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Enhanced potassium storage of carbon nanofibers as binderfree anodes enabled by coupling ultra-small amorphous Sb_(2)O_(3),graphene modification and sulfur doping

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Rare Metals 2024年第1期43卷 51-64页

作者： Zhao Huang yu-kang lou Lin Peng yuan Peng Meng-Meng Wang Ming Zhang College of Railway Transportation Hunan University of TechnologyZhuzhou 412007China College of Semiconductors(College of Integrated Circuits) Changsha Semiconductor Technology and Application Innovation Research InstituteHunan UniversityChangsha 410082China Key Laboratory for Micro-Nano Optoelectronic Devices of Ministry of Education College of Semiconductors(College of Integrated Circuits)Hunan UniversityChangsha 410082China

Considering the intrinsic advantages of natural copiousness and cost-effectiveness of potassium resource,potassium-ion batteries(KIBs) are booming as prospective alternatives to lithium-ion batteries(LIBs) in large-scale energy storage scenarios. Nevertheless, lacking desirable electrodes for reversibly hosting the bulky K+hinders the widespread application of KIBs, and it needs to be urgently solved. Hereon, the porous S-doped Sb_(2)O_(3)-graphene-carbon(SAGC) nanofibers are manufactured through an adjustable and facile approach, which involves electrospinning, in situ etching and sulfuration. The synthesized SAGC is featured by the ultra-small amorphous Sb_(2)O_(3) homogeneously wrapped inside the carbon matrix, as well as the co-incorporation of graphene and sulfur. Tentatively,the SAGC nanofiber sheets are applied as binder-free anodes for KIBs, exhibiting a prominent cycling life(256.72 m Ah·g^(-1) over 150 cycles at 100 m A·g^(-1)) and rate·g^(-1) over 100 cycles at 1 A·g^(-1)). The positive synergy among all the active components accounts for the distinguished performances of the SAGC. By reinforcing the tolerability to the swelling stress, producing the valid electrochemical active sites, and promoting the charge transferring for reversible K+uptake, the SAGC finally renders the excellent cyclability, capacity, and rate capability. Moreover, the extrinsic electrochemical pseudocapacitance characteristics induced by the porous carbon substrate elevate the K-storage capacity of the SAGC as well. It is hoped that the conclusions drawn may offer new insights into a direction for the high-performance binderfree KIB anodes.

关键词： S-doped Sb_(2)O_(3)-graphene-carbon Nanofibers Binder-free Anodes Potassium-ion batteries

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Preparation of silver nanoparticles through the reduction of straw-extracted lignin and its antibacterial hydrogel

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International Journal of Minerals,Metallurgy and Materials 2025年第2期32卷 504-514页

作者： lou Zhang Shuo Li Fu Tang Jingkai Zhang yuetong kang Hean Zhang Lidong Li State Key Laboratory for Advanced Metals and Materials School of Materials Science and EngineeringUniversity of Science and Technology BeijingBeijing 100083China

Silver nanoparticles(Ag NPs)have attracted attention in the field of biomaterials due to their excellent antibacterial ***,the reducing and stabilizing agents used for the chemical reduction of Ag NPs are usually toxic and may cause water *** this work,Ag NPs(31.2 nm in diameter)were prepared using the extract of straw,an agricultural waste,as the reducing and stabilizing *** analysis revealed that the straw extract contained lignin,the structure of which possesses phenolic hydroxyl and methoxy groups that facilitate the reduction of silver salts into Ag *** surfaces of Ag NPs were negatively charged due to the encapsulation of a thin layer of lignin molecules that prevented their *** the prepared Ag NPs were added to the precursor solution of acrylamide,free radical polymerization was triggered without the need for extra heating or light irradiation,resulting in the rapid formation of an Ag NP-polyacrylamide composite *** inhibition zone test proved that the composite hydrogel possessed excellent antibacterial ability due to the presence of Ag *** prepared hydrogel may have potential applications in the fabrication of biomedical materials,such as antibacterial dressings.

关键词： silver nanoparticles hydrogel straw extraction antibacterial

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Study of the Transport Behavior of Multispherical Proppant in Intersecting Fracture Based on Discrete Element Method

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Energy Engineering 2025年第1期122卷 185-201页

作者： Chengyong Peng JianshuWu Mao Jiang Biao Yin Yishan lou CNOOC Research Institute Company Limited Beijing100028China School of Petroleum Engineering Yangtze UniversityWuhan430100China Hubei Key Laboratory of Oil and Gas Drilling and Production Engineering(Yangtze University) Wuhan430100China

To analyze the differences in the transport and distribution of different types of proppants and to address issues such as the short effective support of proppant and poor placement in hydraulically intersecting fractures,this study considered the combined impact of geological-engineering factors on *** reservoir production parameters and the discrete elementmethod,multispherical proppants were ***,a 3D fracture model,based on the specified conditions of the L block,employed coupled(Computational Fluid Dynamics)CFD-DEM(Discrete ElementMethod)for joint simulations to quantitatively analyze the transport and placement patterns of multispherical proppants in intersecting *** indicate that turbulent kinetic energy is an intrinsic factor affecting proppant ***,the efficiency of placement and migration distance of low-sphericity quartz sand constructed by the DEM in the main fracture are significantly reduced compared to spherical ceramic proppants,with a 27.7%decrease in the volume fraction of the fracture surface,subsequently affecting the placement concentration and damaging fracture *** to small-angle fractures,controlling artificial and natural fractures to expand at angles of 45°to 60°increases the effective support length by approximately 20.6%.During hydraulic fracturing of gas wells,ensuring the fracture support area and post-closure conductivity can be achieved by controlling the sphericity of proppants and adjusting the perforation direction to control the direction of artificial fractures.

关键词： Hydraulic fracturing discrete element method proppant sphericity CFD-DEM

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Smart Cellulose‑Based Janus Fabrics with Switchable Liquid Transportation for Personal Moisture and Thermal Management

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Nano-Micro Letters 2025年第1期17卷 333-347页

作者： Jianfeng Xi Yanling lou Liucheng Meng Chao Deng Youlu Chu Zhaoyang Xu Huining Xiao Weibing Wu Jiangsu Co‑Innovation Center of Efficient Processing and Utilization of Forest Resources International Innovation Center for Forest Chemicals and MaterialsJiangsu Provincial Key Lab of Sustainable Pulp and Paper Technology and Biomass MaterialsNanjing Forestry UniversityNanjing 210037People’s Republic of China College of Materials Science and Engineering Nanjing Forestry UniversityNanjing 210037People’s Republic of China Department of Chemical Engineering University of New BrunswickFrederictonNB E3B 5A3Canada Macromolecular Chemistry and Bavarian Polymer Institute University of BayreuthBayreuth 95440Germany

The Janus fabrics designed for personal moisture/thermal regulation have garnered significant attention for their potential to enhance human ***,the development of smart and dynamic fabrics capable of managing personal moisture/thermal comfort in response to changing external environments remains a ***,a smart cellulose-based Janus fabric was designed to dynamically manage personal moisture/*** cotton fabric was grafted with N-isopropylacrylamide to construct a temperature-stimulated transport ***,hydrophobic ethyl cellulose and hydrophilic cellulose nanofiber were sprayed on the bottom and top sides of the fabric to obtain wettability *** fabric exhibits anti-gravity directional liquid transportation from hydrophobic side to hydrophilic side,and can dynamically and continuously control the transportation time in a wide range of 3–66 s as the temperature increases from 10 to 40℃.This smart fabric can quickly dissipate heat at high temperatures,while at low temperatures,it can slow down the heat dissipation rate and prevent the human from becoming too *** addition,the fabric has UV shielding and photodynamic antibacterial properties through depositing graphitic carbon nitride nanosheets on the hydrophilic *** smart fabric offers an innovative approach to maximizing personal comfort in environments with significant temperature variations.

关键词： Directional water transport Cotton fabric Anti-gravity directional liquid transportation Janus wettability

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Multiple dynamic bonds enable high mechanical strength and efficient room-temperature self-healable polyurethane for triboelectric nanogenerators

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Science China Chemistry 2025年

作者： Wenwen Zhang Huixia Xuan Xiaofei Xu Jiaming lou Qingbao Guan Zhengwei You State Key Laboratory for Modification of Chemical Fibers and Polymer Materials Institute of Functional Materials College of Materials Science and Engineering Shanghai Key Laboratory of Lightweight Composite Shanghai Engineering Research Center of Nano-Biomaterials and Regenerative Medicine Donghua University

For room temperature self-healing triboelectric nanogenerators（TENGs）, the inherent contradiction between mechanical strength and self-healing properties was an urgent problem to be solved. Based on the phenol-carbamate bond, this paper proposed a strategy to design a new molecular structure and coordinate the triple dynamic bonds, which provided a feasible strategy to solve this contradiction. With polytetramethylene ether glycol（M_n= 1,000） as the soft segment in the main chain of polyurethane（PU）, meanwhile methylene diphenyl diisocyanate and 4,4′-dihydroxybiphenyl（BP） as the hard segment and chain extension agent, respectively, the combination of tetrad benzene ring endowed the resultant 4BP-PU with π-π interaction. The effective reversible dissociation and association with hydrogen bond not only bestowed 4BP-PU with high mechanical strength（16.14 MPa）, but also promoted high self-healing efficiency（94.8%） at room temperature. 4BP-PU was selected as the elastic substrate between polydimethylsiloxane and copper sheet to prepare a self-healing TENG to collect energy from natural ***, the rational molecular structure design provided new ideas for developing self-healing materials and fabricating energy harvest electronics.

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Role of the globus pallidus in motor and non-motor symptoms of Parkinson's disease

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Neural Regeneration Research 2025年第6期20卷 1628-1643页

作者： Yimiao Jiang Zengxin Qi Huixian Zhu kangli Shen Ruiqi Liu Chenxin Fang Weiwei lou Yifan Jiang Wangrui yuan Xin Cao Liang Chen Qianxing Zhuang Department of Physiology School of MedicineNantong UniversityNantongJiangsu ProvinceChina Department of Neurosurgery Huashan HospitalShanghai Medical CollegeFudan UniversityShanghaiChina National Center for Neurological Disorders ShanghaiChina Shanghai Key Laboratory of Brain Function Restoration and Neural Regeneration ShanghaiChina State Key Laboratory of Medical Neurobiology and MOE Frontiers Center for Brain Science Institute of Brain ScienceFudan UniversityShanghaiChina

The globus pallidus plays a pivotal role in the basal ganglia circuit. Parkinson's disease is characterized by degeneration of dopamine-producing cells in the substantia nigra, which leads to dopamine deficiency in the brain that subsequently manifests as various motor and non-motor symptoms. This review aims to summarize the involvement of the globus pallidus in both motor and non-motor manifestations of Parkinson's disease. The firing activities of parvalbumin neurons in the medial globus pallidus, including both the firing rate and pattern, exhibit strong correlations with the bradykinesia and rigidity associated with Parkinson's disease. Increased beta oscillations, which are highly correlated with bradykinesia and rigidity, are regulated by the lateral globus pallidus. Furthermore,bradykinesia and rigidity are strongly linked to the loss of dopaminergic projections within the cortical-basal ganglia-thalamocortical loop. Resting tremors are attributed to the transmission of pathological signals from the basal ganglia through the motor cortex to the cerebellum-ventral intermediate nucleus circuit. The cortico–striato–pallidal loop is responsible for mediating pallidi-associated sleep disorders. Medication and deep brain stimulation are the primary therapeutic strategies addressing the globus pallidus in Parkinson's disease. Medication is the primary treatment for motor symptoms in the early stages of Parkinson's disease, while deep brain stimulation has been clinically proven to be effective in alleviating symptoms in patients with advanced Parkinson's disease,particularly for the movement disorders caused by levodopa. Deep brain stimulation targeting the globus pallidus internus can improve motor function in patients with tremordominant and non-tremor-dominant Parkinson's disease, while deep brain stimulation targeting the globus pallidus externus can alter the temporal pattern of neural activity throughout the basal ganglia–thalamus network. Therefore, the comp

关键词： anxiety basal ganglia bradykinesia deep brain stimulation depression globus pallidus externus globus pallidus internus lateral globus pallidus medial globus pallidus neural circuit Parkinson's disease

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Recent development of Au arched Pt nanomaterials as promising electrocatalysts for methanol oxidation reaction

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Nano Research 2022年第1期15卷 18-37页

作者： Wenhua lou Asad Ali Pei kang Shen Collaborative Innovation Center of Sustainable Energy Materials Guangxi Key Laboratory of Electrochemical Energy MaterialsGuangxi UniversityNanning 530004China School of Physical Science and Technology Guangxi UniversityNanning 530004China School of Chemistry&Chemical Engineering Guangxi UniversityNanning 530004China

The recent development of Aurum(Au)introduced Platinum(Pt)based nanomaterials is of great significance to direct methanol fuel cell as electrocatalysts for anode reactions,due to its stability and anti-poisoning ***,the performance of PtAu based catalysts with different elements,atomic ratio,and morphology was studied in methanol solution to further improve its electrocatalytic ***,the effects of Au have aroused the researchers'attention in Pt-based *** this review,we summarize the controllable synthesis,mechanism,and catalytic performance of Au introduced Pt-based electrocatalysts such as PtAu core-shell nanostructures,PtAu dendrite,PtAu nanowires,self-supporting Au@Pt NPs,and Au@Pt star-like nanocrystals for the methanol oxidation ***,the challenges and research directions for the future development of PtAu based catalysts are provided.

关键词： methanol oxidation reaction(MOR) direct methanol fuel cell(DMFC) PtAu based catalysts anode catalysts electrocatalysis

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Study on the pointing model of a slant-axis terahertz antenna

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Research in Astronomy and Astrophysics 2020年第4期20卷 115-122页

作者： yu Wang Zheng lou Ying-Xi Zuo Hao-Ran kang Ming-Zhu Zhang Purple Mountain Observatory Chinese Academy of SciencesNanjing 210034China Key Laboratory for Radio Astronomy Chinese Academy of SciencesNanjing 210034China Shanghai Normal University Shanghai 201400China University of Science and Technology of China Hefei 230026China

This paper describes the establishment and verification of an accurate pointing model for a1.2 m aperture slant-axis terahertz antenna.A new analytical pointing model for the slant-axis antenna is presented based on an analogy to that of the alt-azimuth ***,extra error terms are added to the pointing model based on the structure and mechanical analysis of the slant-axis *** verify the pointing model experimentally,a pointing error measurement method based on photogrammetric techniques is *** this method,pointing behaviors of the antenna are accurately measured without the aid of astronomical observations,and major sources of the pointing errors are measured individually by photogrammetry and their respective coefficients are compared with those in the analytical pointing *** results show that an extended pointing model consisting 21 error terms can significantly reduce the residual systematic errors compared with the traditional model,more details are given in the following sections.

关键词： telescopes slant-axis antenna photogrammetry pointing models

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小学英语阅读教学中跨学科素材的关联策略

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教学与管理 2025年第2期 56-59页

作者：娄甜江苏省淮安市天津路小学江苏淮安223001

当前,推动课程综合化实施,加强学科交融,促进学科关联性学习已然成为课程改革的重要内容,这就要求教师在英语教学中树立跨学科意识,培育学生的跨学科素养。在英语阅读教学中积极融合跨学科素材,能够有效促进儿童阅读的深度与广度,提高... 详细信息

当前,推动课程综合化实施,加强学科交融,促进学科关联性学习已然成为课程改革的重要内容,这就要求教师在英语教学中树立跨学科意识,培育学生的跨学科素养。在英语阅读教学中积极融合跨学科素材,能够有效促进儿童阅读的深度与广度,提高儿童阅读的主动性与积极性,彰显跨学科学习的的功能与价值。结合具体的小学英语阅读教学案例,提出建立关联、指向关联、审视关联的跨学科素材融合策略,以期发挥跨学科素材的学科价值与育人价值。

关键词：跨学科素材阅读教学关联性学习小学英语

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Gas Flow Development Through Tandem Heat Exchangers Inside Exhaust Nozzle by Using Porous Medium Model

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Transactions of Nanjing University of Aeronautics and Astronautics 2016年第2期33卷 147-154页

作者： Liu Xiyue Zhang Jingzhou lou Decang kang Yong College of Energy and Power Engineering Jiangsu Province Key Laboratory of Aerospace Power System Nanjing University of Aeronautics and Astronautics Nanjing 210016 P. R. China Collaborative Innovation Center of Advanced Aero-Engine Beijing 100191 P. R. China China Gas Turbine Establishment Chengdu 610500 P. R. China

A computational study on the flow development through tandem double-U-shaped-tubes compact heat exchangers inside exhaust nozzle is *** order to simplify the computational process on modeling the flow field,the compact heat exchanger is modeled as a porous matrix by using an isotropic porous medium assumption,which makes two-dimensional numerical simulation *** the use of an existed quadratic relation which connects the pressure drop with the inlet velocity in the external part of the heat exchanger,the permeability and drag coefficient in the porous medium model are determined and a corresponding computational method validation is also *** schemes of tandem double-U-shaped-tubes compact heat exchangers are numerically *** relative to the baseline scheme,the modified scheme is improved by smoothing the nozzle expansion,varying heat exchanger mounting angle and installing boat-tail ramp at the trailing edge of the last heat *** results show that the pressure losses due to the existence of local recirculation zones and inappropriate distribution of the flow field are reduced in the modified *** pressure loss coefficient is decreased from 1.7% under the baseline scheme to 1.2% under the modified scheme.

关键词： compact heat exchanger exhaust nozzle porous medium pressure loss numerical simulation

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