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Frontiers in Energy 2024年第2期18卷 206-222页

作者： cheng yuan Shiming ZHANG Jiujun ZHANG Institute for Sustainable Energy/College of Sciences Shanghai UniversityShanghai 200444China

Platinum(Pt)-based materials are still the most efficient and practical catalysts to drive the sluggish kinetics of cathodic oxygen reduction reaction(ORR)in proton exchange membrane fuel cells(PEMFCs).However,their catalysis and stability performance still need to be further improved in terms of corrosion of both carbon support and Pt catalyst particles as well as Pt loading *** on the developed synthetic strategies of alloying/nanostructuring Pt particles and modifying/innovating supports in developing conventional Pt-based catalysts,Pt single-atom catalysts(Pt SACs)as the recently burgeoning hot materials with a potential to achieve the maximum utilization of Pt are comprehensively reviewed in this *** design thoughts and synthesis of various isolated,alloyed,and nanoparticlecontained Pt SACs are *** single-atomic Pt coordinating with non-metals and alloying with metals as well as the metal-support interactions of Pt single-atoms with carbon/non-carbon supports are emphasized in terms of the ORR activity and stability of the *** advance further research and development of Pt SACs for viable implementation in PEMFCs,various technical challenges and several potential research directions are outlined.

关键词： oxygen reduction electrocatalysis Pt singleatom catalysts conventional Pt-based catalysts design thoughts and synthesis metal-support interactions

Photonic neuromorphic architecture for tens-of-task lifelong learning

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Light(Science & Applications) 2024年第3期13卷 519-530页

作者： yuan cheng Jianing Zhang Tiankuang Zhou Yuyan Wang Zhihao Xu Xiaoyun yuan Lu Fang Sigma Laboratory Department of Electronic EngineeringTsinghua UniversityBeijing 100084China Beijing National Research Center for Information Science and Technology(BNRist) Beijing 100084China Institute for Brain and Cognitive Science Tsinghua University(THUIBCS)Beijing 100084China

Scalable,high-capacity,and low-power computing architecture is the primary assurance for increasingly manifold and large-scale machine learning *** electronic artificial agents by conventional power-hungry processors have faced the issues of energy and scaling walls,hindering them from the sustainable performance improvement and iterative multi-task *** to another modality of light,photonic computing has been progressively applied in high-efficient neuromorphic ***,we innovate a reconfigurable lifelong-learning optical neural network(L2 ONN),for highly-integrated tens-of-task machine intelligence with elaborated algorithm-hardware *** from the inherent sparsity and parallelism in massive photonic connections,L2 ONN learns each single task by adaptively activating sparse photonic neuron connections in the coherent light field,while incrementally acquiring expertise on various tasks by gradually enlarging the *** multi-task optical features are parallelly processed by multi-spectrum representations allocated with different *** evaluations on freespace and on-chip architectures confirm that for the first time,L2 ONN avoided the catastrophic forgetting issue of photonic computing,owning versatile skills on challenging tens-of-tasks(vision classification,voice recognition,medical diagnosis,etc.)with a single ***,L2 ONN achieves more than an order of magnitude higher efficiency than the representative electronic artificial neural networks,and 14×larger capacity than existing optical neural networks while maintaining competitive performance on each individual *** proposed photonic neuromorphic architecture points out a new form of lifelong learning scheme,permitting terminal/edge AI systems with light-speed efficiency and unprecedented scalability.

关键词： life neural versatile

Defect-mode and Fabry-Perot resonance induced multi-band nonreciprocal thermal radiation

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Science China(Technological Sciences) 2024年第8期67卷 2405-2412页

作者： CHEN ZiHe YU ShiLv yuan cheng CUI XinYou HU Run School of Energy and Power Engineering Huazhong University of Science and TechnologyWuhan 430074China Wuhan Fiberhome Fuhua Electric Co. Ltd.Wuhan 430074China

According to Kirchhoff's radiation law,the spectral-directional absorptivity(α)and spectral-directional emissivity(e)of an object are widely believed to be identical,which places a fundamental limit on photonic energy conversion and *** introduction of Weyl semimetals and magneto-optical(MO)materials into photonic crystals makes it possible to violate Kirchhoff's law,but most existing work only report the unequal absorptivity and emissivity spectra in a single band,which cannot meet the requirements of most practical ***,we introduce a defect layer into the structure composed of one-dimensional(1D)magnetophotonic crystal and a metal layer,which realizes dual-band nonreciprocal thermal radiation under a 3-T magnetic field with an incident angle of 60°.The realization of dual-band nonreciprocal radiation is mainly due to the Fabry-Perot(FP)resonance occurring in the defect layer and the excitation of Tamm plasmon,which is proved by calculating the magnetic field *** addition,the effects of incident angle and structural parameters on nonreciprocity are also *** is more,the number of nonreciprocal bands could be further increased by tuning the defect layer *** the defect layer thickness increases to 18.2μm,tri-band nonreciprocal thermal radiation is realized due to the enhanced number of defect modes in the photonic band gap and the FP resonance occurring in the defect ***,the effect of defect location on nonreciprocity is also *** present work provides a new way for the design of multi-band or even broad-band nonreciprocal thermal emitters.

关键词： Kirchhoff's law multi-band nonreciprocal thermal radiation magnetophotonic crystal Tamm plasmon defect layer Fabry-Perot resonance

DPK:Deep Neural Network Approximation of the First Piola-Kirchhoff Stress

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Advances in Applied Mathematics and Mechanics 2024年第1期16卷 75-100页

作者： Tianyi Hu Jerry Zhijian Yang cheng yuan Institute of Artificial Intelligence School of Computer ScienceWuhan UniversityWuhanHubei 430072China School of Mathematics and Statistics Wuhan UniversityWuhanHubei 430072China Hubei Key Laboratory of Computational Science Wuhan UniversityWuhanHubei 430072China

This paper presents a specific network architecture for approximation of the first Piola-Kirchhoff *** neural network enables us to construct the constitutive relation based on both macroscopic observations and atomistic simulation *** contrast to traditional deep learning models,this architecture is intrinsic symmetric,guarantees the frame-indifference and material-symmetry of ***,we build the approximation network inspired by the Cauchy-Born rule and virial stress *** numerical results and theory analyses are presented to illustrate the learnability and effectiveness of our network.

关键词： Piola-Kirchhoff stress deep neural networks Cauchy-Born rule

New insight into Ca^(2+)-permeable channel in plant immunity

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Journal of Integrative Plant Biology 2024年第3期66卷 623-631页

作者： Wei Wang Hang-yuan cheng Jian-Min Zhou State Key Laboratory of Plant Genomics Institute of Genetics and Developmental BiologyChinese Academy of SciencesBeijing 100101China CAS Center for Excellence in Biotic Interactions University of Chinese Academy of SciencesBeijing 100049China College of Advanced Agricultural Sciences University of Chinese Academy of SciencesBeijing 100049China Hainan Yazhou Bay Seed Laboratory Sanya 572025China

Calcium ions(Ca^(2+)) are crucial intracellular second messengers in eukaryotic cells. Upon pathogen perception, plants generate a transient and rapid increase in cytoplasmic Ca^(2+)levels, which is subsequently decoded by Ca^(2+)sensors and effectors to activate downstream immune responses. The elevation of cytosolic Ca^(2+)is commonly attributed to Ca^(2+)influx mediated by plasma membranelocalized Ca^(2+)–permeable channels. However, the contribution of Ca^(2+)release triggered by intracellular Ca^(2+)-permeable channels in shaping Ca^(2+)signaling associated with plant immunity remains poorly understood. This review discusses recent advances in understanding the mechanism underlying the shaping of Ca^(2+)signatures upon the activation of immune receptors, with particular emphasis on the identification of intracellular immune receptors as non-canonical Ca^(2+)-permeable channels. We also discuss the involvement of Ca^(2+)release from the endoplasmic reticulum in generating Ca^(2+)signaling during plant immunity.

关键词： Ca^(2+)-permeable channels endoplasmic reticulum phosphorylation plant immunity resistosome

Inner-shell ionization cross sections of atoms by positron impact

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Communications in Theoretical Physics 2024年第6期76卷 142-147页

作者： yuan-cheng Wang Jia Ma Li-Guang Jiao Stephan Fritzsche College of Physical Science and Technology Shenyang Normal UniversityShenyang 110034China Helmholtz-Institut Jena D-07743 JenaGermany GSI Helmholtzzentrum für Schwerionenforschung GmbH D-64291 DarmstadtGermany College of Science Shenyang Aerospace UniversityShenyang 110136China College of Physics Jilin UniversityChangchun 130012China Theoretisch-Physikalisches Institut Friedrich-Schiller-Universität Jena07743 JenaGermany

The relativistic binary-encounter-Bethe model with Wannier-type threshold law is employed to obtain the inner-shell ionization cross sections of multi-electron atoms(Ni,Cu,Y,Ag,Au,Yb,Ta,and Pb)for positron impact energies from the thresholds up to 105ke *** is good agreement between the present calculations and the experimental *** constant in the acceleration term derived from the Wannier law is determined to be 0.2 and 0.5 for the K-and L-shells,respectively.

关键词： positron scattering ionization cross section binary-encounter-Bethe model

Printable,flexible ceramic fiber paper based on electrospinning

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Rare Metals 2024年第6期43卷 2739-2746页

作者： Yong-Shuai Xie yuan cheng Yang Lyu Rui Li Jie-Cai Han National Key Laboratory of Science and Technology on Advanced Composites in Special Environments Harbin Institute of TechnologyHarbin 150001China State Key Laboratory of Intelligent Manufacturing Equipment and Technology Huazhong University of Science and TechnologyWuhan 430074China

Based on the fact that it is challenging for the polymer flexible circuit substrates to meet the requirements of serving in high-temperature environments,this work proposed the idea of using printable ceramic fiber paper as a high-temperature flexible circuit substrate.A ceramic fiber paper with all ceramic components had been developed via electrospinning,solving the problems of low strength and severe strength drop at high temperatures of traditional ceramic fiber *** tensile strength of the prepared ceramic fiber paper is 2.63 MPa,and the reliable service temperature is 1200℃.Its bulk density is about 1.5 times that of traditional ceramic fiber *** can be printed with patterns by commercial inkjet printers like ordinary printing paper and has excellent *** feasibility of ceramic fiber paper as a flexible circuit substrate was verified by constructing a simple *** the fiber paper is significantly bent,the circuit still forms a complete path,which proves that it has a strong application potential for high-temperature flexible circuit substrate and is expected to promote the development of flexible electronic devices serving at extreme high-temperature environments.

关键词： Ceramic fiber paper High temperature Inkjet printing Flexible electronic

Efficient piezo-assisted near-infrared-light-driven Cr(Ⅵ)reduction over Bi_(2)S_(3) nanowires transformed from ultrathin Bi_(2)WO_(6) nanosheets

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Rare Metals 2024年第9期43卷 4333-4343页

作者： Qiang Zhang yuan-Hao cheng Wei Liu Hui-Nan Che Yan-Hui Ao Key Laboratory of Integrated Regulation and Resource Development On Shallow Lakes Ministry of EducationCollege of EnvironmentHohai UniversityNanjing 210098China

The utilization of piezo-photocatalytic technol ogy for environmental remediation under full spectrum solar light is promising but still ***,one dimensional Bi_(2)S_(3)nanowires,which can utilize both mechanical energy and near-infrared(NIR)light to remov hexavalent chromium(Cr(Ⅵ))efficiently,were synthe sized by a restrained growth *** reaction rat constants of Cr(Ⅵ)reduction in piezo-photocatalyti process under NIR(800–2500 nm)reached 0.334 min^(-1)which were 3.2 and 12.4 times as that of single piezo and photocatalytic *** formation of polarized electri fields and one-dimensional structure allow ultrafast sepa ration of charge carriers,thereby promoting the catalyti ***,due to the strong penetrability o NIR light,the piezo-photocatalysis performance in turbid solutions under NIR light(0.188 min^(-1))was even com parable to that under visible light(0.186 min^(-1)).Thi study provides a new concept on the development of piezo photocatalytic technology for environmental remediation by utilization of NIR light and natural mechanical energy.

关键词： Piezo-photocatalysis NIR light Bi_(2)S_(3)nanowires Cr(Ⅵ)

A Fluorine-Functionalized 3D Covalent Organic Framework with Entangled 2D Layers

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Chinese Journal of Polymer Science 2024年第8期42卷 1210-1216页

作者： Li-Bang Xiao Zi-Han Wu Jun-Jie Xin yuan-Peng cheng Bo Gui Jun-Liang Sun cheng Wang College of Chemistry and Molecular Sciences Wuhan UniversityWuhan 430072China College of Chemistry and Molecular Engineering Beijing National Laboratory for Molecular SciencesPeking UniversityBeijing 100871China

Constructing three dimensional(3D)covalent organic frameworks(COFs)through the entanglement of two dimensional(2D)nets is a promising but underdeveloped ***,we report the design and synthesis of a fluorine functionalized 3DCOF(3D-An-COF-F)formed by entangled 2D sql *** structure of 3D-An-COF-F was determined by the combination of continuous rotation electron diffraction technique and modelling based on the chemical information from real ***,compared to the isostructural 3D-An-COF without F atom s,3DAn-COF-F showed an improved CO_(2)sorption ability and higher CO_(2)/N_(2)*** study not only demonstrated the generality of constructing 3D COFs with entangled 2D nets by introducing bulky groups vertically in planar building blocks,but also will expand the diversity of 3D COFs for various applications.

关键词： 3D covalent organic frameworks Fluorine Entangled 2D layers Electron diffraction CO_(2)adsorption

p-wave resonances in the exponential cosine screened Coulomb potential

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Communications in Theoretical Physics 2024年第7期76卷 105-113页

作者： yuan-cheng Wang Li Guang Jiao Aihua Liu Yew Kam Ho Stephan Fritzsche College of Physical Science and Technology Shenyang Normal UniversityShenyang 110034China College of Physics Jilin UniversityChangchun 130012China Helmholtz-Institut Jena D-07743 JenaGermany GSI Helmholtzzentrum fur Schwerionenforschung GmbH D-64291 DarmstadtGermany Institute of Atomic and Molecular Physics Jilin UniversityChangchun 130012China Institute of Atomic and Molecular Sciences Academia SinicaTaipei 10617TaiwanChina

We perform benchmark calculations of the p-wave resonances in the exponentially cosine screened Coulomb potential using the uniform complex-scaling generalized pseudo-spectral *** present results show significant improvement in calculation accuracy compared to previous predictions and correct the misidentification of resonance electron configuration in previous *** is found that the resonance states approximately follow an n^(2)-scaling law which is similar to the bound *** birth of a new resonance would distort the trajectory of an adjacent higher-lying resonance.

关键词： complex-scaling method shape resonance generalized pseudospectral method exponential cosine screened Coulomb potential