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International Journal of Coal Science & Technology 2023年第3期10卷 24-40页

作者： Xin Lyu Tong zhang Liang yuan Juejing fang State Key Laboratory of Mining Response and Disaster Prevention and Control in Deep Coal Mines Anhui University of Science and TechnologyHuainan 232001China Institute of Energy Hefei Comprehensive National Science CenterHefei230031China

Under the carbon neutrality goal,coal enterprises must seek breakthroughs from abandoned mines,develop new resources in the new era,turn problems into countermeasures,and participate in the carbon emissions market,for contributing to the accomplishment of the national strategic goal of carbon *** this end,we investigated the relevant national policies and regulations to clarify the boundaries disclosed by the carbon information of enterprises,understood the development direction of carbon storage in abandoned mines,and clarified the transformation and development of carbon storage in aban-doned *** made a few suggestions:(1)China should learn from its past experience and other countries to develop the energy industry with Chinese characteristics and reform the economic system.(2)Coal enterprises must actively respond to the national carbon information disclosure policy,clarify their own responsibilities and carbon emission boundaries.(3)It is necessary to proactively obtain advanced knowledge and plan carbon storage pathways for abandoned mines.(4)Devel-opment problems of coal enterprises should be deduced using ***'dual carbon'goals should be achieved steadily step-by-step.(5)Three measures,*** the existing resource structure,coordinating the information of abandoned mines,and promoting the cultivation of scientific and technological talents.

关键词： Mining engineering Abandoned mines Carbon neutrality Carbon emission rights Carbon tax

Based on non-targeted metabolomics for differential components screening of Rosae Chinensis Flos and Rosae Rugosae Flos and their quality evaluation

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Traditional Medicine Research 2025年第2期10卷 1-15页

作者： Xu Liang Ni-Hui zhang Zhi-Lai Zhan Guang-Lu Chang Yan Gao Xia Li Wen-yuan Gao School of Pharmaceutical Science and Technology Faculty of MedicineTianjin UniversityTianjin 300193China State Key Laboratory for Quality Ensurance and Sustainable Use of Dao-di Herbs China Academy of Chinese Medical SciencesBeijing 100700China Key Laboratory of Modern Chinese Medicine Resources Research Enterprises Tianjin 300402China

Background:Rosa chinensis *** Rosa rugosa *** not only of ornamental value,but also edible flowers and the flower buds have been listed in the Chinese Pharmacopoeia as traditional *** two plants have some differences in efficacy,but the flower buds are easily confused for similar *** addition,large-scale cultivation of ornamental rose flowers may lead to a decrease in the effective components of medicinal ***,it is necessary to study the chemical composition and make quality evaluation of Rosae Chinensis Flos(Yueji)and Rosae Rugosae Flos(Meigui).Methods:In this study,40 batches of samples including Meigui and Yueji from different regions in China were collected to establish high-performance liquid chromatography ***,the fingerprints data was analyzed using principal component analysis,hierarchical cluster analysis,and partial least squares discriminant analysis analysis chemometrics to obtain information on intergroup differences,and non-targeted metabolomic techniques were applied to identify and compare chemical compositions of samples which were chosen from groups with large *** compounds were screened by orthogonal partial least-squares discriminant analysis and S-plot,and finally multi-component quantification was performed to comprehensively evaluate the quality of Yueji and ***:The similarity between the fingerprints of 40 batches roses and the reference print R was 0.73 to 0.93,indicating that there were similarities and differences between the *** principal component analysis and hierarchical cluster analysis of fingerprints data,the samples from different origins and varieties were intuitively divided into four *** least-squares discriminant analysis analysis showed that Meigui and Yueji cluster into two categories and the model was reliable.A total of 89 compounds were identified by high resolution mass spectrometry,mainly were flavonoids and flavon

关键词： Rosa chinensis Jacq. Rosa rugosa Thunb. metabolomics chemometrics multiple component quantification quality evaluation

Degradation of organic contaminants through the activation of oxygen using zero valent copper coupled with sodium tripolyphosphate under neutral conditions

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Journal of Environmental Sciences 2020年第4期32卷 375-384页

作者： Chengwu zhang Lishuang Xuan Jingyi zhang fang yuan Xianglong Kong Chuanyu Qin Key Laboratory of Groundwater Resources and Environment Ministry of EducationJilin UniversityChangchun 130021China Jilin Provincial Key Laboratory of Water Resources and Environment Jilin UniversityChangchun 130021China National and Local Joint Engineering Laboratory for Petrochemical Contaminated Site Control and Remediation Technology Jilin UniversityChangchun 130021China

In this study,sodium tripolyphosphate(STPP)was used to promote the removal of organic pollutants in a zero-valent copper(ZVC)/O2 system under neutral conditions for the first time.20 mg/L p-nitrophenol(PNP)can be completely decomposed within 120 min in the ZVC/O2/STPP *** PNP degradation process followed pseudo-first-order kinetics and the degradation rate of PNP gradually increased upon the decreasing ZVC particle *** optimal pH of the reaction system was *** mechanism investigation showed that Cu+generated by ZVC corrosion was the main reducing agent for the activation of 02 to produce ROS.-OH was identified as the only ROS formed during the degradation of PNP and its production pathway was the double-electron activation of O2(O2→H2 O2→·OH).In this process,STPP did not only promote the release of Cu+through its complexation,but also promoted the production of OH by reducing the redox potential of Cu2+/Cu+.In addition,we could initiate and terminate the reaction by controlling the *** pH8.1,the reaction was *** was recycled to continuously promote the corrosion of ZVC and O2 activation as long as the pH was<*** study provided a new and efficient way for O2 activation and organic contaminants removal.

关键词： Sodium tripolyphosphate Zero valent copper corrosion Oxygen activation pH control

Removal of refractory organics and heavy metals in landfill leachate concentrate by peroxi-coagulation process

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Journal of Environmental Sciences 2022年第6期34卷 43-51页

作者： Dun Liu Ying yuan Yuquan Wei Hao zhang Yanxiao Si fang zhang School of Environment and State Key Joint Laboratory of Environment Simulation and Pollution Control Tsinghua UniversityBeijing 100084China Beijing Advanced Innovation Center for Big Data-based Precision Medicine Beihang UniversityBeijing 100191China

Landfill leachate is a complex effluent and it is difficult to deal with. Electrochemical methods have been considered as a promising alternative technology for treatment of landfill leachate with refractory organic contaminants and heavy metals. Peroxi-coagulation(PC)process with iron anode and modified graphite felt cathode was developed for efficient landfill leachate concentrate treatment. Compared to electro-Fenton(EF) and electrocoagulation(EC) processes, the PC process was more cost-effective due to the combined action of·OH oxidation and iron hydroxides coagulation. A maximal TOC removal of 77.2% ± 1.4% was obtained after 360 min at initial p H = 5.0 and current density of 10 m A/cm^(2). After the PC process, concentrations of all seven heavy metals in the final effluents were below the allowable emission limits given by the present regulatory standards. The method preference for heavy metal removal was PC > EC > EF. Based on the three-dimensional fluorescence spectroscopy coupled with regional integration analysis during the PC treatment, the florescence peaks of both humic acids and fulvic acids disappeared after treatment for 360min. Decreasing trends were observed in the fluorescent regional standard volumes for aromatic protein Ⅰ(31.4%), aromatic protein Ⅱ(63.7%), fulvic acid-like(69.5%), soluble microbial by-product-like(75%) and humic acid-like regions(76.3%). The results indicate that comparing to the EF and EC process, the PC process provide a promising and more cost-effective alternative for the treatment of landfill leachate concentrate.

关键词： Landfill leachate Peroxi-coagulation Electro-Fenton Electrocoagulation Modified cathode

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双针-板结构脉冲气泡放电等离子体固氮研究

原子与分子物理学报 2025年第6期42卷 122-128页

作者：赵少伟张丽方志南京工业大学电气工程与控制科学学院南京211816

大气压低温等离子体可以利用空气直接进行氧化固氮,具有反应条件温和、参数灵活可控、避免温室气体排放等优点.本文利用双针-板电极在水中形成气泡放电等离子体,以空气为放电气体进行了固氮研究,分析了产物浓度和固氮能耗的影响因素.研... 详细信息

大气压低温等离子体可以利用空气直接进行氧化固氮,具有反应条件温和、参数灵活可控、避免温室气体排放等优点.本文利用双针-板电极在水中形成气泡放电等离子体,以空气为放电气体进行了固氮研究,分析了产物浓度和固氮能耗的影响因素.研究结果表明,等离子体中含有丰富的氮原子、氧原子、氢原子、激发态氮分子等活性物种,可高效合成硝态含氮产物.研究发现,脉冲参数、电极间隙、工作气体组分对气泡放电等离子体的固氮性能有重要影响.装置最高NO~-_x合成速率为19.2μmol/min,最小能耗约为11 MJ/mol.此外还发现,电极间隙为6 mm时,固氮性能最优;空气中增加适量氧气(氧气/氮气比例为0.4)可以增强产物合成,降低能耗.

关键词：低温等离子体纳秒脉冲放电气液放电固氮

Mediating role of health literacy in the relationship between social isolation and psychological distress among pre-frail older adults

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World Journal of Psychiatry 2025年第1期15卷 137-144页

作者： Juan fang Li-Hui Li Ming-Qian He Yue Ji Dong-Yan Lu Li-Bing zhang Jin-Lan Yao School of Medicine Huzhou UniversityHuzhou 313000Zhejiang ProvinceChina

BACKGROUND Frailty has become a significant public health *** recent increase in the number of frail older adults has led to increased attention being paid to psycho-logical care services in *** social isolation of pre-frail older adults can impact their psychological *** To explore the mediating effect of health literacy between social isolation and psychological distress among communitydwelling older adults with *** This descriptive cross-sectional study was conducted with 254 pre-frail older individuals aged 60 years and *** isolation,health literacy,and psycholo-gical distress were comprehensively measured using the Lubben Social Network Scale-6,12-item Short-Form Health Literacy Questionnaire,and the Kessler Psy-chological Distress *** were evaluated using the SPSS 27.0 package program and the PROCESS macro *** statistical analyses,correlation analyses,and bootstrap mediation tests were used to assess associations between the *** The results showed that social isolation had an effect on health literacy among pre-frail older adults(β=0.240,P<0.001),social isolation impact on psycho-logical distress pre-frail older adults(β=-0.415,P<0.001);health literacy was identified effect on psychological distress among pre-frail older persons(β=-0.307,P<0.001).Health literacy partially mediated the relationship between social isolation and psychological distress among community-dwelling older adults with pre-frailty,with a mediation effect of-0.074,accounting for 17.83%of the total effect.

关键词： Frail Ageing Psychological distress Health literacy Social isolation

Anti-apoptotic effects of recombinant human granulocyte colony-stimulating factor in focal cerebral ischemic rats

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Neural Regeneration Research 2011年第11期6卷 839-844页

作者： Xia yuan Shiming zhang Wanli Dong Qi fang Department of Neurology First Affiliated Hospital of Soochow University Suzhou 215006 Jiangsu Province China Department of Neurosurgery First Affiliated Hospital of Soochow University Suzhou 215006 Jiangsu Province China

The neuroprotective effects of granulocyte colony-stimulating factor in cerebral ischemia/reperfusion injury are currently contentious. The present study examined the effects of subcutaneous injection of recombinant human granulocyte colony-stimulating factor （50 pg/kg） over 5 days in a model of cerebral ischemia/reperfusion with intraluminal filament occlusion in rats. The results indicated that recombinant human granulocyte colony-stimulating factor reduced brain infarct volume following cerebral ischemia/reperfusion injury in rats, down-regulated the expression of caspase-3 mRNA （a key protease for apoptosis in the cerebral ischemia zone）, lowered the rate of neuronal apoptosis in the cerebral ischemia zone, and notably ameliorated neurological function. These results indicate that recombinant human granulocyte colony-stimulating factor has anti-apoptotic effects on neurons following focal cerebral ischemia/reperfusion injury, and exerts neuroprotective effects.

关键词： recombinant human granulocyte colony-stimulating factor cerebral ischemia/ reperfusion injury anti-apoptosis neural regeneration

Wellposedness for anisotropic rotating fluid equations

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Applied Mathematics(A Journal of Chinese Universities) 2012年第1期27卷 9-33页

作者： fang Dao-yuan WANG Su-mei zhang Ting Department of Mathematics Zhejiang UniversityHangzhou 310027China

The weUposedness problem for an anisotropic incompressible viscous fluid in R3, ro- tating around a vector B（t, x）：= （b1 （t, x）, b2 （t, x）, b3 （t, x））, is studied. The global wellposedness in the homogeneous case （B = e3） with sufficiently fast rotation in the space B0,1/2 is proved. In the inhomogeneous case （B = B（t, xh））, the global existence and uniqueness of the solution in B0,1/2 are obtained, provided that the initial data are sufficient small compared to the horizontal viscosity. Furthermore, we obtain uniform local existence and uniqueness of the solution in the x same function space. We also obtain propagation of the regularity in B2,11/2 under the additional assumption that B depends only on one horizontal space variable.

关键词： the anisotropic Navier-Stokes-Coriolis equation wellposedness anisotropic.

A colorimetric and ratiometric fluorescent chemosensor based on furan-pyrene for selective and sensitive sensing Al^(3+)

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Chinese Chemical Letters 2016年第11期27卷 1673-1678页

作者： yuan zhang yuan fang Nai-zhang Xu Ming-Qun zhang Guan-Zhi Wu Cheng Yao College of Chemistry and Molecular Engineering Nanjing Tech University College of Overseas Education Nanjing Tech University State Key Laboratory of Coordination Chemistry Nanjing University

A new pyrene derivative BF bearing a furan group was synthesized via a one-step reaction as a colorimetric and ratiometric chemosensor for Al3＋ in ethanol-H20 （9：1, v/v, pH 7.2, HEPES buffer） solution. This chemosensor could selectively recognize Al3＋ in the presence of other competing ions. Low limit of detection （LOD） and high association constant revealed its superior sensitivity and binding affinity toward Al3＋, Besides, the probe BF performed perfectly in a reversibility test using EDTA. The mechanism of the interaction has been confirmed by 1H NMR titration. Importantly, chemosensor BF has also been utilized to detect Al3＋ on test paper strips, which showed its ootential for practical applications.

关键词： Pyrene Al3+ Colorimetric Ratiometric Chemosensor Application

Geochemical and Mineralogical Investigation on Different Types of Cenozoic Basalts in the Sanshui Basin:Implications for Magma Mixing Processes

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Journal of Earth Science 2019年第4期30卷 754-762页

作者： Wei zhang Nianqiao fang Xiaobo yuan Lukai Cui Key Laboratory of Marine Geology and Environment Institute of OceanologyChinese Academy of SciencesQingdao 266071China School of Ocean Sciences China University of GeosciencesBeijing 100083China College of Earth Sciences East China Institute of TechnologyNanchang 330013China

Two kinds of basalts with different chemical compositions were obtained in the Sanshui Basin,they share the same eruption period. Although they have significant differences in major and trace element concentrations,their isotopic ratios suggest a similar magma source. Based on mineral geochemical analysis,orthopyroxene with reaction rim and zoned clinopyroxene are observed in Zidong(ZD)basalts,but not found in Wangjiegang(WJG) basalts. Linear scanning of these minerals suggests compositional variation between within-plate tholeiite and within-plate alkali-basalt. Presence of a doublelayer magma chamber under the Sanshui Basin,and occurrence of magma mixing between upper and lower chambers is proposed. This magma mixing leads to different chemical composition and mineral constitution of two kinds of basalts,as well as reaction rim and compositional variation of minerals in ZD basalts.

关键词： Sanshui Basin alkali basalt tholeiite magma mixing magma chamber geochemistry