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Metrological traceable calibration of organic carbon and elemental carbon based on laboratory-generated reference materials

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Journal of Environmental Sciences 2025年第3期149卷 524-534页

作者： yue liu Junjie liu Ji Xiao Jing Ye Lixu Guo Caiqing Yan Center for Environmental Metrology National Institute of Metrology ChinaBeijing 100029China College of Chemistry and Chemical Engineering Taiyuan University of TechnologyTaiyuan 030024China Environment Research Institute Shandong UniversityQingdao 266237China

Carbonaceous aerosol,including organic carbon(OC)and elemental carbon(EC),has significant influence on human health,air quality and climate *** measurement of carbonaceous aerosol is essential to reduce the uncertainty of radiative forcing estimation and source *** accurate separation of OC and EC is controversial due to the charring of ***,the development of reference materials(RM)for the validation of OC/EC separation is an important basis for further *** RMs were mainly based on ambient air sampling,which could not provide traceability of OC and EC *** develop traceable RMs with known OC/EC contents,our study applied an improved aerosol generation and mixing technique,providing uniform deposition of particles on quartz *** generate OC aerosol with similar pyrolytic property of ambient aerosol,both water soluble organic carbon(WSOC)and water insoluble organic carbon(WIOC)were used,and amorphous carbon was selected for EC *** RMs were analyzed using different *** homogeneity within the filter was validated,reaching below 2%.The long-term stability of RMs has been validated with RSD ranged from 1.7%–3.2%.Good correlationwas observed between nominal concentration of RMswithmeasured concentration by two protocols,while the difference of EC concentration was within 20%.The results indicated that the newly developed RMs were acceptable for the calibration of OC and EC,which could improve the accuracy of carbonaceous aerosol ***,the laboratory-generated EC-RMs could be suitable for the calibration of equivalent BC concentration by Aethalometers.

关键词： Carbonaceous aerosol Split point Reference material Laboratory-generated Traceability

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Insight into catalytic performance and reaction mechanism for toluene total oxidation over Cu-Ce supported catalyst

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Journal of Environmental Sciences 2025年第3期149卷 476-487页

作者： Xuan Liang Jin Zhang Juntai Tian Zenghua Xie yue liu Peng liu Daiqi Ye School of Environment and Energy South China University of TechnologyGuangzhou 510006China National Engineering Laboratory for VOCs Pollution Control Technology and Equipment Guangzhou 510006China Guangdong Provincial Key Laboratory of Atmospheric Environment and Pollution Control South China University of TechnologyGuangzhou 510006China Guangdong Provincial Engineering and Technology Research Centre for Environmental Risk Prevention and Emergency Disposal South China University of TechnologyGuangzhou 510006China

Herein,three supported catalysts,CuO/Al_(2)O_(3),CeO_(2)/Al_(2)O_(3),and CuO-CeO_(2)/Al_(2)O_(3),were synthesized by the convenient impregnation method to reveal the effect of CeO_(2)addition on catalytic performance and reaction mechanism for toluene *** with CuO/Al_(2)O_(3),the T_(50)and T_(90)(the temperatures at 50%and 90%toluene conversion,respectively)of CuO-CeO_(2)/Al_(2)O_(3)were reduced by 33 and 39°C,respectively.N_(2)adsorptiondesorption experiment,XRD,SEM,EDS mapping,Raman,EPR,H_(2)-TPR,O_(2)-TPD,XPS,NH_(3)-TPD,Toluene-TPD,and in-situ DRIFTS were conducted to characterize these *** excellent catalytic performance of CuO-CeO_(2)/Al_(2)O_(3)could be attributed to its strong coppercerium interaction and high oxygen vacancies ***,in-situ DRIFTS proved that CuO-CeO_(2)/Al_(2)O_(3)promoted the conversion of toluene to benzoate and accelerated the deep degradation path of *** work provided valuable insights into the development of efficient and economical catalysts for volatile organic compounds.

关键词： Cu-Ce supported catalyst Copper-cerium interaction Oxygen vacancies Toluene oxidation Reaction mechanism

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Cu gradient design to attain high efficient solution-processed CuIn（S,Se）2 solar cells

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Journal of Energy Chemistry 2025年第2期101卷 213-222页

作者： Xuejun Xu Rutao Meng yue liu Han Xu Jianpeng Li Yi Zhang Institute of Photoelectronic Thin Film Devices and Technology State Key Laboratory of Photovoltaic Materials and Cells and Engineering Research Center of Thin Film Optoelectronics Technology Ministry of Education Nankai University

Solution-processed chalcopyrite solar cells are widely regarded as a promising alternative method in reducing the cost compared with vacuum-based *** is noted that the absorber layer usually needs to be prepared under a high insert pressure（～1.6 atm） to suppress element loss or under a mild pressure but additional surface etching is needed for fabricating high efficient solar ***,a copper gradient structured precursor is proposed to prepare CuIn（S,Se）2（CISSe） film under a mild pressure（1.1 atm）.The designed gradient Cu not only promotes crystal grain growth and tailors the defects,but also avoids the surface etching of the formed CISSe film for the fabrication of high efficient solar ***,Cu gradient design decreases the conduction band offset of heterojunction,boosting the carriers transport across the p-n ***,a 13,35% efficient CISSe solar cell,comparable to the high efficient CISSe solar cell prepared by this method under high pressure or with film surface etching,is *** work provides a facile pathway to fabricate high efficient solution-processed chalcopyrite solar cell,avoiding high selenization pressure and film etching,and shows huge potential for solutionprocessed copper-based solar cells.

关键词： Band alignment Carrier transport CISSe Crystal grain growth Cu gradient Defect passivation

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Stretchable All-Small-Molecule Organic Solar Cells Enabled by Polymer Elastomer Confinement

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CHINESE JOURNAL OF POLYMER SCIENCE 2025年第2期43卷 271-277页

作者： Zhang, Chen-Yi liu, Yu-Qiang Li, Hong-Xiang Cui, Xin-yue Wei, Zheng-Dong liu, yue-Heng Li, Ming-Hua Zhang, An-Dong Cheng, Pei Bo, Zhi-Shan Qingdao Univ Coll Text & Clothing State Key Lab Biofibers & Ecotext Qingdao 266071 Peoples R China Sichuan Univ Coll Polymer Sci & Engn State Key Lab Polymer Mat Engn Chengdu 610065 Peoples R China Qingdao Univ Coll Mat Sci & Engn Qingdao 266071 Peoples R China Beijing Normal Univ Coll Chem Beijing Key Lab Energy Convers & Storage Mat Beijing 100875 Peoples R China

Intrinsic stretchability is a promising attribute of polymer organic solar cells (OSCs). However, rigid molecular blocks typically exhibit poor tensile properties, rendering polymers vulnerable to mechanical stress. In this study, we introduce a different approach utilizing all-small-molecule donors and acceptors to fabricate stretchable OSCs. An elastomer, styrene-b-ethylene-butylene-styrene (SEBS), was embedded to modulate film crystallization and stretchability. SEBS effectively confines the growth process of donors and acceptors, leading to enhancement of the crystallization quality, thus contributing to enhanced device efficiencies. Meanwhile, SEBS can absorb and release mechanical stress during stretching, thereby preventing mechanical degradation of donors and acceptors. The mechanical properties of the OSCs were significantly improved by the incorporation of SEBS. Notably, the crack-onset strain increased from 1.03% to 5.99% with SEBS embedding. These findings present a straightforward strategy for achieving stretchable OSCs using all small molecules, offering a different perspective for realizing stretchable devices.

关键词： All-small-molecule Organic solar cells Elastomer Stretchability Flexibility

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Attribution analysis of trends in reference crop evapotranspiration in China

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Journal of Geographical Sciences 2025年第1期35卷 3-16页

作者： liu yue GUO Mengjing LI Jing LYU Na ZHANG Junqi ZHANG Bowen State Key Laboratory of Eco-hydraulics in Northwest Arid Region Xi’an University of TechnologyXi’an710000China

Reference crop evapotranspiration(ET_(0)) is essential for determining crop water requirements and developing irrigation *** this study,ET_(0) was calculated via the FAO-56 Penman-Monteith model,and the spatiotemporal variations in ET_(0) over China from 1960 to 2019 were *** then quantified the contributions of five driving factors(air temperature,wind speed,relative humidity,sunshine hours,and CO_(2) concentration)to the ET_(0) trends via a detrending *** results revealed that nationwide ET_(0) showed no significant(p>0.05)decreasing trend from 1960 to 2019,with a trend of−8.56×10^(−2)mm a^(−2).The average temperature and wind speed were identified as the dominant factors affecting ET_(0)trends at the national *** contributions of the driving factors to the ET_(0) trends were ranked in the following order:average temperature(21.3%)>wind speed(−15.63%)>sunshine hours(−11.99%)>CO_(2) concentration(6.36%)>relative humidity(3.58%).Spatially,the dominant factors influencing the ET_(0) trends varied *** the southeastern region,average temperature and sunshine hours dominated the trends of ET_(0),whereas wind speed and average temperature were the dominant factors in the northwestern *** findings provide valuable insights into the dominant factors affecting ET_(0)trends in China and highlight the importance of considering different driving factors in calculating crop water requirements.

关键词： reference crop evapotranspiration climate change contribution rate trend analysis

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Impacts of near-M_(s)austempering treatment on microstructure evolution and bainitic transformation kinetics of a medium Mn steel

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Journal of Iron and Steel Research International 2025年第1期32卷 249-259页

作者： Yong-gang Yang Xin-yue liu Rui-zhi Li Yu-lai Chen Hong-xiang Wu Guo-min Sun Zhen-li Mi National Engineering Research Center for Advanced Rolling and Intelligent Manufacturing University of Science and Technology BeijingBeijing 100083China Technology Center Ningbo Iron&Steel Co.Ltd.Ningbo 315800ZhejiangChina

The microstructure evolution and bainitic transformation of an Fe-0.19C-4.03Mn-1.48Si steel subjected to near-M_(s)austempering treatment were systematically investigated by combining dilatometer,X-ray diffraction,and electron *** additional austempering treatments with isothermal temperatures above M_(s)were used as *** show that the incubation period for the bainitic transformation occurs when the medium Mn steel is treated with the austempering temperature above M_(s).However,when subjected to near-M_(s)isothermal treatment,the medium Mn steel does not show an incubation period and has the fastest bainitic transformation ***,the largest volume fraction of bainite with a value of 74.7%is obtained on the condition of near-M_(s)austempering treatment after cooling to room *** and microstructure evolution analysis indicates that the elimination of the incubation period and the fastest rate of bainitic transformation are related to the preformed *** advent of preformed martensite allows the specimen to generate more bainite in a limited *** bainitic ferrite nucleation at austenite grain boundaries and through autocatalysis at ferrite/austenite interfaces,a model is established to understand the kinetics of bainite formation and it can describe the nucleation rate of bainitic transformation well when compared to the experimental results.

关键词： Medium manganese steel Bainitic transformation Microstructure Near-M_(s)austempering Transformation modeling

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Quantifying the Driving Effect of Colored Noise in Brownian Motors

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Chinese Physics Letters 2025年第1期42卷 94-98页

作者： Zhichao Zhang yue liu Congmin Wu Dahai He Department of Physics and Jiujiang Research Institute Xiamen UniversityXiamen 361005China School of Mathematical Sciences Xiamen UniversityXiamen 361005China

The colored noise disrupts the detailed balance,enabling directed transport in ratchet systems without additional driving *** a well-established understanding of the conditions for Brownian motors,quantification of the driving effect of colored noise and its connection to deviations from equilibrium remains *** this study,we examined the directed motion of an overdamped Brownian motor within an asymmetric traveling potential subjected to Ornstein–Uhlenbeck colored *** propose a scheme to quantify the driving effect of colored noise by defining an effective force based on the stopping velocity of the traveling potential where directed transport *** results revealed a nonmonotonic dependence of the effective force on the noise correlation time and a monotonic dependence on the noise strength,corresponding to double and single current reversals,*** nonmonotonicity of the current is attributed to the interplay between the fluctuating characteristics and the driving effects of colored noise.

关键词： Brownian colored directed

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Upcycling of polyethylene terephthalate to1,4-cyclohexanedimethanol in water

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Science China Chemistry 2025年

作者： Shuhui Fang Zhiwen Gao Xinrui Shi Min Zhang Wei Zhang yue liu State Key Laboratory of Petroleum Molecular & Process Engineering Shanghai Key Laboratory of Green Chemistry and Chemical ProcessesSchool of Chemistry and Molecular Engineering East China Normal University Engineering Center for Sustainable Carbon Science and Technology East China Normal University Institute of Eco-Chongming

The recycling of waste polyethylene terephthalate（PET）, an extensively used polymer as plastic and fiber materials, has become an urgent topic due to the rapid generation and accumulation of plastic waste into the environment. Current chemical recycling approaches to depolymerize and convert PET into 1,4-cyclohexanedimethanol（CHDM）, an important chemical in the production of advanced polyesters, predominantly use organic solvents, such as alcohols or dioxane. Herein, we developed an environmentally friendly and economically viable pathway for converting PET to CHDM using water as the solvent. In this process, PET is sequentially hydrolyzed in water, hydrogenated to 1,4-cyclohexane dicarboxylic acid（CHDA）, and then reduced to CHDM. The PET conversion rate is self-enhanced in aqueous medium via acid-catalyzed hydrolysis by the generated CHDA intermediate. A Pd-based catalyst（e.g., Pd/C） selectively hydrogenates the arene ring of the PET monomer, terephthalic acid intermediate, and a Ru-Sn/C bimetallic catalyst reduces its COOH to CH2OH group. At optimized reaction conditions, a complete conversion of PET and 80.1% yield of CHDM are obtained. Alternatively, this approach can also efficiently produce CHDA from PET, with a yield up to 86.4%.

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Correction to:Impact of comorbid subthreshold depressive symptoms on cancer-related fatigue and complications in adults with leukemia

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World Journal of Psychiatry 2025年第3期15卷 361-362页

作者： yue-Xian liu Juan Wang Department of Hematology Central Hospital Affiliated to Shandong First Medical UniversityJinan 250013Shandong ProvinceChina

Correction to"liu YX,Wang *** of comorbid subthreshold depressive symptoms on cancer-related fatigue and complications in adults with *** J Psychiatry 2024;14(7):1009-1016[PMID:39050202 DOI:10.5498/wjp.v14.i7.1009]".I... 详细信息

关键词： World Journal of Psychiatry Correction

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China TCM Cardio Bank(CTC Bank):a high-quality,large-sample and real-world research database

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Science Bulletin 2025年第1期70卷 1-3页

作者： Yiwen Li Yanfei liu Mengmeng Zhu Wenting Wang Keji Chen Luqi Huang Fengqin Xu yue liu National Clinical Research Center for TCM Cardiology Xiyuan HospitalChina Academy of Chinese Medical SciencesBeijing 100091China Cardiovascular Disease Group China Center for Evidence-based Medicine of TCMChina Academy of Chinese Medical SciencesBeijing 100091China Beijing Key Laboratory of Traditional Chinese Medicine Basic Research on Prevention and Treatment for Major Diseases Experimental Research CenterChina Academy of Chinese Medical SciencesBeijing 100078China The Second Department of Geriatrics Xiyuan HospitalChina Academy of Chinese Medical SciencesBeijing 100091China China Center for Evidence-based Medicine of TCM China Academy of Chinese Medical SciencesBeijing 100078China

In recent years,real-world research(RWS)has advanced exponentially[1].There has been an increase in the number of retrospective cohort studies in China owing to their time-saving and economic advantages[2].Traditional Chinese medicine(TCM)is being integrated into the RWS *** large amount of multimodal and non-standardized information in the diagnostic and therapeutic treatment of TCM has created obstacles to the evidence-based development of TCM.

关键词： TCM modal database

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