Zhefeng Zhang Rui Yang Liaoning Provincial Key Laboratory of Oral Diseases School and Hospital of StomatologyChina Medical UniversityShenyang 110001China Shi-Changxu Innovation Center for Advanced Materials Institute of Metal ResearchChinese Academy of SciencesShenyang 110016China School of Materials Science and Engineering University of Science and Technology of ChinaHefei 230026China School of Materials Science and Engineering Peking UniversityBeijing 100871China Center for Adaptive System Engineering School of Creativity and ArtShanghaiTech UniversityShanghai 201210China

The authors are very sorry for their carelessness that there are some problems with Fig.3 in the original manuscript.

关键词： composite phase partially

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Covalent organic framework/carbon black/molecularly imprinted polydopamine composites for the selective recognition and electrochemical detection of ciprofloxacin

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Food Science and Human Wellness 2024年

作者： yufeng Sun Yongfeng Chen Xiaomin Pang Geoffrey I.N.Waterhouse Xuguang Qiao Zhixiang Xu Key Laboratory of Food Processing Technology and Quality Control in Shandong Province， College of Food Science and Engineering， Shandong Agricultural University School of Chemical Sciences， The University of Auckland

In this work， a novel electrochemical sensor based on covalent organic framework@carbon black@molecularly imprinted polydopamine （COF@CB@MPDA） was developed for selective recognition and determination of ciprofloxacin （CF）. COF@CB@MPDA possessed good water dispersibility and was synthesized by the self-polymerization of dopamine under alkaline conditions in the presence of the COF， CB and CF. The high surface area COF enhanced the adsorption of CF， whilst CB gave the composites high electrical conductivity to improve the sensitivity of the proposed COF@CB@MPDA/GCE sensor. The specific recognition of CF by COF@CB@MPDA involved hydrogen bonding and van der Waals interactions. Under optimized conditions， the sensor showed a good linear relationship with CF concentration over the range 5.0 × 10-7mol/L and 1.0 × 10-4mol/L， with a limit of detection （LOD） of 9.53 × 10-8mol/L. Further， the developed sensor exhibited high selectivity， repeatability and stability for CF detection in milk and milk powders. The method used to fabricate the COF@CB@MPDA/GCE sensor could be easily adapted for the selective recognition and detection of other antibacterial agents and organic pollutants in the environment.

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Tim4 deficiency reduces CD301b+macrophage and aggravates periodontitis bone loss

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International Journal of Oral Science 2024年第2期16卷 280-292页

作者： Ziming Wang Hao Zeng Can Wang Jiaolong Wang Jing Zhang Shuyuan Qu Yue Han Liu Yang Yueqi Ni Wenan Peng Huan Liu Hua Tang Qin Zhao yufeng Zhang State Key Laboratory of Oral&Maxillofacial Reconstruction and Regeneration Key Laboratory of Oral Biomedicine Ministry of EducationHubei Key Laboratory of StomatologySchool&Hospital of StomatologyTaikang Center for Life and Medical SciencesWuhan UniversityWuhanChina School of Stomatology Nanchang UniversityNanchangChina Institute of Infection and Immunity Science and Technology Innovation CenterShandong First Medical University&Shandong Academy of Medical SciencesJinanChina Medical Research Institute School of MedicineWuhan UniversityWuhanChina

Periodontitis is a common chronic inflammatory disease that causes the periodontal bone destruction and may ultimately result in tooth *** the progression of periodontitis,the osteoimmunology microenvironment in periodontitis is damaged and leads to the formation of pathological alveolar bone ***301b^(+)macrophages are specific to the osteoimmunology microenvironment,and are emerging as vital booster for conducting bone ***,the key upstream targets of CD301b^(+)macrophages and their potential mechanism in periodontitis remain *** this study,we concentrated on the role of Tim4,a latent upstream regulator of CD301b^(+)*** first demonstrated that the transcription level of Timd4(gene name of Tim4)in CD301b^(+)macrophages was significantly upregulated compared to CD301b^(-) macrophages via high-throughput RNA ***,several Tim4-related functions such as apoptotic cell clearance,phagocytosis and engulfment were positively regulated by CD301b^(+)*** single-cell RNA sequencing analysis subsequently discovered that Cd301b and Timd4 were specifically co-expressed in *** following flow cytometric analysis indicated that Tim4 positive expression rates in total macrophages shared highly synchronized dynamic changes with the proportions of CD301b^(+)macrophages as periodontitis ***,the deficiency of Tim4 in mice decreased CD301b^(+)macrophages and eventually magnified alveolar bone resorption in ***,Tim4 controlled the p38 MAPK signaling pathway to ultimately mediate CD301b^(+)macrophages *** a word,Tim4 might regulate CD301b^(+)macrophages through p38 MAPK signaling pathway in periodontitis,which provided new insights into periodontitis immunoregulation as well as help to develop innovative therapeutic targets and treatment strategies for periodontitis.

关键词： period upstream eventually

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Generalized Isospectral-Nonisospectral Modified Korteweg-de Vries Integrable Hierarchies and Related Properties

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Annals of Applied Mathematics 2024年第2期40卷 105-138页

作者： Huanhuan Lu Xinan Ren yufeng Zhang Hongyi Zhang School of Mathematics China University of Mining and TechnologyXuzhouJiangsu 221116China

In this article, a new technique for deriving integrable hierarchy is discussed, i.e., such that are derived by combining the Tu scheme with the vector product. Several classes of spectral problems are introduced by threedimensional loop algebra and six-dimensional loop algebra whose commutators are vector product, and the six-dimensional loop algebra is derived from the enlargement of the three-dimensional loop algebra. It is important that we make use of the variational method to create a new vector-product trace identity for which the Hamiltonian structure of the isospectral integrable hierarchy is worked out. The derived integrable hierarchies are reduced to the modified Korteweg-de Vries(mKdV) equation, generalized coupled mKdV integrable system and nonisospectral mKdV equation under specific parameter selection. Starting from a 3×3 matrix spectral problem, we subsequently construct an explicit N-fold Darboux transformation for integrable system(2.8) with the help of a gauge transformation of the corresponding spectral problem. At the same time, the determining equations of nonclassical symmetries associated with mKdV equation are presented in this paper. It follows that we investigate the coverings and the nonlocal symmetries of the nonisospectral mKdV equation by applying the classical Frobenius theorem and the coordinates of a infinitely-dimensional manifold in the form of Cartesian product.

关键词： Darboux transformation nonlocal symmetry covering manifold contact structure

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