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CoPSe nanoparticles confined in nitrogen-doped dual carbon network towards high-performance lithium/potassium ion batteries

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Chinese Chemical Letters 2025年第1期36卷 568-573页

作者： Zhong-hui sun yu-Qi Zhang Zhen-Yi Gu Dong-Yang Qu Hong-yu Guan Xing-Long Wu Guangdong Engineering Technology Research Center for Photoelectric Sensing Materials and Devices c/o School of Chemistry and Chemical EngineeringGuangzhou UniversityGuangzhou 510006China MOE Key Laboratory for UV Light-Emitting Materials and Technology Northeast Normal UniversityChangchun 130024China

The metal ion batteries have gained widespread attention for wearable electronics due to their competitive energy density and long cycling *** the advanced anode materials is significant for next generation energy storage ***,severe electrode volume changes and sluggish redox kinetics are the critical problems for lithium/potassium ion batteries(LIBs/PIBs)towards large-scale ***,we prepare a novel anode material,which consists of reduced graphene oxide wrapping one-dimensional(1D)N-doped porous carbon nanotube with cobalt phosphoselenide(CoPSe)nanoparticles embedded inside them(r GO@Co PSe/NC).Benefited from the dual carbon decorations and ultrafine nanoparticles structure,it achieves a reversible capacity of 245 mAh/g at 5 A/g after 2000 cycles for LIBs and 215 mAh/g at 1 A/g after 500 cycles for *** pseudocapacitance and GITT measurements are used to investigate the electrochemical kinetics of r GO@Co PSe/NC for *** addition,the lithium ion full cell also shows good electrochemical performance when paired with high capacity LiNi_(0.8)Co_(0.1)Mn_(0.1)O_(2) *** work provides a feasible electrode design strategy for high-efficiency metal ion batteries based on multidimensional nanoarchitecture engineering and composition tailoring.

关键词： Cobalt phosphoselenide Lithium-ion batteries Potassium-ion batteries Reduced graphene oxide Structural stability Full cell

Hierarchically Porous Polypyrrole Foams Contained Ordered Polypyrrole Nanowire Arrays for Multifunctional Electromagnetic Interference Shielding and Dynamic Infrared Stealth

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Nano-Micro Letters 2025年第4期17卷 399-418页

作者： yu-long Liu Ting-yu Zhu Qin Wang Zi-jie Huang De-xiang sun Jing-hui Yang Xiao-dong Qi Yong Wang School of Chemistry Key Laboratory of Advanced Technologies of Materials(Ministry of Education)Southwest Jiaotong UniversityChengdu 610031People’s Republic of China

As modern communication and detection technologies advance at a swift pace,multifunctional electromagnetic interference(EMI)shielding materials with active/positive infrared stealth,hydrophobicity,and electric-thermal conversion ability have received extensive *** the aforesaid requirements simultaneously remains a huge *** this research,the melamine foam(MF)/polypyrrole(PPy)nanowire arrays(MF@PPy)were fabricated via one-step electrochemical *** hierarchical MF@PPy foam was composed of three-dimensional PPy micro-skeleton and ordered PPy nanowire *** to the upwardly grown PPy nanowire arrays,the MF@PPy foam possessed good hydrophobicity ability with a water contact angle of 142.00°and outstanding stability under various harsh ***,the MF@PPy foam showed excellent thermal insulation property on account of the low thermal conductivity and elongated ligament characteristic of PPy nanowire ***,taking advantage of the high conductivity(128.2 S m^(-1)),the MF@PPy foam exhibited rapid Joule heating under 3 V,resulting in dynamic infrared stealth and thermal camouflage *** importantly,the MF@PPy foam exhibited remarkable EMI shielding effectiveness values of 55.77 dB and 19,928.57 dB cm^(2)g^(-1).Strong EMI shielding was put down to the hierarchically porous PPy structure,which offered outstanding impedance matching,conduction loss,and multiple *** innovative approach provides significant insights to the development of advanced multifunctional EMI shielding foams by constructing PPy nanowire arrays,showing great applications in both military and civilian fields.

关键词： Polypyrrole nanowire arrays Hierarchical foam Hydrophobicity Infrared stealth Electromagnetic interference shielding

Atmospheric reductive catalytic fractionation of lignocellulose integrated with one-pot catalytic conversion of carbohydrate yielding valuable lignin monomers and platform chemicals from corn straw

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Green Energy & Environment 2025年第1期10卷 161-172页

作者： Meng-Ying Liu Zhe-hui Zhang Xue-Qi Wang Qian sun Chen Zhang yu Li Zhuohua sun Katalin Barta Feng Peng Tong-Qi yuan State Key Laboratory of Efficient Production of Forest Resources Beijing Forestry UniversityBeijing100083China Beijing Key Laboratory of Lignocellulosic Chemistry Beijing Forestry UniversityBeijing100083China Department of Chemistry Organic and Bioorganic ChemistryUniversity of GrazHeinrichstrasse 28/II8010 GrazAustria

Developing a cost-effective and environmentally friendly process for the production of valuable chemicals from abundant herbal biomass receives great attentions in recent ***,taking advantage of the“lignin first”strategy,corn straw is converted to valuable chemicals including lignin monomers,furfural and 5-methoxymethylfurfural via a two steps *** key of this research lies in the development of a green and low-cost catalytic process utilizing magnetic Raney Ni catalyst and high boiling point ethylene *** utilization of neat ethylene glycol as the sole slovent under atmospheric conditions obviates the need for additional additives,thereby facilitating the entire process to be conducted in glass flasks and rendering it highly convenient for scaling *** the initial step,depolymerization of corn straw lignin resulted in a monomer yield of 18.1 wt%.Subsequently,in a dimethyl carbonate system,the carbohydrate component underwent complete conversion in a one-pot process,yielding furfural and 5-methoxymethylfurfural as the primary products with an impressive yield of 47.7%.

关键词： Atmospheric reductive catalytic fractionation Corn straw Ethylene glycol Raney Ni 5-Methoxymethylfurfural

Study on the off situ reconstruction of the core neutron field based on dual-task hybrid network architecture

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Nuclear Science and Techniques 2025年第1期36卷 175-191页

作者： Pei Cao hui Ding Cheng-Long Cao Zi-hui Yang Guo-Min sun School of Artificial Intelligence and Big Data Hefei UniversityHefei 230001China College of Electronic Engineering National University of Defense TechnologyHefei 230001China Institute of Nuclear Energy Safety Technology HFIPSChinese Academy of SciencesHefei 230027China

The off situ accurate reconstruction of the core neutron field is an important step in realizing real-time reactor *** existing off situ reconstruction method of the neutron field is only applicable to cases wherein a single region changes at a specified location of the ***,when the neutron field changes are complex,the accurate identification of the individual changed regions becomes challenging,which seriously affects the accuracy and stability of the neutron field ***,this study proposed a dual-task hybrid network architecture(DTHNet)for off situ reconstruction of the core neutron field,which trained the outermost assembly reconstruction task and the core reconstruction task jointly such that the former could assist the latter in the reconstruction of the core neutron field under core complex ***,to exploit the characteristics of the ex-core detection signals,this study designed a global-local feature upsampling module that efficiently distributed the ex-core detection signals to each reconstruction unit to improve the accuracy and stability of *** experiments were performed on the simulation datasets of the CLEAR-I reactor to verify the accuracy and stability of the proposed *** results showed that when the location uncertainty of a single region did not exceed nine and the number of multiple changed regions did not exceed ***,the reconstructed ARD was within 2%,RD_(max)was maintained within 17.5%,and the number of RD≥10%was maintained within ***,when the noise interference of the ex-core detection signals was within±2%,although the average number of RD≥10%increased to 16,the average ARD was still within in 2%,and the average RD_(max)was within 22%.Collectively,these results show that,theoretically,the DTHNet can accurately and stably reconstruct most of the neutron field under certain complex core changes.

关键词： Real-time reactor monitoring Core neutron field reconstruction Dual-task hybrid network architecture Global-local feature upsampling module

DTNBP1 Gene Is Associated with Some Symptom Factors of Schizophrenia in Chinese Han Nationality

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Chinese Medical Sciences Journal 2010年第2期25卷 85-89页

作者： yu-hui sun Yan Shen Qi Xu National Laboratory of Medical Molecular Biology Institute of Basic Medical Sciences Chinese Academy of Medical Sciences ＆ Peking Union Medical College Beijing 100005 China

Objective To study the association of DTNBP1 gene with some symptom factors of *** A total of 285 unrelated schizophrenic individuals were recruited from December 2004 to January 2009 for genetic analysis,and their symptom factors were assessed based on the Positive and Negative Syndrome Scale(PANSS).The quantitative trait test was performed by the UNPHASED program(version 3.0.12) to investigate the association between scored positive and negative symptoms and the single nucleotide polymorphisms(SNPs) in DTNBP1 *** The quantitative trait test showed allelic association of rs909706 with the excitement symptom of schizophrenia(P<0.05,adjusted by 10 000 permutations),while the genotype C/G of rs2619539 with a negative symptom,lack of spontaneity and flow of conversation(P<0.05,adjusted by 10 000 permutations).Conclusion DTNBP1 variations are possibly associated with some symptoms of schizophrenia,which could partly explain the relationship between the susceptibility gene DTNBP1 and that disease.

关键词： schizophrenia DTNBP1 gene positive and negative symptoms quantitative trait test

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艾滋病与眼部机会感染

国际眼科杂志 2009年第8期9卷 1572-1574页

作者：孙挥宇北京地坛医院眼科中国北京市100011

随着艾滋病患者的增多,艾滋病并发症:眼部的细菌、病毒、真菌、原虫的感染已经成为临床医师随时可能遇到的疾病,我们就此作简单的论述,希望能给临床医师的工作以帮助。

关键词：艾滋病机会感染

Effect of Heat Treatment on Structure and Electrochemical Properties of Electro-deposited Ni-P Amorphous Alloy

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材料热处理学报 2004年第05B期25卷 1163-1165页

作者： GUOJin-biao WANGyu LIhui-qin sunDong-bai BeijingUniversityofScienceandTechnology Beijing.China

The influences of heat treatment time on structure and the electrochemical behavior of electro-deposited amorphous Ni-P alloy coating were studied. The results show that the as-plated deposits have an amorphous structure, and the deposits crystallize into Ni12P5 and Ni3P at 260 °C, and the corrosion resistance of the as-plated deposits are better than that of the deposits after heat treatment.

关键词：热处理 Ni-P非晶形合金电化学电解沉积

Output Consensus of Heterogeneous Linear MASs via Adaptive Event-Triggered Feedback Combination Control

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IEEE/CAA Journal of Automatica Sinica 2025年第1期12卷 285-287页

作者： Shuo yuan Chengpu yu Jian sun the School of Automation Beijing Institute of Technology the Beijing Institute of Technology Chongqing Innovation Center

Dear Editor,This letter studies output consensus problem of heterogeneous linear multiagent systems over directed graphs. A novel adaptive dynamic event-triggered controller is presented based only on the feedback combination of the agent's own state and neighbors' output,which can achieve exponential output consensus through intermittent communication. The controller is obtained by solving two linear matrix equations, and Zeno behavior is excluded.

关键词： Directed graphs

Sporadic E responds to the 2022 Tonga volcano eruptions recorded by the Meridian Project

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Earth and Planetary Physics 2025年第1期9卷 20-28页

作者： YangYi sun Tao yu Jin Wang Chi Long School of Geophysics and Geomatics China University of Geosciences(Wuhan)Wuhan 430047China School of Physics and Electronic Science Guizhou Normal UniversityGuizhou 550001China

In this study,ionosonde observations over Fuke(19.5°N,109.1°E),Wuhan(30.5°N,114.4°E),and Mohe(53.5°N,122.3°E)were analyzed to demonstrate the responses of the sporadic E()to the severe atmospheric disturbances caused by the Tonga volcanic eruptions on January 15,*** most prominent signature was the disappearance of the layer after~10:00 UT over Wuhan and Fuke,which was attributed to the vertical drift caused by the *** occurred intermittently after 13:00 UT following the arrival of the tropospheric Lamb *** examine the causal mechanism for the intermittence,we also included data of horizontal winds in the mesosphere and lower thermosphere region recorded by the meteor radars at Wuhan and Mohe in this *** wind disturbances with periods of~20 hours contributed to the formation of the layer in the nighttime on January 15.

关键词： sporadic E Tonga eruptions neutral wind disturbances