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Amorphous hybrid tungsten oxide–nickel hydroxide nanosheets used as a highly efficient electrocatalyst for hydrogen evolution reaction

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Nano Research 2024年第4期17卷 2499-2508页

作者： chao lyu Chenghai Dai Yiwei Tan State Key Laboratory of Materials-Oriented Chemical Engineering School of Chemistry and Chemical EngineeringNanjing Tech UniversityNanjing 211816China

There are more challenges for alkaline hydrogen evolution reaction(HER)via simultaneously expediting the electron-coupled water dissociation process(Volmer step)and the following electrochemical H_(2) desorption(Heyrovsky step).Hybrid amorphous electrocatalysts are highly desirable for efficient hydrogen evolution from water-alkali electrolyzers due to the bifunctionality for the different elementary steps of HER and optimal interactions with water molecules and the reactive hydrogen intermediates(Had).Herein,the synthesis of amorphous hybrid ultrathin(tungsten oxide/nickel hydroxide)hydrate(a-[WO_(3)/Ni(OH)_(2)]·0.2H_(2)O)nanosheets on nickel foam(NF)for efficient alkaline HER is *** structural and composition features of a-[WO_(3)/Ni(OH)_(2)]·0.2H_(2)O are characterized in *** resulting a-[WO_(3)/Ni(OH)_(2)]·0.2H_(2)O/NF electrocatalyst with the synergistic effect of both hybrid components for the HER elementary steps shows greatly improved the activity and durability for the HER with a low overpotential of-41 and-163 mV at-10 and-500 mA·cm^(-2),respectively,a Tafel slope as low as-72.9 mV·dec^(-1),and long-term stability of continuous electrolysis for at least 150 h accompanying by inappreciable overpotential change in 1 M *** the hybrid a-[WO_(3)/Ni(OH)_(2)]·0.2H_(2)O,Ni(OH)_(2) and WO_(3) moieties are separately responsible for accelerating dissociative adsorption of water and weakening Had adsorption strength,which is beneficial to the improvement of the alkaline HER activity.

关键词： amorphous nanomaterial bimetallic electrocatalyst tungsten oxide ultrathin nanosheet hydrogen evolution reaction

Single transmembrane GPCR modulating proteins:neither single nor simple

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Protein & Cell 2024年第6期15卷 395-402页

作者： Meng Wang Jianjun lyu chao Zhang Department of Plastic and Reconstructive Surgery Shanghai Ninth People’s HospitalShanghai Jiao Tong University School of MedicineShanghai 200011China Hubei Topgene Research Institute of Hubei Topgene Biotechnology Co. LtdEast Lake High-Tech Development ZoneWuhan 430205China Fundamental Research Center Shanghai Yangzhi Rehabilitation Hospital (Shanghai Sunshine Rehabilitation Center)Tongji UniversityShanghai 200092China

The discovery of G-protein coupled receptor(GPCR)accessory proteins has fundamentally redefined the pharmacological concept of GPCR signaling,demonstrating a more complex molecular basis for receptor specificity on the plasma membrane and impressionable downstream intracellular *** accessory proteins not only contribute to the proper folding and trafficking of receptors but also exhibit selectable receptor preferences.

关键词： specificity GPCR neither

Immersive visualization of 3D subsurface ground model developed from sparse boreholes using virtual reality(VR)

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Underground Space 2024年第4期17卷 188-206页

作者： Borui lyu yu Wang Department of Architecture and Civil Engineering City University of Hong KongKowloon 999077Hong KongChina

Analytics and visualization of multi-dimensional and complex geo-data,such as three-dimensional(3D)subsurface ground models,is critical for development of underground space and design and construction of underground structures(e.g.,tunnels,dams,and slopes)in engineering *** complicated 3D subsurface ground models now can be developed from site investigation data(e.g.,boreholes)which is often sparse in practice,it remains a great challenge to visualize a 3D subsurface ground model with sophisticated stratigraphic variations by conventional two-dimensional(2D)geological *** reality(VR)technology,which has an attractive capability of constructing a virtual environment that links to the physical world,has been rapidly developed and applied to visualization in various disciplines *** on the rapid development of VR,this study proposes a framework for immersive visualization of 3D subsurface ground models in geo-applications using VR *** 3D subsurface model is first developed from limited borehole data in a data-driven ***,a VR system is developed using related software and hardware devices currently available in the markets for immersive visualization and interaction with the developed 3D subsurface ground *** results demonstrate that VR visualization of the 3D subsurface ground model in an immersive environment has great potential in revolutionizing the geo-practices from 2D cross-sections to a 3D immersive virtual environment in digital era,particularly for the emerging digital twins.

关键词： Immersive visualization 3D subsurface model Virtual reality Virtual environment Interaction

Physics-based battery SOC estimation methods:Recent advances and future perspectives

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Journal of Energy Chemistry 2024年第2期89卷 27-40,I0003页

作者： Longxing Wu Zhiqiang lyu Zebo Huang chao Zhang Changyin Wei College of Mechanical Engineering Anhui Science and Technology UniversityChuzhou 233100AnhuiChina Hubei Key Laboratory of Power System Design and Test for Electrical Vehicle Hubei University of Arts and ScienceXiangyang 441053HubeiChina School of Internet Anhui UniversityHefei 230039AnhuiChina School of Mechanical and Electrical Engineering Guilin University of Electronic TechnologyGuilin 541004GuangxiChina

The reliable prediction of state of charge(SOC)is one of the vital functions of advanced battery management system(BMS),which has great significance towards safe operation of electric *** far,the empirical model-based and data-driven-based SOC estimation methods of lithium-ion batteries have been comprehensively discussed and reviewed in various ***,few reviews involving SOC estimation focused on electrochemical mechanism,which gives physical explanations to SOC and becomes most attractive candidate for advanced *** this reason,this paper comprehensively surveys on physics-based SOC algorithms applied in advanced ***,the research progresses of physical SOC estimation methods for lithium-ion batteries are thoroughly discussed and corresponding evaluation criteria are carefully ***,future perspectives of the current researches on physics-based battery SOC estimation are *** insights stated in this paper are expected to catalyze the development and application of the physics-based advanced BMS algorithms.

关键词： Lithium-ion batteries State of charge Electrochemical model Battery management system

Real-Time 3D Ultrasound Imaging System Based on a Hybrid Reconstruction Algorithm

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Chinese Journal of Electronics 2024年第1期33卷 245-255页

作者： Yifei lyu yu SHEN Mingbo ZHANG Junchen WANG School of Mechanical Engineering and Automation Beihang University The First Medical Center General Hospital of Chinese PLA

As a safe and convenient imaging technology in clinical routine diagnosis, ultrasound imaging can provide real-time 2D images of internal tissues and organs. To realize real-time 3D image reconstruction, pixel nearest neighbor interpolation(PNN) reconstruction algorithm and Bezier interpolation algorithm are combined into a hybrid reconstruction algorithm. On this basis, a real-time interactive 3D ultrasound imaging system is *** temporal calibration and spatial calibration, the six degrees of freedom poses of 2D ultrasound images can be accurately collected. The 3D volume reconstructed by the proposed 3D reconstruction algorithm is visualized by volume rendering. A multi-thread software system allows parallel operation of data acquisition, 3D reconstruction,volume visualization and other functions. 3D imaging experiments on a 3D printing femur model, a neck phantom and the neck of human volunteers were performed for systematic evaluation. When the reconstruction voxel size was set to be(0.53 mm3, 1.03 mm3, 1.53 mm3), the reconstruction errors of the femur and trachea model were respectively(0.23 mm, 0.31 mm, 0.56 mm) and(0.62 mm, 0.88 mm, 1.41 mm). Clinical feasibility was demonstrated by application of the 3D ultrasound imaging on the neck of human volunteers.

关键词： Interpolation Three-dimensional displays Ultrasonic imaging Imaging Data visualization Reconstruction algorithms Real-time systems

Effectiveness of colorectal cancer screening integrating non-genetic and genetic risk: a prospective study based on UK Biobank data

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Cancer Biology & Medicine 2024年第8期21卷 712-723页

作者： yu Zhang chao Sheng Zhangyan lyu Hongji Dai Fangfang Song Fengju Song yubei Huang Kexin Chen Department of Epidemiology and Biostatistics Key Laboratory of Molecular Cancer EpidemiologyKey Laboratory of Prevention and Control of Human Major DiseasesMinistry of EducationNational Clinical Research Center for CancerTianjin Medical University Cancer Institute and HospitalTianjin Medical UniversityTianjin 300060China

Objective: Few studies have evaluated the benefits of colorectal cancer(CRC) screening integrating both non-genetic and genetic risk factors. Here, we aimed to integrate an existing non-genetic risk model(QCancer-10) and a 139-variant polygenic risk score to evaluate the effectiveness of screening on CRC incidence and ***: We applied the integrated model to calculate 10-year CRC risk for 430,908 participants in the UK Biobank, and divided the participants into low-, intermediate-, and high-risk groups. We calculated the screening-associated hazard ratios(HRs) and absolute risk reductions(ARRs) for CRC incidence and mortality according to risk ***: During a median follow-up of 11.03 years and 12.60 years, we observed 5,158 CRC cases and 1,487 CRC deaths, respectively. CRC incidence and mortality were significantly lower among screened than non-screened participants in both the intermediateand high-risk groups [incidence: HR: 0.87, 95% confidence interval(CI): 0.81±0.94;0.81, 0.73±0.90;mortality: 0.75, 0.64±0.87;0.70, 0.58±0.85], which composed approximately 60% of the study population. The ARRs(95% CI) were 0.17(0.11±0.24) and 0.43(0.24±0.61), respectively, for CRC incidence, and 0.08(0.05±0.11) and 0.24(0.15±0.33), respectively, for mortality. Screening did not significantly reduce the relative or absolute risk of CRC incidence and mortality in the low-risk group. Further analysis revealed that screening was most effective for men and individuals with distal CRC among the intermediate to high-risk ***: After integrating both genetic and non-genetic factors, our findings provided priority evidence of risk-stratified CRC screening and valuable insights for the rational allocation of health resources.

关键词： Colorectal cancer screening polygenic risk score incidence mortality

Digital twin modeling method for lithium-ion batteries based on data-mechanism fusion driving

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Green Energy and Intelligent Transportation 2024年第5期3卷 52-69页

作者： chao lyu Shaochun Xu Junfu Li Michael Pecht School of Electrical Engineering and Automation Harbin Institute of TechnologyHarbin 150001HeilongjiangChina School of Automotive Engineering Harbin Institute of TechnologyWeihai 264209ShandongChina Center for Advanced Life Cycle Engineering(CALCE) University of MarylandCollege ParkMD 20742USA

Lithium-ion batteries have been rapidly developed as clean energy sources in many industrial fields,such as new energy vehicles and energy *** core issues hindering their further promotion and application are reliability and safety.A digital twin model that maps onto the physical entity of the battery with high simulation accuracy helps to monitor internal states and improve battery *** work focuses on developing a digital twin model via a mechanism-data-driven parameter updating algorithm to increase the simulation accuracy of the internal and external characteristics of the full-time domain battery under complex working *** electrochemical model is first developed with the consideration of how electrode particle size impacts battery *** adding the descriptions of temperature distribution and particle-level stress,a multi-particle size electrochemical-thermal-mechanical coupling model is ***,considering the different electrical and thermal effect among individual cells,a model for the battery pack is constructed.A digital twin model construction method is finally developed and verified with battery operating data.

关键词： Lithium-ion battery Multi-particle size electrochemical-thermalmechanical coupling model Online model parameter updating algorithm Digital twin

Near real-time gravitational wave data analysis of the massive black hole binary with TianQin

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Science China(Physics,Mechanics & Astronomy) 2024年第7期67卷 175-186页

作者： Hong-yu Chen Xiang-yu lyu En-Kun Li Yi-Ming Hu MOE Key Laboratory of TianQin Mission TianQin Research Center for Gravitational Physics&School of Physics and AstronomyFrontiers Science Center for TianQinGravitational Wave Research Center of CNSASun Yat-sen University(Zhuhai Campus)Zhuhai 519082China

Space-borne gravitational wave(GW)detectors can detect the merger of massive black *** early warning and localization of GW events before merging can be used to inform electromagnetic telescopes and conduct multimessenger ***,this requires real-time data transmission and analysis *** geocentric orbit of the space-borne GW detector Tian Qin makes it possible to conduct real-time data *** this study,we develop a search and localization pipeline for massive black hole binaries(MBHBs)with Tian Qin under both regular and real-time data transmission *** demonstrate that,with real-time data transmission,MBHBs can be accurately localized on the *** the approaching merger,each analysis can be finished in only 40 *** an MBHB system at a distance of 1 Gpc,if we receive data every hour,then we can pinpoint its location to within less than 1 deg^(2)on the final day before the merger.

关键词： gravitational wave detectors and experiments black holes data analysis algorithms and implementation data management

Modification of Melting Combustion Kinetic Model of Fine Ash from Entrained-Flow Gasifier

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Journal of Thermal Science 2024年第1期33卷 300-310页

作者： WANG Wenyu LI Wei LU yu REN Qiangqiang lyu Qinggang Institute of Engineering Thermophysics Chinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China Dalian National Laboratory for Clean Energy Chinese Academy of SciencesDalian 116023China

Coal gasification technology is a prominent technology in the coal chemical industry and serves as the fundamental basis for various process industries,including coal-based chemicals,coal-based liquid fuels,Integrated Gasification Combined Cycle(IGCC) power generation,multi-generation systems,hydrogen production,and fuel *** gasification process generates significant quantities of ash residue,with annual emissions exceeding tens of millions of tons and accumulation reaching hundreds of millions of ***,there is an urgent need to investigate methods for its *** combustion of gasified fine ash(GFA) was conducted in a tube furnace,and the conventional shrinking core model was modified to accurately predict the combustion behaviors at different temperatures(900℃-1500℃).We divided the reaction temperatures into three ranges,which is defined as unmelted combustion(TFT) and mixed combustion(DTFT),the surface ash of GFA grains fell off,and the residual carbon and gas-phase reactants were nearly no longer affected by the diffusion resistance,thus significantly accelerated the reaction of internal residual *** order to predict the melt combustion process more accurately,the time term of the shrinkage core model(SCM) is modified,and the effective diffusion coefficient of T>FT is defined.

关键词： fine ash melting combustion kinetic model combustion characteristics