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Steam disinfection enhances bioaccessibility of metallic nanoparticles in nano-enabled silicone-rubber baby bottle teats,pacifiers,and teethers

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Journal of Environmental Sciences 2024年第2期136卷 161-171页

作者： yu Su BinWang Xin Tong Shuchuan Peng Sijin Liu Baoshan Xing Rong ji State Key Laboratory of Pollution Control and Resource Reuse School of the EnvironmentNanjing UniversityNanjing 210023China School of Resources and Environmental Engineering Hefei University of TechnologyHefei 230009China State Key Laboratory of Environmental Chemistry and Ecotoxicology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China Stockbridge School of Agriculture University of MassachusettsAmherstMA 01003USA

Nano-enabled silicone-rubber articles for feeding or chewing could be a source of metallic nanoparticles(NPs)directly exposed to infants and young ***,the impact of steam disinfection on release of NPs and the related potential risks to children's health are ***,we investigated contents and form of Ag and Zn in 57 nano-enabled silicone-rubber baby bottle teats,pacifiers,and teethers of seven countries and examined the impacts of steam disinfection on in vitro bioaccessibility(IVBA)of Ag and Zn in the *** 89%articles had a mixture of Ag-and Zn-containing NPs and the teethers had relatively high Ag and Zn contents(up to 501 and 254μg/g,respectively).Steam disinfection caused rubber decomposition into micro(nano)plastics(0.54-15.7μm)and NP release from the interior of bulk rubber and micro-sized plastics,thus enhancing the IVBA of Ag and Zn by up to 5.5 *** findings provide insights into mechanisms for NP release by steam *** oral exposure risk assessment suggested low health concerns on individual metal release,our study points out the need to assess the potential health risks of child co-exposure to metallic NPs and micro(nano)plastics.

关键词： Silicone rubber Metallic nanoparticles Micro(nano)plastics Bioaccessibility Children's health

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Enhancement and Removal of PM_(2.5)by Cold and Warm Air Masses Accompanying Certain Synoptic Weather Systems across Hangzhou,China during 2014-2020

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Journal of Meteorological Research 2024年第3期38卷 620-634页

作者： Bu yu Feng CHEN Hanqing KANG Bin zhu Hongnian LIU Hangzhou Meteorological Bureau Hangzhou310051China Hangzhou International Urbanology Research Center for Urban Governance Studies Hangzhou311121China Zhejiang Institute of Meteorological Sciences Hangzhou310008China Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration Nanjing University of Information Science&TechnologyNanjing210044China School of Atmospheric Sciences Nanjing UniversityNanjing210023China

Local air pollution is strongly affected by synoptic weather systems,such as fronts,troughs,low-altitude vortices,or high-altitude ***,few studies have analyzed the meteorological properties of cold or warm air masses associated to these systems and their impact on local air *** this study,hourly observations of fine particulate matter(diameter of up to 2.5µm,i.e.,PM_(2.5)),wind(V),temperature(T),pressure(P),and precipitation(R),acquired in Hangzhou in 2014-2020,were *** this analysis,weather patterns were categorized into 27 types;89 and 94 cases illustrating the passage of warm and cold air masses over Hangzhou were identified,respectively;the influence of air mass temperature,wind speed,and wind direction on PM_(2.5) concentrations and local accumulation or removal was *** main results are as follows.(1)Pollution events occurred more frequently for cold than for warm air masses,but average pollutant concentration was lower for cold air masses;(2)48%of the cold air mass cases corresponded to PM_(2.5) decreases and 52%to PM_(2.5) increases,with strong cold air masses(ΔT_(24h)>4°C;∣V∣_(average)>4 m s^(−1))markedly reducing local pollution,but weak cold air masses(ΔT24h4°C)reduced the PM_(2.5) concentration whereas weaker winds(∣V∣_(average)<2 m s^(−1))increased it;and(4)PM_(2.5) concentration decreased sharply within 4 h after the passage of strong cold air masses,but more gradually within 14 h after the passage of strong warm air *** results considerably improve the current understanding of the influence of cold and warm air masses on local pollution patterns.

关键词： weather type air mass enhancement removal meteorological condition

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Effects of acupuncture on hypothalamic–pituitary–adrenal axis:Current status and future perspectives

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Journal of Integrative Medicine 2024年第4期22卷 445-458页

作者： jia-yuan Zheng jing zhu yu Wang Zhan-zhuang Tian Department of Integrative Medicine and Neurobiology School of Basic Medical SciencesState Key Laboratory of Medical Neurobiology and Ministry of Education Frontiers Center for Brain ScienceInstitutes of Brain ScienceInstitute of Acupuncture ResearchAcademy of Integrative MedicineShanghai Key Laboratory for Acupuncture Mechanism and Acupoint FunctionShanghai Medical CollegeFudan UniversityShanghai 200032China Department of Human Anatomy School of Integrative MedicineShanghai University of Traditional Chinese MedicineShanghai 201203China

The hypothalamic–pituitary–adrenal(HPA) axis is a critical component of the neuroendocrine system,playing a central role in regulating the body's stress response and modulating various physiological processes. Dysregulation of HPA axis function disrupts the neuroendocrine equilibrium, resulting in impaired physiological functions. Acupuncture is recognized as a non-pharmacological type of therapy which has been confirmed to play an important role in modulating the HPA axis and thus favorably targets diseases with abnormal activation of the HPA axis. With numerous studies reporting the promising efficacy of acupuncture for neuroendocrine disorders, a comprehensive review in terms of the underlying molecular mechanism for acupuncture, especially in regulating the HPA axis, is currently in need. This review fills the need and summarizes recent breakthroughs, from the basic principles and the pathological changes of HPA axis dysfunction, to the molecular mechanisms by which acupuncture regulates the HPA axis. These mechanisms include the modulation of multiple neurotransmitters and their receptors, neuropeptides and their receptors, and microRNAs in the paraventricular nucleus,hippocampus, amygdala and pituitary gland, which alleviate the hyperfunctioning of the HPA *** review comprehensively summarizes the mechanism of acupuncture in regulating HPA axis dysfunction for the first time, providing new targets and prospects for further exploration of acupuncture.

关键词： Acupuncture Electroacupuncture Hypothalamic-pituitary-adrenal axis Mechanism Neurotransmitter microRNA

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Highly reversible Zn anode enabled by anticatalytic carbon layer with suppressed hydrogen evolution

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Rare Metals 2024年第7期43卷 3044-3054页

作者： Wen-Duo Zhang Chuang Sun yu-Xuan zhu Feng Gao Chao Lai School of Chemistry and Materials Science Jiangsu Normal UniversityXuzhou221116China

Aqueous zinc-ion batteries(AZIBs)have emerged as a promising high-efficiency energy storage system due to the high energy density,low-cost and environmental ***,the practical application of AZIBs is severely restricted by the challenges faced by the Zn anode,which include uncontrollable dendrite growth,corrosion and hydrogen evolution ***,a simple and convenient physical vapor deposition(PVD)method is reported for fabricating uniform graphite as a protection layer on the surface of Zn *** high conductivity graphite layer on Zn anode(denoted as Zn@C)not only benefits the uniform distribution of the electric field,but also provides numerous Zn nucleation sites to regulate and navigate Zn-ion stripping/plating ***,the graphite layer with a poor catalytic activity endows the Zn@C anode with a highly suppressed hydrogen ***,a hydrogen and dendrite free anode is achieved with artificial anticatalytic carbon layer on Zn anode,exhibiting a high reversibility and excellent cycling stability over 2600 h at the current density of 5 mA·cm^(-2)with a capacity of 2.5 mAh·cm^(-2)and longtime cycling stability for assembled full *** work strategically designs the properties of the artificial interface layer to effectively address various challenges simultaneously,which presents insights for the future development of high-performance rechargeable AZIBs.

关键词： Zn metal anode Artificial anticatalytic layer Hydrogen suppression Dendrite free

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Hydrogen-rich water alleviates constipation by attenuating oxidative stress through the sirtuin1/nuclear factor-erythroid-2-related factor 2/heme oxygenase-1 signaling pathway

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World Journal of Gastroenterology 2024年第20期30卷 2709-2725页

作者： Kai-Di Chen Kui-Ling Wang Chen Chen Yi-jia zhu Wen-Wen Tang yu-ji Wang Ze-Peng Chen Lin-Hai He yu-Gen Chen Wei Zhang jiangsu Province Hospital of Chinese Medicine The Affiliated Hospital of Nanjing University of Chinese MedicineNanjing 210029Jiangsu ProvinceChina The No.1 Clinical Medical College Nanjing University of Chinese MedicineNanjing 210029Jiangsu ProvinceChina Department of Colorectal Surgery Jiangsu Province Hospital of Chinese MedicineThe Affiliated Hospital of Nanjing University of Chinese MedicineNanjing 210029Jiangsu ProvinceChina jiangsu Province Key Laboratory of Tumor Systems Biology and Chinese Medicine The Affiliated Hospital of Nanjing University of Chinese MedicineNanjing 210029Jiangsu ProvinceChina jiangsu Collaborative Innovation Center of Chinese Medicine in Prevention and Treatment of Tumor The Affiliated Hospital of Nanjing University of Chinese MedicineNanjing 210029Jiangsu ProvinceChina

BACKGROUND Constipation,a highly prevalent functional gastrointestinal disorder,induces a significant burden on the quality of patients'life and is associated with substantial healthcare ***,identifying efficient therapeutic modalities for constipation is of paramount *** stress is a pivotal contributor to colonic dysmotility and is the underlying pathology responsible for constipation ***,we postulate that hydrogen therapy,an emerging and promising intervention,can serve as a safe and efficacious treatment for *** To determine whether hydrogen-rich water(HRW)alleviates constipation and its potential *** Constipation models were established by orally loperamide to Sprague-Dawley *** freely consumed HRW,and were recorded their 24 h total stool weight,fecal water content,and charcoal propulsion *** samples were subjected to 16S rDNA gene *** non-targeted metabolomic analysis,malondialdehyde,and superoxide dismutase levels were *** tissues were stained with hematoxylin and eosin,Alcian blue-periodic acid-Schiff,reactive oxygen species(ROS)immunofluorescence,and immunohistochemistry for cell growth factor receptor kit(c-kit),PGP 9.5,sirtuin1(SIRT1),nuclear factor-erythroid-2-related factor 2(Nrf2),and heme oxygenase-1(HO-1).Quantitative real-time PCR and western blot analysis were conducted to determine the expression level of SIRT1,Nrf2 and HO-1.A rescue experiment was conducted by intraperitoneally injecting the SIRT1 inhibitor,EX527,into constipated ***460 cells were induced with H2O2 and treated with the metabolites to evaluate ROS and SIRT1 *** HRW alleviated constipation symptoms by improving the total amount of stool over 24 h,fecal water content,charcoal propulsion rate,thickness of the intestinal mucus layer,c-kit expression,and the number of intestinal *** modulated intestinal microbiota imbalance and abnormaliti

关键词： Hydrogen-rich water Constipation Sirtuin1 Oxidative stress Gut microbiota Serum metabolites

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Adjustment mechanism of blasting dynamic-static action in the water decoupling charge

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International Journal of Mining Science and Technology 2024年第6期34卷 821-836页

作者： Hao Zhang Xueyang Xing Yiteng Du Tingchun Li jianxin yu Qingwen zhu College of Civil Engineering and Architecture Shandong University of AeronauticsBinzhou 256600China Shandong Key Laboratory of Civil Engineering Disaster Prevention and Mitigation Shandong University of Science and TechnologyQingdao 266590China School of Civil Engineering Henan Polytechnic UniversityJiaozuo 454003China

Water decoupling charge blasting excels in rock breaking,relying on its uniform pressure transmission and low energy *** water decoupling coefficients can adjust the contributions of the stress wave and quasi-static ***,the quantitative relationship between the two contributions is unclear,and it is difficult to provide reasonable theoretical support for the design of water decoupling *** this study,a theoretical model of blasting fracturing partitioning is *** mechanical mechanism and determination method of the optimal decoupling coefficient are *** reliability is verified through model experiments and a field *** results show that with the increasing of decoupling coefficient,the rock breaking ability of blasting dynamic action decreases,while quasi-static action increases and then *** ability of quasi-static action to wedge into cracks changes due to the spatial adjustment of the blast hole and crushed *** quasi-static action plays a leading role in the fracturing range,determining an optimal decoupling *** optimal water decoupling coefficient is not a fixed value,which can be obtained by the proposed theoretical *** with the theoretical results,the maximum error in the model experiment results is 8.03%,and the error in the field test result is 3.04%.

关键词： Water decoupling blasting Blasting dynamic-static action Optimal decoupling coefficient Adjustment mechanism

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An extended micromechanical-based plastic damage model for understanding water effects on quasi-brittle rocks

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International Journal of Mining Science and Technology 2024年第3期34卷 289-304页

作者： Qiaojuan yu Shigui Du Qizhi zhu Zhanyou Luo Sili Liu Lunyang Zhao Institute of Rock Mechanics Ningbo UniversityNingbo 315211China Ningbo Key Laboratory of Energy Geostructure Ningbo UniversityNingbo 315211China College of Civil and Transportation Engineering Hohai UniversityNanjing 210098China College of Civil Engineering Jiangsu Open UniversityNanjing 210036China South China Institution of Geotechnical Engineering School of Civil Engineering and TransportationSouth China University of TechnologyGuangzhou 510641China

Water effects on the mechanical properties of rocks have been extensively investigated through experiments and numerical ***,few studies have established a comprehensive link between the microscopic mechanisms of water-related micro-crack and the constitutive behaviors of *** this work,we shall propose an extended micromechanical-based plastic damage model for understanding weakening effect induced by the presence of water between micro-crack’s surfaces on quasi-brittle rocks,based on the Mori-Tanaka homogenization and irreversible thermodynamics *** the physical mechanism,water strengthens micro-crack propagation,which induces damage evolution during the pre-and post-stage,and weakens the elastic effective properties of rock *** proposing a special calibration procedure for the determination of model parameters based on the laboratory compression tests,the proposed micromechanical-based model is verified by comparing the model predictions to the experimental *** model effectively captures the mechanical behaviors of quasibrittle rocks subjected to the weakening effects of water.

关键词： Water Micro-crack Damage Micro-mechanics Constitutive model Cohesive force

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Unique electromagnetic wave absorber for three-dimensional framework engineering with copious heterostructures

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Journal of Materials Science & Technology 2024年第3期170卷 129-139页

作者： Liyuan yu Qianqian zhu Zhiqiang Guo yuhang Cheng Zirui jia Guanglei Wu Institute of Materials for Energy and Environment State Key Laboratory of Bio-fibers and Eco-textilesCollege of Materials Science and EngineeringQingdao UniversityQingdao 266071China College of Chemistry and Chemical Engineering Qingdao UniversityQingdao 266071China

In order to obtain high-performance electromagnetic wave absorbers,the adjustment of structure and components is *** on the above requirements,this system forms a three-dimensional frame structure consisting of MXene and transition metal oxides(TMOs)through efficient electrostatic *** three-dimensional network structure has rich heterojunction structures,which can cause a large amount of interface polarization and conduction losses in incident electromagnetic *** structures cause multiple reflections and scattering of electromagnetic waves,which is also an important reason for further increasing electromagnetic wave *** the doping ratio is 1:1,the system has the best impedance matching,the maximum effective absorption bandwidth(EAB max)can reach 5.12 GHz at 1.7 mm,and the minimum reflection loss(RL_(min))is-50.30 dB at 1.8 *** provides a reference for the subsequent formation of 2D-MXene materials into 3D materials.

关键词： MXene Three-dimensional frame Heterojunction structure Conduction loss Electromagnetic wave absorption

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Lactonization of dyes promoted by a coordination cage facilitates cavity-induced chromism as ion mobile detector

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Science China Chemistry 2024年第5期67卷 1554-1560页

作者： Liangliang Zhang yu Liang Zhifeng Xiao yuxuan Meng jinyi Huang Xi Lin ji Li Hong-Cai Zhou yu Fang Strait Institute of Flexible Electronics(SIFE Future Technologies)Fujian Normal University and Strait Laboratory of Flexible Electronics(SLoFE)Fuzhou 350017China State Key Laboratory of Chemo/Bio-Sensing and Chemometrics College of Chemistry and Chemical EngineeringHunan UniversityChangsha 410082China Department of Chemistry Texas A&M UniversityCollege StationTexas 77842-3012USA State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou 350002China Frontiers Science Center for Flexible Electronics(FSCFE) MIIT Key Laboratory of Flexible Electronics(KLoFE)Northwestern Polytechnical UniversityXi’an 710072China

Dye molecules often change colors(so-called “chromism”) according to the environment variation. However, they are rarely induced by a catalytic amount of cavity. Through encapsulation in the cavity of a porous coordination cage(PCC-2), Rhodamine B(1) is transformed from red quinonoid form(1q) into colorless lactone form(1l) in aprotic polar solutions. The μ4-OH groups in the cavity of PCC-2 are shown to stabilize the uncommon zwitterion intermediate(1z), followed by converting to 1l, thus accelerating the equilibrium. The chromism is catalyzed by 0.25 mol% of PCC-2, and the reaction rate is improved by 80,400times. 1@PCC-2 can be further fabricated to a sol-gel that exhibits ion recognition properties. The resulting encapsulation and stabilization of an unconventional intermediate by a catalytic amount of the coordination cage provides fundamental insights into molecular isomerization and has potential use in chemical sensing.

关键词： porous coordination cage Zwitterion intermediate cavity Rhodamine B chromism

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Efficient ammonia production over e_(g)-occupancy-optimized perovskite electrocatalysts

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Nano Research 2024年第6期17卷 4682-4686页

作者： Mingfa Chen yu Zhang Fulong Liu Zhenbao Zhang yuming Dong Yongfa zhu Heqing jiang jiawei zhu Key Laboratory of Synthetic and Biological Colloids Ministry of EducationSchool of Chemical and Material EngineeringJiangnan UniversityWuxi 214122China Qingdao Institute of Bioenergy and Bioprocess Technology Chinese Academy of SciencesQingdao 266101China School of Chemistry and Chemical Engineering Linyi UniversityLinyi 276005China Department of Chemistry Tsinghua UniversityBeijing 100084China

Renewable-energy-driven nitrate(NO_(3)^(−))electroreduction to ammonia(NH_(3))(NERA)has been an attractive technology for decarbonizing NH_(3)production and wastewater *** NERA efficiency requires electrocatalysts that are earth-abundant and show fantastic *** we report a semiempirical activity descriptor of eg occupancy(of surface B-site cations)for identifying inexpensive perovskite oxides with extremely high efficacy toward *** establish the descriptor by systematic investigations of more than 10 perovskite *** investigations demonstrate that their intrinsic NERA activities display a volcano-shaped dependence on eg occupancy and the optimized intrinsic activities are accessible at near-1 eg *** could plausibly be attributed to the favorable overlaps between surface adsorbates and vertically-oriented eg *** importantly,utilizing this descriptor,we predict a highly active,selective,and durable NERA electrocatalyst with a composition of Ba_(0.5)Sr_(0.5)Co_(0.8)Fe_(0.2)O_(3−δ)(BSCF).Because of its close-to-1 e_(g)occupancy(i.e.~1.2),the BSCF features a superior NH_(3)production rate of 0.12 g·h^(−1)·mg_(cat.)^(−1)(Faradaic efficiency of 97.8%)that is at top of the volcano plot,and substantially outperforms most NERA electrocatalysts reported in literature.

关键词： perovskite oxide nitrate electroreduction ammonia electrosynthesis eg occupancy

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