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Nano-Micro Letters 2025年第2期17卷 376-386页

作者： Wei-Min Qin Zhongliang Li Wen‑Xia Su Jia‑Min Hu Hanqin Zou Zhixuan Wu Zhiqin Ruan yue‑Peng cai Kang Li Qifeng Zheng School of Chemistry South China Normal UniversityGuangzhou 510006People’s Republic of China Key Laboratory of Functional Metal‑Organic Compounds of Hunan Province College of Chemistry and Material ScienceHengyang Normal UniversityHengyang 421008People’s Republic of China Guangzhou Key Laboratory of Energy Conversion and Energy Storage Materials Guangzhou 510006People’s Republic of China

Porous organic cages(POCs)with permanent porosity and excellent host–guest property hold great potentials in regulating ion transport behavior,yet their feasibility as solid-state electrolytes has never been testified in a practical ***,we design and fabricate a quasi-solid-state electrolyte(QSSE)based on a POC to enable the stable operation of Li-metal batteries(LMBs).Benefiting from the ordered channels and cavity-induced anion-trapping effect of POC,the resulting POC-based QSSE exhibits a high Li+transference number of 0.67 and a high ionic conductivity of 1.25×10^(−4) S cm^(−1) with a low activation energy of 0.17 *** allow for homogeneous Li deposition and highly reversible Li plating/stripping for over 2000 *** a proof of concept,the LMB assembled with POC-based QSSE demonstrates extremely stable cycling performance with 85%capacity retention after 1000 ***,our work demonstrates the practical applicability of POC as SSEs for LMBs and could be extended to other energy-storage systems,such as Na and K batteries.

关键词： Porous organic cage Cavity-induced anion-trapping Quasi-solid-state electrolyte Homogeneous Li+flux Lithium metal battery

No difference in activity of Sod-1 genotypes of Poa annua to short-term treatment of ambient gaseous organic pollution

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Journal of Environmental Sciences 2005年第5期17卷 866-868页

作者： cai yue-wei CHEN Xiao-yong Shanghai Key Laboratory for Ecological Processes and Restoration in Urban Areas Department of Environmental Sciences East China Normal University Shanghai 200062 China

Our previous studies indicated that genotypes at locus Sod-1 of Poa annua changed clinally along a gradient of gaseous organic pollution. In the present study, we aimed to know whether there were differential responses of activities of different superoxide dismutase （SOD） genotypes to short-term treatment of ambient gaseous organic pollution. Significant bias from Hardy-Weinberg equibrium was observed on locus Sod-1, and no genotype Sod- l-BB was found. Significantly increased activities were observed in most treatments for genotype Sod-1-AA and in one treatment for genotype Sod-1-AB. However, no significant difference in SOD activities was found between the two genotypes. It was interpreted that fitness difference between the two genotypes was small and treatment duration was too short or extent of ambient organic pollution was too low to lead to differential responses. Other environmental factor effects on activities of superoxide dismutases can also explain the results.

关键词： superoxide dismutase genotype activity gaseous organic pollution Poa annua

Faecal microbiota transplantation enhances efficacy of immune checkpoint inhibitors therapy against cancer

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World Journal of Gastroenterology 2021年第32期27卷 5362-5375页

作者： Yong-Bo Kang yue cai Department of Microbiology and Immunology School of Basic Medical SciencesShanxi Medical UniversityJinzhong 030600Shanxi ProvinceChina

Even though immune checkpoint inhibitors(ICIs)are effective on multiple cancer types,there are still many non-responding patients.A possible factor put forward that may influence the efficacy of ICIs is the gut ***,faecal microbiota transplantation may enhance efficacy of ***,the data available in this field are insufficient,and relevant scientific work has just *** a result,the current work reviewed the latest research on the association of gut microbiota with ICI treatments based on anti-programmed cell death protein 1 antibody and anti-cytotoxic T-lymphocyte-associated protein 4 antibody and explored the therapeutic potential of faecal microbiota transplantation in combination with ICI therapy in the future.

关键词： Gut microbiome Immunotherapy Programmed cell death protein 1/programmed cell death protein ligand 1 Cytotoxic T-lymphocyte-associated protein 4 Immune checkpoint inhibitors resistance Faecal microbiota transplantation

New Matrix Loop Algebra and Its Application

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Communications in Theoretical Physics 2008年第8期50卷 321-325页

作者： DONG Huan-He XU yue-cai College of Information Science and Engineering Shandong University of Science and Technology Qingdao 266510 China College of Continuing Education Shangdong University of Science and Technology Taian 271000 China

A new matrix Lie algebra and its corresponding Loop algebra are constructed firstly,as its application,the multi-component TC equation hierarchy is obtained,then by use of trace identity the Hamiltonian structure of the above system is ***,the integrable couplings of the obtained system is worked out by the expanding matrix Loop algebra.

关键词： matrix loop algebra Liouville integrable system Hamiltonian structure integrable couplings

Metal phosphonate-derived cobalt/nickel phosphide@N-doped carbon hybrids as efficient bifunctional oxygen electrodes for Zn-air batteries

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Frontiers of Chemical Science and Engineering 2022年第9期16卷 1367-1376页

作者： cai-yue Wang Meng-Qi Gao Cheng-cai Zhao Li-Min Zhao Hui Zhao School of Materials Science and Engineering Liaocheng UniversityLiaocheng 252000China

The exploration of efficient bifunctional electrocatalysts for oxygen reduction reaction and oxygen evolution reaction is pivotal for the development of rechargeable metal–air *** metal phosphides are emerging as promising catalyst candidates because of their superb activity and low ***,a novel metal phosphonate-derived cobalt/nickel phosphide@N-doped carbon hybrid was developed by a carbothermal reduction of cobalt/nickel phosphonate hybrids with different Co/Ni molar *** metal phosphonate derivation method achieved an intimately coupled interaction between metal phosphides and a heteroatom-doped carbon *** resultant Co_(2)P/Ni_(3)P@NC-0.2 enables an impressive electrocatalytic oxygen reduction reaction activity,comparable with those of state-of-the-art Pt/C catalysts in terms of onset potential(0.88 V),4e‒selectivity,methanol tolerance,and long-term ***,remarkable oxygen evolution reaction activity was also observed in alkaline *** high activity is ascribed to the N-doping,abundant accessible catalytic active sites,and the synergistic effect among the *** work not only describes a highefficiency electrocatalyst for both oxygen reduction reaction and oxygen evolution reaction,but also highlights the application of metal phosphonate hybrids in fabricating metal phosphides with tunable structures,which is of great significance in the energy conversion field.

关键词： metal phosphonate cobalt/nickel phosphide N-doped carbon oxygen electrochemistry Zn−air battery

Localization of nonlocal symmetries and interaction solutions of the Sawada–Kotera equation

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Communications in Theoretical Physics 2021年第6期73卷 6-12页

作者： Jian-wen Wu yue-jin cai Ji Lin Department of Physics Zhejiang Normal UniversityJinhuaZhejiang 321004China

The nonlocal symmetry of the Sawada–Kotera(SK)equation is constructed with the known Lax *** introducing suitable and simple auxiliary variables,the nonlocal symmetry is localized and the finite transformation and some new solutions are obtained *** the other hand,the group invariant solutions of the SK equation are constructed with the classic Lie group *** particular,by a Galileo transformation some analytical soliton-cnoidal interaction solutions of a asymptotically integrable equation are discussed in graphical ways.

关键词： Sawada–Kotera equation nonlocal symmetry interaction solutions

Future prospect of“Gut microbiome composition can predict the response to nivolumab in advanced hepatocellular carcinoma patients”

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World Journal of Gastroenterology 2022年第20期28卷 2248-2250页

作者： Yong-Bo Kang yue cai Department of Microbiology and Immunology School of Basic Medical SciencesShanxi Medical UniversityJinzhong 030600Shanxi ProvinceChina

Recently,we read the article“Gut microbiome composition can predict the response to nivolumab in advanced hepatocellular carcinoma patients”with interest,and it is preliminary suggested that gut microbiota is closely related to therapeutic effect of *** on the meaningful results of this article,several valuable research directions are proposed to enhance the therapeutic effect of immune checkpoint inhibitors on advanced hepatocellular carcinoma.

关键词： Gut microbiome Immunotherapy Immune checkpoint inhibitor resistance Probiotics Faecal microbiota transplantation Hepatocellular carcinoma Prognosis

Asymmetric Fluorinative Dearomatization of Tryptophol Derivatives by Chiral Anion Phase-Transfer Catalysis

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Chinese Journal of Chemistry 2018年第10期36卷 925-928页

作者： Xiao-Wei Liang yue cai Shu-LiYou State Key Laboratory of Organometallic Chemistry Shanghai Institute of Organic Chemistry Chinese Academy of Sciences 345 Lingling Lu Shanghai 200032 China School of Pharmacy East China University of Science and Technology 130Mei-Long Road Shanghai 200237 China

An asymmetric fluorinative dearomatization reaction of tryptophol derivatives was developed via chiral anion phase-transfer catalysis. Vari- ous fluorinated furoindolines were obtained in moderate to excellent yields and enantioselectivity in the presence of Selectfluor. The preliminary mecha- nistic studies suggested the existence of an in situ formed tryptophol boronic ester plays a critical role in determining the enantioselectivity. This method features the facile introduction of a fluorine atom in a highly enantioselective manner and construction of two contiguous quaternary stereogenic cen- ters.

关键词： asymmetric catalysis dearomatization fluorination organocatalysis phase-transfer catalysis tryptophol

An improved siphon drainage method for slope stabilization

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Journal of Mountain Science 2019年第3期16卷 701-713页

作者： SUN Hong-yue WANG Dong-fei SHANG yue-quan cai yue-liang WEI Zhen-lei Ocean College Zhejiang University College of Civil Engineering and Architecture Zhejiang University

The siphon drainage is an effective measure for the slope groundwater control. However,for the traditional siphon drainage, limitations such as siphon lift restriction and poor reliability in longterm service prevent it from being widely used. In this study, an improved siphon drainage method with inclined borehole penetrating the deep part of the slope is proposed to overcome the limitations suffered by the traditional method. Through experimental research, theoretical analysis and engineering practice,the reliability and capability of the proposed method are investigated. The results demonstrate that with the inclined pipe the height difference between the control point of the groundwater level and the orifice can be controlled to be less than the height of the water column corresponding to the local atmospheric pressure. As a result, deep drainage can be *** addition, by controlling the diameter of siphon drainage pipe not larger than 4 mm, a plug flow can be formed in the siphon pipe, which can prevent air accumulation in the siphon process and a continuous and effective siphon drainage is achieved. Through a practical project running smoothly since September 2013, it is found that the proposed method can effectively drain the groundwater deep in the slope and the maximum drawdown of groundwater level in boreholes can reach 8.5 m with an average drainage flow of 5.5 m3/d. The practical results also illustrate that 4 mm siphon pipe can be used to realize deep slope drainage and restart siphon automatically.

关键词： Landslide Drainage Siphon Inclined borehole 4mm diameter siphon pipe

Synthesis and application of an IL-supported diol as protecting group for aldehydes

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Chinese Chemical Letters 2007年第10期18卷 1205-1208页

作者： yue Qin cai Ye Liu Guo Hua Gao Shanghai Key Laboratory of Green Chemistry and Chemical Processes East China Normal University Shanghai 200062 China

A new IL-supported diol, 1-（2,3-dihydroxypropyl）-3-methylimidazolium hexafluorophosphate has been synthesized and characterized by Fr-IR, ^1H NMR, ^13C NMR and MS （ESI）. Its physical properties such as freezing point, solubility and specific gravity and thermal stability were determined. Synthetic utilities of the resultant diol as a protecting group for aldehydes were also investigated.

关键词： IL-supported diol Preparation Characterization Protecting group