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纳米氧化铜-镉单一与联合胁迫对油菜营养品质的影响

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环境科学学报 2024年第4期44卷 381-389页

作者：王诗琪孙约兵农业农村部环境保护科研监测所农业农村部产地环境污染防控重点实验室/天津市农业环境与农产品安全重点实验室天津300191 东北农业大学资源与环境学院哈尔滨150030

采用水培实验,探究了纳米氧化铜(CuO NPs)与镉(Cd)联合胁迫对油菜品质的影响.结果表明,单一CuO NPs(10~50 mg·L^(-1))处理对油菜生长和品质有一定抑制作用,油菜鲜重、可溶性糖、抗坏血酸和总酚含量随CuO NPs浓度增加而降低,与未投加相... 详细信息

采用水培实验,探究了纳米氧化铜(CuO NPs)与镉(Cd)联合胁迫对油菜品质的影响.结果表明,单一CuO NPs(10~50 mg·L^(-1))处理对油菜生长和品质有一定抑制作用,油菜鲜重、可溶性糖、抗坏血酸和总酚含量随CuO NPs浓度增加而降低,与未投加相比,分别降低了9.61%~39.26%、6.88%~45.09%、9.20%~29.14%和10.36%~18.47%,硝酸盐含量则显著升高16.44%~72.61%.在1μmol·L^(-1)Cd处理下,施加CuO NPs后油菜鲜重呈先升高后降低趋势.与空白对照相比,油菜叶片Cd含量降低了21.57%~36.14%,可溶性糖、可溶性蛋白和总酚含量最大分别降低了30.9%、39.61%和27.96%,抗坏血酸含量则增加了44.83%~76.21%,硝酸盐含量大幅升高,最大增加了116.18%,黄酮含量增加不明显.CuO NPs促进了油菜叶部Zn、Mg、Al、K和Ca元素的吸收,抑制了Fe元素吸收.研究表明,CuO NPs、Cd单一及联合胁迫整体上对油菜品质产生了负面影响.

关键词：纳米氧化铜镉胁迫油菜营养品质

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生物炭复配海泡石钝化修复弱碱性镉污染土壤

环境科学学报 2024年第2期44卷 365-374页

作者：王超高珊孙涛张语馨贾宏涛朱荟孙约兵农业农村部环境保护科研监测所农业农村部产地环境污染防控重点实验室/天津市农业环境与农产品安全重点实验室天津300191 新疆农业大学资源与环境学院新疆土壤与植物生态过程重点实验室乌鲁木齐830052 中国地质调查局呼和浩特自然资源综合调查中心呼和浩特010010

通过大田试验,研究了生物炭复配海泡石对弱碱性土壤镉(Cd)有效性、赋存形态和土壤质量以及Cd在玉米体内吸收累积的影响.结果表明,复配材料表面粗糙且含有纤维状结构,结合了海泡石和生物炭的矿物晶体组成.不同钝化处理降低了土壤Cd的有效... 详细信息

通过大田试验,研究了生物炭复配海泡石对弱碱性土壤镉(Cd)有效性、赋存形态和土壤质量以及Cd在玉米体内吸收累积的影响.结果表明,复配材料表面粗糙且含有纤维状结构,结合了海泡石和生物炭的矿物晶体组成.不同钝化处理降低了土壤Cd的有效性,其中,添加0.2%生物炭+0.2%海泡石时土壤有效态Cd含量由0.38 mg·kg^(-1)下降至0.25 mg·kg^(-1),Cd赋存形态由活性较高的可交换态和碳酸盐结合态转化为更稳定的残渣态.施用不同复配比的生物炭和海泡石后,显著降低了玉米各部位Cd含量,与对照相比,3种玉米籽粒中Cd含量分别下降了37.14%~40.55%(蠡玉16)、59.46%~68.78%(郑单958)和40.94%~47.84%(三北218).添加钝化材料较对照处理显著升高了土壤可溶性有机碳含量、土壤脲酶、碱性磷酸酶和过氧化氢酶活性.其中,0.2%生物炭+0.2%海泡石处理对土壤脲酶和碱性磷酸酶活性提升效果最好,0.2%生物炭+0.5%海泡石处理对土壤过氧化氢酶活性提升效果最好.综合考虑,施用0.2%生物炭+0.2%海泡石复配材料对弱碱性Cd污染土壤修复、玉米安全生产及土壤环境质量提升具有较高的应用潜力.

关键词：生物炭海泡石镉污染钝化修复土壤质量

覆盖材料对云贵高原柑橘园土壤理化性质和细菌群落特征以及柑橘品质的影响

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生态学报 2024年第8期44卷 3408-3422页

作者：余高赵仕龙孙约兵罗有亮陈芬铜仁学院贵州省梵净山地区生物多样性保护与利用重点实验室铜仁554300 农业农村部产地环境污染防控重点实验室天津市农业环境与农产品安全重点实验室天津300191

采用田间试验,研究了玉米秸秆覆盖(JF)、白色地膜覆盖(BF)、黑色地膜覆盖(HM)和园艺地布覆盖(YD),以及清耕作为对照(CK)对云贵高原柑橘园土壤理化性质、细菌群落特征及柑橘品质的影响。结果表明,与CK相比,不同覆盖处理下柑橘产量、单果... 详细信息

采用田间试验,研究了玉米秸秆覆盖(JF)、白色地膜覆盖(BF)、黑色地膜覆盖(HM)和园艺地布覆盖(YD),以及清耕作为对照(CK)对云贵高原柑橘园土壤理化性质、细菌群落特征及柑橘品质的影响。结果表明,与CK相比,不同覆盖处理下柑橘产量、单果重、果汁率、可食率、维生素C含量和可溶性固形物等指标均提高,可滴定酸含量则有所降低,进而提高了固酸比,其中以JF处理效果最显著。BF、HM和YD处理降低了土壤pH值,JF处理则相反,不同覆盖处理均能提高土壤温度、含水量、有机质和养分含量,JF处理对土壤有机质、全氮、全磷、全钾、有效磷和速效钾含量的提升作用最明显,BF处理下土壤温度最高。JF、HM和YD处理均能显著提高Chao1指数和Observed species指数,而BF处理则相反。在门水平上,覆盖提高了有益菌放线菌门的相对丰度,降低了致病菌拟杆菌门的相对丰度;在属水平上,覆盖提高了有益菌热酸菌属、朱氏杆菌属、Babeliales、红杆菌属和脱氯单胞菌属的相对丰度,降低了致病菌Saccharimonadales、成对杆菌属、金黄色杆菌属、芽孢八叠球菌属和丛毛单胞菌属的相对丰度。此外,覆盖还使土壤细菌共生网络变得简单而稳定。冗余分析结果表明,土壤全氮和细菌群落红杆菌属是提升柑橘产量和品质的关键因子,其解释率分别为45.67%和39.40%。方差分解分析结果表明,土壤理化性质和细菌群落的共同作用对柑橘产量和品质提升的贡献最大,其解释率为45.0%。综上所述,覆盖能有效改善土壤理化性质,提升土壤养分供应水平,优化细菌群落结构,提高柑橘产量和品质,其中,玉米秸秆覆盖可优先作为云贵高原柑橘园土壤的地表覆盖措施。

关键词：柑橘园覆盖土壤养分特征细菌群落结构柑橘品质

In situ stabilization remediation of cadmium contaminated soils of wastewater irrigation region using sepiolite

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Journal of Environmental Sciences 2012年第10期24卷 1799-1805页

作者： yuebing sun Guohong sun Yingming Xu Lin Wang Dasong Lin Xuefeng Liang Xin Shi Key Laboratory of Original Environmental Quality Safety Ministry of AgricultureTianjin 300191China Tianjin Key Laboratory of Asro-environment and Agro-product Safety Institute of Agro-Environmental ProtectionMinistry of Agriculture7ianjin 300191China Department of Basic Science lianjin Agricultural UniversityTianjin 300384China College of Environment and Resources Jilin UniversityChangchun 130012China

The effects of immobilization remediation of Cd-contaminated soils using sepiolite on soil pH, enzyme activities and microbial communities, TCLP-Cd （toxicity characteristic leaching procedure-Cd） concentration, and spinach （Spinacia oleracea） growth and Cd uptake and accumulation were investigated. Results showed that the addition of sepiolite could increase soil pH, while the TCLP-Cd concentration in soil was decreased with increasing sepiolite. The changes of soil enzyme activities and bacteria number indicated that a certain metabolic recovery occurred after the sepiolite treatments, and spinach shoot biomass increased by 58.5%-65.5% in comparison with the control group when the concentration of sepiolite was ~ 10 g/kg. However, the Cd concentrations in the shoots and roots of spinach decreased with an increase in the rate of sepiolite, experiencing 38.4%-59.1% and 12.6%--43.6% reduction, respectively, in contrast to the control. The results indicated that sepiolite has the potential for success on a field scale in reducing Cd entry into the food chain.

关键词： Cd-contaminated soil immobilization remediation sepiolite soil quality

赤铁矿与巯基坡缕石复配对砷镉复合污染土壤修复效应研究

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农业环境科学学报 2024年第2期43卷 285-293页

作者：景睿裴楠狄雪荣梁学峰秦旭彭云英徐应明黄青青孙约兵东北农业大学资源与环境学院哈尔滨150030 农业农村部产地环境污染防控重点实验室农业农村部环境保护科研监测所天津300191

为探讨巯基坡缕石(MPAL)和赤铁矿(Fe2O3)对土壤重金属污染钝化阻控效应,以江西某农田Cd-As复合污染水稻土为供试土壤,采用盆栽试验研究了巯基坡缕石、赤铁矿单一以及复配处理下土壤pH值、Cd-As有效态与形态分布及水稻生物量和Cd、As、F... 详细信息

为探讨巯基坡缕石(MPAL)和赤铁矿(Fe2O3)对土壤重金属污染钝化阻控效应,以江西某农田Cd-As复合污染水稻土为供试土壤,采用盆栽试验研究了巯基坡缕石、赤铁矿单一以及复配处理下土壤pH值、Cd-As有效态与形态分布及水稻生物量和Cd、As、Fe含量。结果表明:施加不同材料后水稻籽粒生物量较对照显著增加了2.37~2.45倍,土壤中DTPA-Cd含量显著降低16.94%~22.57%(P<0.05)。土壤连续浸提形态分析显示,MPAL和Fe2O3复配处理提高了土壤中无定形态铁氧化物结合态Cd、As含量。MPAL和Fe_(2)O_(3)复配处理下水稻根系Cd和As含量降幅分别达7.14%、25.13%,不同处理下稻米Cd含量降幅为40.00%~60.00%,但籽粒As含量处理间差异不显著。研究表明,巯基坡缕石和赤铁矿复配材料可以有效降低土壤中Cd和As含量,减少水稻对Cd和As的吸收,具备Cd-As复合污染农田修复和安全利用的潜在应用价值。

关键词：巯基坡缕石赤铁矿水稻镉砷复合污染土壤

Effects of sepiolite on stabilization remediation of heavy metal-contaminated soil and its ecological evaluation

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Frontiers of Environmental Science & Engineering 2016年第1期10卷 85-92页

作者： yuebing sun Dan ZHAO Yingming XU Lin WANG Xuefeng LIANG Yue SHEN Key Laboratory of Original Environmental Quality Ministry of Agriculture/Tianjin Key Laboratory of Agro-Environment and Ago-Product Safety Institute of Agro-Environmental Protection Ministry of Agriculture Tianjin 300191 China College of Resources and Environmental Sciences Henan Agricultural University Zhengzhou 450002 China

Stabilization in the remediation of heavy metal contaminated soils has been gaining prominence because of its cost-effectiveness and rapid implementation. In this study, microbial properties such as microbial community and enzyme activities, chemical properties such as soil pH and metal fraction, and heavy metal accumulation in spinach （Spinacia oleracea） were considered in assessing stabilization remediation effectiveness using sepiolite. Results showed that soil pH values increased with rising sepiolite concentration. Sequential extraction results indi- cated that the addition of sepiolite converted significant amounts of exchangeable fraction of Cd and Pb into residual form. Treatments of sepiolite were observed to reduce Cd and Pb translocation from the soil to the roots and shoots of spinach. Concentrations of Cd and Pb exhibited 12.6%-51.0% and 11.5%-46.0% reduction for the roots, respectively, and 0.9%-46.2% and 43.0%- 65.8% reduction for the shoots, respectively, compared with the control group. Increase in fungi and actinomycete counts, as well as in catalase activities, indicated that soil metabolic recovery occurred after sepiolite treatments.

关键词： stabilization remediation heavy metals sepio-lite soil quality spinach (Spinacia oleracea)

Growth responses of the newly-discovered Cd-hyperaccumulator Rorippa globosa and its accumulation characteristics of Cd and As under joint stress of Cd and As

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Frontiers of Environmental Science & Engineering 2007年第1期1卷 107-113页

作者： sun yuebing ZHOU Qixing WEI Shuhe REN Liping Key Laboratory of Terrestrial Ecological Process Institute of Applied EcologyChinese Academy of SciencesShenyang 110016China The Provincial Key Laboratory of the Conservation and Exploitation of Biological Resources in College of Life Sciences Anhui Normal UniversityWuhu 241000China College of Environmental Science and Engineering Nankai UniversityTianjin 300071China

Rorippa globosa has been identified as a newly-found Cd-hyperaccumulating *** the present study,growth responses of Rorippa globosa and its accumulation characteristics of Cd and As were examined under joint stress of Cd and *** results showed that Cd and As had an antagonistic effect on enhancing the growth of Rorippa globosa plants and Cd uptake and accumulation under the low concentration Cd and As *** the concentra-tion of Cd in the soil was 10 mg/kg and the concentration of As was 50 mg/kg,the highest growing height of the plant was up to 35.9 cm and the dry weight of the shoots was up to 2.2 g/pot,***,the accumulation of Cd in the leaves under the joint stress was higher than that at the same level under single Cd ***,there were synergic adverse effects on plant growth and Cd uptake under the combined pollution from a high concentration of Cd and ***,the accumulation of As in the roots was greater than that in the shoots,the translocation factor(TF)was h0.3 and the bioaccumulation factor(BF)was h0.6,thus showing that Rorippa globosa had an excluding effect on As *** results confirmed that Rorippa globosa had a strong tolerant ability to the joint stress of Cd and As,and the potential for phytoremediation of soils contaminated by Cd and As.

关键词： Cd-hyperaccumulator Rorippa globosa combined pollution joint stress phytormediation

Remediation of Heavy Metal-Polluted Agricultural Soils Using Clay Minerals： A Review

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Pedosphere 2017年第2期27卷 193-204页

作者： XU Yi LIANG Xuefeng XU Yingming QIN Xu HUANG Qingqing WANG Lin sun yuebing College of Resources and Environment Hunan Agricultural University Changsha 410128 (China) Innovation Team of Remediation of Heavy Metal-Contaminated Farmlands Agro-Environmental Protection Institute Ministry of Agriculture Tianjin 300191 (China) Key Laboratory of Original Environmental Quality of MOA/ZTianjin Key Laboratory of Agro-Environment and Agro-Product Safety Tianjin 300191 (China)

Heavy metal contamination of agricultural soils poses risks and hazards to humans. The remediation of heavy metal-polluted soils has become a hot topic in environmental science and engineering. In this review, the application of clay minerals for the remediation of heavy metal-polluted agricultural soils is summarized, in terms of their remediation effects and mechanisms, influencing factors, and future focus. Typical clay minerals, natural sepiolite, palygorskite, and bentonite, have been widely utilized for the in-situ immobilization of heavy metals in soils, especially Cd-polluted paddy soils and wastewater-irrigated farmland soils. Clay minerals are able to increase soil pH, decrease the chemical-extractable fractions and bioavailability of heavy metals in soils, and reduce the heavy metal contents in edible parts of plants. The immobilization effects have been confirmed in field-scale demonstrations and pot trials. Clay minerals can improve the environmental quality of soils and alleviate the hazards of heavy metals to plants. As main factors affecting the immobilization effects, the pH and water condition of soils have drawn academic attention. The remediation mechanisms mainly include liming, precipitation, and sorption effects. However, the molecular mechanisms of microscopic immobilization are unclear. F^ture studies should focus on the long-term stability and improvement of clay minerals in order to obtain a better remediation effect.

关键词： bentonite bioavailability immobilization liming effect palygorskite sepiolite soil pH

习近平群众观对毛泽东群众路线思想的发展及其时代价值

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湖南师范大学社会科学学报 2016年第2期45卷 44-49页

作者：孙岳兵中南大学马克思主义学院湖南师范大学

毛泽东结合中国革命和建设的实际,创造性地提出了"一切为了群众,一切依靠群众,从群众中来,到群众中去"的群众路线思想。当前,我国进入了改革攻坚期、矛盾凸显期,面对当今世情、国情、党情的变化,习近平立足解决党的长期执政、党群关系、... 详细信息

毛泽东结合中国革命和建设的实际,创造性地提出了"一切为了群众,一切依靠群众,从群众中来,到群众中去"的群众路线思想。当前,我国进入了改革攻坚期、矛盾凸显期,面对当今世情、国情、党情的变化,习近平立足解决党的长期执政、党群关系、"四风"等方面的问题,在全党深入开展群众路线教育实践活动,提出了"人民对美好生活的向往,就是我们的奋斗目标"、"要更加强化问题导向,注重解决实际问题"等重要论断,继承和发展了毛泽东群众路线思想,开辟了马克思主义群众路线思想的新境界,具有重要的时代价值。

关键词：毛泽东习近平群众路线