检索结果-南通市图书馆

Energy & Environmental Materials 2024年第1期7卷 301-312页

作者： Diab Khalafallah Weibo huang Mingjia Zhi Zhanglian Hong State Key Laboratory of Silicon Material School of Materials Science and EngineeringZhejiang University38 Zheda RoadHangzhou 310027China Mechanical Design and Materials Department Faculty of Energy EngineeringAswan UniversityP.O.Box 81521AswanEgypt

Herein,we demonstrate the synthesis of bifunctional nickel cobalt selenide@nickel telluride(Ni_(x)Co_(12-x)Se@NiTe)core-shell heterostructures via an electrodeposition approach for overall urea electrolysis and *** 3D vertically orientated NiTe dendritic frameworks induce the homogeneous nucleation of 2D Ni_(x)Co_(12-x)Se nanosheet arrays along similar crystal directions and bring a strong interfacial binding between the integrated active *** particular,the optimized Ni_(6)Co_(6)Se@NiTe with an interface coupling effect works in concert to tune the intrinsic *** only needs a low overpotential of 1.33 V to yield a current density of 10 mA cm^(-2)for alkaline urea ***,the full urea catalysis driven only by Ni_(6)Co_(6)Se@NiTe achieves 10 mA cm^(-2)at a potential of 1.38 V and can approach a constant level of the current response for 40 ***,the integrated Ni_(6)Co_(6)Se@NiTe electrode delivers an enhanced specific capacity(223 mA h g^(-1)at 1 A g^(-1))with a high cycling ***,a hybrid asymmetric supercapacitor(HASC)device based on Ni_(6)Co_(6)Se@NiTe exhibits a favorable rate capability and reaches a high energy density of 67.7 Wh kg^(-1)and a power density of 724.8 W kg^(-1)with an exceptional capacity retention of 92.4%after sequential 12000 cycles at 5 A g^(-1).

关键词： bifunctional Ni_(x)Co_(12-x)Se@NiTe core-shell electrodeposition heterointerfaces supercapacitors UOR

(FeO)_(2)FeBO_(3) nanoparticles attached on interconnected nitrogen-doped carbon nanosheets serving as sulfur hosts for lithium-sulfur batteries

在线全文

学校读者我要写书评

暂无评论

Frontiers of Materials Science 2024年第2期18卷 75-88页

作者： Junhai Wang Huaqiu huang Chen Chen Jiandong Zheng Yaxian Cao Sang Woo Joo Jiarui huang School of Material and Chemical Engineering Chuzhou UniversityChuzhou 239000China College of Mechanical Engineering Tongling UniversityTongling 244000China Key Laboratory of Functional Molecular Solids of the Ministry of Education College of Chemistry and Materials ScienceAnhui Normal UniversityWuhu 241002China School of Mechanical Engineering Yeungnam UniversityGyeongsanGyeongbuk 38541Republic of Korea

There are still many challenges including low conductivity of cathodes,shuttle effect of polysulfides,and significant volume change of sulfur during cycling to be solved before practical applications of lithium-sulfur(Li-S)*** this work,(FeO)_(2)FeBO_(3) nanoparticles(NPs)anchored on interconnected nitrogen-doped carbon nanosheets(NcNs)were synthesized,serving as sulfur carriers for Li-S batteries to solve such *** have the cross-linked network structure,which possess good electrical conductivity,large specific surface area,and abundant micropores and mesopores,enabling the cathode to be well infiltrated and permeated by the electrolyte,ensuring the rapid electron/ion transfer,and alleviating the volume expansion during the electrochemical *** addition,polar(FeO)_(2)FeBO_(3) can enhance the adsorption of polysulfides,effectively alleviating the polysulfide shuttle *** a current density of 1.0 A·g^(-1),the initial discharging and charging specific capacities of the(FeO)_(2)FeBO_(3)@NCNs-2/S electrode were obtained to be 1113.2 and 1098.3mA·h·g^(-1),*** 1000 cycles,its capacity maintained at 436.8 mA·h·g^(-1),displaying a decay rate of 0.08%per ***,combining NCNs with(FeO)_(2)FeBO_(3) NPs is conducive to the performance improvement of Li-S batteries.

关键词： (FeO)_(2)FeBO_(3) nitrogen-doped carbon nanosheet cathode lithium-sulfurbattery

Interannual evolution of the chemical composition,sources and processes of PM_(2.5)in Chengdu,China:Insights from observations in four winters

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Journal of Environmental Sciences 2024年第4期138卷 32-45页

作者： Junke Zhang Jiaqi Li Yunfei Su Chunying Chen Luyao Chen Xiaojuan huang Fangzheng Wang Yawen huang gehui Wang Faculty of geosciences and Environmental Engineering Southwest Jiaotong UniversityChengdu 611756China Department of Environmental Science&Engineering Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention(LAP3)Fudan UniversityShanghai 200438China Key Lab of geographic Information Science of the Ministry of Education School of Geographic SciencesEast China Normal UniversityShanghai 200241China

The air quality in China has improved significantly in the last decade and,correspondingly,the characteristics of PM_(2.5)have also *** studied the interannual variation of PM_(2.5)in Chengdu,one of the most heavily polluted megacities in southwest China,during the most polluted season(winter).Our results show that the mass concentrations of PM_(2.5)decreased significantly year-by-year,from 195.8±91.0μg/m~3in winter 2016 to 96.1±39.3μg/m^(3)in winter *** mass concentrations of organic matter(OM),SO_()4^(2-),NH_(4)^(+)and NO_(3)^(-)decreased by 49.6%,57.1%,49.7% and 28.7%,*** differential reduction in the concentrations of chemical components increased the contributions from secondary organic carbon and NO_(3)^(-)and there was a larger contribution from mobile *** contribution of OM and NO_(3)^(-)not only increased with increasing levels of pollution,but also increased year-by-year at the same level of *** sources of PM_(2.5)were identified:combustion sources,vehicular emissions,dust and secondary *** aerosols made the highest contribution and increased year-by-year,from 40.6%in winter 2016 to 46.3% in winter *** contrast,the contribution from combustion sources decreased from 14.4% to 8.7%.Our results show the effectiveness of earlier pollution reduction policies and emphasizes that priority should be given to key pollutants(e.g.,OM and NO_(3)^(-))and sources(secondary aerosols and vehicular emissions)in future policies for the reduction of pollution in Chengdu during the winter months.

关键词： PM_(2.5) Chemical composition Sources Interannual evolution Winter Chengdu

Tandem hydroalkylation and deoxygenation of lignin-derived phenolics to synthesize high-density fuels

在线全文

学校读者我要写书评

暂无评论

Chinese Journal of Chemical Engineering 2024年第2期66卷 104-109页

作者： Rui Yu Zhensheng Shen Yanan Liu Chengxiang Shi Juncong Qu Lun Pan Zhenfeng huang Xiangwen Zhan g Ji-Jun Zou Key Laboratory for green Chemical Technology of Ministry of Education School of Chemical Engineering and TechnologyTianjin UniversityTianjin 300072China Collaborative Innovative Center of Chemical Science and Engineering(Tianjin) Tianjin 300072China Haihe Laboratory of Sustainable Chemical Transformations Tianjin 300192China

Lignin is the most abundant naturally phenolic biomass,and the synthesis of high-performance renewable fuel from lignin has attracted significant *** propose the efficient synthesis of high-density fuels using simulated lignin cracked oil in tandem with hydroalkylation and deoxygenation ***,we investigated the reaction pathway for the hydroalkylation of phenol,which competes with the hydrodeoxygenation form *** then,we investigated the effects of metal catalyst types,the loading amount of metallic,acid dosage,and reactant ratio on the reaction *** phenol hydroalkylation and hydrodeoxygenation were balanced when 180℃ and 5 MPa H_(2)with the alkanes yield of 95%.By extending the substrate to other lignin-derived phenolics and simulated lignin cracked oil,we obtained the polycyclic alkane fuel with high density of 0.918 g·ml^(-1)and calorific value of41.2 MJ·L^(-1).Besides,the fuel has good low-temperature properties(viscosity of 9.3 mm^(2)·s^(-1)at 20℃ and freezing point below-55℃),which is expected to be used as jet *** work provides a promising way for the easy and green production of high-density fuel directly from real lignin oil.

关键词： High-density fuel Biofuel Hydrogenation Alkylation Lignin Phenolics

Scaling Laws Behind Penetrative Turbulence:History and Perspectives

在线全文

学校读者我要写书评

暂无评论

Advances in Atmospheric Sciences 2024年第10期41卷 1881-1900页

作者： Zijing DINg Ruiqi huang Zhen OUYANg School of Energy Science and Engineering Harbin Institute of Technology

An unstably stratified flow entering into a stably stratified flow is referred to as penetrative convection, which is crucial to many physical processes and has been thought of as a key factor for extreme weather conditions. Past theoretical,numerical, and experimental studies on penetrative convection are reviewed, along with field studies providing insights into turbulence modeling. The physical factors that initiate penetrative convection, including internal heat sources, nonlinear constitutive relationships, centrifugal forces and other complicated factors are summarized. Cutting-edge methods for understanding transport mechanisms and statistical properties of penetrative turbulence are also documented, e.g., the variational approach and quasilinear approach, which derive scaling laws embedded in penetrative turbulence. Exploring these scaling laws in penetrative convection can improve our understanding of large-scale geophysical and astrophysical motions. To better the model of penetrative turbulence towards a practical situation, new directions, e.g., penetrative convection in spheres, and radiation-forced convection, are proposed.

关键词： penetrative convection scaling law thermal convection turbulence

Absorbed Bioactive Compounds Replicate guanxinⅡ-Induced Endothelium-Associated in/ex vivo Vasodilation

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

Chinese Journal of Integrative Medicine 2024年第5期30卷 387-397页

作者： XU Min LIU Hao SU Meng-qing LI Lan YU Ai-ling CHEN Ken huang Yun-ke ZHAO Qiu-long huang Wen-ya huang Xi Institute of Traditional Chinese Medicine Related Comorbid Depression Nanjing University of Chinese MedicineNanjing 210029China Department of gynecology Women's HospitalZhejiang University School of MedicineHangzhou 310053China

Objective:To develop an interference-free and rapid method to elucidate guanxinⅡ(gXⅡ)'s representative vasodilator absorbed bioactive compounds(ABCs)among enormous ***:The contents of ferulic acid,tanshinol,and hydroxysafflor yellow A(FTA)in gXⅡ/rat serum after the oral administration of gXⅡ(30 g/kg)were detected using ultra-performance liquid chromatography-mass *** 18 rats were randomly assigned to the control group(0.9%normal saline),gXⅡ(30 g/kg)and FTA(5,28 and 77 mg/kg)by random number table *** coronary flow velocity-time integral(VTI),i.e.,coronary flow or coronary flow-mediated dilation(CFMD),and endothelium-intact vascular tension of isolated aortic rings were *** 12 h of exposure to blank medium or 0.5 mmol/L H_(2)O_(2),endothelial cells(ECs)were treated with post-dose gXⅡof supernatant from deproteinized serum(PgSDS,300μL PgSDS per 1 m L of culture medium)or FTA(237,1539,and 1510 mg/m L)for 10 min as control,H_(2)O_(2),PgSDS and FTA *** oxide(NO),vascular endothelial growth factor(VEgF),endothelin-1(ET-1),superoxide dismutase(SOD),malondialdehyde(MDA)and phosphorylated phosphoinositide 3 kinase(p-PI3K),phosphorylated protein kinase B(p-AKT),phosphorylated endothelial nitric oxide synthase(p-e NOS)were *** was developed as a gXⅡproxy of ex vivo herbal crude ***:PgSDS effectively eliminates false responses caused by crude gXⅡ*** doses equaled the contents in gXⅡ/its post-dose serum,FTA accounted for 98.17%of gXⅡ-added CFMD and 92.99%of PgSDS-reduced vascular *** ECs,FTA/PgSDS was found to have significant antioxidant(lower MDA and higher SOD,PgF,ET-1,PgSDS were markedly abolished by Ng-nitro-L-arginine methyl ester(L-NA,e NOS inhibitor)and wortmannin(PI3K/AKT inhibitor

关键词： ultra-performance liquid chromatography-mass spectrometry endothelium-dependent vasodilation herbal extract guanxinⅡ absorbed bioactive compound

Nb_(2)O_(5) nanocrystals decorated graphene composites as anode materials for high-performance dual-ion batteries

在线全文

学校读者我要写书评

暂无评论

Nano Research 2024年第3期17卷 1535-1541页

作者： Lei Wang Fei huang guoyin Zhu Zhihui Dai Jiangsu Collaborative Innovation Center of Biomedical Functional Materials Jiangsu Key Laboratory of Biofunctional MaterialsSchool of Chemistry and Materials ScienceNanjing Normal UniversityNanjing 210023China Institute of Advanced Materials and Flexible Electronics(IAMFE) School of Chemistry and Materials ScienceNanjing University of Information Science&TechnologyNanjing 210044China School of Chemistry and Molecular Engineering Nanjing Tech UniversityNanjing 211816China

Niobium oxide(Nb_(2)O_(5))is a promising material in photocatalytic,solar cell,electronic like electron field emitters,and especially lithium-ion batteries(LIBs)because of its adjustable morphologies,controllable crystal type,stable structure,and environmental ***,its low electrical conductivity lowers the rate performance and limits the practical applications in ***,we present a one-step solid-state synthesis of orthogonal Nb_(2)O_(5) nanocrystals/graphene composites(Nb_(2)O_(5)/g)as high-performance anode materials in *** from the nanoscale crystalline structure Nb_(2)O_(5) and highly-conductive graphene substrate,the as-prepared Nb_(2)O_(5)/g exhibits excellent electrochemical ***,a reversible structural phase transition between orthogonal Nb_(2)O_(5) and tetragonal Li1-xNbO_(2)(0g with graphite cathode based on PF6-intercalation/deintercalation mechanisms,Nb_(2)O_(5)/g||graphite dual-ion batteries(DIBs)full cell delivers good electrochemical performance in terms of cyclic performance and rate *** believe this work can provide a clear route towards developing advanced transition metal oxide/graphene composite anode and a comprehension of its electrochemical reaction mechanism.

关键词： niobium oxide graphene anode dual-ion batteries graphite intercalation

Stability of water yield in watersheds

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Science China Earth Sciences 2024年第2期67卷 483-496页

作者： Yu YAN Zhiyong LIU Xiaohong CHEN Liyan huang Center for Water Resources and Environment School of Civil EngineeringSun Yat-Sen UniversityGuangzhou510275China Southern Marine Science and Engineering guangdong Laboratory(Zhuhai) Zhuhai519082China

The hydrological system of a watershed is intricately influenced by both underlying characteristics and climate *** the variability in water yield is essential for effective water resources management and water security in the context of changing *** this study,we adopted the Budyko framework and leveraged simulations from the CMIP6 model to investigate the compensation effects of climate and underlying characteristics on watershed water *** on Taylor expansion and Budyko framework,we estimated the sensitivity of watershed water yield to climate and underlying characteristics(the first-and second-order partial derivatives).By combining external watershed characteristics(e.g.,water yield ratios and underlying characteristics)with internal sensitivity coefficients,this study further used vine copula and principal component analysis to quantify the stability of watershed water *** findings show:(1)Water-yield changes related to underlying characteristics could be offset by climate-related water-yield changes across all climate zones,maintaining the water yield ratio steady(i.e.,the compensation effects).(2)However,global watersheds will turn more sensitive to underlying characteristics and less sensitive to climate variation in the *** climate-and underlying-related sensitivities increase in watersheds with arid climates.(3)The stability of watershed water yield will gradually diminish in the *** 1901–1950to 2051–2100,the global stability of 280 watersheds drops from 0.054 to 0.021(i.e.,stability index identified by the joint probability).Particularly,the largest change in stability of water yield reaches-0.347±0.18 in arid *** semi-arid,semihumid,and humid regions,the changes are-0.039±0.010,-0.028±0.005,and-0.005±0.002,*** findings provide a reference for the future sustainable water resources development under climate change,highlighting the vulnerability of the water resources in ari

关键词： Hydrological system stability Compensation effects on water yield Sensitivities Budyko-Fu decomposition framework global watersheds

Fault-tolerant identity-based encryption from SM9

在线全文

学校读者我要写书评

暂无评论

Science China(Information Sciences) 2024年第2期67卷 104-117页

作者： Xiaohong LIU Xinyi huang Zhaohui CHENg Wei WU Fujian Provincial Key Laboratory of Network Security and Cryptology College of Computer and Cyber SecurityFujian Normal University Artificial Intelligence Thrust Information HubThe Hong Kong University of Science and Technology (Guangzhou) Olym Information Security Technology Ltd. Center for Applied Mathematics of Fujian Province School of Mathematics and StatisticsFujian Normal University

This paper initiates the formal study of attribute-based encryption within the framework of SM9,the Chinese National Cryptography Standard for Identity-Based Cryptography, by presenting two new faulttolerant identity-based encryption(FIBE) schemes. Our first scheme uses the same private-key/ciphertext structure as the original SM9 algorithm and operates in a small attribute universe. As a result, it can be effectively and smoothly integrated into the information systems using SM9. In the random oracle model,we prove that our scheme is ciphertext-indistinguishable against fuzzy selective-identity and chosen-plaintext attacks under the(k + 3)-DBDHI assumption. Our second design is a large universe FIBE scheme based on SM9 that is ciphertext-indistinguishable against chosen-plaintext attacks in the random oracle model under the(f, g)-gDDHE assumption. Finally, we compare the communication and computing costs of our schemes to those of other classical ones. The comparison shows that our schemes have comparable performance as others. We believe that our findings will accelerate the applications of SM9 in modern information systems such as cloud computing and blockchain.

关键词： attribute-based encryption identity-based encryption fault-tolerant SM9

Meromorphic Functions Sharing Two Values

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

Wuhan University Journal of Natural Sciences 2024年第1期29卷 7-12页

作者： ZHAO Ying huang Zhigang School of Mathematical Sciences Suzhou University of Science and TechnologySuzhou 215009JiangsuChina

Let f and g be two nonconstant meromorphic functions,and n be a positive *** f^(n)(z)and g^(n)(z)share 1 CM(counting multiplicities),f(z)and g(z)share∞IM(ignoring multiplicities),and N(r,1f)+N(r,1g)=S(r,f)+S(r,g),then either f(z)≡tg(z)or f(z)g(z)≡t,where t^(n)=*** an application,shared values problems of a meromorphic function related to its shifts and difference operators are also investigated.

关键词： meromorphic function shared values difference operator shift