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An effective'salt in dimethyl sulfoxide/water'electrolyte enables high-voltage supercapacitor operated at-50℃

Journal of Energy Chemistry 2024年第6期93卷 361-367,I0009页

作者： Yingbin Liu chang yu Xuedan Song Siyi Hou Shuqin Lan Jinhe yu yuanyang Xie Jieshan Qiu State Key Lab of Fine Chemicals Frontier Science Center for Smart MaterialsSchool of Chemical EngineeringLiaoning Key Lab for Energy Materials and Chemical EngineeringDalian University of TechnologyDalian 116024LiaoningChina School of Chemistry Frontier Science Center for Smart MaterialsLiaoning Key Lab for Energy Materials and Chemical EngineeringDalian University of TechnologyDalian 116024LiaoningChina College of Chemical Engineering State Key Laboratory of Chemical Resource EngineeringBeijing University of Chemical TechnologyBeijing 100029China

Compared with organic electrolytes,aqueous electrolytes exhibit significantly higher ionic conductivity and possess inherent safety features,showcasing unique advantages in ***,challenges remain for low-salt aqueous electrolytes operating at high voltage and low ***,we report a low-salt(0.87 m,m means mol kg^(-1))'salt in dimethyl sulfoxide/water'hybrid electrolyte with non-flammability via hybridizing aqueous electrolyte with an organic co-solvent of dimethyl sulfoxide(hydrogen bond acceptor).As a result,the 0.87 m hybrid electrolyte exhibits enhanced electrochemical stability,a freezing temperature below-50℃,and an outstanding ionic conductivity of 0.52mS cm~(-1)at-50℃.Dimethyl sulfoxide can anchor water molecules through intermolecular hydrogen bond interaction,effectively reinforcing the stability of water in the hybrid ***,the interaction between dimethyl sulfoxide and water molecules diminishes the involvement of water in the generation of ordered ice crystals,finally facilitating the low-temperature performance of the hybrid *** paired with the 0.87 m'salt in dimethyl sulfoxide/water'hybrid electrolyte,the symmetric supercapacitor presents a 2.0 V high operating voltage at 25℃,and can operate stably at-50℃.Importantly,the suppressed electrochemical reaction of water at-50℃further leads to the symmetric supercapacitor operated at a higher voltage of 2.6 *** modification strategy opens an effective avenue to develop low-salt electrolytes for high-voltage and low-temperature aqueous supercapacitors.

关键词： Dimethyl sulfoxide Co-solvent High voltage Low temperature Supercapacitors

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Phase Patterning of Poly(oxime-ester)for Information Encryption by Photo-induced Isomerization

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Chinese Journal of Polymer Science 2024年第10期42卷 1488-1494,I0010页

作者： yu-Fan Yang yun Bai Yi-Bao Li chang-Fei He School of Chemistry and Chemical Engineering Gannan Normal UniversityGanzhou341000China

Crystal polymers or liquid crystal elastomers undergo a phase transition that results in a change in the corresponding optical properties,which has the potential to be applied in areas such as information encryption and *** utilization of these materials for patterning purposes requires different phase transition ***,once prepared,altering the phase transition temperature of them presents significant ***,a poly(oxime-ester)(POE)network is developed to achieve high-resolution and multilevel patterning by photo-induced *** as-prepared POE exhibits the ability to transition from an opaque state to a transparent state under temperature stimuli,with the transition temperature and kinetics dependent on UV light exposure ***,complex patterns and information can be encrypted through different selective regional exposure time and decrypted under specific temperature or cooling ***,we illustrate an example of temporal communication,where cooling time or temperature serves as the encoded *** research expands the application scope of advanced encryption materials,showcasing the potential of POE in dynamic information encryption and decryption processes.

关键词： Poly(oxime-ester) Isomerization Phase patterning Information encryption

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Stage separation of recoverable liquid launch vehicle by using moving pulsating ball analogue for propellant sloshing

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Chinese Journal of Aeronautics 2024年第2期37卷 360-370页

作者： yu LU Baozeng yuE Bailong HAO Bole MA Feng LIU yuanyuan chang School of Aerospace Engineering Beijing Institute of TechnologyBeijing 100081China Beijing Institute of Astronautical Systems Engineering Beijing 100076China

In the process of stage separation of recoverable liquid launch vehicles,because of the large amount of residual fuel in the storage tanks,the influence of liquid sloshing on separation safety must be *** calculation simplicity and operation practicability,the Moving Pulsating Ball Model(MPBM)of large amplitude liquid sloshing is introduced into the calculation of launch vehicle stage *** the dynamic equation of the model with the energy relationship during"breathing movement",the formula calculating the force of liquid on the rigid body is *** with the calculations of commercial CFD calculation software,the accuracy of MPBM model is ***,all the external forces and moments are applied to the rigid body of the stages,so that the translational and rotational dynamic equations of the stages are obtained *** to the relative position of the two stages,the geometric shape of the interstage section and the engine of the second stage,the minimum clearance in the separation process can be decided to guarantee that the separation process is safe.

关键词： Moving Pulsating Ball Model(MPBM) Dynamics of stage separation Large amplitude sloshing Recoverable liquid launch vehicle Flight dynamics

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Sustainability-oriented social responsibility and corporate innovation

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China Journal of Accounting Research 2024年第2期17卷 193-215页

作者： Li chang Qian yu School of Accounting Dongbei University of Finance and EconomicsChina

This paper empirically examines how sustainability-oriented social responsibility influences corporate innovation quantity and radical innovation from the perspectives of environment-and employee-oriented social *** forms of social responsibility are found to contribute significantly to corporate *** environment-oriented responsibility increases innovation by increasing R&***-oriented responsibility increases innovation by helping firms retain talent;by motivating employees,employeeoriented social responsibility promotes both innovation quantity and radical ***,both environment-and employee-oriented responsibility can alleviate financing constraints,and the positive effects of environment-and employee-oriented responsibility on radical innovation and innovation quantity,respectively,increase total factor ***lowing sustainable development theory,this paper analyzes the heterogeneous mechanisms of the influences of environment-and employee-oriented social responsibility on corporate innovation and provides empirical evidence of high-quality,innovation-driven corporate development through social responsibility.

关键词： Sustainable Development Theory Corporate Social Responsibility Innovation Quantity Radical Innovation

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Robust Feedback Controller for Exponential Stability of Nonlinear Systems with Mismatched Uncertainties

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Journal of Systems Engineering and Electronics 2002年第2期13卷 92-97页

作者： yu kai, Zhao chang’an & Li ShiyongDepartment of Control Science and Technology, Harbin Institute of Technology, Harbin 150001, P. R. China(Received June 28, 2001) Department of Control Science and Technology Harbin Institute of Technology Harbin 150001 P. R. China

The robust stabilization of nonlinear systems with mismatched uncertainties is investigated. Based on the stability of the nominal system, a new approach to synthesizing a class of continuous state feedback controllers for uncertain nonlinear dynamical systems is proposed. By such feedback controllers, the exponential stability of uncertain nonlinear dynamical systems can be guaranteed. The approach can give a clear insight to system analysis. An illustrative example is given to demonstrate the utilization of the approach developed. Simulation results show that the method presented is practical and effective.

关键词： Exponential stability Nonlinear dynamical systems Uncertainty State feedback controller.

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Solid-state lithium-ion batteries for grid energy storage:opportunities and challenges

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Science China Chemistry 2024年第1期67卷 43-66页

作者： Xin chang yu-Ming Zhao Boheng yuan Min Fan Qinghai Meng yu-Guo Guo Li-Jun Wan CAS Key Laboratory of Molecular Nanostructure and Nanotechnology CAS Research/Education Center for Excellence in Molecular SciencesBeijing National Laboratory for Molecular Sciences(BNLMS)Institute of ChemistryChinese Academy of Sciences(CAS)Beijing 100190China University of Chinese Academy of Sciences Beijing 100049China

The energy crisis and environmental pollution drive more attention to the development and utilization of renewable *** the capricious nature of renewable energy resource,it has difficulty supplying electricity directly to consumers stably and efficiently,which calls for energy storage systems to collect energy and release electricity at peak *** to their flexible power and energy,quick response,and high energy conversion efficiency,lithium-ion batteries stand out among multiple energy storage technologies and are rapidly deployed in the *** superior performance and ensuring the safety of energy storage systems,intrinsically safe solid-state electrolytes are expected as an ideal alternative to liquid *** this review,we systematically evaluate the priorities and issues of traditional lithium-ion batteries in grid energy *** lithium-ion batteries containing liquid electrolytes,solid-state lithium-ion batteries have the potential to play a more significant role in grid energy *** challenges of developing solid-state lithium-ion batteries,such as low ionic conductivity of the electrolyte,unstable electrode/electrolyte interface,and complicated fabrication process,are discussed in ***,the safety of solid-state lithium-ion batteries is *** the obtained insights,inspiring prospects for solid-state lithium-ion batteries in grid energy storage are depicted.

关键词： lithium-ion batteries grid energy storage solid-state electrolytes interface stability

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Intrinsic pentagon defect engineering in multiple spatial-scale carbon frameworks for efficient triiodide reduction

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Journal of Energy Chemistry 2024年第8期95卷 20-28,I0002页

作者： Siyi Hou Xuedan Song chang yu Jiangwei chang Yiwang Ding Yingbin Liu Xiubo Zhang Weizhe Liu Jieshan Qiu State Key Lab of Fine Chemicals Liaoning Key Lab for Energy Materials and Chemical EngineeringFrontier Science Center for Smart MaterialsSchool of Chemical EngineeringDalian University of TechnologyDalian 116024LiaoningChina Liaoning Key Lab for Energy Materials and Chemical Engineering Frontier Science Center for Smart MaterialsSchool of ChemistryDalian University of TechnologyDalian 116024LiaoningChina State Key Laboratory of Chemical Resource Engineering College of Chemical EngineeringBeijing University of Chemical TechnologyBeijing 100029China

Intrinsic topological defect engineering has been proven as a promising strategy to elevate the electrocatalytic activity of carbon ***,the controllable construction of high-density and specific topological defects in carbon frameworks to reveal the relationship between reactivity and defect structure remains a challenging ***,the intrinsic pentagon carbon sites that can favor electron overflow and enhance their binding affinity towards the intermediates of catalytic reaction are firstly presented by the work function and the p-band center *** experimentally verify this,the cage-opening reaction of fullerene is proposed and utilized for synthesizing carbon quantum dots with specific pentagon configuration(CQDs-P),subsequently utilizing CQDs-P to modulate the micro-scale defect density of three-dimensional reduced graphene oxide(rGO)viaπ-π*** multiple spatial-scale rGO-conjugated CQDs-P structure simultaneously possesses abundant pentagon and edge defects as catalytic active sites and long-range-orderedπelectron delocalization system as conductive *** defects-rich CQDs-P/rGO-4 all-carbon-based catalyst exhibits superb catalytic activity for triiodide reduction reaction with a high photoelectric conversion efficiency of 8.40%,superior to the Pt reference(7.97%).Theoretical calculations suggest that pentagon defects in the carbon frameworks can promote charge transfer and modulate the adsorption/dissociation behavior of the reaction intermediates,thus enhancing the electrocatalytic activity of the *** work confirms the role of intrinsic pentagon defects in catalytic reactions and provides a new insight into the synthesis of defects-rich carbon catalysts.

关键词： Defect engineering Pentagon carbon Carbon quantum dots Electrocatalytic activity Triiodide reduction

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Acute exercise is associated with specific executive functions in college students with ADHD:A preliminary study

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Journal of Sport and Health Science 2015年第1期4卷 89-96页

作者： Jennifer I.Gapin Jeffrey D.Labban Sara C.Bohall Joshua S.Wooten yu-kai chang Department of Kinesiology and Health Education Southern Illinois University Edwardsville The School of Health and Human Sciences Office of ResearchThe University of North Carolina at Greensboro Graduate Institute of Athletics and Coaching Science National Taiwan Sport University

Purpose： The relationship between acute exercise and executive functions in college students with attention deficit hyperactivity disorder （ADHD） has not been clearly established. The purpose of this preliminary study was to examine the difference in cognitive performance between college students with and without ADHD and to explore the effects of acute exercise on multiple aspects of executive functions and on serum brain derived neurotrophic factor （BDNF）. Methods： College students （normal： n = 10; ADHD： n = 10） performed the Stroop Test, Trail Making Test, and Digit Span Test prior to and after an acute exercise intervention. Blood samples were obtained prior to the pre-test cognitive test performance and then again after exercise and prior to the post-test cognitive test performance. Results： Students with ADHD exhibited impaired executive functions, particularly on inhibition. Additionally, while acute exercise improved all aspects of executive functions in those without ADHD, acute exercise only improved inhibitory performance for those with ADHD. Further, BDNF was not influenced by acute exercise regardless of the subjects＇ ADHD status. Conclusion： These results provide preliminary evidence for exercise as a potential adjunct treatment for benefitting inhibition in college students with ADHD.

关键词： Cognition Executive function Neurotrophins Physical activity

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Risk assessment of oil and gas investment environment in countries along the Belt and Road Initiative

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Petroleum Science 2024年第2期21卷 1429-1443页

作者： Bao-Jun Tang chang-Jing Ji yu-Xian Zheng Kang-Ning Liu Yi-Fei Ma Jun-yu Chen Center for Energy and Environmental Policy Research Beijing Institute of TechnologyBeijing100081China School of Management and Economics Beijing Institute of TechnologyBeijing100081China Collaborative Innovation Center of Electric Vehicles in Beijing BeijingChina Sustainable Development Research Institute for Economy and Society of Beijing BeijingChina Institute of Carbon Neutrality ShanghaiTech UniversityShanghai201210China

With the implementation of the Belt and Road Initiative, China is deepening its cooperation in oil and gas resources with countries along the Initiative. In order to better mitigate risks and enhance the safety of investments, it is of significant importance to research the oil and gas investment environment in these countries for China's overseas investment macro-layout. This paper proposes an indicator system including 27 indicators from 6 dimensions. On this basis, game theory models combined with global entropy method and analytic hierarchy process are applied to determine the combined weights, and the TOPSIS-GRA model is utilized to assess the risks of oil and gas investment in 76 countries along the Initiative from 2014 to 2021. Finally, the GM(1,1) model is employed to predict risk values for 2022-2025. In conclusion, oil and gas resources and political factors have the greatest impact on investment environment risk, and 12 countries with greater investment potential are selected through cluster analysis in conjunction with the predicted results. The research findings may provide scientific decisionmaking recommendations for the Chinese government and oil enterprises to strengthen oil and gas investment cooperation with countries along the Belt and Road Initiative.

关键词： Belt and Road Initiative Oil and Gas Investment Risk assessment

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DOA estimation of high-dimensional signals based on Krylov subspace and weighted l_(1)-norm

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Journal of Systems Engineering and Electronics 2024年第3期35卷 532-540,F0002页

作者： YANG Zeqi LIU Yiheng ZHANG Hua MA Shuai chang kai LIU Ning Lyu Xiaode Aerospace Information Research Institute Chinese Academy of SciencesBeijing 100094China National Key Laboratory of Microwave Imaging Technology Beijing 100190China School of Electronic Electrical and Communication Engineering University of Chinese Academy of SciencesBeijing 100049China Northern Institute of Electronic Equipment Beijing 100191China

With the extensive application of large-scale array antennas,the increasing number of array elements leads to the increasing dimension of received signals,making it difficult to meet the real-time requirement of direction of arrival(DOA)estimation due to the computational complexity of *** subspace algorithms require estimation of the covariance matrix,which has high computational complexity and is prone to producing spurious *** order to reduce the computational complexity of DOA estimation algorithms and improve their estimation accuracy under large array elements,this paper proposes a DOA estimation method based on Krylov subspace and weighted l_(1)-*** method uses the multistage Wiener filter(MSWF)iteration to solve the basis of the Krylov subspace as an estimate of the signal subspace,further uses the measurement matrix to reduce the dimensionality of the signal subspace observation,constructs a weighted matrix,and combines the sparse reconstruction to establish a convex optimization function based on the residual sum of squares and weighted l_(1)-norm to solve the target *** results show that the proposed method has high resolution under large array conditions,effectively suppresses spurious peaks,reduces computational complexity,and has good robustness for low signal to noise ratio(SNR)environment.

关键词： direction of arrival(DOA) compressed sensing(CS) Krylov subspace l_(1)-norm dimensionality reduction

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