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Particle Distribution Informed by Chain Rigidity in Diblock Copolymer Melts: The Effect of Entropy

Chinese Journal of Polymer Science 2024年第3期42卷 388-399,I0009页

作者： yuguo Chen Shuanhu qi Ying jiang School of Chemistry Beihang UniversityBeijing 100191China

We study the effect of chain rigidity on tailoring the nanoparticle locations for neutral and selective particles embedded in the lamellar morphology formed by semiflexible diblock copolymer chains using self-consistent field calculations. The nanoparticles are modeled through a cavity function, and the semiflexible chains are represented by the continuous Kratsky-Porod chain model. In general situation, the nanoparticles prefer to stay at the interface in order to reduce the interface areas and thus the system free energy. However, the particle distribution at the domain center is subtle, and the underlying physics is intrinsically different depending on the polymer flexibility. In the case of flexible chains, the entropy just contributes a constant shift to the free energy when the nanoparticles move around the domain center indicating that the local metastable state if appears at the domain center is wholly attributed to the local minimum in the enthalpy. If the polymers are rigid, the variation of the particle distribution at the domain center has a close relation with the polymer rigidity and nanoparticle size. In the case of strongly rigid polymers with small nanoparticles, a nearly uniform particle distribution at the domain center is observed, while in other cases, a local enhancement of particle distribution there is found. In contrast to the case of flexible chains, further analysis reveals the crucial role of entropy in controlling the shape of particle distributions at the phase domain. Specifically, the local metastable state appears in the domain center is determined by the large entropy there which arises from the weak coupling of bond orientations that allows the polymer chains to be relatively relaxed. When the particle becomes selective, its distribution in the phase domain exhibits a shift almost uniformly rather than changes its profile, and the underlying physics still holds. In all, our study establishes a strong coupling between the chain rigi

关键词： Semiflexible diblock copolymer Nanoparticle distribution Self-consistent field theory Entropic effect

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Reformulating natural language queries using sequence-to-sequence models

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Science China(Information Sciences) 2019年第12期62卷 254-256页

作者： Xiaoyu LIU Shunda PAN qi ZHANG yu-Gang jiang Xuanjing HUANG School of Computer Science Fudan University

Dear editor,In recent years, reformulating natural language queries has attracted significant amount of attention from both industry and academia. However,there is a lexical chasm between natural language queries and ... 详细信息

关键词： Reformulating natural language queries using sequence-to-sequence models

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Oligouridylates Formation with N-(O,O'-Diisopropyl)-Phosphoryl Alanine in the presence of Poly(β-(N^7-Adeninyl)Ethyl Methacrylate)

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Chinese Chemical Letters 2001年第4期12卷 313-316页

作者： Hong qi XIANG Jian Jun HU Yang jiang yu Fen ZHAO Bioorganic Phosphorus Laboratory Department of ChemistrySchool of Life Science and EngineeringTsinghua UniversityBeijing 100084

The oligouridylates formation with N-(O,O-diisopropyl)-phosphoryl alanine in the presence of poly((-(N7-adeninyl)ethyl methacrylate) was studied. An increased yield by the presence of the polymeric nucleic acid analo... 详细信息

关键词： N-phosphoryl amino acid nucleoside interaction polymeric nucleic acid analog.

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Adaptive fault-tolerant control for non-minimum phase hypersonic vehicles based on adaptive dynamic programming

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Chinese Journal of Aeronautics 2024年第3期37卷 290-311页

作者： Le WANG Ruiyun qi Bin jiang State Key Laboratory of Mechanics and Control for Aerospace Structures Nanjing University of Aeronautics and AstronauticsNanjing 210016China College of Automation Engineering Nanjing University of Aeronautics and AstronauticsNanjing 211106China

In this paper,a novel adaptive Fault-Tolerant Control(FTC)strategy is proposed for non-minimum phase Hypersonic Vehicles(HSVs)that are affected by actuator faults and parameter *** strategy is based on the output redefinition method and Adaptive Dynamic Programming(ADP).The intelligent FTC scheme consists of two main parts:a basic fault-tolerant and stable controller and an ADP-based supplementary *** the basic FTC part,an output redefinition approach is designed to make zero-dynamics stable with respect to the new ***,Ideal Internal Dynamic(IID)is obtained using an optimal bounded inversion approach,and a tracking controller is designed for the new output to realize output tracking of the nonminimum phase HSV *** the ADP-based compensation control part,an ActionDependent Heuristic Dynamic Programming(ADHDP)adopting an actor-critic learning structure is utilized to further optimize the tracking performance of the HSV control ***,simulation results are provided to verify the effectiveness and efficiency of the proposed FTC algorithm.

关键词： Hypersonic vehicle Fault-tolerant control Non-minimum phase system Adaptive control Nonlinear control Adaptive dynamic programming

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One-pot synthesis of N-aryl propargylamine from aromatic boronic acid,aqueous ammonia,and propargyl bromide under microwave-assisted conditions

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Chinese Chemical Letters 2014年第5期25卷 779-782页

作者： yu-Bo jiang Wen-Sheng Zhang Hui-Ling Cheng yu-qi Liu Rui Yang Faculty of Science Kunming University of Science and Technology School of Science and Technology Jiaozuo Teachers’ College

A facile,one-pot synthesis of N-aryl propargylamine from aromatic boronic acid,aqueous ammonia,and propargyl bromide has been achieved under microwave-assisted *** reactions can be smoothly completed within a total 10 min through a two-step procedure,including copper-catalyzed coupling of aromatic boronic acids with aqueous ammonia and following propargylation by propargyl bromide.

关键词： One-pot Microwave N-Aryl propargylamine Aromatic boronic acid Aqueous ammonia Propargyl bromide

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Deciphering the molecular mechanisms of Simiaowan in the treatment of hyperuricemia: in vivo and in silico approaches

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Traditional Medicine Research 2025年第2期10卷 37-54页

作者： Yong-Chang Zeng Jun-Hong Wu Dan-Dan Xu Kang He Chang-qing Liu Li-Fei Song Zheng-Zhi Wu qian-qian jiang Shao-yu Liang Department of Neurology The First Affiliated Hospital of Shenzhen UniversityShenzhen 518020China Pharmaceutical Department The Affiliated TCM Hospital of Guangzhou Medical UniversityGuangzhou 510000China School of Pharmacy Guizhou University of Traditional Chinese MedicineGuiyang 550025China Guangzhou Zeli Medical Technology Co. Ltd.Guangzhou 510700China

Background:Simiaowan(SMW),a well-known traditional Chinese medicine,has been employed to treat hyperuricemia(HUA)and gout for ***,the bioactive components and underlying mechanisms have not been *** objective of this study was to identify the active components and potential mechanisms of SMW by integrating pharmacological experimentation,serum pharmacochemistry,network pharmacology and molecular ***:HUA rats modelling by high-fat/high-sugar diet and potassium oxonate/adenine oral administration were used to evaluate the pharmacodynamic effects of ***-Q-Exactive-MS/MS was employed to detect the bioactive components present in SMW-containing *** pharmacology and molecular docking were utilized to elucidate the potential targets and underlying ***:SMW effectively ameliorated HUA rats via the inhibition of uric acid(UA)production,promotion of UA excretion,improvement of lipid and glucose metabolic abnormalities,antioxidant,anti-inflammatory and anti-insulin resistance effects.A total of 73 compounds detected in SMW-containing serum were identified as potential active components,with alkaloids,flavonoids,organic acids,and terpenoids emerging as the primary active *** 203 corresponding targets were obtained as SMW anti-HUA/gout targets,which mainly participated in apoptosis,insulin resistance,TNF,PI3K-Akt,HIF-1,NF-κB,MAPK,IL-17 and TLR signaling *** docking indicated that active compounds(***,phellodendrine,quercetin,formononetin,ferulic acid)had superior binding abilities to the key targets(*** carrier family 22 member 12(URAT1),solute carrier family 22 member 6(OAT1),ATP-binding cassette sub-family G member 2(ABCG2),solute carrier family 2,facilitated glucose transporter member 9(GLUT9),xanthine dehydrogenase/oxidase(XDH),transcription factor p65(RELA),toll-like receptor 4(TLR4),prostaglandin G/H synthase 2(PTGS2),caspase-3(CASP3),insulin(INS)).Conclusion:S

关键词： hyperuricemia network pharmacology serum pharmacochemistry Simiaowan UPLC-Q-Exactive-MS/MS

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Approximate analytical solutions for threedimensional ascent trajectory of a solid-fuel launch vehicle with time-varying mass flow rate

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Chinese Journal of Aeronautics 2024年第10期37卷 275-293页

作者： qi yu Wanchun CHEN Wenbin yu School of Astronautics Beihang UniversityBeijing 102206China

In the scenario that a solid-fuel launch vehicle maneuvers in outer space at high angles of attack and sideslip for energy management,Approximate Analytical Solutions(AAS)for the threedimensional(3D)ascent flight states are derived,which are the only solutions capable of considering time-varying Mass Flow Rate(MFR)at *** uneven MFR makes the thrust vary nonlinearly and thus increases the difficulty of the problem *** AAS are derived based on a 3D Generalized Ascent Dynamics Model(GADM)with a normalized mass as the independent *** simplify some highly nonlinear terms in the GADM,several approximate functions are introduced carefully,while the errors of the approximations relative to the original terms are regarded as minor ***,a finite series with positive and negative exponents,called Exponent-Symmetry Series(ESS),is proposed for function approximation to decrease the highest exponent in the AAS so as to reduce computer round-off *** calculate the ESS coefficients,a method of seeking the Optimal Interpolation Points(OIP)is proposed using the leastsquares-approximation *** to the artful design of the approximations,the GADM can be decomposed into two analytically solvable subsystems by a perturbation method,and thus the AAS are obtained ***,to help implement the AAS,two indirect methods for measuring the remaining mass and predicting the burnout time in flight are put forward using information from *** results verify the superiority of the AAS under the condition of time-varying MFR.

关键词： Approximate analytical solutions 3D ascent trajectory Solid-fuel launch vehicle Uneven thrust Energy management

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Supervised learning of enhancing convolutional Hash for image retrieval

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The Journal of China Universities of Posts and Telecommunications 2019年第4期26卷 51-61页

作者： Zhai qi jiang Mingyan School of Information Science and Engineering Shandong University

Deep convolutional neural network(CNN)makes great breakthroughs in computer ***,many works have demonstrated that the performance of the CNN depends on the stacked convolutional *** is obvious that the features of the fully connected layers lose the topological structures of images,and the convolutional layer features contain a large amount of redundant information that interferes with the performance of ***,we propose an effective supervised deep Hashing method,enhancing convolutional deep Hashing(ECDH),which learns the binary codes from the strengthened convolutional ***,an enhanced convolutional Hash layer is constructed between the top convolutional layer and the output layer,enhancing the local features of the convolutional layer outputs while learning the binary codes by optimizing an objective *** proposed method works well for existing deep learning models such as Alex neural network(AlexNet),visual geometry group neural network(VGGNet),residual neural network(ResNet),and is easier to be *** with state-of-the-art methods,extensive experiments show that the proposed method achieves better retrieval performance.

关键词： CNN Hashing image retrieval Hamming distance

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南美洲沉积型铜矿遥感地质解译及成矿带划分

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世界地质 2016年第4期35卷 1138-1144页

作者：贾大成穆宏玉姜琦刚李远华杨长保吉林大学地球探测科学与技术学院长春130026

针对南美洲沉积型铜矿类型和成矿带划分,基于Google Earth遥感影像,对典型矿床进行遥感地质解译,建立了不同沉积铜矿类型的遥感地质解译标志。基于Landsat--ETM遥感影像,依据沉积型铜矿分布、控矿地质条件和遥感影像特征,将南美洲沉积... 详细信息

针对南美洲沉积型铜矿类型和成矿带划分,基于Google Earth遥感影像,对典型矿床进行遥感地质解译,建立了不同沉积铜矿类型的遥感地质解译标志。基于Landsat--ETM遥感影像,依据沉积型铜矿分布、控矿地质条件和遥感影像特征,将南美洲沉积型铜矿划分为滨太平洋一级成矿带和北部二叠纪、中部古近纪和南部白垩纪等3个次一级成矿带。

关键词：沉积型铜矿床解译标志遥感地质解译成矿带划分南美洲

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A review of brain imaging biomarker genomics in Alzheimer’s disease:implementation and perspectives

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Translational Neurodegeneration 2022年第1期11卷 294-330页

作者： Lanlan Li Xianfeng yu Can Sheng Xueyan jiang qi Zhang Ying Han Jiehui jiang School of Information and Communication Engineering Shanghai UniversityShanghai 200444China School of Biomedical Engineering Hainan UniversityHaikou 570228China Department of Neurology Xuanwu Hospital of Capital Medical UniversityBeijing 100053China Institute of Biomedical Engineering School of Life ScienceShanghai UniversityShanghai 200444China.

Alzheimer’s disease(AD)is a progressive neurodegenerative disease with phenotypic changes closely associated with both genetic variants and imaging *** imaging biomarker genomics has been developed in recent years to reveal potential AD pathological mechanisms and provide early *** technique integrates multimodal imaging phenotypes with genetic data in a noninvasive and high-throughput *** this review,we summarize the basic analytical framework of brain imaging biomarker genomics and elucidate two main implementation scenarios of this technique in AD studies:(1)exploring novel biomarkers and seeking mutual interpretability and(2)providing a diagnosis and prognosis for AD with combined use of machine learning methods and brain imaging biomarker ***,we highlight the necessity of brain imaging biomarker genomics,discuss the strengths and limitations of current methods,and propose directions for development of this research field.

关键词： Imaging biomarker genomics Alzheimer’s disease Evolving technologies Implementation

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