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Boosting the adsorption and removal of dye from water by COOH-functionalized carbon nanotubes

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Green Chemical Engineering 2023年第1期4卷 88-98页

作者： Binran Zhao Yiyi Zhao Peng Liu yu-long men yun-Xiang Pan School of Chemical Engineering Northwest UniversityXi'an710069China Department of Chemical Engineering School of Chemistry and Chemical EngineeringShanghai Jiao Tong UniversityShanghai200240China

Water pollution caused by dye is a serious ***,we use a novel discharge process to functionalize carbon nanotube(CNT)by COOH groups to form CNT30 for removing methyl red(MR)from *** pristine CNT,75%MR is removed in 60 min,with an adsorption capacity of 68.44 mg *** CNT30,85%MR is fast removed in only 5 min,and the removal efficiency reaches to 95%after 30 min,with an adsorption capacity of80.33 mg ***,a higher MR removal efficiency is achieved in a much shorter time on ***,CNT30 has an outstanding reusability,with the MR removal efficiency decreasing by only 7%after ten *** COOH groups on CNT30 improve the hydrophilicity of CNT30,thus promoting the interaction of MR in water with *** hydrogen bonding and electrostatic interaction of MR with the COOH groups on CNT30 could be the force to drive MR adsorption on *** higher COOH content could be the origin for the better performance of CNT30 in removing dye from *** discharge process developed herein is operated in O2,without using harmful substances,and the COOH content on CNT can be efficiently tuned by simply changing discharge *** is different from the chemical modification widely used to functionalize CNT by strong oxidants,e.g.,HNO_(3).The present work is of great significance to realize green construction of materials for more efficiently removing dye from water.

关键词： Carbon nanotube Oxygen-containing functional group Dye Water pollution Discharge process

Efficient photocatalysis triggered by thin carbon layers coating on photocatalysts:recent progress and future perspectives

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Science China Chemistry 2020年第10期63卷 1416-1427页

作者： yu-long men Peng Liu Xingcui Peng yun-Xiang Pan Institute of Nano Biomedicine and Engineering Shanghai Engineering Research Centre for Intelligent Diagnosis and Treatment InstrumentDepartment of Instrument Science and EngineeringSchool of Electronic Information and Electrical EngineeringShanghai Jiao Tong UniversityShanghai 200240China

Solar-energy-driven photocatalysis,such as photocatalytic reduction of CO2,is promising simultaneously for the energy and environmental *** thin carbon layers with the thickness less than 10 nm on photocatalysts has been developed as an efficient strategy for enhancing the photocatalytic efficiency in recent *** the present review,we summarize the crucial progress on carbon-coated *** for the improved light absorption,charge separation,reactant adsorption and photocatalytic stability on carbon-coated photocatalysts as well as the applications of carbon-coated photocatalysts are *** opportunities and challenges associated with carbon-coated photocatalysts are shown at the end of the *** hope that the present review can trigger more deep insights on carbon-coated photocatalysts and provide new opportunities for developing low-cost but efficient photocatalysts.

关键词： carbon-coated photocatalysts light absorption charge separation reactant adsorption photocatalytic stability

Recent progresses on improving CO_(2)adsorption and proton production for enhancing efficiency of photocatalytic CO_(2)reduction by H_(2)O

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Green Chemical Engineering 2020年第1期1卷 33-39页

作者： Peng Liu Xingcui Peng yu-long men yun-Xiang Pan Dept.of Instrument Science and Engineering School of Electronic Information and Electrical EngineeringShanghai Jiao Tong UniversityShanghai200240PR China Dept.of Chemical Engineering School of Chemistry and Chemical EngineeringState Key Laboratory of Metal Matrix CompositesShanghai Jiao Tong UniversityShanghai200240PR China

Photocatalytically reducing CO_(2)by H_(2)O into valuable carbon-containing chemicals is one of the greatest concerns for both scientific and industrial communities,due to its great potential in solving energy and environmental ***,the photocatalytic reduction efficiency is still much lower than the need of large-scale ap*** of photocatalysts in adsorbing CO_(2)and splitting H_(2)O to produce protons are crucial factors determining the photocatalytic reduction *** research efforts have been devoted to addressing the issues on CO_(2)adsorption and proton *** present review discusses the recent progresses in improving CO_(2)adsorption and proton production on photocatalysts for increasing the photocatalytic reduction *** research opportunities and challenges are also *** is hoped that the present review can stimulate more deep insights on adsorption of CO_(2)and production of proton for increasing the photocatalytic reduction efficiency。

关键词： Carbon dioxide Photocatalysis Adsorption of carbon dioxide Production of proton Water splitting

Photocatalytic CO2 reduction highly enhanced by oxygen vacancies on Pt-nanoparticle-dispersed gallium oxide

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Nano Research 2016年第6期9卷 1689-1700页

作者： yun-Xiang Pan Zheng-Qing Sun Huai-Ping Cong yu-long men Sen Xin Jie Song Shu-Hong yu School of Chemistry and Chemical Engineering Hefei University of Technology Hefei 230009 China Division ofNanomaterials & Chemistry Hefei National Laboratory for Physical Sciences at the Microscale Department of Chemistry CAS Center for Excellence in Nanoscience University of Science and Technology of China Hefei 230026 China Institute of Nano Biomedicine and Engineering Department of Instrument Science and Engineering School of Electronic Information and Electrical Engineering Shanghai Jiao Tong University Shanghai 200240 China

Photocatalytic CO2 reduction on metal-oxide-based catalysts is promising for solving the energy and environmental crises faced by mankind. The oxygen vacancy （Vo） on metal oxides is expected to be a key factor affecting the efficiency of photocatalytic CO2 reduction on metal-oxide-based catalysts. Yet, to date, the question of how an Vo influences photocatalytic CO2 reduction is still unanswered. Herein, we report that, on Vo-rich gallium oxide coated with Pt nanoparticles （Vo-rich Pt/Ga203）, CO2 is photocatalytically reduced to CO, with a highly enhanced CO evolution rate （21.0umol.h-1） compared to those on Vo-poor Pt/Ga2O3 （3.9 gmol-h-1） and Pt/TiO2（P25）（6.7 gmol.h-1）. We demonstrate that the Vo leads to improved CO2 adsorption and separation of the photoinduced charges on Pt/Ga203, thus enhancing the photocatalytic activity of Pt/Ga203. Rational fabrication of an Vo is thereby an attractive strategy for developing efficient catalysts for photocatalytic CO2 reduction.

关键词： photocatalytic CO2reduction oxygen vacancy metal-oxide-based catalyst C02 adsorption

Simultaneously quantifying hundreds of acylcarnitines in multiple biological matrices within ten minutes using ultrahigh-performance liquid-chromatography and tandem mass spectrometry

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Journal of Pharmaceutical Analysis 2024年第1期14卷 140-148页

作者： Jingxian Zhang Qinsheng Chen Lianglong Zhang Biru Shi men yu Qingxia Huang Huiru Tang State Key Laboratory of Genetic Engineering School of Life SciencesHuman Phenome InstituteZhangjiang Fudan International Innovation CenterMetabonomics and Systems Biology Laboratory at Shanghai International Centre for Molecular PhenomicsZhongshan HospitalFudan UniversityShanghai200032China Wuhan Laboratory for Shanghai Metabolome Institute(SMI)Ltd. Wuhan430000China

Acylcarnitines are metabolic intermediates of fatty acids and branched-chain amino acids having vital biofunctions and pathophysiological significances. Here, we developed a high-throughput method for quantifying hundreds of acylcarnitines in one run using ultrahigh performance liquid chromatography and tandem mass spectrometry (UPLC-MS/MS). This enabled simultaneous quantification of 1136 acylcarnitines (C0–C26) within 10-min with good sensitivity (limit of detection 0.992), accuracy (relative error 0.998) for predicting retention time (tR) of acylcarnitines with no standards and built a database of their multiple reaction monitoring parameters (tR, ion-pairs, and collision energy). Furthermore, we quantified 514 acylcarnitines in human plasma and urine, mouse kidney, liver, heart, lung, and muscle. This provides a rapid method for quantifying acylcarnitines in multiple biological matrices.

关键词： Acylcarnitine UPLC-MS/MS Quantitative structure-retention relationship Molecular phenotype

Control of 2-D Semi-Markov Jump Systems:A View from Mode Generation Mechanism

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IEEE/CAA Journal of Automatica Sinica 2024年第1期11卷 258-260页

作者： yunzhe men Jian Sun Jie Chen the National Key Laboratory of Autonomous Intelligent Unmanned Systems the School of AutomationBeijing Institute of TechnologyBeijing 100081 the Beijing Institute of Technology Chongqing Innovation Center Chongqing 401120China the Department of Control Science and Engineering Tongji UniversityShanghai 201804 the National Key Laboratory of Autonomous Intelligent Unmanned Systems Beijing Institute of TechnologyBeijing 100081China

Dear Editor,Two-dimensional(2-D) systems have wide applications in image data processing,gas absorption and fluid dynamics analysis [1]-[3].When there exist abrupt changes in 2-D systems,they are usually modeled by 2-D Markov jump systems(MJSs) or 2-D semi-Markov jump systems(SMJSs).This letter investigates the control of 2-D SMJSs based on a novel mode generation mechanism,which could avoid mode ambiguousness phenomenon caused by the evolution of system mode in two different *** criterion that guarantees the almost surely exponential stability of the system is obtained.A thermal process is studied to demonstrate the availability of the proposed method.

关键词： Markov mode system

Climate warming is likely to weaken the performance of two-phase closed thermosyphon on the Qinghai-Tibet Plateau

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Advances in Climate Change Research 2024年第1期15卷 90-100页

作者： Guan-Li JIANG Zi-Teng FU Xin-yu men Hong-Ting ZHAO Si-Ru GAO Yong-Zhi LI Qing-Bai WU State Key Laboratory of Frozen Soil Engineering Northwest Institute of Eco-Environment and ResourcesChinese Academy of SciencesLanzhou 730000China Beiluhe Observation and Research Station on Frozen Soil Engineering and Environment in the Qinghai-Tibet Plateau Northwest Institute of Eco-Environment and ResourcesChinese Academy of SciencesLanzhou 730000China Muli Field Scientific Observation and Research Station for Gas Hydrate China Geological SurveyBeijing 100083China University of Chinese Academy of Sciences Beijing 100049China School of Civil Engineering and Architecture Jiaxing Nanhu UniversityJiaxing 314001China

Over the years,numerous geotechnical approaches have been implemented to mitigate the adverse effects of climate warming on various infrastructures in the permafrost region of the Qinghai-Tibet Plateau(QTP),such as the Qinghai-Tibet Highway and Railway,and achieved the expected engineering ***,little attention has been given to whether the performance of these geotechnical approaches has changed during the ongoing process of climate *** investigate the performance variation of one of these geotechnical approaches,which is two-phase closed thermosyphon(TPCT),during sustained climate warming,we conducted a statistical analysis of soil temperature monitoring data in 2003-2020 from eight regular embankments and six TPCT embankments in our permafrost monitoring *** results indicate that TPCT undeniably has a cooling effect on the permafrost beneath embankments,even rapidly eliminated previously formed taliks beneath ***,further analysis reveals that the performance of TPCT has been weakening during sustained climate warming,which has confirmed by the re-forming of the taliks beneath embankment where they had been previously *** on the current understanding,we attributed the weakening of thermosyphon performance to a significant reduction in the air temperature freezing index caused by ongoing climate *** this study,we aimed to draw attention to the evolving performance of geotechnical approaches in permafrost regions amid climate warming,prompting necessary engineering innovations to address this situation and ensure the sustainable development of the permafrost region on the QTP.

关键词： Two-phase closed thermosyphon Climate warming Supra-permafrost talik Permafrost degradation Qinghai-Tibet Highway

Cold storage alters the fat-trehalose trade-off,decreases the flight ability,and maintains the high survival rate and flight speed of Osmia excavata(Hymenoptera:Megachilidae)

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Insect Science 2024年第3期31卷 927-936页

作者： Yingying Song Li Liu Fang Ouyang Hongying Cui Wenxiu Guo Suhong Lv Baohua Ye Lili Li Yi yu Xingyuan men Institute of Plant Protection Shandong Academy of Agricultural SciencesJinanChina College of Plant Protection Shandong Agricultural UniversityJinanChina State Key Laboratory of Integrated Management of Pest Insects and Rodents Institute of ZoologyChinese Academy of SciencesBejingChina

Osmia solitary bees are important pollinators of various crops *** has been widely used to synchronize the emergence time of Osmia species from cocoons with the blooming time of different crops,but the fitness of Osmia after refrigeration remains ***,the effects of long-term refrigeration at 0℃on the vitality,flight ability,and metabolism of Osmia excavata,which is known as the"king of pollination"in China,were *** survival rate(>90%before 120 d),weight loss rate(long-term *** content of fats,which have antifreeze and energy storage properties,was not significantly altered in *** before 130 d of refrigeration,which might explain why the survival rates and flight speed of *** remained high after long-term ***,the flight duration and distance decreased significantly(Plong-term refrigeration;however,long-term refrigeration may decrease pollination *** findings highlight new research directions that could improve the ecological service function of refrigerated ***.

关键词： ecological service value flight ability Osmia pollination efficiency refrigeration vitality

A combined evaluation of the characteristics and antibiotic resistance induction potential of antibiotic wastewater during the treatment process

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Journal of Environmental Sciences 2024年第4期138卷 626-636页

作者： Sun Miao Yanyan Zhang Cong men Yiou Mao Jiane Zuo State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China School of Energy and Environmental Engineering Beijing Key Laboratory of Resource-Oriented Treatment of Industrial PollutantsUniversity of Science and Technology BeijingBeijing 100083China High School Affiliated to Renmin University of China Beijing 100080China Tsinghua Shenzhen International Graduate School Shenzhen 518055China

Antibiotic wastewater contains a variety of pollutant stressors that can induce and promote antibiotic resistance(AR)when released into the *** these substances are mostly in concentrations lower than those known to induce AR individually,it is possible that antibiotic wastewater discharge might still promote the AR transmission risk via additive or synergistic ***,the comprehensive effect of antibiotic wastewater on AR development has rarely been evaluated,and its treatment efficiency remains ***,samples were collected from different stages of a cephalosporin production wastewater treatment plant,and the potential AR induction effect of their chemical mixtures was explored through the exposure of the antibiotic-sensitive Escherichia coli K12 *** with raw cephalosporin production wastewater significantly promoted mutation rates(3.6×10^(3)-9.3×10^(3)-fold)and minimum inhibition concentrations(6.0-6.7-fold)of *** against ampicillin and *** may be attributed to the inhibition effect and oxidative stress of cephalosporin wastewater on *** AR induction effect of cephalosporin wastewater decreased after the coagulation sedimentation treatment and was completely removed after the full treatment process.A Pearson correlation analysis revealed that the reduction in the AR induction effect had a strong positive correlation with the removal of organics and biological *** indicates that the antibiotic wastewater treatment had a collaborative processing effect of conventional pollutants,toxicity,and the AR induction *** study illustrates the potential AR transmission risk of antibiotic wastewater and highlights the need for its adequate treatment.

关键词： Antibiotic wastewater treatment plant Antibiotic resistance Antibiotic resistance induction effect Correlation analysis Biological toxicity