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Decade Milestone Advancement of Defect-Engineered g-C_(3)N_(4) for Solar Catalytic Applications

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Nano-Micro Letters 2024年第4期16卷 153-218页

作者： Shaoqi Hou Xiaochun Gao Xingyue Lv Yilin Zhao Xitao Yin Ying liu Juan fang Xingxing yu Xiaoguang Ma Tianyi Ma Dawei Su School of Mathematical and Physical Sciences Faculty of ScienceUniversity of Technology Sydney(UTS)SydneyNSW 2007Australia Laboratory of Plasma and Energy Conversion School of Physics and Optoelectronic EngineeringLudong University186 Middle Hongqi RoadYantai 264025People’s Republic of China School of Energy and Environmental Engineering University of Science and Technology BeijingBeijing 100083People’s Republic of China Department of Chemistry The University of Tokyo7‑3‑1 HogoBunkyoTokyoJapan School of Science STEM CollegeRMIT UniversityMelbourneVIC 3000Australia

Over the past decade, graphitic carbon nitride(g-C_(3)N_(4)) has emerged as a universal photocatalyst toward various sustainable carbo-neutral technologies. Despite solar applications discrepancy, g-C_(3)N_(4) is still confronted with a general fatal issue of insufficient supply of thermodynamically active photocarriers due to its inferior solar harvesting ability and sluggish charge transfer dynamics. Fortunately, this could be significantly alleviated by the “all-in-one” defect engineering strategy, which enables a simultaneous amelioration of both textural uniqueness and intrinsic electronic band structures. To this end, we have summarized an unprecedently comprehensive discussion on defect controls including the vacancy/non-metallic dopant creation with optimized electronic band structure and electronic density, metallic doping with ultraactive coordinated environment(M–N_(x), M–C_(2)N_(2), M–O bonding), functional group grafting with optimized band structure, and promoted crystallinity with extended conjugation π system with weakened interlayered van der Waals interaction. Among them, the defect states induced by various defect types such as N vacancy, P/S/halogen dopants, and cyano group in boosting solar harvesting and accelerating photocarrier transfer have also been emphasized. More importantly, the shallow defect traps identified by femtosecond transient absorption spectra(fs-TAS) have also been highlighted. It is believed that this review would pave the way for future readers with a unique insight into a more precise defective g-C_(3)N_(4) “customization”, motivating more profound thinking and flourishing research outputs on g-C_(3)N_(4)-based photocatalysis.

关键词： Defect engineering g-C_(3)N_(4) Electronic band structures Photocarrier transfer kinetics Defect states

Assessment and Enhancement of FRC of Power Systems Considering Thermal Power Dynamic Conditions

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CSEE Journal of Power and Energy Systems 2024年第4期10卷 1371-1383页

作者： Feng Hong Yalei Pang Weiming Ji Lu Liang fang fang Junhong Hao Jizhen liu State Key Laboratory of Alternate Electric Power System with Renewable Energy Sources and School of Control and Computer Engineering North China Electric Power UniversityBeijing 102206China State Key Laboratory of Alternate Electric Power System with Renewable Energy Sources School of Energy Power and Mechanical EngineeringNorth China Electric Power UniversityBeijing 102206China

Frequency stability and security have been a vital challenge as large-scale renewable energy is integrated into power *** contrast,the proportion of traditional thermal power units decreases during the decarbonization transformation process,resulting in poor frequency *** paper aims to explore the potential of frequency regulation support,dynamic assessment,and capacity promotion of thermal power plants in the transition *** the dynamic characteristics of the main steam working fluid under different working conditions,a nonlinear observer is constructed by extracting the main steam pressure and valve opening degree *** real-time frequency modulation capacity of thermal power units can provide a dynamic state for the power grid.A dynamic adaptive modification for primary frequency control(PFC)of power systems,including wind power and thermal power,is proposed and *** power dynamic allocation factor is adaptively optimized by predicting the speed droop ratio,and the frequency modulation capability of the system is improved by more than 11%under extreme ***,through the Monte Carlo simulation of unit states of the system under various working conditions,the promotion of the frequency regulation capacity with high wind power penetration(WPP)is verified.

关键词： Dynamic evaluation frequency regulation power system predictive modeling wind penetration

Design,synthesis,and biological evaluation of 1,2,4-triazole derivatives as potent antitubercular agents

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Chinese Chemical Letters 2024年第3期35卷 326-331页

作者： yu Wen Shichun Lun yuxue Jiao Wei Zhang Tianyu Hu Ting liu Fan Yang Jie Tang Bing Zhang William R.Bishai Li-fang yu Shanghai Engineering Research Center of Molecular Therapeutics and New Drug Development School of Chemistry and Molecular EngineeringEast China Normal UniversityShanghai 200062China Center for Tuberculosis Research Department of MedicineDivision of Infectious DiseaseJohns Hopkins School of MedicineBaltimoreMD21231-1044United States Shanghai Institute for Advanced Immunochemical Studies and School of Life Science and Technology ShanghaiTech UniversityShanghai 201210China Shanghai Key Laboratory of Green Chemistry and Chemical Process School of Chemistry and Molecular EngineeringEast China Normal UniversityShanghai 200062China

Inhibition of mycobacterial membrane protein large 3(MmpL3)thereby affecting the mycolic acid biosynthetic pathway has been proven to be an effective strategy for developing antitubercular *** on the X-ray crystal structure of MmpL3 inhibitor complexes,a series of novel 1,2,4-triazole derivatives were designed,synthesized and evaluated antitubercular activity against Mtb strain *** structure–activity relationship exploration resulted in the identification of compounds 21 and 28,which possess potent antitubercular activity against Mtb strain H37Rv[minimum inhibitory concentration(MIC)=0.03–0.13μg/mL]and the clinical isolates of multidrug resistance(MDR)and extensive drug resistance(XDR)tuberculosis(MIC=0.06–1.0μg/mL).Moreover,compounds 21 and 28 showed neglectable cytotoxicity(IC_(50)≥32μg/mL)to the mammalian Vero cells and favorable physicochemical and pharmacokinetic properties according to the in silico absorption,distribution,metabolism and excretion(ADME)***,the potential target of representative 1,2,4-triazole 28 was identified to be MmpL3 using a microscale thermophoresis(MST)assay.

关键词： Tuberculosis MDR and XDR-TB MmpL3 inhibitor 1 2 4-Triazole Structure-based drug design

Improved performance of LiMn_(0.8)Fe_(0.2)PO_(4) by addition of fluoroethylene carbonate electrolyte additive

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Chinese Chemical Letters 2024年第6期35卷 229-233页

作者： Guihuang fang Wei Chen Hongwei Yang Haisheng fang Chuang yu Maoxiang Wu Faculty of Metallurgy and Energy Engineering Kunming University of Science and TechnologyKunming 650093China Key Laboratory of Optoelectronic Materials Chemistry and Physics Fujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou 350002China State Key Laboratory of Advanced Electromagnetic Engineering and Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074China

The addition of electrolyte additives is an effective strategy for tuning the property of the electrolyte to engineer the electrode/electrolyte interface,and there exist obvious discrepancies regarding the effect of fluoroethylene carbonate(FEC)as an electrolyte additive on the performance of *** FEC is introduced into the electrolyte of the LiMn_(0.8)Fe_(0.2)PO_(4)/Li cell and its effect on the properties of the LiMn_(0.8)Fe_(0.2)PO_(4) is *** is found that the addition of FEC in the electrolyte has a positive effect on the performance of the LiMn_(0.8)Fe_(0.2)PO_(4) cathode,which can be attributed to the reduced products generated by the interfacial side-reactions on the LiMn_(0.8)Fe_(0.2)PO_(4) cathode surface and the decreased metal dissolution in the FEC-containing electrolyte,thanks to the higher oxidation resistance of FEC and the easier and stronger binding of FEC and PF_6^(-).

关键词： Lithium-ion batteries LiMn_(0.8)Fe_(0.2)PO_(4) Cathode Electrolyte additives Fluoroethylene carbonate

An integrative mathematical model of microwave ion thruster for mHz-frequency thrust noise analysis

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Chinese Journal of Aeronautics 2024年第4期37卷 121-136页

作者： Xiang NIU Hui liu Daren yu Plasma Propulsion Laboratory Harbin Institute of TechnologyHarbin 150001China

Many high-precision space missions need thrusters to produce thrust with low noise to compensate for disturbances and ensure satellite platform stability. Microwave ion thruster is characterized with a wide thrust range and potential for these missions. A cost-effective and accurate mathematical model is crucial for mHz-frequency thrust noise analysis and feedback controller design. The Particle-In-Cell(PIC) and global models are two common simulation tools. The PIC model is characterized with high accuracy but huge computation cost, which is difficult to analyze long-time performance characteristics. Now, the global model is only used for the discharge chamber with low accuracy and cannot reflect ion extraction properties. In this paper, an integrative mathematical model is built for a 1-cm microwave ion thruster and can reflect ion beamlet divergence and impingement on the Accelerator Grid(AG). Simulation results show good agreement with experiments at 0.06 sccm. However, the model demonstrates worse consistency with experiments when the flux increases to 0.1 sccm, which may be because the influence of neutral gas on the Electron Cyclotron Resonance(ECR) is not considered in the model. A long-time(1000 s) simulation is conducted with this model under 35 μN. It takes 3 hrs, and the thrust noise reaches 1 μN/Hz^(0.5) at 1 mHz.

关键词： Electric propulsion Microwave ion thruster Integrative model Sheath property Ion beamlet divergence Thrust noise Plasma

Performance analysis and multi-objective optimization based on a modified irreversible Stirling cycle

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Science China(Technological Sciences) 2024年第6期67卷 1668-1684页

作者： XU Lei yu MinJie liu ZhiChun liu Wei School of Energy and Power Engineering Huazhong University of Science and TechnologyWuhan430074China

The efficiency of the actual Stirling engine is much lower than the ideal Carnot cycle *** obtain more precise efficiency for Stirling engines,this paper proposes a modified Stirling cycle with a more accurate heat transfer process in Stirling engines based on a thermodynamic function called available *** finite-time thermodynamic method is used to analyze the model performance under constant heat source temperature,finite temperature difference heat transfer,and incomplete regenerative processes.A new polytropic process is introduced to model the heat transfer between the working fluid and external heat sources in which only heat above ambient temperature is converted into technical *** regenerator is divided into numerous smaller heat reservoirs with individual temperature to analyze the incomplete regenerative *** expressions of the output power and thermal efficiency are obtained based on the modified irreversible Stirling cycle,and the effects of irreversible losses are analyzed to evaluate the performance of the proposed *** indicate that the efficiency of the modified cycle is much lower than that of the ideal Stirling cycle with an isothermal *** the increase of the average heat transfer temperature difference,there exists an optimum value for the power of the irreversible *** optimum power of the model was obtained for varying thermodynamic parameters by optimizing the average heat transfer temperature difference between the hot and cold *** optimize the irreversible model,the multi-objective optimization analysis is carried out based on NSGA-Ⅱ,which results in an optimized output power of 40.87 kW and an optimized thermal efficiency of 44%.

关键词： stirling cycle regenerative processes isopotential processes multi-objective optimization finite time thermodynamics

UKF‐MOT:An unscented Kalman filter‐based 3D multi‐object tracker

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CAAI Transactions on Intelligence Technology 2024年第4期9卷 1031-1041页

作者： Meng liu Jianwei Niu yu liu Collective Intelligence&Collaboration Laboratory China North Artificial Intelligence and Innovation Research InstituteBeijingChina China North Vehicle Research Institute BeijingChina State Key Laboratory of Software Development Environment School of Computer Science and EngineeringBeihang UniversityBeijingChina State Key Laboratory of Virtual Reality Technology and Systems School of Computer Science and EngineeringBeihang UniversityBeijingChina School of Computer Science and Engineering Beihang UniversityBeijingChina

Multi‐object tracking in autonomous driving is a non‐linear *** better address the tracking problem,this paper leveraged an unscented Kalman filter to predict the object's *** the association stage,the Mahalanobis distance was employed as an affinity metric,and a Non‐minimum Suppression method was designed for *** the detections fed into the tracker and continuous‘predicting‐matching’steps,the states of each object at different time steps were described as their own continuous *** conducted extensive experiments to evaluate tracking accuracy on three challenging datasets(KITTI,nuScenes and Waymo).The experimental results demon-strated that our method effectively achieved multi‐object tracking with satisfactory ac-curacy and real‐time efficiency.

关键词： autonomous vehicle transportation

Molecular crowding electrolytes for stabilizing Zn metal anode in rechargeable aqueous batteries

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Chinese Chemical Letters 2024年第7期35卷 445-451页

作者： Li Lin Song-Lin Tian Zhen-yu Hu yu Zhang Li-Min Chang Jia-Jun Wang Wan-Qiang liu Qing-Shuang Wang fang Wang School of Materials Science and Engineering Changchun University of Science and TechnologyChangchun 130022China School of Life Science and Technology Changchun University of Science and TechnologyChangchun 130022China Key Laboratory of Preparation and Applications of Environmental Friendly Materials of the Ministry of Education Jilin Normal UniversityChangchun 130103China Zhongshan Institute of Changchun University of Science and Technology Zhongshan 528437China

A solid electrolyte interphase(SEI)with a robust mechanical property and a high ionic conductivity is imperative for high-performance zinc metal ***,it is difficult to form such a SEI directly from an *** this work,a molecular crowding effect is based on the introduction of Zn(OTF)_(2)and Zn(ClO_(4))_(2)to 2 mol/L ZnSO_(4)*** and experiments indicate that the Zn(OTF)_(2)and Zn(ClO_(4))_(2)not only create a molecularly crowded electrolyte environment to promote the interaction of Zn^(2+)and OTF^(-),but also participate in the reduction to construct a robust and high ionic-conductive SEI,thus promoting metal zinc deposition to the(002)crystal *** this molecular crowding electrolyte,a high current density of 1 mA/cm^(2)can be obtained by assembling symmetric batteries with Zn as the anode for over 1000 *** in a temperature environment of-10℃,a current density of 1 mA/cm^(2)can be obtained by assembling symmetric batteries with Zn for over 200 ***//Bi_(2)S_(3)/VS4@C cells achieve a CE rate of up to 99.81%over 1000 ***,the utilization of a molecular crowding electrolyte is deemed a highly effective approach to fabricating a sophisticated SEI for a zinc anode.

关键词： Zinc ion batteries Anode Electrolyte Solid electrolyte interphase Molecular crowding effect

Seed-assisted growth for high-performance perovskite solar cells:A review

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Journal of Energy Chemistry 2024年第9期96卷 588-610页

作者： Zhimin fang Ting Nie Jianning Ding Shengzhong(Frank)liu Institute of Technology for Carbon Neutralization Yangzhou UniversityYangzhou 225127JiangsuChina Dalian National Laboratory for Clean Energy iChEMDalian Institute of Chemical PhysicsChinese Academy of SciencesDalian 116023LiaoningChina Key Laboratory of Applied Surface and Colloid Chemistry Ministry of EducationShaanxi Key Laboratory for Advanced Energy DevicesShaanxi Engineering Lab for Advanced Energy TechnologySchool of Materials Science and EngineeringShaanxi Normal UniversityXi’an 710119ShaanxiChina

The rapid increase in the power conversion efficiency(PCE)of perovskite solar cells(PSCs)is closely related to the development of deposition techinique for perovskite *** high-quality perovskite film enables efficient charge transportation and less trap states,which are eventually translated into enhanced device ***-assisted growth(SAG)is a potential technique for depositing highly-crystallized perovskite films with preferential crystal orientation among the numerous approaches related to crystallization *** this review,we summarize the recent advances in the SAG technique for both one-step and two-step processed perovskite ***,seeding at the buried interface and on the top surface are also *** present different seeds and their corresponding seeding mechanism in detail,such as inorganic nanomaterials,organic ammoniums,alkali metal halides,and perovskite ***,challenges and perspectives are proposed to investigate the potential expansion of seeding engineering in high-performance PSCs,particularly large-area devices.

关键词： Perovskite solar cell Seed Crystallization Efficiency