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Regulating the oxidation state of Pd to enhance the selective hydrogenation for 5-hydroxymethylfurfural

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Chinese Journal of Chemical Engineering 2024年第8期72卷 60-68页

作者： Xin Li yue Ma Xuning Wang Jianguo Wu Dong Cao Daojian Cheng State Key Laboratory of Organic-Inorganic Composites and College of Chemical Engineering Beijing University of Chemical TechnologyBeijing 100029China

The highly selective hydrogenation of 5-hydroxymethylfurfural to 2,5-dihydroxymethylfuran is an important reaction in the field of biomass hydrogenation,because it is a bridge between biomass resources and chemical ***,we precisely constructed carbon nitride supported Pd-based catalysts by a simple impregnation-reduction *** changing the reduction temperature,catalysts with different oxidation state could be precisely ***,the important correlation between the ratio of Pd^(0)/Pd^(2+)and catalytic activity is revealed during the selective hydrogenation of *** Pd/g—C_(3.N_(4)—3.0 catalyst with a Pd^(0)/Pd^(2+)ratio of 3.2 showed the highest catalytic activity,which could get 96.9%5-hydroxymethylfurfural conversion and 90.3.2,5-dihydroxymethylfuran *** density functional theory calculation revealed that the synergistic effect between Pd0and Pd2+in Pd/g—C_(3.N_(4)—3.0 system could boost the adsorption of the substrate and the dissociation of *** this work,we highlight the important correlation between metal oxidation state and catalytic activity,which provides valuable insights for the rational design of precious metal catalysts for hydrogenation reactions.

关键词： Pd/g-C_(3.N_(4) Selective hydrogenation 5-hydroxymethylfurfural 2,5-dihydroxymethylfuran Oxidation state

Distributed active vibration control for helicopter based on diffusion collaboration

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Chinese Journal of Aeronautics 2024年第8期37卷 208-232页

作者： Yang YUAN Yang LU Xunjun MA Jingliang LI Huiyu yue National Key Laboratory of Helicopter Aeromechanics Nanjing University of Aeronautics and AstronauticsNanjing 210016China Wuhan Second Ship Design and Research Institute Wuhan 430205China

The active vibration control technology has been successfully applied to several helicopter ***,with the increasing of control scale,traditional centralized control algorithms are experiencing significant increase of computational complexity and physical implementation *** address this issue,a diffusion collaboration-based distributed Filtered-x Least Mean Square algorithm applied to active vibration control is proposed,drawing inspiration from the concept of data fusion in wireless sensor *** algorithm distributes the computation load to each node,and constructs the active vibration control network topology of large-scale system by discarding the weak coupling secondary paths between nodes,achieving distributed active vibration *** order to thoroughly validate the effectiveness and superiority of this algorithm,a helicopter fuselage model is designed as the research ***,the excellent vibration reduction performance of the proposed algorithm is confirmed through ***,specialized node control units are developed,which utilize STM3. microcontroller as the processing ***,a distributed control system is constructed based on multi-processor *** on this foundation,a large-scale active vibration control experimental platform is *** on the platform,experiments are carried out,involving the 4-input 4-output system and the 8-input 8-output *** experimental results demonstrate that under steady-state harmonic excitation,the proposed algorithm not only ensures control effectiveness but also reduces computational complexity by 50%,exhibiting faster convergence speed compared with traditional centralized *** time-varying external excitation,the proposed algorithm demonstrates rapid tracking of vibration changes,with vibration amplitudes at all controlled points declining by over 94%,proving the strong robustness and adaptive capability of the algorithm

关键词： Helicopter Active vibration control Diffusion collaboration Distributed control Experiment

Characteristics and triggering mechanisms of early negative Indian Ocean Dipole

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Acta Oceanologica Sinica 2024年第3期43卷 59-65页

作者： yue Fang Shuangwen Sun Yongcan Zu Jianhu Wang Lin Feng First Institute of Oceanography and Key Laboratory of Marine Science and Numerical ModelingMinistry of Natural ResourcesQingdao 266061China Laboratory for Regional Oceanography and Numerical Modeling Qingdao Marine Science and Technology CenterQingdao 266237China Shandong Key Laboratory of Marine Science and Numerical Modeling Qingdao 266061China

Negative Indian Ocean Dipole(nIOD)can exert great impacts on global climate and can also strongly influence the climate in *** nIOD is a major type of nIOD,which can induce more pronounced climate anomalies in summer than La Niña-related ***,the characteristics and triggering mechanisms of early nIOD are *** results based on reanalysis datasets indicate that the early nIOD and La Niña-related nIOD are the two major types of nIOD,and the former accounts for over one third of all the nIOD events in the past six *** two types of nIODs are similar in their intensities,but are different in their spatial patterns and seasonal *** early nIOD,which develops in spring and peaks in summer,is one season earlier than the La Niña-related *** spatial pattern of the wind anomaly associated with early nIOD exhibits a winter monsoon-like pattern,with strong westerly anomalies in the equatorial Indian Ocean and eastly anomalies in the northern Indian *** to the triggering mechanism of early positve IOD,the early nIOD is induced by delayed Indian summer monsoon *** results of this study are helpful for improving the prediction skill of IOD and its climate impacts.

关键词： Indian Ocean Dipole(IOD) triggering mechanism Indian summer monsoon seasonal cycle negative IOD

Stability of bedded rock slopes subjected to hydro-fluctuation and associated strength deterioration

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第8期16卷 3233-3257页

作者： Bin Xu Xinrong Liu yue Liang Xiaohan Zhou Zuliang Zhong School of River and Ocean Engineering Chongqing Jiaotong UniversityChongqing400074China School of Civil Engineering Chongqing UniversityChongqing400045China

Reservoir-induced earthquakes(RIEs)occur frequently in the Three Gorges Reservoir Area(TGRA)and the rock mass strength of the hydro-fluctuation belt(HFB)deteriorates severely due to the reservoirinduced seismic *** models of typical bedded rock slopes(BRSs),***(GIS),moderately(MIS),and steeply(SIS)inclined slopes,were proposed according to field *** dynamic response mechanism and stability of the BRSs,affected by the rock mass deterioration of the HFB,were investigated by the shaking table test and the universal distinct element code(UDEC)***,the amplification coefficient of the peak ground acceleration(PGA)of the slope was gradually attenuated under multiple seismic loads,and the acceleration response showed obvious“surface effect”and“elevation effect”in the horizontal and vertical directions,***“S-type”cubic function and“steep-rise type”exponential function were used to characterize the cumulative damage evolution of the slope caused by microseismic waves(low seismic waves)and high seismic waves,*** to the dynamic responses of the acceleration,cumulative displacement,rock pressure,pore water pressure,damping ratio,natural frequency,stability coefficient,and sliding velocity of the slope,the typical evolution processes of the dynamic cumulative damage and instability failure of the slope were generalized,and the numerical and experimental results were *** the dynamic effects of the slope height(SH),slope angle(SA),bedding plane thickness(BPT),dip angle of the bedding plane(DABP),dynamic load amplitude(DLA),dynamic load frequency(DLF),height of water level of the hydro-fluctuation belt(HWLHFB),degradation range of the hydro-fluctuation belt(DRHFB),and degradation shape of the hydro-fluctuation belt(DSHFB),the sensitivity of factors influencing the slope dynamic stability using the orthogonal analysis method(OAM)was DLA>DRHFB>SA>SH>DLF>HWLHFB>DSHFB>DABP>BPT.

关键词： Bedded rock slopes Hydro-fluctuation belt Shaking table test UDEC simulation Dynamic response mechanism

The role of proteasomes in tumorigenesis

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Genes & Diseases 2024年第4期11卷 155-169页

作者： Xiangyi Zhou Ruqing Xu yue Wu Li Zhou Tingxiu Xiang Department of Oncology The First Affliated Hospital of Chongqing Medical UniversityChongqing 400016China Chongqing Key Laboratory of Translational Research for Cancer Metastasis and Individualized Treatment Chongqing University Cancer HospitalChongqing 400030China

Protein homeostasis is the basis of normal life activities,and the proteasomefamily plays an extremely important function in this *** proteasome 2os is a concentric circle structure with twoαrings and twoβrings *** proteasome 2os can perform both ATP-dependent and non-ATP-dependent ubiquitination proteasome degradation by binding to various subunits(such as 19S,11S,and 200 PA),which is performed by its active subunitβ1,β2,andβ*** proteasome can degrade misfolded,excess proteins tomaintain *** the same time,it can be utilized by tumors to degrade over-proliferate and unwanted proteins to support their *** can affect the development of tumors from several aspects including tumor signaling pathways such as NF-kB and p53.cell cycle,immune regulation,and drug ***-encoding genes have been found to be overexpressed in a variety of tumors,providing a potential novel target for cancer *** addition,proteasome inhibitors such as bortezomib,carfilzomib,and ixazomib have been put into clinical application as the first-line treatment of multiple *** and more studies have shown that it also has different therapeutic effects in other tumors such as hepatocellular carcinoma,non-small cell lung cancer,glioblastoma,and ***,proteasome inhibitors are not much effective due to their tolerance and singleness in other ***,further studies on their mechanisms of action and drug interactions are needed to investigate their therapeutic potential.

关键词： Bortezomib Cancer therapy Immunoproteasome Multiplemyeloma Proteasome 20S Proteasome inhibitor Thymoproteasom

Parallel Vision ■ Image Synthesis/Augmentation

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IEEE/CAA Journal of Automatica Sinica 2024年第3期11卷 782-784页

作者： Wenwen Zhang Wenbo Zheng Qiang Li Fei-yue Wang the School of Computer Science Shaanxi Normal UniversityXi’an 710119China the School of Computer Science and Technology Wuhan 430070China the State Key Laboratory for Management and Control of Complex Systems Institute of AutomationChinese Academy of SciencesBeijing 100190China

Dear Editor,Scene understanding is an essential task in computer *** ultimate objective of scene understanding is to instruct computers to understand and reason about the scenes as humans *** vision is a research fram... 详细信息

关键词： instru explanation computer

Weakly-supervised instance co-segmentation via tensor-based salient co-peak search

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Frontiers of Computer Science 2024年第2期18卷 83-92页

作者： Wuxiu QUAN Yu HU Tingting DAN Junyu LI yue ZHANG Hongmin CAI School of Computer Science Guangdong Polytechnic Normal UniversityGuangzhou 510665China School of Computer Science and Engineering South China University of TechnologyGuangzhou 510006China

Instance co-segmentation aims to segment the co-occurrent instances among two *** task heavily relies on instance-related cues provided by co-peaks,which are generally estimated by exhaustively exploiting all paired candidates in point-to-point ***,such patterns could yield a high number of false-positive co-peaks,resulting in over-segmentation whenever there are mutual *** tackle with this issue,this paper proposes an instance co-segmentation method via tensor-based salient co-peak search(TSCPS-ICS).The proposed method explores high-order correlations via triple-to-triple matching among feature maps to find reliable co-peaks with the help of co-saliency *** proposed method is shown to capture more accurate intra-peaks and inter-peaks among feature maps,reducing the false-positive rate of co-peak *** having accurate co-peaks,one can efficiently infer responses of the targeted *** on four benchmark datasets validate the superior performance of the proposed method.

关键词： weakly-supervised co-segmentation co-peak tensormatching deep network instance segmentation

Exercise-induced adaptation of neurons in the vertebrate locomotor system

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Journal of Sport and Health Science 2024年第2期13卷 160-171页

作者： yue Dai Yi Cheng Renkai Ge Ke Chen Liming Yang Key Lab of Adolescent Health Assessment and Exercise Intervention of Ministry of Education College of Physical Education and Health CareEast China Normal UniversityShanghai 200241China Shanghai Key Laboratory of Multidimensional Information Processing School of Communication and Electronic EngineeringEast China Normal UniversityShanghai 200241China School of Physical Education and Health Care East China Jiaotong UniversityNanchang 330013China Key Laboratory of High Confidence Software Technologies of Ministry of Education School of Computer SciencePeking UniversityBeijing 100871China

Vertebrate neurons are highly dynamic cells that undergo several alterations in their functioning and physiologies in adaptation to various external *** particular,how these neurons respond to physical exercise has long been an area of active *** of the vertebrate locomotor system’s adaptability suggest multiple mechanisms are involved in the regulation of neuronal activity and properties during *** this brief review,we highlight recent results and insights from the field with a focus on the following mechanisms:(a)alterations in neuronal excitability during acute exercise;(b)alterations in neuronal excitability after chronic exercise;(c)exercise-induced changes in neuronal membrane properties via modulation of ion channel activity;(d)exercise-enhanced dendritic plasticity;and(e)exercise-induced alterations in neuronal gene expression and protein *** hope is to update the community with a cellular and molecular understanding of the recent mechanisms underlying the adaptability of the vertebrate locomotor system in response to both acute and chronic physical exercise.

关键词： Dendritic plasticity Excitability Exercise Ion channel modulation Neuron adaptation

A scalable one-pot strategy for the development of polymer electrolytes adaptable to room-temperature high-voltage lithium batteries

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Chinese Chemical Letters 2024年第3期35卷 461-467页

作者： yue Guo Xinxin Qu Zhen Li Ruiyuan Tian Xiaokong Liu State Key Laboratory of Supramolecular Structure and Materials College of ChemistryJilin UniversityChangchun 130012China Key Laboratory of Physics and Technology for Advanced Batteries(Ministry of Education) College of PhysicsJilin UniversityChangchun 130012China

Poly(ethylene oxide)(PEO)polymer electrolytes(PEs)have been commercially applied in LiFePO_(4)||Li solid-state lithium batteries(SSLBs).However,it remains challenging to develop PEO-based PEs applicable to the high-voltage SSLBs with higher energy density,owing to the poor electrochemical stability of ***,we report a scalable strategy for fabricating PEO-based PEs with high-voltage compatibility,by exploiting a new mechanism to stabilize the cathode-electrolyte interface in the highvoltage *** protocol only involves a one-pot synthesis procedure to covalently crosslink the PEO chains,in the presence of high-content lithium bis(trifluoromethylsulphonyl)imide(LiTFSI)salts and N,N-dimethylformamide(DMF).LiTFSI-DMF supramolecular aggregates are formed and firmly embedded in the polymer network,endowing the PE with high room-temperature ionic *** dissociated and highly concentrated TFSI^-anions can enter the Helmholtz layer close to the high-voltage cathode,leading to the formation of a thin and homogeneous cathode electrolyte interface(CEI),mainly composed of LiF,on the *** CEI with high electrochemical stability can effectively stabilize the cathode-electrolyte interface,enabling long-term stable cycling of the high-voltage LiCoO_(2)||Li and nickelrich NCM_(622)||Li batteries at room *** simplicity and scalability of the strategy makes the reported PEO-based PE potentially applicable in high-voltage SSLBs in practice.

关键词： Lithium batteries Polymer electrolytes Poly(ethylene oxide) Energy density High-voltage cathodes